Frequency locking of a 1324 nm DFB laser to an optically pumpedrubidium vapor

Some experimental results and a simple theoretical model on a dither-free frequency-locking technique of a DFB laser operating at 1324 nm are presented. A resonance observed through absorption in an ⁸⁷ Rb vapor optically pumped by a modulated 795-nm laser diode tuned to the D₁ line is used. This approach has the advantage of producing sub-Doppler resonances. Such a technique could be used to generate an unmodulated 1324-nm wavelength reference     

Frequency-locked,injection-seeded,pulsed narrowband optical parametric generator

A frequency-locked, injection-seeded, pulsed optical parametric generator (OPG) has been developed for short-range infrared differential absorption lidar (DIAL) applications. The periodically poled lithium niobate OPG is pumped by a passively Q-switched Nd:YAG microlaser and is seeded by a distributed feedback (DFB) diode laser. The OPG is designed for DIAL measurement of a narrow R-branch transition of methane at 3.2704 microm. The output of the OPG is a two-pulse sequence with a 100-micros temporal separation between the pulses, where the first pulse is absorbed by methane and the second pulse is not absorbed. The first pulse is actively locked to the methane absorption feature by use of the derivative of the transmission spectrum through a reference cell. Although the device was not optimized for output power, the 3.27-microm OPG output energies of the first and second pulses are 5.5 and 5.9 microJ, respectively, producing 21 mW when operated at 1818 Hz.     

Frequency stabilization of a diode laser with a thin Cs-vapor cell

We propose a novel method of stabilizing laser oscillation frequency that uses a sub-Doppler spectrum of atoms in a thin vapor cell. An extended-cavity diode laser is frequency-locked to a hyperfine component of the Cs-D(2) line. In the Allan-variance measurements on the beat note between two lasers thus stabilized, a frequency stability of 6.6x10(-11) is achieved at an averaging time of 5.8 s. The frequency can be controlled even when the laser beam intensity is as small as 70 nW/cm(2).     

Bessel-beam-pumped tunable distributed-feedback laser

A distributed-feedback (DFB) dye laser that is pumped by a standing Bessel-beam wave is constructed. Because of the long line focus of the Bessel beam, the laser medium is pumped in only a very thin filament (a few micrometers) along the optical axis. At the same time, longitudinal-mode selection is achieved because of the DFB effect. It is demonstrated that when the effective wavelength of the Bessel pump beam is varied, the Bragg wavelength for DFB is altered, and as a result the output wavelength can be tuned.     

Holographic DFB Dye Lasers

A new simple type of DFB dye laser is proposed. The laser consists of a dye cell and a transparent phase holographic grating mounted on the front window of the cell. In the experiment, high-quality stable transparent holographic gratings were recorded in bichromated gelatine with a single mode He-Cd laser. When pumped perpendicular to the surface of the grating the DFB laser emitted a narrow spectral line independently of the width and the position of the pump spectrum. A linewidth of 0·01 nm was measured under pumping with broadband radiation of 20 nm spectral width. Either a set of holographic gratings of a different period or a fan-shaped grating may be used in the laser for stepped or continuous spectral tuning.     

Absolute frequency control of a 1560 nm (192 THz) DFB laser lockedto a rubidium absorption line using a second-harmonic-generated signal

We demonstrate second-harmonic generation from a DFB laser at 1560 nm in a type I critically phase-matched KNbO₃ crystal. We obtain 2.2 nW at 780 mm with 11.3 mW at 1560 nm incident on the crystal. The conversion efficiency is 17.2 pW/(mW)². The 780 nm beam is used to interrogate a resonance of the ⁸⁷Rb-D₂ line at 780 nm and lock the laser frequency. To characterize the absolute frequency stability, two 1560 nm DFB lasers are respectively stabilized on a Doppler resonance of the ⁸⁷Rb-D₂ line (780.246 nm) and of the ⁸⁵Rb-D₂ line (780.244 nm). The square root of the Allan variance measured from the beat note is around 1.5×10^-9 for averaging times between 3 and 100 s. To improve the precision of the frequency locking, we realize a setup to observe a saturated absorption profile. We use a 780 nm stabilized laser as a pump and the SHG signal as a probe. A saturated absorption profile is observed over the Doppler envelope. Work is under progress to use this saturated resonance for an improved frequency control     

Frequency stabilization of distributed-feedback laser diodes at 1572 nm for lidar measurements of atmospheric carbon dioxide

We demonstrate a wavelength-locked laser source that rapidly steps through six wavelengths distributed across a 1572.335 nm carbon dioxide (CO(2)) absorption line to allow precise measurements of atmospheric CO(2) absorption. A distributed-feedback laser diode (DFB-LD) was frequency-locked to the CO(2) line center by using a frequency modulation technique, limiting its peak-to-peak frequency drift to 0.3 MHz at 0.8 s averaging time over 72 hours. Four online DFB-LDs were then offset locked to this laser using phase-locked loops, retaining virtually the same absolute frequency stability. These online and two offline DFB-LDs were subsequently amplitude switched and combined. This produced a precise wavelength-stepped laser pulse train, to be amplified for CO(2) measurements.     

Testing carbon sequestration site monitor instruments using a controlled carbon dioxide release facility

Two laser-based instruments for carbon sequestration site monitoring have been developed and tested at a controlled carbon dioxide (CO(2)) release facility. The first instrument uses a temperature tunable distributed feedback (DFB) diode laser capable of accessing the 2.0027-2.0042 microm spectral region that contains three CO(2) absorption lines and is used for aboveground atmospheric CO(2) concentration measurements. The second instrument also uses a temperature tunable DFB diode laser capable of accessing the 2.0032-2.0055 mum spectral region that contains five CO(2) absorption lines for underground CO(2) soil gas concentration measurements. The performance of these instruments for carbon sequestration site monitoring was studied using a newly developed controlled CO(2) release facility. A 0.3 ton CO(2)/day injection experiment was performed from 3-10 August 2007. The aboveground differential absorption instrument measured an average atmospheric CO(2) concentration of 618 parts per million (ppm) over the CO(2) injection site compared with an average background atmospheric CO(2) concentration of 448 ppm demonstrating this instrument's capability for carbon sequestration site monitoring. The underground differential absorption instrument measured a CO(2) soil gas concentration of 100,000 ppm during the CO(2) injection, a factor of 25 greater than the measured background CO(2) soil gas concentration of 4000 ppm demonstrating this instrument's capability for carbon sequestration site monitoring.     

Intracavity absorption spectroscopy with a tunable multimode traveling-wave ring Ti:sapphire laser

A tunable multimode unidirectional traveling-wave Ti:sapphire laser was developed to measure in situ the atmospheric absorption spectra using intracavity absorption spectroscopy. The effective absorption path length was 2100 km. O2 and H2O vapor lines in atmosphere with absorption coefficients of 10(-6)-10(-8) cm(-1) were measured with uncertainties <5%, and the absorption coefficients were in agreement with those estimated from the HITRAN database. By tuning the wavelength, a weak absorption line with an absorption coefficient of 10(-9) cm(-1) was measured with a sensitivity of 2×10(-10) cm(-1). The sensitivity was limited by the residual parasitic variation that appeared in the spectrum.     

Progress in the realization of a frequency standard at 192.1 THz(1560.5 nm) using 87Rb D2-line and second harmonicgeneration

Second harmonic generation of a 192.1 THz semiconductor distributed feedback (DFB) laser is achieved using a KNbO₃ crystal in a resonant ring cavity. Optical feedback from this cavity is used to stabilize the laser frequency and reduce its linewidth. A second harmonic power of 5.5 μW is generated with 38 mW incident on the cavity. We use the second harmonic signal to observe saturated absorption lines and orientation signals in rubidium vapor. Injection-locking of a 780 nm Fabry-Perot laser using the second harmonic signal is also demonstrated. With this scheme, we observe saturated absorption lines in rubidium     

Extraction efficiency of saturated-gain high-power dye laser amplifiers: effect of nonlinear signal absorption

The effect of nonlinear signal absorption (NLSA) due to ground-state absorption and excited-state absorption in a transversely pumped high-power dye laser amplifier is theoretically examined with a one-dimensional steady-state model for a dye amplifier pumped by a copper vapor laser. A well-approximated analytical expression for the extraction efficiency is derived, from which the effect of NLSA in reducing the amplifier efficiency can be appreciated immediately and can also be interpreted in terms of certain characteristic lengths. The reduction in efficiency due to NLSA is found to be largely independent of the pump power, provided that the signal power is increased linearly with the pump power to continue to saturate the amplifier gain and suppress amplified spontaneous emission.     

Kilohertz pulse repetition frequency slab Ti:sapphire lasers with high average power (10 W)

High-average-power broadband 780-nm slab Ti:sapphire lasers, pumped by a kilohertz pulse repetition frequency copper vapor laser (CVL), were demonstrated. These lasers are designed for damage-free power scaling when pumped by CVL's configured for maximum output power (of order 100 W) but with poor beam quality (M(2) ~ 300). A simple Brewster-angled slab laser side pumped by a CVL produced 10-W average power (1.25-mJ pulses at 8 kHz) with 4.2-ns FWHM pulse duration at an absolute efficiency of 15% (68-W pump power). Thermal lensing in the Brewster slab laser resulted in multitransverse mode output, and pump absorption was limited to 72% by the maximum doping level for commercially available Ti:sapphire (0.25%). A slab laser with a multiply folded zigzag path was therefore designed and implemented that produced high-beam-quality (TEM(00)-mode) output when operated with cryogenic cooling and provided a longer absorption path for the pump. Excessive scattering of the Ti:sapphire beam at the crystal surfaces limited the efficiency of operation for the zigzag laser, but fluorescence diagnostic techniques, gain measurement, and modeling suggest that efficient power extraction (>15 W TEM(00), >23% efficiency) from this laser would be possible for crystals with an optical quality surface polish.     

Single-frequency Sb-based distributed-feedback lasers emitting at 2.3 microm above room temperature for application in tunable diode laser absorption spectroscopy

GaInAsSb/GaAlAsSb/GaSb distributed-feedback (DFB) laser diodes based on a type I active region were fabricated by molecular beam epitaxy at the Centre d'Electronique et de Micro-Optoélectronique de Montpellier (CEM2). The DFB processing was done by Nanoplus Nanosystems and Technologies GmbH. The devices work in the continuous-wave regime above room temperature around an emission wavelength of 2.3 microm with a side-mode suppression ratio greater than 25 dB and as great as 10 mW of output power. The laser devices are fully characterized in terms of optical and electrical properties. Their tuning properties made them adaptable to tunable diode laser absorption spectroscopy because they exhibit more than 220 GHz of continuous tuning by temperature or current. The direct absorption of CH4 is demonstrated to be possible with high spectral selectivity.     

Wavelength tuning and spectral properties of distributed feedback diode lasers with a short external optical cavity

We report on the wavelength tuning and spectral properties of distributed feedback (DFB) diode lasers operated with a plane external cavity (XC) mirror positioned as close as possible to the diode-laser front facet. These lasers generate single-frequency near IR radiation at wavelengths of 1392, 1580, 1602, and 1653 nm. A piezoelectric variation of the XC length provided continuous single-frequency tuning to as high as 19 GHz. A further benefit of XC DFB lasers is a residual amplitude modulation per gigahertz tuning of less than 10(-3). The XC feedback also suppresses residual side-mode oscillations to less than 60 dB. The laser's total intensity noise is close to the shot noise limit. The laser linewidth (measured in a beat note experiment) is less than 90 kHz within an acquisition time of 40 ms. The advantageous properties of XC DFB lasers for molecular spectroscopy are demonstrated by recording R(3) 2nu(3) overtone spectra of methane by single-scan single-pass absorption or frequency-modulation spectroscopy.     

Multimode distributed feedback laser emission in a dye-doped optically pumped polymer thin-film

We report on particular features of thin film distributed feedback (DFB) lasers. Devices are optically pumped using a Lloyd-mirror interferometer. For a given DFB grating period, the number of lasing modes is film thickness dependent. Spectral content of the devices is analysed using planar waveguide theory. An excellent agreement between the theoretical transverse electric mode structure and the laser emission spectrum is found.     

Precise wavelength control of a single-frequency pulsed Ho:Tm:YLF laser

We demonstrate wavelength control of a single-frequency diode-pumped Ho:Tm:YLF laser by referencing its wavelength to an absorption line of carbon dioxide. We accomplish this wavelength control by injection seeding with a cw Ho:Tm:YLF laser that can be tuned over or stabilized to carbon dioxide or water vapor lines. We show that the pulsed laser can be scanned precisely over an absorption line of carbon dioxide by scanning the injection seed laser wavelength. We locked the pulsed laser to within 18.5 MHz of the absorption line center by stabilizing the injection seed on the line center. The single-frequency pulsed output, intended for use as a transmitter for differential absorption lidar detection of atmospheric carbon dioxide and water vapor and for coherent detection of wind, is 100 mJ per pulse at a 5-Hz repetition rate.     

Wavelength-modulation laser hygrometer for ultrasensitive detection of water vapor in semiconductor gases

Water vapor is measured by use of a near-infrared diode laser and wavelength-modulation absorption spectroscopy. Humidity levels as low as 5 nmol/mol [1 nmol/mol = 1 ppb (1 ppb equals 1 part in 10(9))] of water vapor in air are measured with a sensitivity of better than 0.2 nmol/mol (3varsigma). The sensitivity, linearity, and stability of the technique are determined in experiments conducted at the National Institute of Standards and Technology, Gaithersburg, Maryland, by use of the low frost-point humidity generator over the range from 5 nmol/mol to 2.5 mumol/mol of water vapor in air. The pressure-broadening coefficients for water broadened by helium [0.0199(6) cm(-1) atm(-1) HWHM] and by hydrogen chloride [0.268(6) cm(-1) atm(-1) HWHM] are reported for the water line at 1392.5 nm.     

Characteristics of a dye laser amplifier transversely pumped by copper vapor lasers with a two-dimensional calculation model

A two-dimensional rate equation model, taking into consideration the transverse absorption loss of pump laser power, is proposed to evaluate the characteristics of a dye laser amplifier with a large input laser beam diameter pumped by high average power copper vapor lasers. The calculations are in good agreement with the measurements taken with a Rhodamine 6G dye, and the model can be used for evaluation of the dye concentration at any wavelength.     

Sum-frequency-generation system for differential absorption lidar measurement of atmospheric nitrogen dioxide

A sum-frequency-generation system for differential absorption lidar measurement of atmospheric nitrogen dioxide in the lower troposphere was developed. The system uses a combination of a pair of KD*P crystals and a tunable dye laser with LDS 765 dye pumped by the second harmonic of a Nd:YAG laser to generate lambdaon and lambdaoff alternatively. Compared with the conventional system that uses Coumarin 445 dye pumped by the third harmonic, the output energy and long-term stability were improved. By use of this system, atmospheric NO2 concentrations of approximately 10-50 ppb were measured, with an instrumental error of approximately 7 ppb.     

Infrared intracavity laser absorption spectroscopy with a continuous-scan Fourier-transform interferometer

High-quality broadband infrared high-resolution spectra were obtained by use of the intracavity laser absorption spectroscopy technique with a Ti:sapphire laser in combination with a continuous-scan Fourier-transform (FT) interferometer. With electronic filtering used to smooth out the fluctuations of the laser power, the absorption of atmospheric water vapor in the range of 12,450-12,700 cm(-1) was recorded at a resolution of 0.05 cm(-1). A signal-to-noise ratio of greater than 300 was observed in this spectrum, corresponding to a minimum detectable absorption of approximately 2 x 10(-9) cm(-1). Comparison with previous measurements by use of a conventional FT technique shows that this method gives absorption spectra with highly accurate line positions along with reasonable line intensities. Investigation of the evolution of intracavity laser absorption spectra with the generation time is also shown to be possible with a continuous-scan FT spectrometer by use of the interleave rapid-scan method.