PWR（U）乏燃料中超铀元素在混合堆快裂变包层内嬗变研究

从中子学角度对ＰＷＲ（Ｕ）乏燃料中的超铀元素（２３８Ｐｕ，２３９Ｐｕ，２４１Ｐｕ，２４１Ａｍ，２４３Ａｍ，２３７Ｎｐ，２４４Ｃｍ）在聚变－裂变混合堆快裂变包层内嬗变的可行性进了研究。利用一维中子输运和燃耗计算程序ＢＩＤＥＣＡＹ译不同燃料组分的四个快裂变包层进行分析计算。结果表明，在聚变－裂变混合堆快裂变包层内安全，高效地嬗变ＰＷＲ（Ｕ）乏燃料中的超铀元素是可能的。     

聚变-裂变混合能源堆一维计算模型燃耗分析

聚变-裂变混合能源堆包括聚变中子源和以天然铀为燃料、水为冷却剂的次临界包层,主要目标是生产电力。利用输运燃耗耦合程序系统MCORGS计算了混合能源堆一维模型的燃耗,给出了中子有效增殖因数k_eff、能量放大倍数M、氚增殖比TBR等物理量随时间的变化。通过分析能谱和重要核素随燃耗时间的变化,说明混合能源堆与核燃料增殖、核废料嬗变混合堆的不同特点。本文给出的结果可作为混合堆中子输运、燃耗分析程序校验的参考数据,为混合堆概念研究提供了基础数据。     

氦气、水和熔盐冷却的混合堆中子学性能研究

氦气、水、熔盐(Flibe)在强磁场中流动不存在严重的MHD问题,因此适合在基于磁约束的聚变-裂变混合堆中作为冷却剂.针对氦气、水、Flibe这3种冷却剂对混合堆包层中子学性能的影响进行研究,分析包层中能谱特点及燃料增殖特性.通过燃耗计算,研究氚增殖率(TBR)、能量倍增因子(M)、keff等随运行时间的变化.中子学输运采用三维蒙特卡罗程序MCNP.计算结果表明,不同的冷却剂对混合堆系统中子能谱影响很大:氦冷系统的能谱最硬,主要发生快中子裂变,氚增殖效果最好;水冷系统的能谱最软,产能最多,但需提高TBR;Flibe冷系统的能谱较硬,产能最少.     

功率展平的压水堆乏燃料发电包层中子学初步研究

聚变裂变混合堆在增殖核燃料、嬗变长寿命核废料及固有安全性等方面具有较大优势,同时,它比纯聚变堆在工程及技术方面要求低,因此较聚变堆更易实现。本工作基于目前国际聚变实验堆（ITER）所能达到的技术水平,提出一种直接利用乏燃料进行发电的聚变裂变混合堆包层概念,利用在不同位置放置不同乏燃料体积分数的方法对燃料增殖区实现了功率展平。计算结果表明：功率展平后的包层功率不均匀系数更小,且包层中燃料区的能量输出要比不展平情况下的能量输出高约21.7%。燃料富集度到运行末期最大可达5.23%。从中子学角度初步论证了该包层的可行性。     

聚变裂变混合发电堆水冷包层中子学设计分析

主要针对聚变裂变混合发电堆FDS-EM水冷包层的能量倍增因子M和氚增殖率TBR等中子学参数进行优化计算。FDS-EM包层主要设计目标是在氚自持的基础上获得约1 GW的电功率,并且尽可能长时间连续运行不换料。通过初步设计分析给出一个使用核废料(压水堆卸出的废料钚、锕系加上贫铀)作为裂变燃料,能够实现氚自持、能量倍增因子约为90等设计目标,且连续运行至少10年不换料的中子学方案。     

聚变-裂变混合能源堆球模型参数敏感性分析

在聚变-裂变混合能源堆球模型基础上,使用蒙特卡罗方法中子学程序对中子源、铀水体积比、产氚区等相关参数进行了中子学的敏感性计算。分析了各参数对混合能源堆能量放大倍数M和氚增殖比TBR的影响,并总结其基本规律,为开展进一步的混合能源堆概念设计提供了重要参考。     

利用D-T聚变中子源转化长寿命裂变产物的中子学可行性研究

从中子学角度研究长寿命裂变产物在Tokamak型D-T聚变堆包层中转化的可行性.提出了用可裂变Pu增殖中子的混合包层转化方案,研制了相应的燃耗计算程序及数据库,并对所提方案进行了计算和分析.结果表明,在可预见的聚变堆芯技术条件下,所研究的概念性包层可对长寿命裂变产物进行有效转化.     

球床包层聚变—裂变混合堆热工安全分析

球床包层混合堆与板状元件包层混合堆相比较，前者在核燃料生产和安全方面可能具有更多的优越性。本应用ＴＨＥＲＭＩＸ程序和辅助程序对我国开发的托卡马克堆芯氮气冷却球床包层聚变－裂变合堆的包层进行了热工计算。计算中考虑了不同的燃料球材料及稳态，卸压和断流事故工况。计算结果表明，只要选用合适的燃料球材料和设置适当的控制保护系统，具有快速卸料罐的托卡马克堆芯氦气包层聚变－裂变混合堆的概念设计在安全上的可行的。     

聚变-裂变混合堆外中子源效应

聚变-裂变混合堆(FFHR)作为聚变驱动次临界系统(FDS),具有良好的物理性能,能够实现产能、氚增殖、嬗变核废料等功能。采用COUPLE程序研究了水冷混合堆包层的铀水比和中子倍增剂对中子源效率的影响。结果表明:包层能谱越硬,外中子源效率越高;适当加入中子倍增剂Be可使外中子源效率增加。研究结果对进一步改进聚变-裂变混合堆的概念设计具有一定的指导意义。     

混合堆增殖乏燃料组件中子学特性初步研究

本文主要对聚变-裂变混合堆增殖乏燃料在压水堆组件中使用的可能性进行了初步研究。根据聚变 裂变混合堆增殖乏燃料的特点,给出了的聚变-裂变混合堆增殖乏燃料压水堆组件设计方案,分析组件的燃料温度系数、慢化剂温度系数等参数。结果表明：聚变 裂变混合堆乏燃料组件的特性与全铀组件的特性相似。在相同的易裂变同位素质量百分比情况下,本文给出的组件设计方案的功率不均匀系数更小。研究结果可为未来实现聚变 裂变混合堆和压水堆联合循环系统提供技术支持。     

Numerical Study on Effects of Fuel Mixture Fraction and Li-6 Enrichment on Neutronic Parameters of a Fusion–Fission Hybrid Reactor

This study presents the effects of mixture fractions of nuclear fuels (mixture of fissile–fertile fuels and mixture of two different fertile fuels) and ⁶Li enrichment on the neutronic parameters (the tritium breeding ratio, TBR, the fission rate, FR, the energy multiplication ratio, M, the fissile breeding rate, FBR, the neutron leakage out of blanket, L, and the peak-to-average fission power density ratio, Γ) of a deuterium–tritium (D–T) fusion neutron-driven hybrid blanket. Three different fertile fuels (²³²Th, ²³⁸U and ²⁴⁴Cm), and one fissile fuel (²³⁵U) were selected as the nuclear fuel. Two different coolants (pressurized helium and natural lithium) were used for the nuclear heat transfer out of the fuel zone (FZ). The Boltzmann transport equation was solved numerically for obtaining the neutronic parameters with the help of the neutron transport code XSDRNPM/SCALE4.4a. In addition, these calculations were performed by also using the MCNP4B code. The sub-limits of the mixture fractions and ⁶Li enrichment were determined for the tritium self-sufficiency. The considered hybrid reactor can be operated in a self-sufficiency mode in the cases with the fuel mixtures mixed with a fraction of equal to or greater than these sub-limits. Furthermore, the numerical results show that the fissile fuel breeding and fission potentials of the blankets with the helium coolant are higher than with the lithium coolant.     

Effect of Nuclear Data Libraries on Tritium Breeding in a (D–T) Fusion Driven Reactor

In design a Deuterium–Tritium (D–T) fusion driven hybrid reactor, neutronics and nuclear data libraries have an essential role for reliable neutronics calculations. Therefore, nuclear data libraries are very important to calculate of the neutronic parameters and selection of tritium breeder materials to be used in the blanket. In this study tritium breeding performances of candidate tritium breeding materials, namely, Li₂O, LiH, Li₂TiO₃, Li₂ZrO₃ and Li₄SiO₄ in a (D–T) driven fusion–fission (hybrid) reactor is investigated based on three dimensional (3-D) and one dimensional (1-D) neutronic calculations. 3-D and 1-D neutron transport calculations are performed with Monte Carlo transport code (MCNP 4C), SCALE 5 and ANISN nuclear data codes to determine the tritium breeding ratio (TBR) of the blanket. The effects of different nuclear data libraries on TBR are examined and TBR calculation results are comparatively investigated.     

Temperature distribution in mixed ThO2–UO2 fuel rods located in blanket of an inertial fusion energy breeder

Investigations of neutronic analysis and temperature distribution in fuel rods located in a blanket driven ICF (Inertial Confinement Fusion) have been performed for various mixed fuels and coolants under a first wall load of 5 MW/m². The fuel rods containing ThO₂ and UO₂ mixed by various mixing methods for achieving a flat fission power density are replaced in the blanket and cooled with different coolants; natural lithium, flibe, eutectic lithium and helium for the nuclear heat transfer. It is assumed that surface temperature of the fuel rod increases linearly from 500 °C (at top) to 700 °C (at bottom) during cooling fuel zone. Neutronic and temperature distribution calculations have been performed by MCNP4B Code and HEATING7, respectively. In the blanket fueled with pure UO₂ and cooled with helium, M (fusion energy multiplication ratio) increases to 3.9 due to uranium having higher fission cross-section than thorium. The high fission energy released in this blanket, therefore, causes proportionally increasing of temperature in the fuel rods to 823 °C. However, the M is 2.00 in the blanket fueled with pure ThO₂ and cooled with eutectic lithium because of more capture reaction than fission reaction. Maximum and minumum values of TBR (tritium breeding ratio) being one of main neutronic paremeters for a fusion reactor are 1.07 and 1.45 in the helium and the natural lithium coolant blanket, respectively. These consequences bring out that the investigated reactor can produce substantial electricity in situ during breeding fissile fuel and can be self-sufficient in the tritium required for the DT fusion driver in all cases of mixed fuels and coolant types. Quasi-constant fission power density profiles in FFB (fissile fuel breeding) zone are obtained by parabolically increasing mixture fraction of UO₂ in radial and axial directions for all coolant types. Such as, in the helium coolant blanket and the case of PMF (parabolically mixed fuel), Γ (peek-to-average fission power density ratio) of the blanket is reduced to 1.1, and the maximum temperatures of the fuel rods in radial direction of the FFB zone are also quasi-constant. At the same time, in the case of PMF, for all coolant types, the temperature profiles in the radial direction of the fuel rods rise proportionally with surface temperature from the top to the bottom of fuel rods in the axial direction. In other words, for each radial temperature profile in the axial direction, temperature differences between centerline and surface of the fuel rods are quasi-constant. According to the coolant types, these temperature diffences vary between 30 and 45 °C.     

Effects of lithium burn-up on TBR in DEMO reactor SlimCS

Lithium in a breeding blanket is burned up through neutron nuclear reactions in fusion DEMO reactors. Effects of decrease of solid breeder materials due to lithium burn-up on tritium breeding ratio (TBR) are not systematically calculated in the past. For the SlimCS blanket design, TBR is calculated taking into account the lithium burn-ups by one dimensional Sn radiation transport calculation code ANISN in this study. The ⁶Li burn-ups are 8–79% after 10-year operation. TBR due to ⁶Li decreases to 40% of the initial one in some layer, while it increases in some layers. The TBR integrated over all the blanket decreases to around 96% of the initial one. The study makes it clear that the reduction of the TBR due to the lithium burn-up is not so large.     

Integral neutronics experiments in analytical mockups for blanket of a hybrid reactor

The paper describes recent progress in integral neutronics experiments in the analytical mockups for the blanket in a fusion-fission hybrid energy reactor. A conceptual blanket of the hybrid reactor is mainly loaded with natural uranium and lithium material. In the fission fuel region, uranium material and light water are arranged alternately. The mockups of the conceptual blanket are designed and used for checking neutron property of the blanket by integral experiments. Based on materials available, the spherical fission mockup for fission research and plutonium production consists of three layers of depleted uranium shells and several layers of polyethylene and graphite shells. The spherical lithium mockup for tritium production consists of depleted uranium and LiPb alloy shells. The cubic mockup consists of natural uranium and polyethylene and its structure is basically consistent with one of the fuel region. In the mockups with the D-T neutron source, the plutonium production rates, uranium fission rates and tritium production rates are measured, separately. The measured results are compared to the calculated ones with MCNP-4B code and ENDF/B-VI library data.     

Neutronic performance of new coolants in a fusion–fission (hybrid) reactor

Selection of coolant used in the fuel zone of a fusion–fission (hybrid) reactor affects the neutronic performance of the blanket much. Recently, two coolants namely, Flinabe and Li₂₀Sn₈₀ have been investigated to use in fusion reactors as tritium breeder and energy carrier due to their advantages of low melting point, low vapor pressure. In this study, neutronic performance of these coolants in a hybrid reactor using Canada Deuterium Uranium Reactor (CANDU) spent fuel was investigated for an operation period of 48 months. And also that of natural lithium and Flibe was also examined for comparison. Neutron transport calculations were conducted on a simple experimental hybrid blanket in a cylindrical geometry with the help of the SCALE4.3 system by solving the Boltzmann transport equation with the XSDRNPM code in 238 neutron groups and a S₈–P₃ approximation.     

Rejuvenation of spent fuel in the force-free helical reactor (FFHR)

This study considers spent fuel rejuvenation potential of the force-free helical reactor (FFHR), which is a relevant heliotron-type D-T fusion reactor. For this purpose, three different spent fuels were selected, i.e.: (1) CANDU, (2) PWR-UO₂, and (3) PWR-MOX spent fuels. The spent fuel (volume fraction of 60%), spherically prepared and cladded with SiC (volume fraction of 10%), was located in the fuel zone (FZ) in the blanket of the FFHR. The FZ was cooled with high-pressured helium gas (volume fraction of 30%) for the nuclear heat transfer. The neutronic calculations were performed by solving the Boltzmann transport equation with the help of the neutron transport code XSDRNPM-S/SCALE4.3. The calculations of the time dependent atomic densities of the isotopes were performed for an operation period (OP) of up to 4 years by 75% plant factor (η) under a first-wall neutron load (P) of 1.5 MW/m². The temporal variations of the atomic densities of the isotopes in the spent fuel composition and other physical parameters were calculated for a discrete time interval (Δt) of 1/12 year (one month), by using the interface program (code). In all investigated spent fuel cases, the tritium self-sufficiency is maintained for DT fusion driver along the OP. The CANDU spent fuel becomes usable in a conventional CANDU reactor after a regeneration time of ∼6 months. The CFFE value approaches 3.5% in the blanket fuelled with the PWR-UO₂ and -MOX spent fuels after 40 and 34 months, respectively. The plutonium component can never reach a nuclear weapon grade quality during spent fuel rejuvenation. Consequently, the blanket has high neutronic performance for the rejuvenation of the spent fuels.     

Neutronic analysis of an inertial fusion energy breeder with SiCf/SiC

Neutronic performance of a blanket driven ICF (Inertial confinement fusion) neutron based on SiC_f/SiC composite material is investigated for fissile fuel breeding. The investigated blanket is fueled with ThO₂ and cooled with natural lithium or (LiF)₂BeF₂ or Li₁₇Pb₈₃ or ⁴He coolant. MCNP4B Code is used for calculations of neutronic data per DT neutron. Calculations have show that values of TBR (tritium breeding ratio) being one of the main neutronic paremeters of fusion reactors are greater than 1.05 in all type of coolant, and the breeder hybrid reactor is self-sufficient in the tritium required for the DT fusion driver. Calculations show that natural lithium coolant blanket has the highest TBR (1.298) and M (fusion energy multiplication) (2.235), Li₁₇Pb₈₃ coolant blanket has the highest FFBR (fissile fuel breeding ratio) (0.3489) and NNM (net neutron multiplication) (1.6337). ⁴He coolant blanket has also the best Γ (peek-to-average fission power density ratio) (1.711). Values of neutron leakage out of the blanket in all type of coolants are quite low due to SiC reflector and B₄C shielding.     

Analysis of Time-Dependent Tritium Breeding Capability of Water Cooled Ceramic Breeder Blanket for CFETR

Attaining tritium self-sufficiency is an important mission for the Chinese Fusion Engineering Testing Reactor(CFETR) operating on a Deuterium-Tritium(D-T) fuel cycle. It is necessary to study the tritium breeding ratio(TBR) and breeding tritium inventory variation with operation time so as to provide an accurate data for dynamic modeling and analysis of the tritium fuel cycle. A water cooled ceramic breeder(WCCB) blanket is one candidate of blanket concepts for the CFETR. Based on the detailed 3D neutronics model of CFETR with the WCCB blanket,the time-dependent TBR and tritium surplus were evaluated by a coupling calculation of the Monte Carlo N-Particle Transport Code(MCNP) and the fusion activation code FISPACT-2007.The results indicated that the TBR and tritium surplus of the WCCB blanket were a function of operation time and fusion power due to the Li consumption in breeder and material activation.In addition, by comparison with the results calculated by using the 3D neutronics model and employing the transfer factor constant from 1D to 3D, it is noted that 1D analysis leads to an over-estimation for the time-dependent tritium breeding capability when fusion power is larger than 1000 MW.