Wall-loss distribution of charge breeding ions in an electron cyclotron resonance ion source

The ion loss distribution in an electron cyclotron resonance ion source (ECRIS) was investigated to understand the element dependence of the charge breeding efficiency in an electron cyclotron resonance (ECR) charge breeder. The radioactive (111)In(1+) and (140)Xe(1+) ions (typical nonvolatile and volatile elements, respectively) were injected into the ECR charge breeder at the Tokai Radioactive Ion Accelerator Complex to breed their charge states. Their respective residual activities on the sidewall of the cylindrical plasma chamber of the source were measured after charge breeding as functions of the azimuthal angle and longitudinal position and two-dimensional distributions of ions lost during charge breeding in the ECRIS were obtained. These distributions had different azimuthal symmetries. The origins of these different azimuthal symmetries are qualitatively discussed by analyzing the differences and similarities in the observed wall-loss patterns. The implications for improving the charge breeding efficiencies of nonvolatile elements in ECR charge breeders are described. The similarities represent universal ion loss characteristics in an ECR charge breeder, which are different from the loss patterns of electrons on the ECRIS wall.     

Charge breeding results and future prospects with electron cyclotron resonance ion source and electron beam ion source (invited)

The Californium Rare Ion Breeder Upgrade (CARIBU) of the Argonne National Laboratory ATLAS facility will provide low-energy and reaccelerated neutron-rich radioactive beams for the nuclear physics program. A 70 mCi (252)Cf source produces fission fragments which are thermalized and collected by a helium gas catcher into a low-energy particle beam with a charge of 1+ or 2+. An electron cyclotron resonance (ECR) ion source functions as a charge breeder in order to raise the ion charge sufficiently for acceleration in the ATLAS linac. The final CARIBU configuration will utilize a 1 Ci (252)Cf source to produce radioactive beams with intensities up to 10(6) ions∕s for use in the ATLAS facility. The ECR charge breeder has been tested with stable beam injection and has achieved charge breeding efficiencies of 3.6% for (23)Na(8+), 15.6% for (84)Kr(17+), and 13.7% for (85)Rb(19+) with typical breeding times of 10 ms∕charge state. For the first radioactive beams, a charge breeding efficiency of 11.7% has been achieved for (143)Cs(27+) and 14.7% for (143)Ba(27+). The project has been commissioned with a radioactive beam of (143)Ba(27+) accelerated to 6.1 MeV∕u. In order to take advantage of its lower residual contamination, an EBIS charge breeder will replace the ECR charge breeder in the next two years. The advantages and disadvantages of the two techniques are compared taking into account the requirements of the next generation radioactive beam facilities.     

Beam injection improvement for electron cyclotron resonance charge breeders

The injection of a 1+ beam into an electron cyclotron resonance (ECR) charge breeder is classically performed through a grounded tube placed on its axis at the injection side. This tube presents various disadvantages for the operation of an ECR charge breeder. First experiments without a grounded tube show a better use of the microwave power and a better charge breeding efficiency. The optical acceptance of the charge breeder without decelerating tube allows the injection of high intensity 1+ ion beams at high energy, allowing metals sputtering inside the ion source. The use of this method for refractory metallic ion beams production is evaluated.     

Ion beam capture and charge breeding in electron cyclotron resonance ion source plasmas

Beam capture of injected ions and charge breeding in electron cyclotron resonance (ECR) charge breeder ion source plasmas has been investigated utilizing an ECR plasma modeling code, the generalized ECR ion source model, and a Monte Carlo beam capture code. Beam capturing dynamics, charge breeding in the plasma, and the extracted charged ion states are described. Optimization of ion beam energy is performed for (1) high beam capture efficiency and (2) high charge state ion beam extractions. A sample case study for ANL-ECR has been performed. Ions entering ECR ion source plasma are slowed down mostly by the background ions. Assuming Maxwellian plasma ions, maximum beam energy loss occurs when the beam velocity is around the background thermal velocity in magnitude. It is also found that beam capture location affects charge state distribution. For instance, with a majority of beam ions captured near the middle of the device higher currents for higher charge states are obtained. The beam ions captured near the entry have a higher probability of backstreaming after they are captured. For this reason, the optimum beam energy of the injected Ar(+) beam ions for charge breeding is generally higher than the optimum input beam energy for maximum beam energy loss.     

Development of electron beam ion source charge breeder for rare isotopes at Californium Rare Isotope Breeder Upgrade

Recently, the Californium Rare Isotope Breeder Upgrade (CARIBU) to the Argonne Tandem Linac Accelerator System (ATLAS) was commissioned and became available for production of rare isotopes. Currently, an electron cyclotron resonance ion source is used as a charge breeder for CARIBU beams. To further increase the intensity and improve the purity of neutron-rich ion beams accelerated by ATLAS, we are developing a high-efficiency charge breeder for CARIBU based on an electron beam ion source (EBIS). The CARIBU EBIS charge breeder will utilize the state-of-the-art EBIS technology recently developed at Brookhaven National Laboratory (BNL). The electron beam current density in the CARIBU EBIS trap will be significantly higher than that in existing operational charge-state breeders based on the EBIS concept. The design of the CARIBU EBIS charge breeder is nearly complete. Long-lead components of the EBIS such as a 6-T superconducting solenoid and an electron gun have been ordered with the delivery schedule in the fall of 2011. Measurements of expected breeding efficiency using the BNL Test EBIS have been performed using a Cs(+) surface ionization ion source for external injection in pulsed mode. In these experiments we have achieved ～70% injection∕extraction efficiency and breeding efficiency into the most abundant charge state of ～17%.     

Performance and operation of advanced superconducting electron cyclotron resonance ion source SECRAL at 24 GHz

SECRAL (superconducting ECR ion source with advanced design in Lanzhou) ion source has been in routine operation for Heavy Ion Research Facility in Lanzhou (HIRFL) accelerator complex since May 2007. To further enhance the SECRAL performance in order to satisfy the increasing demand for intensive highly charged ion beams, 3-5 kW high power 24 GHz single frequency and 24 GHz +18 GHz double frequency with an aluminum plasma chamber were tested, and some exciting results were produced with quite a few new record highly charged ion beam intensities, such as (129)Xe(35+) of 64 eμA, (129)Xe(42+) of 3 eμA, (209)Bi(41+) of 50 eμA, (209)Bi(50+) of 4.3 eμA and (209)Bi(54+) of 0.2 eμA. In most cases SECRAL is operated at 18 GHz to deliver highly charged heavy ion beams for the HIRFL accelerator, only for those very high charge states and very heavy ion beams such as (209)Bi(36+) and (209)Bi(41+), SECRAL has been operated at 24 GHz. The total operation beam time provided by SECRAL up to July 2011 has exceeded 7720 hours. In this paper, the latest performance, development, and operation status of SECRAL ion source are presented. The latest results and reliable long-term operation for the HIRFL accelerator have demonstrated that SECRAL performance for production of highly charged heavy ion beams remains improving at higher RF power with optimized tuning.     

Liquid metal alloy ion source based metal ion injection into a room-temperature electron beam ion source

We have carried out a series of measurements demonstrating the feasibility of using the Dresden electron beam ion source (EBIS)-A, a table-top sized, permanent magnet technology based electron beam ion source, as a charge breeder. Low charged gold ions from an AuGe liquid metal alloy ion source were injected into the EBIS and re-extracted as highly charged ions, thereby producing charge states as high as Au(60 +). The setup, the charge breeding technique, breeding efficiencies as well as acceptance and emittance studies are presented.     

Performance of the Argonne National Laboratory electron cyclotron resonance charge breeder

An electron cyclotron resonance charge breeder for the Californium rare ion breeder upgrade (CARIBU), a new radioactive beam facility for the Argonne Tandem Linac Accelerator System (ATLAS), has been constructed and commissioned. Charge breeding efficiencies up to 15.6% have been realized for stable beams with a typical breeding time of 10 ms∕charge state. The CARIBU system has been undergoing commissioning tests utilizing a 100 mCi (252)Cf fission source. A charge breeding efficiency of 14.8 ± 5% has been achieved for the first radioactive beam of (143)Cs(27+).     

Design of a compact electron cyclotron resonance ion source for medium charge state light ions

At the Australian Nuclear Science and Technology Organization we are developing a new isotope ratio mass spectrometer based on the measurement of multiple charge state ions. We have carried out a review of our existing ECR ion source and identified a number of design flaws. For the new instrument, we are producing a new ECR source and have refined the design, in particular by using 3D simulations to improve the magnetic confinement field and by a combination of simulations and experiments to improve the design of the microwave coupling.     

Status and special features of the Atomki ECR ion source

The ECR ion source has been operating in ATOMKI (Debrecen) since 1996. During the past 15 years lots of minor and numerous major technical modifications have been carried out on the ECRIS. Many of these changes aimed the increasing of beams charge, intensity, and the widening of the ion choice. Another group of the modifications were performed to develop special, non-standard operation modes or to produce peculiar plasmas and beams.     

The on-line charge breeding program at TRIUMF's Ion Trap For Atomic and Nuclear Science for precision mass measurements

TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN) constitutes the only high precision mass measurement setup coupled to a rare isotope facility capable of increasing the charge state of short-lived nuclides prior to the actual mass determination in a Penning trap. Recent developments around TITAN's charge breeder, the electron beam ion trap, form the basis for several successful experiments on radioactive isotopes with half-lives as low as 65 ms and in charge states as high as 22+.     

Operation of the CAPRICE electron cyclotron resonance ion source applying frequency tuning and double frequency heating

The properties of the electromagnetic waves heating the electrons of the ECR ion sources (ECRIS) plasma affect the features of the extracted ion beams such as the emittance, the shape, and the current, in particular for higher charge states. The electron heating methods such as the frequency tuning effect and the double frequency heating are widely used for enhancing the performances of ECRIS or even for the routine operation during the beam production. In order to better investigate these effects the CAPRICE ECRIS has been operated using these techniques. The ion beam properties for highly charged ions have been measured with beam diagnostic tools. The reason of the observed variations of this performance can be related to the different electromagnetic field patterns, which are changing inside the plasma chamber when the frequency is varying.     

Experimental investigations of silicon tetrafluoride decomposition in ECR discharge plasma

The results of first experiments on the investigation of plasma of electron cyclotron resonance (ECR) discharge, sustained by CW radiation of technological gyrotron with frequency 24 GHz are considered. The parameters of nitrogen plasma of ECR discharge in magnetic field up to 1 T were investigated by Langmuir probe in the pressure range 10(-4)-10(-2) mbar under different values of microwave power. Depending on gas pressure and power of microwave radiation, the typical temperature and density of electrons could attain values of 1-5 eV and 10(11)-10(12) cm(-3), respectively. The prospects for using of ECR discharge for plasma chemical decomposition of silicon tetrafluoride (SiF(4)) have been experimentally demonstrated. Plasma was created from SiF(4) and hydrogen (H(2)) gas mixture and heated by microwave radiation in ECR conditions. Using the method of mass-spectrometry analysis of the gas at the outlet from the reactor and the weighting method, the content of the resultants of SiF(4) decomposition as a function of process parameters was investigated. It was shown that SiF(4) decomposition degree strongly depends on the microwave power, gas pressure in the reactor, gas flow rates, and can attain the value of 50%. The possible applications of PECVD method based on ECR discharge for production of isotopically pure elements with high deposition rate are discussed.     

Measurement of the high energy component of the x-ray spectra in the VENUS electron cyclotron resonance ion source

High performance electron cyclotron resonance (ECR) ion sources, such as VENUS (Versatile ECR for NUclear Science), produce large amounts of x-rays. By studying their energy spectra, conclusions can be drawn about the electron heating process and the electron confinement. In addition, the bremsstrahlung from the plasma chamber is partly absorbed by the cold mass of the superconducting magnet, adding an extra heat load to the cryostat. Germanium or NaI detectors are generally used for x-ray measurements. Due to the high x-ray flux from the source, the experimental setup to measure bremsstrahlung spectra from ECR ion sources is somewhat different from that for the traditional nuclear physics measurements these detectors are generally used for. In particular, the collimation and background shielding can be problematic. In this paper, we will discuss the experimental setup for such a measurement, the energy calibration and background reduction, the shielding of the detector, and collimation of the x-ray flux. We will present x-ray energy spectra and cryostat heating rates depending on various ion source parameters, such as confinement fields, minimum B-field, rf power, and heating frequency.     

Advanced light ion source extraction system for a new electron cyclotron resonance ion source geometry at Saclay

One of the main goal of intense light ion injector projects such as IPHI, IFMIF, or SPIRAL2, is to produce high current beams while keeping transverse emittance as low as possible. To prevent emittance growth induced in a dual solenoid low energy transfer line, its length has to be minimized. This can be performed with the advanced light ion source extraction system concept that we are developing: a new ECR 2.45 GHz type ion source based on the use of an additional low energy beam transport (LEBT) short length solenoid close to the extraction aperture to create the resonance in the plasma chamber. The geometry of the source has been considerably modified to allow easy maintenance of each component and to save space in front of the extraction. The source aims to be very flexible and to be able to extract high current ion beams at energy up to 100 kV. A specific experimental setup for this source is under installation on the BETSI test bench, to compare its performances with sources developed up to now in the laboratory, such as SILHI, IFMIF, or SPIRAL2 ECR sources. This original extraction source concept is presented, as well as electromagnetic simulations with OPERA-2D code. Ion beam extraction in space charge compensation regime with AXCEL, and beam dynamics simulation with SOLMAXP codes show the beam quality improvement at the end of the LEBT.     

Design of the injection beamline for the Californium Rare Isotope Breeder Upgrade electron beam ion source charge breeder

The design of the ion injection line connecting the electron beam ion source (EBIS) charge breeder and the Californium Rare Isotope Breeder Upgrade radio frequency quadrupole cooler-buncher at the Argonne Tandem Linear Accelerator System was investigated with particle tracking simulations. The injection line was configured to accommodate several differential pumping sections, individual optical components were optimized to minimize emittance growth, and the ion beam parameters were matched with the EBIS electron beam acceptance to minimize losses upon injection.     

The effect of the additive concentration in emulsions to the tribological behavior of a cold rolling tube under sliding contact

The industrial steel tube in the cold rolling processes under liquid lubrication was simulated in a recovered cutting machine to study the tribological performances of an emulsion with four different concentrations of an emulsifier. The test machine was equipped with a device to measure the electrical contact resistance (ECR) between the rubbing surfaces of a steel tube and a roller. The ECR readings were useful to identify the existence of a surface absorption layer (a boundary layer film) between the contact surfaces and thus to realize the tribological effects. The tribological properties, including the friction coefficient, the electrical contact resistance, the wear loss of the tube and the worn surface area, were evaluated at these emulsifier concentrations. The displacement energy and the spraying coefficients for these emulsifier concentrations were applicable to interpret their relationships with the wear loss of the steel tube. The measures of the ECR are found to have a tendency more related to the values of the friction coefficient. Stribeck curves were also established for four emulsions; they are useful for assisting in the explanation for why a high friction coefficient in some cases does not necessarily produce a high wear loss. They were also provided to investigate the effects of the emulsifier concentrations on the friction coefficients at various lubrication stages. The emulsion with a dilute ratio of 50:1 proved to be the optimum choice of the four emulsifier concentrations because it leads to the lowest friction coefficient, the smallest wear loss and the worn surface as to the test time of 60 minutes.     

The electron cyclotron resonance ion source with arc-shaped coils concept (invited)

The main limitation to further improve the performance of ECR ion sources is set by the magnet technology related to the multipole magnet field used for the closed minimum-B structure. The JYFL ion source group has sought different approaches to improve the strength of the minimum-B structure required for the production of highly charged ion beams. It was found out that such a configuration can be realized with arc shaped coils. The first prototype, electron cyclotron resonance ion source with arc-shaped coils (ARC-ECRIS), was constructed and tested at JYFL in 2006. It was confirmed that such an ion source can be used for the production of highly charged ion beams. Regardless of several cost-driven compromises such as extraction mirror ratio of 1.05-1.2, microwave frequency of 6.4 GHz, and beam line with limited capacity, Ar(4+) beam intensity of up to 2 μA was measured. Subsequent design study has shown that the ARC-ECRIS operating at the microwave frequency above 40 GHz could be constructed. This specific design would be based on NbTi-wires and it fulfills the experimental magnetic field scaling laws. In this article, the ARC-ECRIS concept and its potential applications will be described.     

The preliminary tests of the superconducting electron cyclotron resonance ion source DECRIS-SC2

A new compact version of the "liquid He-free" superconducting ECR ion source, to be used as an injector of highly charged heavy ions for the MC-400 cyclotron, is designed and built at the Flerov Laboratory of Nuclear Reactions in collaboration with the Laboratory of High Energy Physics of JINR. The axial magnetic field of the source is created by the superconducting magnet and the NdFeB hexapole is used for the radial plasma confinement. The microwave frequency of 14 GHz is used for ECR plasma heating. During the first tests, the source shows a good enough performance for the production of medium charge state ions. In this paper, we will present the design parameters and the preliminary results with gaseous ions.     

Multigan®: first experimental results

A new design of a multicharged ion source based on the MONO1000 ECRIS has been presented at the last ECR ion source (ECRIS) Workshop 2010. [L. Maunoury et al., in Proceedings of the XIXth International Workshop on ECR Ion Sources, Grenoble, France, 23-26 August 2010] This source has not only two opening at both ends but also a large space in the middle of the source enabling a direct contact with the ECR plasma. The source has been assembled mechanically and put on a test bench at the Pantechnik company. The primary tests have shown that the plasma ignition occurred at low pressure (10(-6) mbar) and low RF power (10 W). The first experimental results ( = 1.30 for Ar and 1.85 for Xe) demonstrated the potential of this ion source in production of multicharged ion beams.