Fission Gas Induced Cladding Deformation of LWR Fuel Rods under Reactivity Initiated Accident Conditions

Behavior of irradiated fuel rods under power burst conditions by accidental reactivity insertion in light water reactors (LWRs) has been studied in the Nuclear Safety Research Reactor (NSRR). In the experiments, cladding hoop deformation, which reached up to about 10%, was much larger than that of the fresh rods. The current LWR fuel behavior analysis codes, which only take account of the thermal expansion of the fuel pellets for the deformation calculation, under-predicted the plastic deformation of the cladding to be less than about 1%. Fission gas release during the pulse irradiation tests reached as high as 22% in the NSRR irradiated fuel tests. In order to describe these test results, a model of grain boundary fission gases to cause the cladding deformation has been developed and installed in a fuel behavior simulation code, FRAP-T6. In the model, the over-pressurized gases by the pulse irradiation cause grain boundary separation and stress the cladding during the tests. The model assumes that the gases remain in the fuel during the early part of pulse irradiation and are released to the open volume in the rod after the cladding deformation. The model, in combination with a fuel thermal expansion model, GAPCON, which was validated through fresh fuel tests, reproduces the NSRR test results reasonably well.     

Transient Elongation of a Fresh Fuel Rod under Reactivity Initiated Accident Conditions

In-pile experiments of fresh fuel rods under reactivity initiated accident (RIA) conditions have been performed in the Nuclear Safety Research Reactor at the Japan Atomic Energy Research Institute in order to understand the basic pellet cladding mechanical interaction (PCMI) behavior. Rapid fuel pellet expansion due to a power excursion would cause radial and longitudinal deformation of the cladding. This PCMI could be one of the possible incipient failure modes of an embrittled cladding of a high burnup fuel under the RIA conditions.

Basic PCMI behavior was studied by measuring cladding deformation of a fresh fuel rod without complicated irradiation effects. The transient elongation measurements of the fuel with two kinds of gap width indicated not only PCMI-induced cladding elongation, but also reduction of the pellet stack displacement by the cladding constraint. In the tests under a high-pressure and high-temperature condition simulating an operation condition of BWRs, additional ridge-type cladding deformation was generated due to the axial collapse of the cladding. A preliminary analysis for interpretation of the tests was made using a computer code for the transient analysis of fuel rods, FRAP-T6.     

Behavior of 60 to 78MWd/kgU PWR Fuels under Reactivity-Initiated Accident Conditions

To provide a data base for the regulatory guide of light water reactors, behavior of reactor fuels during off-normal and postulated accident conditions such as reactivity-initiated accident (RIA) is being studied in the Nuclear Safety Research Reactor (NSRR) program of the Japan Atomic Energy Agency (JAEA). The paper presents recent results obtained from the NSRR power burst experiments with high burnup fuels, and discusses effects of pellet expansion as PCMI (Pellet-Cladding Mechanical Interaction) loading and cladding embrittlement primarily due to hydrogen absorption. Results from the recent four experiments on high burnup (about 60 to 78 MWd/kgU) PWR UO₂ rods with advanced cladding alloys showed that the fuel rods with improved corrosion resistance have larger safety margin against the PCMI failure than conventional Zircaloy-4 rods. The tests also suggested that the smaller inventory of inter-granular gas in the pellets with the large grain could reduce the fission gas release during the RIA transient; and high burnup structure in pellet periphery (so-called rim structure) does not have strong effect on reduction of the failure threshold because the PCMI load is produced primarily by solid thermal expansion.     

Experimental Study on the Fuel Behavior during Reactivity Accident at Power Operation Condition

In the Nuclear Safety Research Reactor (NSRR) program of Japan Atomic Energy Research Institute (JAERI), the fuel behavior in reactivity initiated accidents (RIAs) has been studied through irradiation tests with simulated power burst using fresh or preirradiated test fuel rods. In order to investigate possible influence of the difference of initial temperature profile in the fuel pellet on the fuel failure behavior, two tests were conducted with fresh fuel rods for RIAs at power operation using the newly developed NSRR operation mode and the results were compared with the results of previous irradiation tests which were for RIAs at zero power.

In the tests for RIAs at power, the reactivity of 2.0$ or 2.3$ was inserted rapidly after the linear heat rate of the test fuel rod was kept constant at 39kW/m for 5s. It has been shown through this study with fresh fuel rods that the fuel enthalpy of the failure threshold for RIAs at power is the same as that for RIAs at zero power and that the failure mechanism is the same as that of RIA at zero power. It has been clarified that there is no obvious influence of initial temperature distribution on the fuel behavior during RIAs in case of fresh fuels. The evaluation method of fuel enthalpy with which the fuel failure threshold is described was also studied.     

Behavior of Coated Fuel Particle of High-Temperature Gas-Cooled Reactor under Reactivity-Initiated Accident Conditions

In order to clarify the failure mechanism and determine the failure limit of the High-Temperature Gascooled Reactor (HTGR) fuel under reactivity-initiated accident (RIA) conditions, pulse irradiations were performed with unirradiated coated fuel particles at the Nuclear Safety Research Reactor (NSRR). The energy deposition ranged from 0.578 to 1.869 kJ/gUO₂, in the pulse irradiations and the estimated peak temperature at the center of the fuel particle ranged from 1,510 to 3,950 K. Detailed examinations after the pulse irradiations showed that the coated fuel particles failed above 1.40 kJ/gUO₂, where the peak fuel temperature reached over the melting point of UO₂ fuel. It was concluded that the coated fuel particle was failed by the mechanical interaction between the melted and swelled fuel kernel and the coating layer under RIA conditions.     

MOX Fuel Performance Experiment Specified for Japanese PWR Utilisation in the HBWR

In order to obtain high burn-up MOX fuel irradiation performance data, SBR and MIMAS MOX fuel rods with Pufissile enrichment of about 6 wt% have been irradiated in the HBWR. In-pile performance data of MOX have been obtained, and the peak burn-up of MOX pellet have reached to 66 GWd/tM as of October 2004. MOX fuel temperature is confirmed to have no significant difference compared to UO₂, if taking into account adequately for thermal conductivity degradation due to PuO₂ addition and burn-up development, and measured fuel temperature agrees well with HB-FINE code calculation up to high burn-up region. Fission gas release of MOX is possibly larger than UO₂ based on temperature and pressure assessment. No significant difference is confirmed between SBR and MIMAS MOX on FGR behaviour. MOX fuel swelling rate agrees well with solid swelling rate. Cladding elongation data shows onset of PCMI in high power region. Ramp test data from other experiment programs with various types of MOX fabrication route confirms superior PCI resistance of MOX compared to UO₂, due to enhanced creep rate of MOX. The irradiation is expected to continue until achieving of 70 GWd/tM (MOX pellet peak).     

Effect of Fuel Pellet Eccentricity with Cladding on Fuel Rod Thermal Behavior under Reactivity Initiated Accident Condition

Fuel rod behavior under Reactivity Initiated Accident (RIA) conditions has been studied in the Nuclear Safety Research Reactor (NSRR), JAERI. In the experiments, cladding thermal behavior was observed to be influenced by the fuel pellet eccentricity to produce large azimuthal temperature variation in the cladding. The maximum azimuthal cladding temperature difference was measured to be as large as 150°C by thermocouples attached to opposite sides of the cladding around the circumference, though the thermocouples did not always detect the maximum temperature difference around the circumference. The actual temperature differences in the fuel rods subjected to less than 290 cal/g?UO₂ were estimated to be 350°C at maximum based on metallographies. A simple calculation considering gap conductance variations also showed that the maximum temperature difference became 350°C under fully eccentrical condition in the fuel rod subjected to 260 cal/g?UO₂. Moreover, as the rod damage such as cladding deformation, melting and failure occurs unevenly around the circumference due to the fuel pellet eccentricity in general, the fuel pellet eccentricity should influence the fuel rod failure under RIA conditions.     

Transient Cooling Process of Fuel Rod in Reactivity Initiated Accident

Out-of-pile experiments were performed with Zircaloy-4 rods in subcooled water environment to study the basic phenomena occurring in the transient cooling process undergone by a fuel rod during a reactivity-initiated accident (RIA) affecting a light water reactor (LWR). The experimental results show that the cooling process of the fuel rod during an RIA can be divided into three phases separated by the quenching temperature T_q and the rewetting temperature T_q .

It is also noted from the experimental results that with increasing degree of subcooling, T_q tends to rise to levels far exceeding the maximum liquid superheat temperature of water; T_q , on the other hand, is little affected by the cooling water temperature, and remains close to that of the maximum superheat temperature.

Numerical calculations indicate conclusively that radial heat transfer to coolant water is the dominant factor that governs the transient cooling process in an RIA affecting the cold start-up of a BWR, rather than the axial heat conduction through rod which is considered to be the basic mechanism of cooling that governs the reflooding process during a LOCA.     

Influence of Cladding-Peripheral Hydride on Mechanical Fuel Failure under Reactivity-Initiated Accident Conditions

In order to investigate the influence of hydrogen embrittlement on fuel failure under reactivity-initiated accident (RIA) conditions, pulse irradiation experiments were performed with unirradiated fuel rods at the Nuclear Safety Research Reactor (NSRR). Fresh cladding was pre-hydrided so that the other factors of cladding degradation, such as irradiation damage and oxidation, were excluded. Hydride clusters are circumferentially oriented and localized in the cladding periphery in order to simulate ‘hydride rim’ which is formed in high burnup PWR cladding. The present study demonstrated hydride-assisted pellet-cladding mechanical interaction (PCMI) failure which has been observed in high burnup fuel experiments. The fuel enthalpy at failure was lower when the cladding had a thicker hydride rim where surface cracks were easily generated. It indicates that the failure limit is highly correlated with the stress intensity factor assuming that the crack depth is equivalent to the hydride rim thickness. Hence, we conclude that hydride rim formation is the primary factor of decreasing the failure limit for high burnup fuels. Based on the experimental results together with an analysis on cladding mechanical state during PCMI, the present study suggests a process of through-wall crack generation which is originated with brittle cracking within the hydride rim.     

Analysis of MOX Fuel Behavior in Halden Reactor by FEMAXI-6 Code

Capabilities of the FEMAXI-6 code to analyze the behavior of high burnup MOX fuels in LWRs have been evaluated. Coolant conditions, detailed power histories and specifications of the MIMAS-MOX fuel rods, rod 10 and rod 11, of IFA-597.4–7 irradiated in the Halden reactor were input, and calculated rod internal pressures and pellet center temperatures were compared with the measured data for the range of 0-31 MWd/kgUO₂. Some sensitivity studies were conducted mainly with respect to pellet thermal conductivity and swelling rate to investigate the changes in thermal behavior and their effects on fission gas release.

In the irradiation period up to about 23 MWd/kgUO₂, the calculated pellet center temperatures sufficiently agreed with the measured data and also the calculated rod internal pressures reproduced the tendency of an increase in the measured rod internal pressures. These results suggest that fission gas release from MOX fuels can be reasonably predicted by a diffusion process that is modeled in UO₂ pellet grains. On the other hand, the steep increase in the measured rod internal pressures observed at the power ramp around 23 MWd/kgUO₂ cannot be reproduced by FEMAXI-6 and can be regarded as the result of a relatively large amount of gas release, which possibly caused a pellet-cladding-gap closure through pellet gas-bubble swelling.     

Transient Behavior of Low Enriched Uranium Silicide Plate-Type Fuel for Research Reactors during Reactivity Initiated Accident Conditions

Abstract

This paper describes the results of transient experiments using a low enriched uranium silicide miniplate fuel for research reactor. The pulse irradiation was performed in the Nuclear Safety Research Reactor (NSRR) at the Japan Atomic Energy Research Institute (JAERI).

The results obtained in this study are summarized as follows :

(1) The tested fuel plates were damaged with energy depositions above 94 cal/g·fuel, but remained intact below 82cal/g·fuel. A failure threshold should therefore exist between these two values.

(2) Four of the fuel plates that showed peak cladding surface temperatures <330°C were damaged by the thermal stress during quenching. These damaged fuel plates revealed small intergranular cracks that propagated perpendicularly to the axial direction of the plate, from the Al cladding surface to the fuel core, without significant dimensional changes. On the other hand, when peak cladding surface temperatures were >400°C, the test fuel plates were damaged mainly by melting of the Al cladding, accompanying significant dimensional changes.

(3) The thermal stress of the damaged fuel plates calculated on the basis of the maximum transient temperature drop during quenching was greater than the tensile stress that occurred during fabrication.     

Modeling for Void Reactivity Effect by Subcooled Boiling under Reactivity Initiated Accident Condition of BWR

A simple mechanistic model is presented to evaluate the subcooled void reactivity effect under a Reactivity Initiated Accident (RIA) at cold critical condition of BWR. This model consists of a drift flux model for vapor velocity and a vapor mass conservation model with a term of vapor source on a heated wall, and it was incorporated into a homogeneous and equilibrium thermal-hydraulic code EUREKA-JINS. A sample analysis by this model showed that the subcooled void reactivity effect leads to reduction of the maximum fuel enthalpy by about 20 cal/g UO₂ in the case of RIA at cold critical condition. Though the reduced value is dependent on the reactor core condition, this result indicates the significance of subcooled void reactivity effect in the accident, while the effect can be neglected in the hot stand-by case where, at most, only 4 cal/g UO₂ is reduced for the maximum fuel enthalpy.     

Releases of Cesium and Poorly Volatile Elements from UO2 and MOX Fuels under Severe Accident Conditions

Radionuclide release from fuel under severe accident conditions has been investigated in the VEGA program at the Japan Atomic Energy Agency. In this program, three types of fuel, two UO₂ fuels irradiated at PWR and BWR and a MOX fuel irradiated at the ATR Fugen, were heated up to about 3130K in helium atmosphere at 0.1 MPa. Comparison of experimental data and evaluation with computer code analyses showed that Cs release is essentially identical among the three fuels. The Cs release from fuel may differ below about 1770K due to a difference in migration to grain boundaries during irradiation. The difference was not also observed for releases of poorly volatile elements, namely, U, Pu, Sr and Mo between UO₂ and MOX fuels. The release rate of Pu became slightly higher than that of U at 3130 K. The release rate of Sr increased at 3130 K, while that of Mo was quite low at temperatures above 2310 K.     

LWR Fuel Safety Research with Particular Emphasis on RIA/LOCA and Other Conditions

Fuel safety research at Japan Atomic Energy Research Institute (JAERI) is reviewed on the major subjects including studies on fuel behavior under postulated Reactivity Initiated Accident (RIA), postulated Loss of Coolant Accident (LOCA) and normal operating conditions. Nuclear Safety Research Reactor (NSRR) at JAERI has been utilized extensively for the studies of fuel behavior under RIA conditions. For the studies of fuel rod and cladding behavior under LOCA conditions, outpile experiments were conducted. The work on this subject has been concluded. Pellet Cladding Interaction (PCI) has been major subject on fuel integrity study during normal operating conditions. Irradiation experiments at Halden Boiling Water Reactor (HBWR) as well as code development are described.     

Thermal Stress Analysis of High-Burnup LWR Fuel Pellet Pulse-Irradiated in Reactivity-Initiated Accident Conditions

For RIA-simulated experiments in the NSRR with high-burnup PWR fuel and BWR fuel, numerical analyses were performed to evaluate the temporal changes of profiles of temperature and thermal stress in pellet induced by pulse power, using the RANNS code. The pre-pulse states of rods were calculated using the fuel performance code FEMAXI-6 along the irradiation histories in commercial reactors and the results were fed to the RANNS analysis as initial conditions of the rod. One-dimensional FEM was applied to the mechanical analysis of the fuel rod, and the calculated cladding permanent strain was compared with the measured value to confirm the validity of the PCMI calculation. The calculated changes in the profiles of temperature and stress in the pellet during an early transient phase were compared with the measured data such as the internal gas pressure rise, cracks and grain structure in the post-test pellet, anddiscussed in terms of PCMI and grain separation. The analyses indicate that the pellet cracking appearances coincided with the calculated tensile stress state and that the compressive thermal stress suppresses the fission gas bubble expansion leading to grain separation.     

Effects of Rod Pre-Pressurization on Light Water Reactor Fuel Behavior during Reactivity Initiated Accident Conditions

Previously pressurized (pre-pressurized) fuel rod tests recently performed in the Nuclear Safety Research Reactor (NSRR) investigate the effects of initial internal pressure on fuel rod behavior during reactivity initiated accident (RIA) conditions. A single PWR type fuel rod was contained within a waterfilled, ambient temperature and ambient pressure capsule. The fuel rod was then heated by the pulsing operation of the NSRR.

Results from the tests show that the effect of pre-pressurization was significant for the fuel rods with initial internal pressure of 0.8 MPa and above, and fuel rod failure occurred from rupture of the cladding with lower threshold energy deposition for failure as the initial internal pressure was increased. The cladding rupture was governed mainly by the cladding temperature rise, not by the rod internal pressure rise during the transient. The relationships between cladding burst pressure and cladding burst temperature and between cladding strain and cladding temperature at cladding rupture obtained in the present study under an RIA condition agree with the results obtained from various in- and ex-reactor experiments under a LOCA condition, although the obtained time-averaged strain rate of the Zircaloy cladding was much greater than that in a LOCA condition.     

Effects of Coolant Flow on Light Water Reactor Fuel Behaviors during Reactivity Initiated Accident

This paper describes the in-pile experimental results to study the influences of coolant flow on fuel behaviors under reactivity initiated accident (RIA) conditions performed in the Nuclear Safety Research Reactor (NSRR). A single PWR type test fuel rod was irradiated by a large neutron pulse in the NSRR to simulate a prompt power excursion of RIA's. The effects of coolant flow were studied at a coolant flow velocity of 0.3~1.8m/s and a coolant temperature of 20~90°C under the atmospheric pressure. It was found that the cooling conditions had considerable influences on fuel thermal behaviors under prompt heat-up. The increase of coolant flow velocity and subcooling enhanced heat transfer coefficient at cladding surface during film boiling, which resulted in large decrease of maximum cladding temperature and film boiling duration, and consequently in the increase of fuel failure threshold energy. The data tendencies are summarized and the influences of coolant flow are discussed with some computer analyses.     

Irradiation Performance of Fast Reactor MOX Fuel Assemblies Irradiated to High Burnups

Mixed oxide fuel assemblies (MFA-1 and MFA-2 assemblies) were irradiated in the fast flux test facility to evaluate the irradiation performance of fast reactor core fuels at high burnups and high fast neutron fluences. The MFA-1 and MFA-2 assemblies achieved respective peak pellet burnups of 147 and 162GWd/t, and resisted to respective peak fast neutron fluences (E > 0:1 MeV) of 21:4 _ 1026 and 23:8 _ 1026 n/m2, without any indication of fuel pin breaching. Structural components of these assemblies were made of modified type 316 stainless steel and 15Cr-20Ni base advanced austenitic stainless steel. Postirradiation examinations of these assemblies revealed dimensional changes of fuel pins and assembly ducts due to irradiation-induced void swelling and irradiation creep, and fuel cladding local oval distortions due to bundle-duct interaction (BDI). The swelling resistance of 15Cr-20Ni base advanced austenitic stainless steel fuel pin cladding was almost the same as that of the modified type 316 stainless steel cladding, while the assembly duct of the former material had a slightly higher swelling resistance than that of the latter material. Analyses of fuel pin bundle deformations indicated that these assemblies likely mitigate BDI mainly by fuel pin bowings and cladding oval distortions.