Novel approach for design of low index contrast multimode interference devices

Self-imaging theory is widely accepted as a good method in designing multimode interference (MMI) couplers, but it is also true that self-imaging theory is not suitable for low-contrast structures. An improved self-imaging theory is proposed in this paper for the optimal design of low-contrast 1 × N MMI couplers. The average effective width of the MMI waveguide and the average effective propagation constant of the MMI waveguide are used in the improved self-imaging theory. An approach is given to find the average effective width. We use this approach in the optimal design of a 1?×?4 silica MMI coupler, and the results show that the improved self-imaging theory is more accurate than conventional self-imaging theory for low-contrast structures.     

Observation of a fast-formed absorption grating and a slowly formed phase grating in undeveloped dichromated gelatin

Real-time diffraction efficiency is measured during hologram formation in undeveloped dichromated gelatin (DCG) film. The main features of real-time diffraction efficiency of undeveloped DCG reveal double peaks with increasing exposure time. Adopting the grating translation technique, we show that the first peak originates from the absorption grating and that the latter is related to the phase grating. To explain such complicated hologram-formation dynamics, we present a phenomenological model for mixed gratings associated with photoinduced refractive-index changes and absorption changes. We have compared the model results with the experimental results, which show good agreement.     

Electrochemical assay of nonlabeled DNA chip and SNOM imaging by using streptavidin-biotin interaction

The assay of DNA biosensor-based nucleic acid recognition using microfabrication technology provides for high sensitivity, good surface coverage and reproducibility. We have achieved efficient immobilization and hybridization of nonlabeled DNA using cyclic voltammetry (CV), square wave voltammetry (SWV) and scanning near-field optical microscopy (SNOM) techniques. The increased electrochemical response observed following the immobilization of biotinlyated ssDNA probe suggests that nucleic acid is a somewhat better medium for electronic transfer. We demonstrated the high coverage of immobilized FITC-labeled biotinylated DNA probe on a streptavidin-modified surface using SNOM imaging. SNOM imaging of FITC-labeled complementary DNA also exhibited fluorescent light spots of hybridization distributed throughout. No fluorescent light was observed with the hybridization of non-complementary DNA.     

Direct observation of surface mode excitation and slow light coupling in photonic crystal waveguides

A scanning near-field optical microscope (SNOM) is used to systematically study the properties of guided modes in linear and slow-light regimes of silicon-on-insulator (SOI)-based photonic crystal waveguides (PhCWs) with different terminations of the photonic lattice. High quality SNOM images are obtained for light at telecom wavelengths propagating in the PhCW, demonstrating directly, for the first time to our knowledge, drastic widening of the PhCW guided mode in the slow-light regime and excitation of surface waves at the PhCW interface along with their feeding into the guided mode for the lattice terminations corresponding to significantly reduced coupling loss.     

Near-field microscopy and lithography of light-emitting polymers

We describe the application of scanning near-field optical microscopy (SNOM) to the study of the photophysical and self-organization properties of thin films of blends of conjugated polymers, and also to the lateral nanoscale patterning of conjugated-polymer structures. Such thin-film plastic semiconductor nanostructures offer significant potential for use in opto-electronic devices. The implementation of SNOM we employ is the most established form in which a probe with a sub-wavelength aperture is scanned in close proximity to the sample surface. We consider the nature of the near-field optical distribution, which decays within the first ca. 100 nm of these semiconductor materials, and address the identification of topographic artefacts in near-field optical images. While the topographic information obtained simultaneously with optical data in any SNOM experiment enables an easy comparison with the higher-resolution tapping-mode atomic force microscopy, the spectroscopic contrast provided by fluorescence SNOM gives an unambiguous chemical identification of the different phases in a conjugated-polymer blend. Both fluorescence and photoconductivity SNOM indicate that intermixing of constituent polymers in a blend, or nanoscale phase separation, is responsible for the high efficiency of devices employing these materials as their active layer. We also demonstrate a scheme for nano-optical lithography with SNOM of conjugated-polymer structures, which has been employed successfully for the fabrication of poly(-phenylene vinylene) nanostructures with 160 nm feature sizes.     

Ray-tracing method for isotropic inhomogeneous refractive-index media from arbitrary discrete input

We have developed a ray-tracing simulation procedure for optically isotropic gradient refractive-index media. The procedure can take discrete points of arbitrary distribution for the definition of refractive-index distributions and lens surfaces. It is useful for simulating ray trajectories in real lens systems. The procedure is applied to a ray-tracing simulation of the Luneburg lens and a radial gradient optical fiber. The simulation results are compared with the analytical solutions, and it is shown that they are in precise agreement.     

Fluorescence resonance energy transfer scanning near-field optical microscopy

The method of fluorescence resonance energy transfer scanning near-field optical microscopy (FRET SNOM) consists in the separation of a FRET pair between an SNOM tip and a sample. The donor (or acceptor) centre is located at the tip apex and scanned in the vicinity of a sample while acceptor fluorescence (or donor-fluorescence quenching) is detected. It is shown that the spatial resolution for such an approach is governed not by the aperture size but by the FRET characteristic radius (F?rster radius), and thus can attain the value of 2-7 nm with the same (or higher) sensitivity as characteristic for the aperture SNOM. The theoretical fundamentals of the method, its experimental realization and connections with other types of near-field optical microscopy are discussed. Coherent FRET SNOM, which can be realized at liquid helium temperatures, and its possible applications for quantum informatics, are briefly outlined.     

Observation of the dynamics of live cardiomyocytes through a free-running scanning near-field optical microscopy setup

We report the observation of live-cell dynamics by noncontact scanning near-field optical microscopy (SNOM) modified to work with living biological samples that are fully immersed in liquid. We did not use the SNOM setup in strictly near-field conditions (we used 1-mum constant-height mode); however, we could examine the dynamics of rhythmically beating cardiac myocytes in culture with extremely high vertical sensitivity below the nanometric range. We could halt scans at any point to record localized contraction profiles of the cell membrane. We show that the contractions of the organisms changed shape dramatically within adjacent areas. We believe that the spatial dependency of the contractions arises because of the measurement system's ability to resolve the behavior of individual submembrane actin bundles. Our results, combining imaging and real-time recording in localized areas, reveal a new, to our knowledge, noninvasive method for using SNOM setups for studying the dynamics of live biological samples.     

Measurement of refractive-index change at a liquid-solid interface close to the critical angle

We measured the refractive-index change on a liquid sample, using the reflection of a polarized Gaussian laser beam close to the angle of total reflection. We applied this technique to a solution of nickel (ii) phthalocyanine tetrasulfonated (NiPTS) in water-ethanol (1/1 v/v), in which the nonlinearity of the refractive index is due to optically induced thermal effects. We show that close to the angle of total reflection the sensitivity of this technique is four times bigger than at normal incidence.     

Refractive-index structure parameter in the planetary boundary layer: comparison of measurements taken with a 10.6-microm coherent lidar, a 0.9-microm scintillometer, and in situ sensors

An optical technique is described that determines the path-averaged value of a refractive-index structure parameter at 10.6 mum by use of a pulsed coherent CO(2) lidar in direct detection and hard-target returns. The lidar measurements are compared with measurements taken by a 0.9-mum scintillometer and temperature probe (with humidity corrections). The experimental results show good agreement for C(n)(2) >/= (-14) m(-2/3). With respect to practical applications the new technique permits C(n)(2) lidar measurements in a neutral meteorological situation to an unstably stratified convective boundary layer over long ranges (1 km or more).     

Dilute-melt, proton-exchange slab waveguides in LiNbO 3 : a new fabrication and characterization method

A method of dilute-melt proton exchange employing a mixture of glycerol and KHSO4 with lithium benzoate added is used to fabricate planar waveguides in c -cut LiNbO3 . With this exchange melt system the waveguide refractive-index profiles can be fabricated with a high degree of reproducibility. In contrast with the traditional dilute-melt method, which uses benzoic acid and lithium benzoate, the need for sealed containers during the exchange process can be avoided when the glycerol, KHSO4 , and lithium benzoate system is used for the exchange process. A new characterization method for determining the waveguide refractive-index profile from the measured-mode indexes is introduced. The main advantage of this characterization method compared with other methods is that it also applies to single-mode waveguides. Using the new characterization method, we investigate in detail the relation between waveguide refractive-index change and composition of this glycerol, KHSO4 and lithium benzoate exchange melt system.     

Modeling and experimental observation of an on-chip two-dimensional far-field interference pattern

In this paper, we model and experimentally observe the far-field radiation produced by interfering beams propagating in two-dimensional (2D) slab waveguides. Using a transmission-line analogy, we compare the 2D propagation with standard three-dimensional (3D) far-field representations and derive the 2D conditions for using standard far-field approximations. Then we test our theoretical results by experimentally observing the 2D far-field pattern produced by a 1×3 multimode interference (MMI) coupler on a silicon nanomembrane. The MMI outputs are connected to a slab silicon waveguide, and the far field is observed at the edge of the silicon slab. This represents the observation of 2D far-field pattern produced by an array of on-chip radiators.     

Design and modeling of ultrashort MMI-based couplers

In this work, based on the Gaussian-modes theory, modeling and analysis of ultrashort (<10 µm) MMI couplers is performed. Using the introduced model, temporal behaviors and also other features such as insensitivity to input polarization, insensitivity to operating wavelength and manufacturing tolerances of these devices are studied. In addition, the optimal refractive-index structures with no sensitivity to the polarization are obtained. A comparison is made between this model and the semi-sinusoidal model and it is shown that the Gaussian model is necessary to handle these ultrashort devices. In addition, accuracy of the model is justified using a comparison with results of direct simulations obtained using the FEMLAB environment and FDTD method.     

Near-Field Surface-Enhanced Raman Imaging of Dye-Labeled DNA with 100-nm Resolution

Raman chemical imaging on a scale of 100 nm is demonstrated for the first time. This is made possible by the combination of scanning near-field optical microscopy (SNOM or NSOM) and surface-enhanced Raman scattering (SERS), using brilliant cresyl blue (BCB)-labeled DNA as a sample. SERS substrates were produced by evaporating silver layers on Teflon nanospheres. The near-field SERS spectra were measured with an exposure time of 60 s and yielded good signal-to-noise ratios (25:1). The distinction between reflected light from the excitation laser and Raman scattered light allows the local sample reflectivity to be separated from the signal of the adsorbed DNA molecules. This is of general importance to correct for topographic coupling that often occurs in near-field optical imaging. The presented data show a lateral dependence of the Raman signals that points to special surface sites with particularly high SERS enhancement.     

Realization of a multichannel integrated Young interferometer chemical sensor

We report on the design, realization, and characterization of a four-channel integrated optical Young interferometer device that enables simultaneous and independent monitoring of three binding processes. The generated interference pattern is recorded by a CCD camera and analyzed with a fast-Fourier-transform algorithm. We present a thorough theoretical analysis of such a device. The realized device is tested by monitoring glucose solutions that induce well defined phase changes between output channels. The simultaneous measurement of three different glucose concentrations shows the multipurpose feature of such devices. The observed errors, caused by the mismatching of spatial frequencies of individual interference patterns with those determined from the CCD camera, are reduced with different reduction schemes. The phase resolution for different pairs of channels was approximately 1 x 10(-4) fringes, which corresponds to a refractive-index resolution of approximately 8.5 x 10(-8). The measured sensitivity coefficient of the phase change versus refractive-index change of approximately 1.22 x 10(3) x 2pi agrees well with the calculated coefficient of approximately 1.20 x 10(3) x 2pi.     

Deterministic beam fanning in Fe-doped stoichiometric lithium niobate crystals

We investigated the beam-fanning effect in Fe-doped stoichiometric lithium niobate (Fe:SLN) crystals that were grown by the top-seeded solution growth method. Deterministic beam fanning (DBF) was measured in Z-cut Fe:SLN crystal for incident light propagating along the c+ and c- axes. The dependence of beam-fanning factors on incident power density was also studied. The experimental results of DBF in the Z-cut Fe:SLN crystal were in good agreement with a theoretical simulation based on a two-wave mixing model. The results compared with those for Fe-doped congruent lithium niobate crystals indicate that the beam-fanning process in Fe:SLN is deterministic because of its much-reduced intrinsic density of defects.     

Precise Measurement of Thermal-Induced Refractive-Index Change in BaTiO(3) on the Basis of Anisotropic Self-Diffraction

We propose a method for precise measurement of the temperature-dependent refractive-index change in BaTiO(3) by use of anisotropic self-diffraction (ASD). In this method the refractive-index change corresponds to the angle deviation of the diffraction pattern. Because only the geometry of the ASD is used for measuring, the precision of measurement is independent of crystal thickness and environmental perturbation. The accuracy of the refractive-index change achieved is 10(-4) when the resolution of the measurement of the angle is ~0.04 degrees . Both the theory and the experiment are demonstrated.     

Refractive-Index Changes of Standard Telecommunication Fiber through Exposure to Femtosecond Laser Pulses at 810 cm

We report on permanent refractive-index changes as great as 6 x 10(-3) in standard fibers on irradiation with tightly focused femtosecond (120-fs) near-IR (lambda = 800-nm) pulses. The refractive-index increase was measured through changes in the transmission spectrum of an UV photowritten Bragg-grating-based Fabry-Perot interferometer. We depict the dependence of the index variation on exposure time. The changes in refractive index can be optimized after a few seconds of irradiation. The measured induced excess loss increases during near-IR exposure.