使用离散钍铀燃料组件的CANDU6堆物理特性初步研究

为研究钍铀燃料在CANDU6堆中的应用,采用DRAGON/DONJON程序,对使用离散型钍铀燃料37棒束组件的CANDU6堆进行时均堆芯分析。结果表明,组件采用235U富集度为2.5%的铀棒以及第1、2、3圈布置钍棒的37棒束组件,堆芯在8棒束换料、3个燃耗分区的方案下,组件的冷却剂空泡反应性较使用天然铀的37棒束组件（NU-37组件）与采用混合钍铀元件棒的37棒束组件更负;堆芯最大时均通道/棒束功率满足小于6700?kW/860?kW的限值;燃料转化能力比采用NU-37组件时更高;卸料燃耗可到达13400?MW·d/t(U)。研究表明,所设计的离散型钍铀燃料37棒束组件可用于现有CANDU6堆芯,且无需对堆芯结构及控制机构作重大改造;燃料组件和堆芯设计方案可为钍铀燃料在CANDU6堆芯的应用提供参考。      

A model for coolant void reactivity evaluation in assemblies of CANDU cells

Coolant void reactivity is a very important safety parameter in CANDU reactor analysis. Here we evaluate the coolant void reactivity in a 2 × 2 heterogeneous assembly of CANDU cells using the code DRAGON. Since the current version of DRAGON can only treat the coolant void reactivity for a single CANDU cell, an approximate model for the geometry must be considered to perform assembly calculations in a 2 × 2 pattern. The model we propose consists of replacing the annular fuel pins by equivalent square fuel pins. The equivalence between annular fuel pins and square fuel pins is brought about by homogenizing the fuel plus its sheath and subsequently conserving the reaction rates between the two geometries using a SPH equivalence procedure. The approximate CANDU cells constructed using square pins were used to perform the transport calculations in 2 × 2 assembly patterns. In addition, the model was used to evaluate coolant void reactivity in 2 × 2 checkerboard voiding patterns. These calculations reflect more accurately the actual voiding situation being studied. This helps in assessing the effects due to the coupling of neutrons born in one cell to those born in the neighbouring cells.     

Comparison of thorium-based fuels with different fissile components in existing boiling water reactors

With the aim of investigating the technical feasibility of fuelling a conventional BWR (Boiling Water Reactor) with thorium-based fuel, computer simulations were carried out in a 2D infinite lattice model using CASMO-5. Four different fissile components were each homogenously combined with thorium to form mixed oxide pellets: Uranium enriched to 20% U-235 (LEU), plutonium recovered from spent LWR fuel (RGPu), pure U-233 and a mixture of RGPu and uranium recovered from spent thorium-based fuel. Based on these fuel types, four BWR nuclear fuel assembly designs were formed, using a conventional assembly geometry (GE14-N). The fissile content was chosen to give a total energy release equivalent to that of a UOX fuel bundle reaching a discharge burnup of about 55 MWd/kgHM. The radial distribution of fissile material was optimized to achieve low bundle internal radial power peaking. Reactor physical parameters were computed, and the results were compared to those of reference LEU and MOX bundle designs. It was concluded that a viable thorium-based BWR nuclear fuel assembly design, based on any of the fissile components, can be achieved. Neutronic parameters that are essential for reactor safety, like reactivity coefficients and control rod worths, are in most cases similar to those of LEU and MOX fuel. This is also true for the decay heat produced in irradiated fuel. However when Th is mixed with U-233, the void coefficient (calculated in 2D) can be positive under some conditions. It was concluded that it is very difficult to make savings of natural uranium by mixing LEU (20% U-235) homogenously with thorium and that mixing RGPu with thorium leads to more efficient consumption of Pu compared to MOX fuel.     

等效天然铀燃料中子学性能分析

采用10种回收铀（RU）和贫铀（DU）成分情形,根据等效天然铀（NUE）燃料混合比计算程序ALPHA算得配成NUE燃料的混合比。以标准CANDU 6栅元结构为载体,采用WIMS程序,通过比较NUE燃料与天然铀（NU）燃料的中子学性能参数,以及NUE燃料入堆示范验证试验中实际入堆的燃料信息,对NUE燃料与NU燃料的中子学性能等效性进行了论证分析。研究表明,与NU燃料相比,各种情形下NUE燃料在无限增殖系数、卸料燃耗、冷却剂空泡反应性以及燃料温度效应等中子学性能参数上吻合较好,NUE燃料与NU燃料具备较好的中子学等效性,可应用于重水堆核电站,实现回收铀的有效利用。     

CANDU堆先进燃料循环的展望

介绍ＣＡＮＤＵ堆的天然铀燃料循环以及最近开发的适合未来近期的先进燃料循环。高中子经济性,不停堆换料以及简单的燃料束设计,使得ＣＡＮＤＵ堆具有非常优良的燃料循环灵活性和多样性。     

Coupled neutronics/thermal hydraulics evaluation for thorium based fuels in thermal spectrum SCWR

Thorium can supplement the current limited reserves of uranium. In current study, analyses are performed for thorium based fuels in thermal neutron spectrum Super Critical Water Reactor (SCWR). Thorium based fuels are studied in two roles. First role being replacement of conventional uranium dioxide fuel while the other being burner of Reactor Grade Plutonium (RG-Pu) in thermal neutron spectrum SCWR. Coupled neutron physics/thermal hydraulics analyses are performed due to large density variation of coolant over the active fuel length. Analyses reveal that thorium-uranium MOX fuels lead to smaller burnup values as compared to equivalent enriched uranium dioxide but possess the advantage of smaller excess reactivity at Beginning of Life (BOL). This can lead to savings in the form of Burnable Poisons (BP). Smaller fuel average temperature values are obtained for thorium-uranium MOX fuels as compared to uranium dioxide fuel option. Coated fuel option utilizing mixed thorium-uranium mono nitride fuel can help further decrease fuel average temperature values for thorium based fuels. U-233, produced in thorium uranium fuels, contribution towards fission energy produced is smaller as compared to plutonium produced in conventional uranium dioxide fuel. In terms of proliferation resistance, approximately 40% less quantity of plutonium is produced for thorium-uranium MOX fuels (for studied compositions) as compared to equivalent enriched uranium dioxide fuel. But, there is not much difference between the discharged plutonium vector compositions. Thorium–Plutonium based fuels lead to significantly harder spectrum which results in larger spread in radial power density and eventually causes larger values for thermal hydraulic parameters like fuel and clad temperature. Due to almost no production of plutonium, thorium based fuels can be a very good option to burn RG-Pu in thermal spectrum SCWR. Thorium based fuels destroyed almost 74% initially loaded RG-Pu as compared to 60% for uranium based MOX. HEU based thorium fuels can be a very good option for replacing conventional uranium dioxide fuels as very small quantities of plutonium is produced. This option, although, has regulatory issues due to use of HEU material.     

Accuracy of nuclear design of fast and thermal neutron coupled core by SRAC

Supercritical-pressure light water cooled fast reactor adopts the blanket fuel assemblies with depleted uranium fuel and zirconium hydride layer in the core for negative coolant void reactivity. Thermal neutrons are generated in the core of fast reactor. It is called “fast and thermal neutron coupled core”. The purpose of the present study is to examine the accuracy of assembly and core calculations including preparation of the macroscopic cross sections with the SRAC code system for “fast and thermal neutron coupled core” in comparison with the Monte Carlo codes, MVP and MVP-BURN. Accuracy of the neutron multiplication factor and coolant void reactivity calculation has been evaluated in four types of cores of different fractions of the blanket fuel assembly with zirconium hydride rods. The conventional analysis is based on the macroscopic cross sections which are prepared with infinite lattice. The conventional SRAC calculation underestimates the neuron multiplication factor for all types of cores. Other findings are that the conventional SRAC calculation overestimates coolant void reactivity for the cores without zirconium hydride rods, and underestimates coolant void reactivity for the core of all blanket fuel assemblies having zirconium hydride rods. To overcome these problems, it has been proposed that the macroscopic cross sections of seed fuel assembly are prepared with the model that a seed fuel assembly is surrounded by blanket fuel assemblies in order to take into account the effects of the surrounding fuel assemblies. Evaluations show that accuracy of the neutron multiplication factor by the SRAC calculation can be improved by the proposed method.     

Pu-breeding feasibility in PWR

This study addresses the issue of alternative pathways for breeding plutonium in a 900 MWe three loop thermal pressurized water reactor (PWR), either fueled with uranium fuel (3.5% U-235) or with mixed fuel (20% MOX). During the operation of a nuclear reactor the in-core neutron flux and the ex-core neutron flux are monitored with flux detectors. At the places where those detectors operate, the guide thimbles and the vessel wall, respectively, the neutron flux can be used to irradiate material samples. This paper investigates whether it would be possible to produce plutonium by breeding it at the walls of a PWR vessel and/or in the guide thimbles. The neutron flux in the reactor and the corresponding multi-group spectra are estimated with Monte Carlo simulations for different positions at the vessel wall of a PWR operating with either UO₂ or MOX. Then the irradiation of fresh uranium samples at the vessel wall and in the guide thimbles are calculated and the isotopic composition of the irradiated samples are determined. The minimum irradiation period and the necessary minimum amount of fresh uranium to breed different grades of plutonium are derived.     

Calculation of the void reactivity of CANDU lattices using the code system

The reactivity effect of coolant voiding in CANDU-type fuel lattices has been calculated with different methods using the code system. The known positive void reactivity coefficient of the original lattice was correctly obtained. A modified fuel bundle containing dysprosium and slightly enriched uranium to eliminate the positive reactivity effect was also calculated. Owing to the increased heterogeneity of this modified fuel the one-dimensional cylindrical calculation with XSDRN proved to be inadequate. Code options allowing bundle geometry were successfully used for the calculation of the strongly space dependent flux and spectrum changes which determine the void reactivity.     

A 3D stylized half-core CANDU benchmark problem

A 3D stylized half-core Canadian deuterium uranium (CANDU) reactor benchmark problem is presented. The benchmark problem is comprised of a heterogeneous lattice of 37-element natural uranium fuel bundles, heavy water moderated, heavy water cooled, with adjuster rods included as reactivity control devices. Furthermore, a 2-group macroscopic cross section library has been developed for the problem to increase the utility of this benchmark for full-core deterministic transport methods development. Monte Carlo results are presented for the benchmark problem in cooled, checkerboard void, and full coolant void configurations.     

Conceptual Design Study of 180 MWt Small-Sized Reduced-Moderation Water Reactor Core

Conceptual design of a Small-sized Reduced-Moderation Water Reactor (S-RMWR) core, which has the thermal output of 180 MW, the conversion ratio of 1.0 and the void reactivity coefficient of negative value, has been constructed. S-RMWR is a technology demonstration reactor which also conducts material and fuel testing for commercial use of Reduced-Moderation Water Reactor (RMWR) in large-scale power plants. It has a very tight triangular fuel rod lattice and a high coolant void fraction. The RMWR core axially has two short and flat uranium plutonium mixed oxide (MOX) regions with an internal blanket region in between, in order to avoid a positive void reactivity coefficient. The MOX regions are sandwiched between upper and lower blanket regions, in order to increase a conversion ratio.

In this small reactor core, leakage of neutrons is expected to be larger than in a large core. Therefore, a core design concept different from that for a large core is necessary. Core burnup calculations and nuclear and thermal-hydraulic coupled calculations were performed in the present study with SRAC and MOSRA codes. MVP code was also used to obtain control rod worth. Because of its large neutron leakage, keeping the void reactivity coefficient negative is easier for S-RMWR than RMWR. Thus, the heights of MOX region can be taller and the plutonium enrichment can be lower than in RMWR. On the other hand, to achieve the conversion ratio of 1.0, radial blanket and stainless steel reflector assemblies are necessary, whereas they are not needed for RMWR.     

改进Flower型超临界水冷快堆初步增殖研究

超临界水冷快堆集快堆和轻水堆两种特性。整个堆芯冷却剂流量仅为现BWR的1/8,中子能谱硬于普通PWR,故有一定的核燃料增殖能力。本文建立不同Flower型超临界水冷快堆堆芯物理模型,研究堆芯分区布置、冷却剂密度分层、seed及blanket组件P/D值设计、MOX燃料设计、燃料富集度分区分层布置、blanket内部通道采用贫铀冷却等方案,分析堆芯的空泡反应性、功率分布及增殖比。通过比较,得到了超临界水冷快堆的优化设计方案。     

在重水堆中用贫铀作为核燃料的应用研究

对以贫铀和钚组成ＭＯＸ核燃料替代ＣＡＮＤＵ堆中的天然铀的可能性进行了探讨、从而开一用于核能的途径。经过初步验算,得出了用＾２３５Ｕ含量为０．２５％的贫化铀浓缩残渣和钚组成ＭＯＸ核燃料可以替代ＣＡＮＤＵ堆中的天然铀来维持重水堆中的链式反就,达到核能利用的的目的。并展望了贫铀应用的前景。     

Verification of a Nuclear Analysis System for Fast Reactors using BFS-62 Critical Experiment

Critical experiments have been analyzed to verify a nuclear analysis system for fast reactors used in Japan Nuclear Cycle Development Institute (JNC). The experiments were performed in a collaboration work between JNC and the Institute of Physics and Power Engineering of Russia to dispose Russian surplus weapons plutonium, focusing on the effect of the introduction of uranium-plutonium mixed-dioxide (MOX) fuel and stainless steel reflector into the current BN-600 core that is comprised of UO₂ fuel and blanket.

The analysis results agreed well with measured values on most of the nuclear characteristics. The accuracies are comparable to those obtained for the conventional MOX fueled fast reactors. It suggests that the JNC analysis system can analyze accurately nuclear characteristics in uranium fueled cores as well.

A significant improvement was achieved on the sodium void reactivity by employing an ultra fine group cell calculation system. A change in adjoint neutron spectrum mostly contributes to the improvement.

A discrepancy of more than 20% was found on the fission rate distribution of ²³⁵U or ²³⁹Pu in stainless steel reflector regions, which cannot be solved by introducing continuous Monte Carlo calculation or different nuclear data sets.     

Analysis of fuel temperature effects on reactivity of light water reactor fuel assemblies by using MVP-2 adopting an exact resonance elastic scattering model

Using the continuous-energy Monte Carlo code MVP-2 adopting a resonance elastic scattering model considering the thermal motion of a target nucleus (the exact model) for major heavy nuclides, analysis of fuel temperature effects on reactivity of mockup UO₂ and MOX fuel assemblies for light water reactors was performed, and the results were compared with those of the conventional asymptotic model. A base condition was a hot operating condition with an in-channel void fraction of 40% and fuel temperature of 520 ℃ for the BWR fuel assemblies and a hot zero-power condition with fuel temperature of 284 ℃ for the PWR fuel assemblies. The fuel temperature of a high-temperature condition was 1500 ℃ for both types of assemblies. The calculated results showed that the exact model made the neutron multiplication factors at the high-temperature condition lower by ?220 to ?440 pcm (10^?5 Δk) and the Doppler reactivity between the base- and high-temperature conditions more negative by 7% to 10% compared with those obtained by the asymptotic model. The energy-dependent reaction rates of capture and ν-fission were also analyzed to study the detail mechanism in the effect of the exact model on the assembly reactivity.     

Hafnium clad fuels for fast spectrum BWRs

We show that by use of hafnium cladding, a fast neutron spectrum is achievable in the top of uprated BWRs. Monte Carlo calculations have been made for Hf clad inert matrix nitride and low fertile MOX fuels, with fuel segments located in the upper part of an uprated BWR, where the coolant void fraction exceeds 70%. The nitride fuel results in the hardest neutron spectrum, but the low fertile MOX fuel still yields fission probabilities for even neutron number nuclides similar to those of sodium cooled reactors. The inert matrix nitride fuel configuration yields high burning rates, permitting to stabilise TRU inventories with less than 50% BWR cores of the here suggested type in the power park. The core with low fertile MOX fuel is less efficient, but still a zero net producer of TRU. Fuel and coolant temperature feedbacks are affected by introduction of absorbing elements in the fuel, but remain within acceptable ranges for the low fertile MOX fuel. Although control rod worths are reduced, shutdown margins are sufficient to ensure sub-criticality in cold conditions. From a materials point of view, the behaviour of hafnium clad MOX fuel would be similar to zircalloy clad MOX fuel already used extensively in nuclear industry. Thus, if dynamic stability of the core can be ensured, the here proposed fuel may be considered as a low cost solution for transmutation of minor actinides on industrial scale.     

Improvement of power coefficient by using burnable poison in the CANDU reactor

For stable operation of a power reactor, the power coefficient (PC) of the nuclear reactor should be less than or equal to zero. In the CANDU reactor loaded with the recovered uranium (RU) which has a uranium enrichment of ∼0.9 wt% U²³⁵, the PC is estimated to be clearly positive over a wide power range of interest, owing to the generic positive coolant temperature coefficient (CTC) and weak fuel temperature coefficient (FTC) in the CANDU reactor. In order to improve the PC of the CANDU reactor without seriously compromising the economy, introduction of the burnable poison (BP) has been proposed in this work and a physics study has been performed to find the optimal BP material and its optimal loading scheme for the CANDU reactor loaded with the CANFLEX-RU fuel. Four potential BPs (Dy, Er, Eu, and Hf) were evaluated to find the optimal BP and various loading options of the selected BP were evaluated to determine the optimal loading scheme of the BP. From the viewpoint of the achievable fuel discharge burnup, it was found that Er is evaluated to be the best BP and the BP should be loaded within the central two fuel rings because the BP loading on the inner ring is more effective for reducing the CTC. The discharge burnup of the Er-loaded CANFLEX-RU fuel was 38% higher than that of the standard natural uranium (NU) fuel. The fuel discharge burnup can be increased further if the fuel enrichment is increased. It is shown that the discharge burnup of 1.0 wt%-enriched uranium fuel is 1.7 times higher than that of the NU fuel. This study has shown that the use of the BP is feasible to render the PC of the CANDU reactor negative, even though the slight reduction of the fuel burnup is inevitable, and thus the reactor safety can be greatly improved by the use of the BP in the CANDU reactor.     

Utilization of spent PWR fuel-advanced nuclear fuel cycle of PWR／CANDU synergism

High neutron economy, on line refueling and channel design result in the unsurpassed fuel cycle flexi-bility and variety for CANDU reactors. According to the Chinese national conditions that China has both PWR and CANDU reactors and the closed cycle policy of reprocessing the spent PWR fuel is adopted, one of the advanced nu-clear fuel cycles of PWR/CANDU synergism using the reprocessed uranium of spent PWR fuel in CANDU reactor is proposed, which will save the uranium resource (-22.5%), increase the energy output (-41%), decrease the quantity of spent fuels to be disposed (-2/3) and lower the cost of nuclear poower, Because of the inherent flexibility of nuclearfuel cycle in CANDU reactor, and the low radiation level of recycled uranium(RU), which is acceptable for CANDU reactor fuel fabrication, the transition from the natural uranium to the RU can be completed without major modifica-tion of the reactor core structure and operation mode.It can be implemented in Qinshan Phase Ⅲ CANDU reactors with little or no requirement of big investment in new design. It can be expected that the reuse of recycled uranium of spent PWR fuel in CANDU reactor is a feasible and desirable strategy in China.     

Lattice Parameter Measurements on Cluster-Type Fuel for Advanced Thermal Reactor

Abstract

The behavior of neutrons in a highly heterogeneous unit cell consisting of D₂O moderator, H₂O coolant and a 28-pin fuel cluster contained in a pressure tube has been studied through lattice parameter measurements covering three different ²³⁵U enrichments, four coolant void fractions and two lattice pitches. A single-region core configuration was adopted, with which measurements were made to determine—in relation to coolant void fraction—the critical D₂O level, as well as various lattice parameters

A strong dependence on coolant void was observed for the critical level and the lattice parameters, in the case of the smaller 22.5 cm pitch lattice, due to the positive effect on core reactivity exerted by the slowing-down faculty of H₂O in the epithermal energy region. With the larger 25.0 cm pitch, however, no meaningful dependence on void fraction was shown by any of the measured values, and this was ascribed to a compensating negative effect due to enhanced thermal neutron self-shielding in the fuel region produced by the H₂O coolant.

The results of cell calculations obtained by means of the METHUSELAH-II code showed generally good agreement with experimentally determined data, for both critical D₂O levels and lattice parameters, in the case of coolant-filled lattices (0, 30 and 70% void fractions). For lattices devoid of coolant (100% void fraction), however, discrepancies in lattice parameters—particularly in p ²⁸—produced corresponding deviations in core reactivity amounting to 1% in excess of those incurred with other void fractions.     

Neutronics and material attractiveness for PWR thorium systems using monte carlo techniques

Thorium (Th) oxide fuel offers a significant advantage over traditional low-enriched uranium and mixed uranium/plutonium oxide (MOX) fuel irradiated in a Light Water Reactor. The benefits of using thorium include the following: 1) unlike depleted uranium, thorium does not produce plutonium, 2) thorium is a more stable fuel material chemically than LEU and may withstand higher burnups, 3) the materials attractiveness of plutonium in Th/Pu fuel at high burnups is lower than in MOX at currently achievable burnups, and 4) thorium is three to four times more abundant than uranium. This paper quantifies the irradiation of thorium fuel in existing Light Water Reactors in terms of: 1) the percentage of plutonium destroyed, 2) reactivity safety parameters, and 3) material attractiveness of the final uranium and plutonium products. The Monte Carlo codes MCNP/X and the linkage code Monteburns were used for the calculations in this document, which is one of the first applications of full core Monte Carlo burnup calculations. Results of reactivity safety parameters are compared to deterministic solutions that are more traditionally used for full core computations.Thorium is fertile and leads to production of the fissile isotope ²³³U, but it must be mixed with enriched uranium or reactor-/weapons-grade plutonium initially to provide power until enough ²³³U builds in. One proposed fuel type, a thorium-plutonium mixture, is advantageous because it would destroy a significant fraction of existing plutonium while avoiding the creation of new plutonium. ²³³U has a lower delayed neutron fraction than ²³⁵U and acts kinetically similar to ²³⁹Pu built in from ²³⁸U. However, as with MOX fuel, some design changes may be required for our current LWR fleet to burn more than one-third a core of Th/Pu fuel and satisfy reactivity safety limits. The calculations performed in this research show that thorium/plutonium fuel can destroy up to 70% of the original plutonium per pass at 47 GWd/MTU, whereas only about 30% can be destroyed using MOX. Additionally, the materials attractiveness of the final plutonium product of irradiated plutonium/thorium fuel is significantly reduced if high burnups (∼94 GWD/MTU) of the fuel can be attained.