Radon concentration measurements in bituminous coal mines

Radon measurements were carried out in Kozlu, Karadon and Uzülmez underground coal mines of Zonguldak bituminous coal basin in Turkey. Passive-time integrating method, which is the most widely used technique for the measurement of radon concentration in air, was applied by using nuclear etched track detectors (CR-39) in the study area. The radon concentration measurements were performed on a total of 42 points in those three mines. The annual exposure, the annual effective dose and lifetime fatality risk, which are the important parameters for the health of workers, were estimated based on chronic occupational exposure to the radon gas, which is calculated using UNCEAR-2000 and ICRP-65 models. The radon concentrations at several coal production faces are higher than the action level of 1000 Bq m(-3). It is suggested that the ventilation rates should be rearranged to reduce the radon concentration.     

Radon progeny in Egyptian underground phosphate mines

In addition to the workers in uranium mines, the staff of other underground mines, such as workers in underground phosphate mines, can be exposed to 222Rn and its progeny. In this study the individual radon progeny concentrations were measured in three Egyptian underground phosphate mines to estimate the occupational exposure of the workers at those sites. A filter method was used to measure individual radon progeny concentrations (218Po, 214Pb and 214Po). The reported mean values of radon progeny concentrations exceed the action levels which are recommended by ICRP 65 (1993). Based on the measured individual radon progeny concentrations (218Po, 214Pb and 214Po) in these mines, the annual effective dose for the workers has been calculated using the lung dose model of ICRP 66 (1994). According to the obtained results, some countermeasures were recommended in this study to minimise these exposure levels.     

Radon dose calculation methodology for underground workers in the Czech Republic

The project focused on classifying the level of irradiation from natural ionising radiation sources for workers in publicly accessible caves and in caves used for speleotherapy, with applicability to other underground workplace. A correct and accurate procedure (and calculation) is defined for determining the effective dose that workers are exposed to in caves, based on the results of integral measurements of radon volume activity and on the length of time spent by workers in the caves. A review was made of various approaches for evaluating lung irradiation found in the literature. Experimental measurements of cave atmosphere characteristics (continuous measurement of radon volume activity, continuous and integral measurements of radon decay products, interior climatic parameters and aerosol spectra) were the main sources for the methodology.     

Characterisation of an electronic radon gas personal dosemeter

The monitoring of radon exposure at workplaces is of great importance. Up to now passive measurement systems have been used for the registration of radon gas. Recently an electronic radon gas personal dosemeter came onto the market as an active measurement system for the registration of radon exposure (DOSEman; Sarad GmbH, Dresden, Germany). In this personal monitor, the radon gas diffuses through a membrane into a measurement chamber. A silicon detector system records spectroscopically the alpha decays of the radon gas and of the short-lived progeny 218Po and 214Po gathered onto the detector by an electrical field. In this work the calibration was tested and a proficiency test of this equipment was made. The diffusion behaviour of the radon gas into the measurement chamber, susceptibility to thoron, efficiency, influence of humidity, accuracy and the detection limit were checked.     

Real-time measurement of individual occupational radon exposures in tombs of the Valley of the Kings, Egypt

The active radon exposure meter developed recently at the German Research Center for Environmental Health (Helmholtz Zentrum München) was used to measure radon concentrations in 12 tombs located in the Valley of the Kings, Egypt. Radon concentrations in air between 50 ± 7 and 12 100 ± 600 Bq m(-3) were obtained. The device was also used to measure individual radon exposures of those persons working as safeguards inside the tombs. For a measurement time of 2-3 d, typical individual radon exposures ranged from 1800 ± 400 to 240 000 ± 13 000 Bq h m(-3), depending on the duration of measurement and radon concentration in the different tombs. Based on current ICRP dose conversion conventions for workers and on equilibrium factors published in the literature for these tombs, individual effective dose rates that range from 1.5 ± 0.3 to 860 ± 50 μSv d(-1) were estimated. If it is assumed that the climatic conditions present at the measurement campaign persist for about half a year, in this area, then effective doses up to ～ 66 mSv could be estimated for half a year, for some of the safeguards of tombs where F-values were known. To reduce the exposure of the safeguards, some recommendations are proposed.     

Thoron and decay products, beyond UNSCEAR 2006 Annex E

Uranium and thorium series radionuclides are present in all soils and rocks. Thus, radon and thoron, the radioactive noble gases originating in the uranium ((238)U) and thorium ((232)Th) decay chains is ubiquitous and everyone is exposed to both radon and thoron gases and their particulate radioactive decay products. As described in UNSCEAR Annex E (2006), radon and its decay products have been recognised for many years as a hazard to underground miners. More recently, the risks from exposure to residential radon have been demonstrated through residential case-control epidemiological studies. However, as discussed by UNSCEAR, exposures to thoron and its decay products have often been relatively ignored. Moreover, unlike radon the effects of exposure to thoron and its decay products are not available from epidemiology and thus, a dosimetric approach is required to assess risks. UNSCEAR continues to recommend the use of a dose conversion factor for thoron decay products of 40 nSv (Bq h m(-3))(-1). UNSCEAR Annex E suggests there is an emerging problem, namely, that the contribution of (220)Rn (thoron) gas to the (222)Rn (radon) gas measurement signal is not well known. Until recently, this has largely been ignored. This is an important consideration as measurements at work and homes are the basis for investigating lung cancer exposure-response relationships. Based on UNSCEAR Annex E, this paper provides an overview of the sources and levels of thoron and its associated decay products at home and work. In addition, this paper provides an overview of the thoron dosimetry considered by UNSCEAR Annex E and some recent results.     

Radon concentration measurements in the Amasra coal mine, Turkey

In this study, the results of atmospheric radon measurements that were performed for the Amasra underground coal mine in Zonguldak bituminous coal basin (Turkey) are presented. The radon measurements were performed for 40 days between November 2004 and December 2004 using passive nuclear etched track detectors. The radon concentrations vary from a minimum value 49 Bq m(-3) in a site located at +40 m to a maximum value 223 Bq m(-3) in a site located at -100 m. Mean concentration is 117 (Bq m(-3)). This value is well below the action level of 500-1,500 Bq m(-3) recommended by the International Commission on Radiological Protection (ICRP) (1993). The mean effective dose value for workers of this mine of 3.4 microSv per day was obtained. This result shows that protection against radiological hazards would not be necessary for workers of this mine((2)).     

International standardisation work on the measurement of radon in air and water

Radon is considered to be the main source of human exposure to natural radiation. As stated by the World Health Organization, the exposure due to the inhalation of indoor radon is much greater than the one via the ingestion of water as radon degasses from water during handling. In response to these concerns about the universal presence of radon, environmental assessment studies are regularly commissioned to assess the radon exposure of public and workers. The credibility of such studies relies on the quality and reliability of radon analysis as well as on the sample representativeness of the radiological situation. The standard-setting approach, based on consensus, seemed to lend itself to a settlement of technical aspects of potential comparison. At present, two Working Groups of the International Standardization Organization are focussing on drafting standards on radon and its decay products measurement in air and water. These standards, which aim for a set of rigorous metrology practices, will be useful for persons in charge of the initial characterisation of a site with respect to natural radioactivity as well as to those performing the routine surveillance of specific sites.     

Miners' exposure to radon and its decay products in some Iranian non-uranium underground mines

Measurements of radon, radon decay products and gamma exposure rate in 12 non-uranium underground mines have been carried out in order to estimate the occupational radiation exposure of miners. Continuous measurements of radon using pulse ionisation chambers and scintillation cell techniques were employed for these studies. Progenies of radon were collected on filter paper, and then a three-count procedure was used for the measurement. The equilibrium state between radon and its decay products has been determined. Concentrations of natural radionuclides ((226)Ra, (232)Th and (40)K) in ore and soil samples taken from various locations in each mine have been measured using a Canberra High Purity Germanium detector. Based on these measurements two ranges of dose were evident. Doses ranged from 0.1 to 1.52 mSv y(-1) for nine mines and from 10 to 31 mSv y(-1) for the other three mines. A separate grouping of the mines was recognised from radon concentrations, which varied from 2 Bq m(-3) to 10 kBq m(-3). In three of these mines, working level (WL) concentrations of the order of 36-1771 mWL were determined in different working areas. In all other mines, the concentrations were observed to be <45 mWL.     

Radon dynamics and reduction in an underground mine in Brazil. Implications for workers' exposure

This work was aimed at studying the behaviour of 222Rn in an experimental underground copper mine in Brazil with a single entrance. The 222Rn concentrations, meaured by using a dynamic radon measuring technique. varied between 30.5 Bq.m(-3), during ventilated conditions applied to the mine galleries, and 19.4 x 10(3) Bq.(-3) for non-ventilated conditions and when operational mining activities were conducted inside. High radon concentration surges were observed after blasting and drilling activities. In the cases of inadequate ventilation, it was estimated that workers could be subjected to exposures as high as 10 microSv.h(-1), only due to 222Rn and its short-lived progeny. The results show the importance of real-time measurements to evaluate radon dynamics during mining operations.     

Assessment of test duration effect in indoor radon measurement by Monte Carlo simulations

To better understand the effect of various test durations on indoor radon measurement results in Canada, Monte Carlo simulations were performed for test durations of 1 month (30 d), 2 months (61 d), 3 months (91 d) and 6 months (183 d). For each of the specified test durations, a total of 1500 Monte Carlo simulations were performed. Each simulation was compared with the result of a 1-y measurement. On average, the radon concentration estimated from a 30-d test differed by about ±22 % from the value of a 1-y measurement. The difference reduced to about ±17 % for a 61-d test, ±14 % for a 91-d test and ±9 % for a half-year test. Health Canada's recommendation of a 3-month radon test performed during the heating season resulted in an estimated radon concentration, on average, ～20 % higher than the value determined from a 1-y measurement. This ensures a conservative estimate of the annual average radon concentration, as there is some risk at any radon level. Therefore, to avoid an underestimation of radon exposure and to ensure appropriate levels of precision and accuracy are met, the results from this study suggest that a radon measurement duration of 3 months or longer during the heating season (from October through to April) is needed.     

Workplace monitoring for exposures to radon and to other natural sources in Europe: integration of monitoring for internal and external exposures

Part of the action of the EURADOS working group (European Radiation Dosimetry Group) on "Harmonisation of Individual Monitoring in Europe" was to investigate how the results from personal dosemeters for external radiation, from monitoring for internal exposure and from workplace monitoring, can be combined into a complete and consistent system of individual monitoring. To facilitate this work, the "EURADOS questionnaire Q3" relating to radon and other natural sources of radiation in the workplace was distributed to relevant institutes across Europe. A total of 24 countries replied to the questionnaire. This study offers an important overview on actual regulations, national standards and reference levels for protection of employees from radon and other natural sources in different workplace scenarios. Information was also collected on individual monitoring and area monitoring to determine individual doses in workplaces with elevated levels of natural radiation. The article discusses in detail the results obtained showing by country the reference level in workplaces for radon gas and other natural sources. In both instances, exposures in mines, other underground workplaces, industry workplaces/waterworks, offices, schools and day-care homes were considered. The resultant data clearly indicate that there is a need for harmonisation among countries, not least in the areas of regulation and use of reference levels in the workplace.     

In vivo measurements of 210Pb in skull and knee geometries as an indicator of cumulative 222Rn exposure in a underground coal mine in Brazil

Cumulative exposure to radon can be evaluated by measuring (210)Pb in bone. The skull and knee are two convenient parts of the skeleton for in vivo measuring (210)Pb because these regions of the body present a high concentration of bone, the detectors are easily positioned and the likelihood of cross contribution from other organs or tissues is low. A radiological survey of non-uranium mines in Brazil indicated that an underground coal mine in Paraná, located in the south of Brazil, exhibited a high radon concentration. In vivo measurements of 32 underground coal miners were performed in the IRD-CNEN Whole Body Counter shielded room using an array of four high-resolution germanium detectors. Estimations of (210)Pb in the total skeleton were determined from direct in vivo measurements of (210)Pb in the head and knees. In vivo measurements of (210)Pb in 6 out of 32 underground coal miners ranged from 80 to 164 Bq, suggesting that these workers were significantly exposed to (222)Rn.     

Anomalous indoor radon concentration in a dwelling in Qatif City, Saudi Arabia

An indoor radon survey was carried out recently in nine cities of Saudi Arabia using nuclear track detectors (NTD)-based passive radon detectors. The survey included Qatif City in the Eastern Province of Saudi Arabia, where 225 detectors were collected back successfully. It was found that the average indoor radon concentration in the dwellings was 22 +/- 15 Bq m(-3). However, one of the dwellings showed an anomalous radon concentration of 535 +/- 23 Bq m(-3). This finding led to a detailed investigation of this dwelling using active and passive techniques. In the active technique, an AlphaGUARD 2000 PRQ radon gas analyser was used. In the passive technique, CR-39 based passive radon detectors were used in all the rooms of the dwelling. Radon exhalation from the wall and the floor was also measured using the can technique. The active measurement confirms the passive one. Before placing the passive radon detectors in all the rooms of the two-storey building, the inhabitant was advised to ventilate his house regularly. The radon concentration in the different rooms was found to vary from 124 to 302 Bq m(-3). Radon exhalation from the floor and the wall of the room with the anomalous radon concentration was found to vary from 0.5 to 0.8 Bq m(-2) h(-1). These low radon exhalation rates suggest that the anomalous radon concentration is most probably due to underground radon diffusion into the dwelling through cracks and joints in the concrete floor.     

Radon exposures from the use of natural gas in buildings

Low levels of natural radioactivity in the ground produce radon-222 and its decay products which can be entrained with gas streams and become distributed with gas supplies to commercial and domestic users. Levels of radon in blended gas received by most users are comparable with the levels that are present naturally in buildings as a result of ingress from the ground and this is further diluted during the combustion process. For typical rates of gas usage with an average radon level of about 200 Bq x m(-3), the estimated dose from the use of natural gas is estimated at 4 microSv, less than 1% of the dose from radon exposure at the average level in UK homes. Commercial users may receive somewhat higher doses, and the estimate for a critical group is a few tens of microsievert. The total radon emission to the environment is estimated at about 10(13) Bq x y(-1) which represents less than 10(-4) of the natural emission rate from the ground. There is some variability of radon levels in gas from different sources and it would be prudent to keep this source of exposure under review. A standard sampling and measurement protocol has been developed in conjunction with a technical group representing the industry.     

Towards the use of small amounts of activated charcoal along with well-type NaI(Tl) detector for indoor radon measurements

The feasibility of using small quantities of activated charcoal and a 7.6 cm x 7.6 cm NaI(Tl) well-type detector was investigated for indoor radon measurements. Vials, filled with 10 g of charcoal, were exposed for different indoor radon concentration levels typical of Kuwait dwellings. After exposure, the vials were sealed and kept for 3 h to allow radon to come into radioactive equilibrium with its progenies and were then analysed by gamma-ray spectrometry using the well-type NaI(Tl) detector. The variation of radon absorption by the vials filled with charcoal with exposure time was also studied. A comparative study of the present technique with the standard technique of using 70 g charcoal canisters and flat NaI detector was also performed. After establishing the suitability of the technique, the charcoal vials were then used to investigate the effect of air-ventilation on the concentration levels of the indoor radon. Results show that there is a reduction in the radon concentration level (up to 25%) when the air-ventilation system was switched on. The paper presents the results of the study on the feasibility of combining small amounts of activated charcoal with a well-type NaI(Tl) detector in the measurement of indoor radon concentrations.     

Significance of independent radon entry rate and air exchange rate assessment for the purpose of radon mitigation effectiveness proper evaluation: case studies

Two new single-family houses identified as insufficient with regard to existing radon barrier efficiency, have been selected for further examination. A complex set of radon diagnosis procedures has been applied in order to localise and quantify radon entry pathways into the indoor environment. Independent assessment of radon entry rate and air exchange rate has been carried out using the continuous indoor radon measurement and a specific tracer gas application. Simultaneous assessment of these key determining factors has turned out to be absolutely crucial in the context of major cause identification of elevated indoor radon concentration.     

Are radon gas measurements adequate for epidemiological studies and case control studies of radon-induced lung cancer?

The lung dose derived from radon is not attributed to the radon gas itself, but instead to its short-lived progeny. However, in many epidemiological studies as well as in case control studies of the radon risk, the excess number of cancers are related to the radon gas exposure, and not to the radon progeny exposure. A justification for such an approach has resorted to the assumption that there is self-compensation between the radiation doses from the unattached and attached fractions. In the present study, we used the Jacobi model to calculate the radon progeny concentrations in a room by varying the attachment rate and then calculated the resulting lung dose. It was found that self-compensation was not fully realised, and the effective dose can vary by a factor up to approximately 2 for the same radon gas concentration. In conclusion, the radon gas concentration alone does not provide adequate information on the effective dose.     

An assessment of annual whole-body occupational radiation exposure in Ireland (1996-2005)

Whole-body occupational exposure to artificial radiation sources in Ireland for the years 1996-2005 has been reviewed. Dose data have been extracted from the database of the Radiological Protection Institute of Ireland, which contains data on >95% of monitored workers. The data have been divided into three sectors: medical, industrial and education/research. Data on exposure to radon in underground mines and show caves for the years 2001-05 are also presented. There has been a continuous increase in the number of exposed workers from 5980 in 1996 to 9892 in 2005. Over the same time period, the number of exposed workers receiving measurable doses has decreased from 676 in 1996 to 189 in 2005 and the collective dose has also decreased from 227.1 to 110.3 man millisievert (man mSv). The collective dose to workers in the medical sector has consistently declined over the 10-y period of the study while that attributable to the industrial sector has remained reasonably static. In the education/research sector, the collective dose typically represents 5% or less of the total collective dose from all practices. Over the 10 y of the study, a total of 77 914 annual dose records have been accumulated, but only 4040 (<6%) of these represent measurable radiation doses in any given year. Over the same time period, there were 283 instances in which exposed workers received individual annual doses >1 mSv and 21 of these exceeded 5 mSv. Most of the doses >1 mSv were received by individuals working in diagnostic radiology (which also includes interventional radiology) in hospitals and site industrial radiography. There has been only one instance of a dose above the annual dose limit of 20 mSv. Evaluating the data for the period 2001-05 separately, the average annual collective dose from the medical, industrial and educational/research sectors are approximately 60, 70 and 2 man mSv with the average dose per exposed worker who received a measurable dose being 0.32, 0.79 and 0.24 mSv, respectively. Diagnostic radiology and site industrial radiography each represents >60% of the collective dose in their respective sectors. Available data on radon exposure in one underground mine and in three show caves indicate an annual collective dose of 75 man mSv from these work activities. By comparison, previous estimates of exposure of Irish air crew to cosmic radiation have given rise to an estimated collective dose of 12 000 man mSv. It can be concluded therefore that the natural radioactivity sources account for well >90% of all occupational exposure in Ireland. This evaluation does not include an estimate of exposure to radon in above-ground workplaces-these data are currently being evaluated and their inclusion will increase both the total occupational collective dose as well as the percentage of that dose due to natural radiation.     

The overview of internal exposure monitoring in Lithuania

This study deals with analysis of situation and results of internal exposure monitoring of radiation workers and population in Lithuania. Radiation workers are assessed for internal exposures by direct methods--whole body counting or organ counting by gamma spectrometry at the Radiation Protection Centre and Ignalina Nuclear Power Plant (INPP). Results of monitoring of INPP and nuclear medicine workers show that no significant activities were detected. The annual committed effective doses of workers are <1 mSv. The measured average activity of 40K in males and females was 3.7 +/- 1.0 and 2.5 +/- 0.7 kBq, respectively. Mixed diet sampled at hospitals in 2001-5 was analysed for (90)Sr and (137)Cs activity concentrations. Average effective dose due to 90Sr and 137Cs in mixed diet was 0.6 +/- 0.2 and 0.47 +/- 0.13 microSv, respectively. Indoor radon measurements were done in multi-storey houses. Average concentration was 15.1 +/- 1.0 Bq m(-3). The annual effective dose aused by radon was 0.38 mSv.