聚变堆交叉冷却固态包层中子学设计优化

针对聚变堆固态包层设计路线,提出了一个交叉排列氦冷固态包层概念。设计采用Be、Li₂TiO₃分层球床。两种尺寸的氦气冷却管道交叉排列,分两个回路同时冷却,以增加系统安全可靠性。分析比较了4种⁶Li富集度布置方案。结果表明：径向远离第一壁降低⁶Li富集度较为合理,靠近第一壁的增殖层⁶Li富集度不能过低,以减少长期运行中Li的消耗对氚增殖性能的影响。借助蒙特卡罗程序MCNP建立11.25°对称模型,全堆包层氚增殖率为1.176,包层寿期内产氚性能稳定,在包层寿命运行时间内的燃耗分布相对均匀。     

氚增殖剂Li4SiO4 陶瓷小球的制备工艺

欧洲和中国聚变堆固态产氚包层（TBM）的氚增殖剂倾向于采用直径0.5～2mm的Li₄SiO₄陶瓷小球填充床。本工作探讨锂陶瓷小球的性能指标设计,研究挤压-滚圆、烧结法制备Li₄SiO₄小球的工艺可行性,测试分析小球的密度、直径、球形度、晶粒尺寸、压碎载荷等性能。研究表明：挤压-滚圆成型、1050℃无压烧结的Li₄SiO₄陶瓷小球密度为90.4%TD,堆积密度为52.9%TD;平均直径为0.95mm,标准偏差为0.15mm;球形度为1.10;平均压碎载荷为18.50N,标准偏差为2.76N;平均晶粒尺寸为14μm;相结构由Li₄SiO₄主晶相、少量Li₂SiO₃和Li₂Si₂O₅等组成。采用优化的挤压 滚圆、烧结工艺可制备出合格的Li₄SiO₄陶瓷小球产品。     

聚变堆氦冷固态包层结构和6Li富集度对产氚率的影响

在聚变堆固态包层基本参数基础上，建立简化20°模型，包层分第1壁装甲、第1壁冷却板、氚增殖区和支撑结构。分别选择Li₄SiO₄和Li₂O做增殖材料，应用MCNP程序，研究第1壁结构布置和6Li富集度对产氚率的影响。结果表明：₆Li富集度适宜选择在30％~80％之间；第1壁选择Be装甲可提高产氚率；冷却管板的厚度应取3cm以下，以避免对产氚造成不利的影响。     

中国氦冷固态实验包层2×6模块中子学计算分析

为了满足ITER对波纹度的要求,核工业西南物理研究院提出了新的减少低活化铁素体钢的氦冷固态（HCSB）实验包层模块（TBM）设计方案。采用MCNP程序及ITER全堆MCNP模型,对新设计的2×6HCSB-TBM进行三维中子学计算分析,给出了模块产氚率、核热沉积和功率密度分布等结果。在ITER运行因子为22%时,HCSB-TBM的产氚率为12.68mg/d。TBM内总核热沉积为522.5kW,最高功率密度为11.8W/cm³,出现在氚增殖区Li₄SiO₄中。计算结果可为TBM进一步的结构、热工水力学优化及其他系统设计提供中子学数据。     

超临界水冷固态实验包层中子学与热工水力特性研究

基于国际热核聚变实验堆(ITER)实验包层方案,提出了一个超临界水冷固态实验包层概念设计方案。设计采用Be作为中子倍增剂,Li4SiO4作为氚增殖剂,CLAM钢作为结构材料。包层第一壁采用多层盘道设计以提高第一壁出口温度,内部采用增殖剂与中子倍增剂分层布置以提高热沉积与氚增殖率。为验证包层设计的可行性,分析计算了三维包层氚增殖率与热沉积的分布,然后根据中子学计算得到的结果对超临界水冷固态实验包层进行了数值模拟研究。结果表明:包层功率密度分布较合理;氚增殖率满足运行中氚自持的要求;在冷却剂出口温度达到500℃条件下材料温度不超过限值。该设计方案能满足中子学设计与热工水力的要求。     

随机填充球床通道内氦气流动特性实验研究

在聚变堆氦冷固态包层氚增殖区,球床通道内氦气流动压降特性对泵功率的设计具有重要意义。以氦冷固态包层氚增殖区为背景,研究了氦气流速、球床颗粒直径及球床通道长度对球床通道内氦气流动压降特性的影响。实验段采用20 mm×20 mm×500 mm的矩形通道,实验中氦气流速为0.1～0.6 m/s,球床颗粒直径为0.5、0.8、1.0、1.5、2.0 mm。实验结果表明,压降与氦气流速以及球床通道长度呈正相关,与球床颗粒直径呈负相关。对比Ergun关系式发现,在球床颗粒直径较小时,Ergun关系式预测值低于实验值,这主要是由于氦气可压缩性的影响。通过动量方程,理论推导出经可压缩性修正的Ergun关系式,结果发现修正后的Ergun关系式预测值与实验值符合良好。本研究为氦冷固态包层氚增殖区设计提供了数据支撑,为球床通道内流动特性的数值模拟提供了验证手段。     

高氚增殖比包层的设计及热工水力分析

本文设计了一种高氚增殖比包层(HBRB),该包层采用多孔U-10Zr合金作为中子倍增剂,Li4SiO4球床作为增殖剂,低活化马氏体(RAFM)钢作为结构材料。在详细研究包层加工工艺、流量分配、中子性能等问题的基础上,完成了包层内部详细结构设计。利用中子学软件分析计算了包层的氚增殖比(TBR)和热沉积分布,并根据计算结果对包层进行热力耦合分析。结果表明:包层TBR较高,且核性能稳定;冷却剂的流量分配情况和压降合理;包层内各组件冷却充分,温度和结构材料热应力不超过限值。     

MnO2/碳气凝胶粉末复合电极材料制备与性能研究

以间苯二酚(R)和甲醛为原料，碳酸钠（C）为催化剂，制备了碳气凝胶粉末（CRF），并以KBrO₃和MnSO₄•H₂O为原料，采用水热法制备了MnO₂/CRF复合材料。采用N₂吸附、X射线衍射技术对所制备的复合材料进行了表征。结果表明，水热法制备的MnO₂材料为纯的软锰矿相，且碳气凝胶粉的加入并未影响MnO₂的晶体结构。在1mol/LKOH电解液中进行的循环伏安和计时电位扫描测试表明，电极材料电化学性能稳定，具有较好的可逆性；在1mA电流密度下进行充放电测试时，电极比电容为146.6F/g；再循环500次后，电极仍能保持稳定的电容，显示出该电极材料是一理想的电化学电极材料。     

堆内辐照氚增殖剂球床有效热导率分析

氘-氚聚变反应堆中,固态氚增殖剂包层能不断为聚变反应提供氚核素,是实现聚变反应堆商用的关键技术之一。由锂陶瓷小球堆积形成的球床形式的固态氚增殖剂包层具有比表面积大、产氚效率高等优点,是我国重点发展的氚增殖剂包层形式。氚增殖剂球床须能支撑在堆内辐照时的高温环境,这就要求氚增殖剂球床有较好的导热特性。球床的有效热导率在球床设计和辐照过程中的安全分析十分重要,因此在中国先进研究堆（CARR）开展了氚增殖剂球床在堆内辐照环境下的有效热导率测量实验。根据MCNP计算得出的球床发热功率,结合实验测量的球床温度分布反推得到氚增殖剂球床的有效热导率,并与广泛应用于球床有效热导率计算的改进型ZBS模型计算结果以及堆外实验结果进行对比分析,理论值与实验值能较好吻合。     

堆内辐照氚增殖剂球床有效热导率分析

氘-氚聚变反应堆中,固态氚增殖剂包层能不断为聚变反应提供氚核素,是实现聚变反应堆商用的关键技术之一。由锂陶瓷小球堆积形成的球床形式的固态氚增殖剂包层具有比表面积大、产氚效率高等优点,是我国重点发展的氚增殖剂包层形式。氚增殖剂球床须能支撑在堆内辐照时的高温环境,这就要求氚增殖剂球床有较好的导热特性。球床的有效热导率在球床设计和辐照过程中的安全分析十分重要,因此在中国先进研究堆(CARR)开展了氚增殖剂球床在堆内辐照环境下的有效热导率测量实验。根据MCNP计算得出的球床发热功率,结合实验测量的球床温度分布反推得到氚增殖剂球床的有效热导率,并与广泛应用于球床有效热导率计算的改进型ZBS模型计算结果以及堆外实验结果进行对比分析,理论值与实验值能较好吻合。     

硅酸锂球床传热传质特性与吹扫气体流动的DEM-CFD耦合模拟

氦冷固态增殖包层是中国聚变工程实验堆（CFETR）的3种候选包层概念之一,氚增殖球床是包层的核心部件,采用硅酸锂颗粒作为氚增殖材料。球床结构对氚在球床内的输运行为及流动和传热均有重要影响。本文基于离散单元法（DEM）生成了满足氚增殖球床填充率要求的随机堆积结构,通过CFD计算获取了球床结构下氚在吹扫气体内的等效扩散系数及吹扫气体的流动特性,包括速度分布、压力分布及进出口压降;开展了外加热流及有内热源两种工况下球床等效导热系数的模拟。计算结果表明,球床结构下氚在吹扫气体内的等效扩散系数为二元气体扩散系数的40%;受球床结构影响,球床内存在流动迟滞区,壁面出现流动加速;拟合得到Ergun方程的黏性阻力系数C1=87;有内热源工况下的球床等效导热系数低于外加热流工况下的球床等效导热系数。     

Status and progress of Indian LLCB test blanket systems for ITER

The lead–lithium ceramic breeder (LLCB) TBM and its auxiliary systems are being developed by India for testing in ITER machine. The LLCB TBM consists of lithium titanate as ceramic breeder (CB) material in the form of packed pebble beds. The FW structural material is ferritic martensitic steel cooled by high-pressure helium gas and lead–lithium eutectic (Pb–Li) flowing separately around the ceramic breeder pebble bed to extract the nuclear heat from the CB zones. Low-pressure helium is purged inside the CB zone for in situ extraction of bred tritium. Currently the LLCB blanket design optimization is under progress. The performance of tritium breeding and high-grade heat extraction is being evaluated by neutronic analysis and thermal–hydraulic calculations for different LLCB cooling configurations and geometrical design variants. The LLCB TBM auxiliary systems such as, helium cooling system (HCS), lead–lithium cooling system (LLCS), tritium extraction system (TES) process design are under progress. Safety analysis of the LLCB test blanket system (TBS) is under progress for the contribution to preliminary safety report of ITER-TBMs. This paper will present the status of the LLCB TBM design, process integration design (PID) of the auxiliary systems and preliminary safety analysis results.     

Experimental measurement of effective thermal conductivity of packed lithium-titanate pebble bed

Lithium titanate is a promising solid breeder material for the fusion reactor blanket. Packed lithium titanate pebble bed is considered for the blanket. The thermal energy; that will be produced in the bed during breeding and the radiated heat from the reactor core absorbed must be removed. So, the experimental thermal property data are important for the blanket design. In past, a significant amount of works were conducted to determine the effective thermal conductivity of packed solid breeder pebble bed, in helium atmosphere, but no flow of gas was considered. With increase in gas flow rate, effective thermal conductivity of pebble bed increases. Particle size and void fraction also affect the thermal properties of the bed significantly. An experimental facility with external heat source was designed and installed. Experiments were carried out with lithium-titanate pebbles of different sizes at variable gas flow rates and at different bed wall temperature. It was observed that effective thermal conductivity of pebble bed is a function of particle Reynolds number and temperature. From the experimental data two correlations have been developed to estimate the effective thermal conductivity of packed lithium-titanate pebble bed for different particle Reynolds number and at different temperatures. The experimental details and results are discussed in this paper.     

球床包层聚变—裂变混合堆热工安全分析

球床包层混合堆与板状元件包层混合堆相比较，前者在核燃料生产和安全方面可能具有更多的优越性。本应用ＴＨＥＲＭＩＸ程序和辅助程序对我国开发的托卡马克堆芯氮气冷却球床包层聚变－裂变合堆的包层进行了热工计算。计算中考虑了不同的燃料球材料及稳态，卸压和断流事故工况。计算结果表明，只要选用合适的燃料球材料和设置适当的控制保护系统，具有快速卸料罐的托卡马克堆芯氦气包层聚变－裂变混合堆的概念设计在安全上的可行的。     

氚增殖剂球床组件堆内辐照物理热工计算分析

为验证在中国先进研究堆(CARR)内进行国际热核聚变实验堆(ITER)氚增殖包层模块(TBM)辐照实验的可行性和安全性,进行了氚增殖剂球床组件堆内辐照物理及热工计算分析。氚增殖剂包层模块主要是固态氚增殖剂陶瓷球床。本文采用Monte Carlo粒子输运模拟程序对氚增殖剂球床进行堆内建模,计算球床的中子注量率、能量沉积和产额,得到不同功率下球床的中子注量率、发热功率和产氚速率以及球床组件引入反应堆的反应性。根据物理计算得到的组件各部件发热情况建立热工计算一维模型,通过更改反应堆功率得到满足实验要求的工况并采用三维程序进行验证。物理与热工计算分析的结果表明,在反应堆运行功率为20 MW的工况下球床组件各部件的温度均不超过限值。     

Investigation of the packing structure of pebble beds by DEM for CFETR WCCB

Li₂TiO₃/Be₁₂Ti mixed pebble beds with multi-sized particles are one of the potential candidates for the WCCB (water-cooled ceramic breeder blanket) of the CFETR (China Fusion Engineering Test Reactor). To meet the neutronics requirements of a WCCB, a study of the packing structure of the concerned pebble bed is necessary. In this paper, the discrete element method (DEM) is applied to produce a prototypical blanket pebble bed by directly simulating the contact state of each individual particle using basic interaction laws. According to the current simulation, the packing factor of a mono-sized pebble bed is 0.62–0.64, while the value will become more than 0.75 for Li₂TiO₃/Be₁₂Ti mixed breeding pebble bed with a diameter ratio of not less than 5 as well as an appropriate mixed volume ratio, and thus can meet the neutronics requirements.     

Requirements for helium cooled pebble bed blanket and R&D activities

This work aims to give an outline of the design requirements of the helium cooled pebble bed (HCPB) blanket and its associated R&D activities. In DEMO fusion reactor the plasma facing components have to fulfill several requirements dictated by safety and process sustainability criteria. In particular the blanket of a fusion reactor shall transfer the heat load coming from the plasma to the cooling system and also provide tritium breeding for the fuel cycle of the machine. KIT has been investigating and developed a helium-cooled blanket for more than three decades: the concept is based on the adoption of separated small lithium orthosilicate (tritium breeder) and beryllium (neutron multiplier) pebble beds, i.e. the HCPB blanket. One of the test blanket modules of ITER will be a HCPB type, aiming to demonstrate the soundness of the concept for the exploitation in future fusion power plants. A discussion is reported also on the development of the design criteria for the blanket to meet the requirements, such as tritium environmental release, also with reference to the TBM.The selection of materials and components to be used in a unique environment as the Tokamak of a fusion reactor requires dedicated several R&D activities. For instance, the performance of the coolant and the tritium self-sufficiency are key elements for the realization of the HCPB concept. Experimental campaigns have been conducted to select the materials to be used inside the solid breeder blanket and R&D activities have been carried out to support the design. The paper discusses also the program of future developments for the realization of the HCPB concept, also focusing to the specific campaigns necessary to qualify the TBM for its implementation in the ITER machine.     

A Measurement Platform Scheme and Data Post-processing Method for Thermal Conductivity of Li<Subscript>4</Subscript>SiO<Subscript>4</Subscript> Pebble Bed

The effective thermal conductivity of tritium breeder pebble bed is an important thermal parameter and must be known for the thermo-mechanical design of solid tritium breeder blankets. In order to obtain the parameter, experimental measurement is an effective method. A measurement platform was designed by University of Science and Technology of China for CFETR solid blanket scheme to measure the immediate thermal conductivity data and study the effect of pebble bed temperature, the purge gas pressure and pebble deformation on the thermal conductivity of pebble bed. Measurements were performed based on about 1 mm diameter Li₄SiO₄ pebbles in the temperature range between 100 and 800 °C, with purge gas pressure ranging from 0.1 to 0.3 MPa. This paper described a measurement platform scheme by thermal probe method. On the other hand, for the sake of increasing the precision of thermal conductivity data transformed from temperature data, some improvements for the data post-processing using Monte Carlo inversion method were made in this paper too.