Global temperature stabilization via controlled albedo enhancement of low-level maritime clouds

An assessment is made herein of the proposal that controlled global cooling sufficient to balance global warming resulting from increasing atmospheric CO2 concentrations might be achieved by seeding low-level, extensive maritime clouds with seawater particles that act as cloud condensation nuclei, thereby activating new droplets and increasing cloud albedo (and possibly longevity). This paper focuses on scientific and meteorological aspects of the scheme. Associated technological issues are addressed in a companion paper. Analytical calculations, cloud modelling and (particularly) GCM computations suggest that, if outstanding questions are satisfactorily resolved, the controllable, globally averaged negative forcing resulting from deployment of this scheme might be sufficient to balance the positive forcing associated with a doubling of CO2 concentration. This statement is supported quantitatively by recent observational evidence from three disparate sources. We conclude that this technique could thus be adequate to hold the Earth's temperature constant for many decades. More work--especially assessments of possible meteorological and climatological ramifications--is required on several components of the scheme, which possesses the advantages that (i) it is ecologically benign--the only raw materials being wind and seawater, (ii) the degree of cooling could be controlled, and (iii) if unforeseen adverse effects occur, the system could be immediately switched off, with the forcing returning to normal within a few days (although the response would take a much longer time).     

Sea-going hardware for the cloud albedo method of reversing global warming

Following the review by Latham et al. (Latham et al. 2008 Phil. Trans. R. Soc. A 366) of a strategy to reduce insolation by exploiting the Twomey effect, the present paper describes in outline the rationale and underlying engineering hardware that may bring the strategy from concept to operation. Wind-driven spray vessels will sail back and forth perpendicular to the local prevailing wind and release micron-sized drops of seawater into the turbulent boundary layer beneath marine stratocumulus clouds. The combination of wind and vessel movements will treat a large area of sky. When residues left after drop evaporation reach cloud level they will provide many new cloud condensation nuclei giving more but smaller drops and so will increase the cloud albedo to reflect solar energy back out to space. If the possible power increase of 3.7W m-2 from double pre-industrial CO2 is divided by the 24-hour solar input of 340W m-2, a global albedo increase of only 1.1 per cent will produce a sufficient offset. The method is not intended to make new clouds. It will just make existing clouds whiter. This paper describes the design of 300 tonne ships powered by Flettner rotors rather than conventional sails. The vessels will drag turbines resembling oversized propellers through the water to provide the means for generating electrical energy. Some will be used for rotor spin, but most will be used to create spray by pumping 30 kgs-1 of carefully filtered water through banks of filters and then to micro-nozzles with piezoelectric excitation to vary drop diameter. The rotors offer a convenient housing for spray nozzles with fan assistance to help initial dispersion. The ratio of solar energy reflected by a drop at the top of a cloud to the energy needed to make the surface area of the nucleus on which it has grown is many orders of magnitude and so the spray quantities needed to achieve sufficient global cooling are technically feasible.     

Retrieval of total ozone abundances from the ultraviolet region of spectra recorded with an ultraviolet-visible spectrometer

A method is described for deriving total ozone abundances from zenith-sky intensities measured by an UV-visible spectrometer, known as the System of Analysis of Observations at Zenith (SAOZ). Total ozone abundances are determined by comparison of intensity ratios measured at two wavelengths in the UV region with ratios computed with a radiative transfer model. The wavelength pair 320-307 nm was used in this study. Spectra recorded by the SAOZ spectrometer in Oslo (60 degrees N) from the beginning of May 1995 to the end of August 1995 were analyzed, and the results were compared with total ozone measured with a Brewer instrument. The relative difference in derived ozone abundances for the whole period, including days with thin and medium-thick cloud covers, is -0.18 +/- 1.46%. We study the effects of clouds and varying ground albedo on the derived total ozone. Clouds result in an overestimation of the derived total ozone. The error increases with the optical depth tau of the cloud from approximately 2% for an optically thin cloud (tau = 0.5) to approximately 10% for a thick cloud (tau = 50). The ratio between measured intensities at 550 and 350 nm, the so-called color index, can be used as a measure of the cloud optical depth for thin and medium-thick clouds. The effects of thin and medium-thick clouds on the derived ozone abundances can be compensated for by use of an empirical relationship found between the measured color index and the error in the inferred ozone abundances caused by cloud scattering. We also study the influence of changes in the ground albedo and in the ozone profiles on derived total ozone values.     

云层厚度对蓝绿激光通信性能的影响分析

针对机载激光发射器位于云层上方或云层中央时,云层的存在会降低激光通信性能的问题,仿真分析了不同类型的云层对激光能量衰减、信噪比、最大码元传输速率与误码率的影响。得到结论:云的存在主要造成激光能量衰减,影响最大传输速率与误码率,但对信噪比影响较小。链路余量大于18.9 dB的通信系统,链路上允许存在4 km的云层。云层对最大通信速率与误码率的影响主要是时间扩展造成码间串扰。卷云对通信性能几乎无影响;积云对通信性能的影响较大;层云、层积云和积雨云对通信性能的影响更大,但三种云的差异很小,可不作区分;高层云和雨层云对通信性能影响最大,其中雨层云的影响比高层云更大。     

Evolution of bubble clouds induced by pulsed cavitational ultrasound therapy - histotripsy

Mechanical tissue fractionation can be achieved using successive, high-intensity ultrasound pulses in a process termed histotripsy. Histotripsy has many potential clinical applications where noninvasive tissue removal is desired. The primary mechanism for histotripsy is believed to be cavitation. Using fast-gated imaging, this paper studies the evolution of a cavitating bubble cloud induced by a histotripsy pulse (10 and 14 cycles) at peak negative pressures exceeding 21MPa. Bubble clouds are generated inside a gelatin phantom and at a tissue-water interface, representing two situations encountered clinically. In both environments, the imaging results show that the bubble clouds share the same evolutionary trend. The bubble cloud and individual bubbles in the cloud were generated by the first cycle of the pulse, grew with each cycle during the pulse, and continued to grow and collapsed several hundred microseconds after the pulse. For example, the bubbles started under 10 microm, grew to 50 microm during the pulse, and continued to grow 100 microm after the pulse. The results also suggest that the bubble clouds generated in the two environments differ in growth and collapse duration, void fraction, shape, and size. This study furthers our understanding of the dynamics of bubble clouds induced by histotripsy.     

Boreal forests, aerosols and the impacts on clouds and climate

Previous studies have concluded that boreal forests warm the climate because the cooling from storage of carbon in vegetation and soils is cancelled out by the warming due to the absorption of the Sun's heat by the dark forest canopy. However, these studies ignored the impacts of forests on atmospheric aerosol. We use a global atmospheric model to show that, through emission of organic vapours and the resulting condensational growth of newly formed particles, boreal forests double regional cloud condensation nuclei concentrations (from approx. 100 to approx. 200 cm(-3)). Using a simple radiative model, we estimate that the resulting change in cloud albedo causes a radiative forcing of between -1.8 and -6.7 W m(-2) of forest. This forcing may be sufficiently large to result in boreal forests having an overall cooling impact on climate. We propose that the combination of climate forcings related to boreal forests may result in an important global homeostasis. In cold climatic conditions, the snow-vegetation albedo effect dominates and boreal forests warm the climate, whereas in warmer climates they may emit sufficiently large amounts of organic vapour modifying cloud albedo and acting to cool climate.     

Physically based parameterizations of the short-wave radiative characteristics of weakly absorbing optically thick media: application to liquid-water clouds

We propose the physically based parameterization of the radiative characteristics of liquid-water clouds as functions of the wavelength, effective radius, and refractive index of particles, liquid-water path, ground albedo, and solar and observation angles. The formulas obtained are based on the approximate analytical solutions of the radiative transfer equation for optically thick, weakly absorbing layers and the geometrical optics approximation for local optical characteristics of cloud media. The accuracy of the approximate formulas was studied with an exact radiative transfer code. The relative error of the approximate formula for the reflection function at nadir observations was less then 15% for an optical thickness larger than 10 and a single-scattering albedo larger than 0.95.     

Integrating biomass, sulphate and sea-salt aerosol responses into a microphysical chemical parcel model: implications for climate studies

Aerosols are known to influence significantly the radiative budget of the Earth. Although the direct effect (whereby aerosols scatter and absorb solar and thermal infrared radiation) has a large perturbing influence on the radiation budget, the indirect effect (whereby aerosols modify the microphysical and hence the radiative properties and amounts of clouds) poses a greater challenge to climate modellers. This is because aerosols undergo chemical and physical changes while in the atmosphere, notably within clouds, and are removed largely by precipitation. The way in which aerosols are processed by clouds depends on the type, abundance and the mixing state of the aerosols concerned. A parametrization with sulphate and sea-salt aerosol has been successfully integrated within the Hadley Centre general circulation model (GCM). The results of this combined parametrization indicate a significantly reduced role, compared with previous estimates, for sulphate aerosol in cloud droplet nucleation and, consequently, in indirect radiative forcing. However, in this bicomponent system, the cloud droplet number concentration, N(d) (a crucial parameter that is used in GCMs for radiative transfer calculations), is a smoothly varying function of the sulphate aerosol loading. Apart from sea-salt and sulphate aerosol particles, biomass aerosol particles are also present widely in the troposphere. We find that biomass smoke can significantly perturb the activation and growth of both sulphate and sea-salt particles. For a fixed salt loading, N(d) increases linearly with modest increases in sulphate and smoke masses, but significant nonlinearities are observed at higher non-sea-salt mass loadings. This non-intuitive N(d) variation poses a fresh challenge to climate modellers.     

Approach to photorealistic halo simulations

A multiple-scattering Monte Carlo model that can produce near-photographic quality images is developed and used to simulate several dramatic halo displays. The model atmosphere contains an absorbing ozone layer plus two clear, molecular air layers with Rayleigh scattering surrounding a cloud layer and an atmospheric boundary layer with aerosol particles subject to Lorentz-Mie scattering. Halos are produced by right hexagonal or pyramidal crystals that reflect and refract according to geometric optics without diffraction, although "junk" crystals with a pronounced forward-scattering peak but no halo peaks may be included to simulate typical, faint halos. Model parameters include ozone height and content, surface and cloud pressure, cloud optical thickness, crystal shapes, orientations and abundances, atmospheric turbidity, aerosol radius, and albedo. Beams for each wavelength are sorted into small bins as halo beams if they have been scattered once only by a single crystal and otherwise as sky beams, which are smoothed and combined with the halo beams to produce images. Multiple scattering generally vitiates halos, but extremely rare halos, such as Kern's arc, can be produced if a significant fraction of crystals in optically thick clouds have identical shapes and are highly oriented. Albedo is a model by-product with potential value in climate studies.     

平面参数空间的实时三维点云配准方法

针对具有多平面结构的室内环境的三维定位和环境建模,提出了一种在平面参数空间进行配准的实时三维点云配准方法。该方法首先使用一种改进的三维霍夫变换算法快速提取点云中的平面特征,然后使用迭代算法在平面的参数空间中寻找最近平面,最后使用这些平面的对应关系来估计两帧点云之间的位姿变换关系。在一个实验室场景中进行的对比实验表明,该算法能够达到与传统迭代最近点(ICP)算法相似的精度,而且速度大大提升。在仅使用普通笔记本CPU的情况下即可实现实时的点云拼接。     

Classification of particle effective shape ratios in cirrus clouds based on the lidar depolarization ratio

A shape classification technique for cirrus clouds that could be applied to future spaceborne lidars is presented. A ray-tracing code has been developed to simulate backscattered and depolarized lidar signals from cirrus clouds made of hexagonal-based crystals with various compositions and optical depth, taking into account multiple scattering. This code was used first to study the sensitivity of the linear depolarization rate to cloud optical and microphysical properties, then to classify particle shapes in cirrus clouds based on depolarization ratio measurements. As an example this technique has been applied to lidar measurements from 15 mid-latitude cirrus cloud cases taken in Palaiseau, France. Results show a majority of near-unity shape ratios as well as a strong correlation between shape ratios and temperature: The lowest temperatures lead to high shape ratios. The application of this technique to space-borne measurements would allow a large-scale classification of shape ratios in cirrus clouds, leading to better knowledge of the vertical variability of shapes, their dependence on temperature, and the formation processes of clouds.     

Glory of clouds in the near infrared

Spectrally resolved visible and infrared images of marine stratus clouds were acquired from the NASA ER-2 high-altitude aircraft during the 1987 First International Cloud Climatology Program Regional Experiment. The images were obtained by cross-track scanning radiometers. Data images at nearinfrared wavelengths show frequent and readily apparent brightness features that are due to glory single scattering. The observations and subsequent analysis by radiative transfer calculations show that the glory is a significant feature of near-infrared solar reflectance from water clouds. Glory observations and calculations based on in-cloud microphysics measurements agree well. The most dramatic difference from the visible glory is that the scattering angles are significantly larger in the near infrared. The glory is also apparently more distinct in the near infrared than in the visible, as scattering size parameters are in a range that effectively produces a glory feature, and also there is less obscuration bymultipe-scattering reflectance because of absorption of radiation by droplets in the near infrared. For both the visible and the near infrared, the principal factors that wash out the glory are dispersion and, to a lesser degree, the effective radius of the cloud droplet-size distribution. The obscuration by multiple scattering in optically thick clouds is secondary. Rather than being a novelty, glory observations would be an accurate and unambiguous technique to sense the droplet size of water clouds remotely.     

Multipurpose spectral imager

A small spectral imaging system is presented that images static or moving objects simultaneously as a function of wavelength. The main physical principle is outlined and demonstrated. The instrument is capable of resolving both spectral and spatial information from targets throughout the entire visible region. The spectral domain has a bandpass of 12 A. One can achieve the spatial domain by rotating the system's front mirror with a high-resolution stepper motor. The spatial resolution range from millimeters to several meters depends mainly on the front optics used and whether the target is fixed (static) or movable relative to the instrument. Different applications and examples are explored, including outdoor landscapes, industrial fish-related targets, and ground-level objects observed in the more traditional way from an airborne carrier (remote sensing). Through the examples, we found that the instrument correctly classifies whether a shrimp is peeled and whether it can disclose the spectral and spatial microcharacteristics of targets such as a fish nematode (parasite). In the macroregime, we were able to distinguish a marine vessel from the surrounding sea and sky. A study of the directional spectral albedo from clouds, mountains, snow cover, and vegetation has also been included. With the airborne experiment, the imager successfully classified snow cover, leads, and new and rafted ice, as seen from 10.000 ft (3.048 m).     

Observation of Raman scattering by cloud droplets in the atmosphere

In a recent field campaign, the NASA Goddard Space Flight Center scanning Raman lidar measured, in the water vapor channel, Raman scattering from low-level clouds well in excess of 100% relative humidity. The excess scattering has been interpreted to be spontaneous Raman scattering by liquid water in the cloud droplets. A review of research on Raman scattering by microspheres indicates that the technique may provide a remote method to observe cloud liquid water. The clouds studied appear, from Mie scattering, to have two distinct layers with only the upper layer showing significant Raman scattering from liquid water in the droplets.     

Studies on Low Altitude Clouds Over New Delhi,India Using Lidar

This study reports the altitude distribution of physical and optical properties of clouds in the lower troposphere over the urban tropical region Delhi using an UV (355 nm) lidar which is capable of operating in both day and night time. Most of the low altitude clouds are observed above the planetary boundary layer during the observation period. The low altitude cloud bottom and top height varies between 0.58 ± 0.21 and 1.5 ± 0.61 km respectively during the observation period. The depolarization ratio of the observed clouds varies from 0.18 ± 0.01 to 1.2 ± 0.58. The role of the atmospheric region below the cloud in the growth process of the cloud cell is studied. Cloud turbulence is derived to show its role in maintaining the strength of the cloud.     

Error analysis of Raman differential absorption lidar ozone measurements in ice clouds

A formalism for the error treatment of lidar ozone measurements with the Raman differential absorption lidar technique is presented. In the presence of clouds wavelength-dependent multiple scattering and cloud-particle extinction are the main sources of systematic errors in ozone measurements and necessitate a correction of the measured ozone profiles. Model calculations are performed to describe the influence of cirrus and polar stratospheric clouds on the ozone. It is found that it is sufficient to account for cloud-particle scattering and Rayleigh scattering in and above the cloud; boundary-layer aerosols and the atmospheric column below the cloud can be neglected for the ozone correction. Furthermore, if the extinction coefficient of the cloud is ?0.1 km(-1), the effect in the cloud is proportional to the effective particle extinction and to a particle correction function determined in the limit of negligible molecular scattering. The particle correction function depends on the scattering behavior of the cloud particles, the cloud geometric structure, and the lidar system parameters. Because of the differential extinction of light that has undergone one or more small-angle scattering processes within the cloud, the cloud effect on ozone extends to altitudes above the cloud. The various influencing parameters imply that the particle-related ozone correction has to be calculated for each individual measurement. Examples of ozone measurements in cirrus clouds are discussed.     

Homomorphism between cloudy and clear spectral radiance in the 800-900-cm(-1) atmospheric window region

The sensitivity of a new algorithm for cloud detection over a sea surface has been assessed on the basis of extensive simulations of clear and cloudy radiance spectra, including water and ice and low- and high-altitude clouds. The new algorithm makes use of autocorrelation and cross correlation between an observed spectrum and either a synthetic or a laboratory spectrum and can be used to determine quantitatively the degree of homogeneity of two spectra in the 800-900-cm(-1) region (11.11-12.5 microm). The scheme is intended for high-spectral-resolution observations and could form the basis for an operational stand-alone cloud-detection algorithm for next-generation sounding spectrometers. Application of the scheme to real observations is presented and discussed.     

Shallow layer simulation of heavy gas released on a slope in a calm ambient. Part I. Continuous releases

Although much research considers heavy gas dispersion over flat ground, less is known about the physics of dense gas dispersion on a slope. Here, the appropriateness of shallow layer models for the simple case of releases over a slope in a calm ambient is assessed. This two-part paper assesses the value of shallow layer modelling using the established shallow layer model TWODEE [J. Hazard. Mater. 66 (3) (1999) 211; J. Hazard. Mater. 66 (3) (1999) 227; J. Hazard. Mater. 66 (3) (1999) 239] and the experimental results of Schatzmann et al. [M. Schatzmann, K. Marotzke, J. Donat, Research on continuous and instantaneous heavy gas clouds, contribution of sub-project EV 4T-0021-D to the final report of the joint CEC project, Technical Report, Meteorological Institute, University of Hamburg, February 1991]. Part I considers continuous releases, and part II considers instantaneous releases; both use the same model with the same entrainment coefficients. For continuous releases, cloud arrival times are generally well predicted, and cloud concentrations are generally correct to within a factor of two. Shallow layer models thus appear to be capable of physically accurate simulation of continuous releases over a slope in a calm ambient.     

Extinction efficiency in the infrared (2-18 µm) of laboratory ice clouds: observations of scattering minima in the Christiansen bands of ice

Extinction measurements with a laser diode (0.685 μm) and a Fourier transform infrared spectrometer (2-18 μm) were performed on laboratory ice clouds (5 μm ≤ D ≤ 70 μm) grown at a variety of temperatures, and thus at a variety of crystal habits and average projected crystal area. Ice clouds were grown by nucleation of a supercooled water droplet cloud with a rod cooled with liquid nitrogen. The ice crystals observed were mainly plates and dendrites at the coldest temperatures (≈-15 °C) and were mainly columns and needles at warmer temperatures (≈-5 °C). The crystals were imaged with both a novel microscope equipped with a video camera and a heated glass slide and a continuously running Formvar replicator. The IR spectral optical-depth measurements reveal a narrow (0.5-μm-width) extinction minimum at 2.84 μm and a wider (3-μm-width) minimum at 10.5 μm. These partial windows are associated with wavelengths where the real part of the index of refraction for bulk ice has a relative minimum so that extinction is primarily due to absorption rather than scattering (i.e., the Christiansen effect). Bulk ice has absorption maxima near the window wavelengths. IR extinction efficiency has a noticeable wavelength dependence on the average projected crystal area and therefore on the temperaturedependent crystal properties. The average-size parameters in the visible for different temperatures ranged from 64 to 128, and in the IR they ranged from 2.5 to 44. The extinction efficiency and the single-scatter albedo for ice spheres as computed from Mie scattering also show evidence of the Christiansen effect.     

Multiple-scattering lidar retrieval method: tests on Monte Carlo simulations and comparisons with in situ measurements

A multiple-field-of-view (MFOV) lidar measurement and solution technique has been developed to exploit the retrievable particle extinction and size information contained in the multiple-scattering contributions to aerosol lidar returns. We describe the proposed solution algorithm. The primary retrieved parameters are the extinction coefficient at the lidar wavelength and the effective particle diameter from which secondary products such as the extinction at other wavelengths and the liquid-water content (LWC) of liquid-phase clouds can be derived. The solutions are compared with true values in a series of Monte Carlo simulations and with in-cloud measurements. Good agreement is obtained for the simulations. For the field experiment, the retrieved effective droplet diameter and LWC for the available seven cases studied are on average 15% and 35% (worst case) smaller than the measured data, respectively. In the latter case, the analysis shows that the differences cannot be attributed solely to lidar inversion errors. Despite the limited penetration depth (150-300 m) of the lidar pulses, the results of the studied cases indicate that the retrieved lidar solutions remain statistically representative of measurements performed over the full cloud extent. Long-term MFOV lidar monitoring could thus become a practical and economical option for cloud statistical studies but more experimentation on more varied cloud conditions, especially for LWC, is still needed.