Beta Spectrometry with Magnetic Calorimeters

Absolute activity measurements of alpha, beta and gamma emitting radioactive sources are important in numerous fields such as therapeutic radiology and the characterization of nuclear waste. Conventional ionization and liquid scintillation detectors, which are commonly used for these applications, have an energy dependent quantum efficiency and severe limitations in energy resolution. As a novel alternative we have developed a detector based on a metallic magnetic calorimeter (MMC) with a gold absorber that covers the full solid angle of 4π around the radioactive source. Deposition of energy in the absorber causes a temperature rise and results in a change of magnetization of a parametric Au:Er sensor, which can be measured by a low-noise high-bandwidth dc-SQUID. The detector has equal sensitivity for beta and gamma radiation. In this paper we describe a detector which has a deviation from linear behavior for energies up to 700 keV of smaller than 0.5% and an overall quantum efficiency for beta particles in this energy range close to unity. We show the data of our experiments measuring the decay of ³⁶Cl and compare the results to the theoretically expected spectrum for this second order forbidden non-unique β-decay. We discuss the observed contributions to noise, the quantum efficiency and the achieved energy resolution.     

Development of integrated ΔE-E silicon detector telescope using silicon planar technology

An integrated ΔE-E silicon detector telescope using silicon planar technology has been developed. The technology developed is based on standard integrated circuit technology and involves double sided wafer processing. The ΔE and E detectors have been realized in a PIN configuration with a common buried N⁺ layer. Detectors with ΔE thicknesses of 10, 15 and 25 μm, and E detector with thickness of 300 μm have been fabricated and tested with alpha particles using ²³⁸Pu-²³⁹Pu dual alpha source. The performance of the detector with ΔE detector of thickness 10 μm and E detector of thickness 300 μm has been studied for identification of charged particles using 12 MeV ⁷Li⁺ ion beam on carbon target. The results of these tests demonstrate that the integrated detector telescope clearly separates the charged particles, such as alpha particles, protons and ⁷Li. Due to good energy resolution of the E detector, discrete alpha groups corresponding to well known states of ¹⁵N populated during the reaction could be clearly identified.     

Observations on dual-ended readout of 100 mm long LYSO crystals

We are investigating using dual-ended readout of axially oriented long thin scintillator crystals in detectors for a compact geometry, small ring diameter animal PET system. The axial position of interaction is determined from the light sharing between two photodetectors at opposite ends of the crystal. We examine the light output, energy resolution and axial spatial resolution of 1.5-5×2×100 mm³ polished LYSO crystals by irradiating with an electronically collimated beam of 511 keV photons oriented perpendicular to the long axis and read out at either end by position sensitive photomultiplier tubes (PSPMTs). Three reflector materials, namely Teflon, 3 M enhanced specular reflector (ESR) and black paint are examined for the 2×2×100 mm³ crystal size. The light output increases and energy resolution improves with the crystal cross-section. Generally, the spatial resolution worsens with increase in crystal cross-section. For the 2×2×100 mm³ crystal size, the mean energy resolutions of the photopeak over the nine irradiation positions were 14.4±0.4%, 16.0±1.2% and 28.3±2.1% with mean spatial resolutions of 7.0±1.0, 9.4±3.3 and 26.0±5.0 mm using ESR, Teflon and black paint, respectively. ESR reflector gave the best light output, energy and axial spatial resolutions. These characterization results of PSPMT-based dual-ended long LYSO crystals will be useful in the design of detector modules for a highly compact geometry preclinical PET system using this detector technology.     

Development of an energy-binned photon-counting detector for X-ray and gamma-ray imaging

The aim of this study is to develop an energy-binned photon-counting (EBPC) detector that enables us to provide energy information of x-rays with a reasonable count statistics. We used Al-pixel/CdTe/Pt semiconductor detectors, which had an active area of 8 mm×144 mm and consisted of 18 modules aligned linearly. The size of a CdTe detector module was 8 mm×8 mm and the thickness of the CdTe crystal was 1 mm. Each module consisted of 40×40 pixels and the pixel size was 200 μm×200 μm. We applied the bias voltage of −500 V to the Pt common electrode. The detector counted the number of x-ray photons with four different energy windows, and output four energy-binned images with pixel depths of 12, 12, 11 and 10 bits at a frame rate of 1200 Hz (300 Hz×4 energy bins). The basic performance of the detector was evaluated in several experiments. The results showed that the detector realized the photon counting rate of 0.4×10⁶ counts/sec/pixel (10⁷ counts/sec/mm²), energy resolution 4.4% FWHM at 122 keV. The integral uniformity of the detector was about 1% and the differential uniformity was about 1%. In addition, the image quality was examined with a resolution chart and step-wedge phantoms made of aluminum and polymethyl methacrylate. And we compared the quality of an acquired image with that acquired with an energy integration detector. The results of these experiments showed that the developed detector had desirable intrinsic characteristics for x-ray photon counting imaging.     

Metallic Magnetic Calorimeters for Particle Detection

The principles and theory of operation of a magnetic calorimeter, made of a dilute concentration of paramagnetic ions in a metallic host, is discussed in relation to the use of such a device as a detector of x-rays. The response of a calorimeter to the absorption of energy depends upon size, heat capacity, temperature, magnetic field, concentration of spins and interactions among them. The conditions that optimize the performance of a calorimeter are derived. Noise sources, especially that due to thermodynamic fluctuations of the electrons in the metal, are analyzed. Measurements have been made on detectors in which Er serves as the paramagnetic ion and Au as the host metal. The measured resolution of a detector with a heat capacity of 10^–12 J/K was 12 eV at 6 keV. In a detector suitable for use with hard x-rays up to 200 keV a resolution of 120 eV was obtained. Calculations indicate that the performance of both detectors can be improved by an order of magnitude. At temperatures below 50 mK, the time response of the Au : Er calorimeters to an energy deposition indicates the presence of an additional heat capacity, which we interpret as arising from the quadruple splitting of the Au nuclei in the electric field gradients introduced by the presence of the Er ions.     

Cryogenic detection of particles with a SQUID-assisted thermocouple Au:Fe-Nb and silicon absorber

The feasibility of thermoelectric detection in cryogenic detectors was demonstrate at elevated temperature of 1 K with a 33 mm³ volume silicon absorber placed in electrical field. Au:Fe-Nb thermocouple was used as a thermometer, installed directly on the heat absorber. The resolution, provided by Au:Fe-Nb thermocouple with SQUID read-out was 2.10^–7 K/Hz^1/2, which is one order of magnitude less than expected, and was limited by a noise of SQUID electronics.     

Evaluation of silicon active pixel sensors for alpha particle detection

Alpha particles can be used as a test stimulus offering several advantages for probing materials of micrometre thicknesses. In this work a silicon CMOS Active Pixel Sensor (APS) is evaluated for alpha particle detection and imaging. These devices can replace traditionally used solid-state track detectors, giving advantages of increased sensitivity, improved linearity and higher dynamic range. CMOS APSs offer high detection efficiency, low noise and digital readout. Qualitative and quantitative analysis of the back-illuminated back-thinned (BT) and standard sensor response to 5.5 MeV alpha particles is presented. Alpha particle detection efficiency was estimated and energy resolution was measured. Imaging capabilities were assessed and quantified. Cluster centroiding algorithms were implemented for image quality improvement.     

Development of Large Bismuth Absorbers for Magnetic Calorimeters Applied to Hard X-ray Spectrometry

Bismuth is an interesting material for magnetic calorimeter absorbers applied to high energy resolution X-ray spectrometry; it has a low specific heat and high atomic number. However, past detector developments with Bi absorbers were confronted with the low thermal conductivity of bismuth that degraded the energy resolution and deformed the detector response function (non-Gaussian energy peak). In the present study, we have investigated the performances of large bulk bismuth absorbers ( \(1\times 1\times 0.16\)  mm \(^{3}\) ) thermally coupled to metallic magnetic sensors. Despite a very good baseline energy resolution, detectors with monolithic bismuth absorbers have degraded FWHM energy resolutions with any type of thermal coupling between the absorber and the sensor tested. In comparison tests with BiCu and BiAg bilayer absorbers demonstrated much better performances.     

Small pixel CZT detector for hard X-ray spectroscopy

A new small pixel cadmium zinc telluride (CZT) detector has been developed for hard X-ray spectroscopy. The X-ray performance of four detectors is presented and the detectors are analysed in terms of the energy resolution of each pixel. The detectors were made from CZT crystals grown by the travelling heater method (THM) bonded to a 20×20 application specific integrated circuit (ASIC) and data acquisition (DAQ) system. The detectors had an array of 20×20 pixels on a 250 μm pitch, with each pixel gold-stud bonded to an energy resolving circuit in the ASIC. The DAQ system digitised the ASIC output with 14 bit resolution, performing offset corrections and data storage to disc in real time at up to 40,000 frames per second. The detector geometry and ASIC design was optimised for X-ray spectroscopy up to 150 keV and made use of the small pixel effect to preferentially measure the electron signal. A ²⁴¹Am source was used to measure the spectroscopic performance and uniformity of the detectors. The average energy resolution (FWHM at 59.54 keV) of each pixel ranged from 1.09±0.46 to 1.50±0.57 keV across the four detectors. The detectors showed good spectral performance and uniform response over almost all pixels in the 20×20 array. A large area 80×80 pixel detector will be built that will utilise the scalable design of the ASIC and the large areas of monolithic spectroscopic grade THM grown CZT that are now available. The large area detector will have the same performance as that demonstrated here.     

Advances in silicon carbide X-ray detectors

The latest advances in SiC X-ray detectors are presented: a pixel detector coupled to a custom ultra low noise CMOS preamplifier has been characterized at room and high temperature. An equivalent noise energy (ENE) of 113 eV FWHM, corresponding to 6.1 electrons r.m.s., has been achieved with the detector/front-end system operating at +30 °C. A Fano factor of F=0.10 has been estimated from the ⁵⁵Fe spectrum. When the system is heated up to +100 °C, the measured ENE is 163 eV FWHM (8.9 electrons r.m.s.). It is determined that both at room and at high temperature the performance are fully limited by the noise of the front-end electronics. It is also presented the capability of SiC detectors to operate in environments under unstable temperature conditions without any apparatus for temperature stabilization; it has been proved that a SiC detector can acquire high resolution X-ray spectra without spectral line degradation while the system temperature changes between +30 and +75 °C.     

GaN-based PIN alpha particle detectors

GaN-based PIN alpha particle detectors are studied in this article. The electrical properties of detectors have been investigated, such as current-voltage (I-V) and capacitance-voltage (C-V). The reverse current of all detectors is in nA range applied at 30 V, which is suitable for detector operation. The charge collection efficiency (CCE) is measured to be approximately 80% but the energy resolution is calculated to be about 40% mostly because the intrinsic layer is not sufficiently thick enough.     

Performance measurements from LYSO scintillators coupled to a CMOS position sensitive SSPM detector

We have designed a 5×5 mm² position sensitive solid-state photomultiplier (PS-SSPM) using a complementary metal-oxide-semiconductor (CMOS) process that provides imaging capability on the micro-pixel level. The PS-SSPM has 11,664 micro-pixels total, with each having an active area and micro-pixel pitch of 30×30 μm² and 44.3 μm, respectively. The PS-SSPM was then examined for its performance characteristics such as its energy and spatial resolution, and LYSO scintillator array imaging capabilities. When coupled to 5×5×3 mm³ LYSO, the energy resolution at 511 keV (²²Na) was measured as a function of bias, and corrected for the PS-SSPM non-linear output. The resolution is 14% (FWHM) at 511 keV with 30 V bias. The LYSO coincidence timing resolution was 9.4 ns (FWHM) at 511 keV. Spatial resolution studies were conducted using a focused (∼30 μm beam spot diameter) pulsed 635 nm diode laser. Scintillator array imaging studies were conducted at 511 keV using a 6×6 LYSO array, having 500 μm pixels (530 μm pitch) and 5 mm tall.     

Microfabrication of Transition-Edge Sensor Arrays of Microcalorimeters with <Superscript>163</Superscript>Ho for Direct Neutrino Mass Measurements with HOLMES

HOLMES is aiming at a direct measurement of neutrino mass by performing a calorimetric measurement of the energy released in the decay of ¹⁶³Ho. In such approach, the ¹⁶³Ho source, with the required activity, needs to be embedded in the detector. HOLMES will deploy a large array of transition-edge sensor microcalorimeters with implanted ¹⁶³Ho ions. While good progress has been made in optimizing single pixel design and fabrication to achieve the target resolution, a major challenge is the fabrication of arrays of such microcalorimeters with the required amount of ¹⁶³Ho ions embedded in the detectors absorber. We describe the multi-step microfabrication process implemented to produce the detector arrays for HOLMES. One crucial part of such process is the ability to perform co-deposition of gold during the ¹⁶³Ho implantation process on the detectors absorber. We describe the UHV target chamber, with integrated gold deposition system, we have built to achieve this goal.     

Evaluation of large deuterated scintillators for fast neutron detection (E=0.5-20 MeV) using the D(d,n)He, C(d,n) and Al(d,n) reactions

The response of large deuterated liquid scintillators (up to 10 cm diameter by 15 cm) to neutrons 0.5-20 MeV has been studied using the 2.5 MeV neutron generator at the University of Michigan, and the d(d,n), ¹³C(d,n), ²⁷Al(d,n) and other reactions at the University of Notre Dame FN tandem accelerator. The latter utilize 9 and 16 MeV deuteron beams including a pulsed beam, which permitted time-of-flight measurements. Combining pulse-shape discrimination and time-of-flight allows gating on specific neutron energy groups to determine the detector response to specific neutron energies. This will permit accurate simulation of the detector response functions for applications of these detectors in nuclear research and homeland security applications.     

Lithographically patterned magnetic calorimeter X-ray detectors with integrated SQUID readout

We describe the design, fabrication and performance of a fully lithographically patterned magnetic microcalorimeter X-ray detector. The detector is fabricated on the same chip as a low-noise SQUID that measures the change in the magnetic sensor film's magnetization as the film is heated by absorbed X-rays. Our proof-of-principle detectors use a 100 μm×100 μm–2 μm paramagnetic Au:Er film coupled to a low-noise on-chip SQUID via a meandering superconducting pickup loop that also provides the magnetic field bias to the film. Absorption of 6 keV X-rays in the film causes heating on the order of 1 mK with a decay time of 1 ms or less, the fastest reported using a magnetic calorimeter. However, the resolution is currently poor due to poor Au:Er film properties and non-optimized coupling to the SQUID. We describe the design and fabrication of this device and present measurements of the heat capacity, decay time constant and effective thermal conductance of the microcalorimeter as a function of temperature. Because the SQUID and calorimeter are lithographically patterned on the same substrate, this technology can be readily applied to the fabrication of arrays of multiplexed magnetic microcalorimeter detectors.     

High Energy Resolution Cryogenic Alpha Spectrometers Using Magnetic Calorimeters

We report the recent progress on high resolution alpha spectrometers that use metallic magnetic calorimeters. The detector is composed of a meander-type magnetic calorimeter and a gold-foil absorber. The thermal connection between the magnetic sensor and the absorber consists of annealed gold wires. The signal rise time is found to be as expected, with the electronic thermal conductance of gold wires. The energy resolution of a 3.2?keV FWHM is obtained for 5.5?MeV alpha particles with possibilities for further improvements.     

Cryogenic composite detectors for the dark matter experiments CRESST and EURECA

Weakly interacting massive particles (WIMPs) are candidates for non-baryonic dark matter. WIMPs are supposed to interact with baryonic matter via scattering off nuclei producing a nuclear recoil with energies up to a few 10 keV with a very low interaction rate of 10⁻⁶ events per kg of target material and day in the energy region of interest. The dark matter experiment cryogenic rare event search with superconducting thermometers (CRESST) and the European underground rare event calorimeter array (EURECA) project are aimed at the direct detection of WIMPs with the help of very sensitive modularised cryogenic detectors that basically consist of a transition edge sensor (TES) in combination with a massive absorber crystal. In the CRESST experiment the search for coherent WIMP-nucleon scattering events is validated by the detection of two processes. In the scintillating absorber single crystal, CaWO₄, heat (phonons) and scintillation light are produced and detected with two independent cryogenic detectors: a phonon channel and a separate light channel.The development of such cryogenic detectors and the potential ton-scale production are investigated in this paper. To decouple the TES production from the choice of the target material in order to avoid heating cycles of the absorber crystal and to allow pretesting of the TESs, a composite detector design (CDD) for the detector production has been developed and studied. An existing thermal detector model has been extended to the CDD, in order to investigate, understand, and optimize the performance of composite detectors. This extended model, which has been worked out in detail, can be expected to provide a considerable help when tailoring composite detectors to the requirements of various experiments.     

Microstructured Magnetic Calorimeter with Meander-Shaped Pickup Coil

In the last years metallic magnetic calorimeters (MMC) showed an energy resolution of a few eV for x-rays up to 10 keV. This makes MMCs a promising and powerful tool for many applications where photons or energetic massive particles have to be detected—like absolute activity measurements of radioactive isotopes, high resolution x-ray spectroscopy and x-ray fluorescence material analysis. However, in order to fulfill all requirements of these applications and to allow to reach the maximum resolving power a consequent micro-fabrication of the MMC detectors is needed. The micro-fabrication of metallic magnetic calorimeters requires reliable deposition and patterning processes for niobium structures with high critical currents and for paramagnetic sensors. As one result of our advances in microstructuring a fully microfabricated MMC which consists of a meander shaped niobium thin film pickup coil and a 3 μm thick sputter deposited paramagnetic Au:Er temperature sensor will be presented. Deposition of energy in the paramagnetic sensor causes a rise in temperature and results in a change of magnetization, which is measured by a low noise high bandwidth dc-SQUID. The sputter deposited Au:Er films we report on are working well and show thermodynamic properties close to the ones known from bulk material down to temperatures of 45 mK.      

Characterization of bismuth tri-iodide single crystals for wide band-gap semiconductor radiation detectors

Bismuth tri-iodide is a wide band-gap semiconductor material that may be able to operate as a radiation detector without any cooling mechanism. This material has a higher effective atomic number than germanium and CdZnTe, and thus should have a higher gamma-ray detection efficiency, particularly for moderate and high energy gamma-rays. Unfortunately, not much is known about bismuth tri-iodide, and the general properties of the material need to be investigated. Bismuth tri-iodide does not suffer from some of the material issues, such as a solid state phase transition and dissociation in air, that mercuric iodide (another high-Z, wide band-gap semiconductor) does. Thus, bismuth tri-iodide is both easier to grow and handle than mercuric iodide. A modified vertical Bridgman growth technique is being used to grow large, single bismuth tri-iodide crystals. Zone refining is being performed to purify the starting material and increase the resistivity of the crystals. The single crystals being grown are typically several hundred mm³. The larger crystals grown are approximately 2 cm³. Initial detectors are being fabricated using both gold and palladium electrodes and palladium wire. The electron mobility measured using an alpha source was determined to be 260±50 cm²/Vs. An alpha spectrum was recorded with one of the devices; however the detector appears to suffer from polarization.     

Development of Metallic Magnetic Calorimeters for High Precision Measurements of Calorimetric 187Re and 163Ho Spectra

The measurement of calorimetric spectra following atomic weak decays, beta?(β) and electron capture (EC), of nuclides having a very low Q-value, can provide an impressively high sensitivity to a non-vanishing neutrino mass. The achievable sensitivity in this kind of experiments is directly connected to the performance of the used detectors. In particular an energy resolution of a few eV and a pulse formation time well below 1?μs are required. Low temperature Metallic Magnetic Calorimeters (MMCs) for soft X-rays have already shown an energy resolution of 2.0?eV FWHM and a pulse rise-time of about 90?ns for fully micro-fabricated detectors. We present the use of MMCs for high precision measurements of calorimetric spectra following the β-decay of ¹⁸⁷Re and the EC of ¹⁶³Ho. We show results obtained with detectors optimized for ¹⁸⁷Re and for ¹⁶³Ho experiments respectively. While the detectors equipped with superconducting Re absorbers have not yet reached the aimed performance, a first detector prototype with a Au absorber having implanted ¹⁶³Ho ions already shows excellent results. An energy resolution of 12?eV FWHM and a rise time of 90?ns were measured.