共查询到20条相似文献,搜索用时 15 毫秒
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《Advanced Materials Technologies》2017,2(9)
Ultrafast Kerr effect switching in near‐infrared two‐photon absorption (TPA)‐free and free‐carrier‐absorption (FCA)‐free nonstoichiometric silicon carbide (Six C1−x ) microring waveguides is performed and investigated. With pulsed return‐to‐zero on–off‐keying (PRZ‐OOK) stream for the Si‐rich Six C1−x ‐based all‐optical switches, the inversely modulated probe reveals an asymmetric bit shape data extinction ratio (ER) of only 8.7 dB owing to the TPA + FCA effect. By eliminating the FCA effects in nearly stoichiometric Six C1−x microring waveguide, the high‐speed wavelength conversion of a data stream with an ER of 14 dB can be observed when coinciding the probe wavelength with the transmission dip. Slightly deviating the probe wavelength from the transmission dip, most probe power still remains in bus waveguide to cause a strong FCA effect to degrade the ER down to 7.4 dB. A symmetrically converted and inverted data stream with high on/off extinction can be observed in the C‐rich Six C1−x ‐based microring waveguide with completely suppressed trailing‐edge response. To further approach the upper limitation on bandwidth, the wavelength‐converted and sign‐reversible PRZ‐OOK data switching at a bit rate up to 12 Gbit s−1 can be obtained with similar ER of better than 20 dB, as contributed mainly by the enhanced Kerr nonlinearity in the C‐rich Six C1−x . 相似文献
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Yogesh Kumar Srivastava Manukumara Manjappa Longqing Cong Harish N. S. Krishnamoorthy Vassili Savinov Prakash Pitchappa Ranjan Singh 《Advanced materials (Deerfield Beach, Fla.)》2018,30(29)
The mechanism of Cooper pair formation and its underlying physics has long occupied the investigation into high temperature (high‐Tc) cuprate superconductors. One of the ways to unravel this is to observe the ultrafast response present in the charge carrier dynamics of a photoexcited specimen. This results in an interesting approach to exploit the dissipation‐less dynamic features of superconductors to be utilized for designing high‐performance active subwavelength photonic devices with extremely low‐loss operation. Here, dual‐channel, ultrafast, all‐optical switching and modulation between the resistive and the superconducting quantum mechanical phase is experimentally demonstrated. The ultrafast phase switching is demonstrated via modulation of sharp Fano resonance of a high‐Tc yttrium barium copper oxide (YBCO) superconducting metamaterial device. Upon photoexcitation by femtosecond light pulses, the ultrasensitive cuprate superconductor undergoes dual dissociation–relaxation dynamics, with restoration of superconductivity within a cycle, and thereby establishes the existence of dual switching windows within a timescale of 80 ps. Pathways are explored to engineer the secondary dissociation channel which provides unprecedented control over the switching speed. Most importantly, the results envision new ways to accomplish low‐loss, ultrafast, and ultrasensitive dual‐channel switching applications that are inaccessible through conventional metallic and dielectric based metamaterials. 相似文献
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Yong Xu Marwan Deb Grégory Malinowski Michel Hehn Weisheng Zhao Stéphane Mangin 《Advanced materials (Deerfield Beach, Fla.)》2017,29(42)
Current‐induced magnetization manipulation is a key issue for spintronic applications. This manipulation must be fast, deterministic, and nondestructive in order to function in device applications. Therefore, single‐ electronic‐pulse‐driven deterministic switching of the magnetization on the picosecond timescale represents a major step toward future developments of ultrafast spintronic systems. Here, the ultrafast magnetization dynamics in engineered Gdx [FeCo]1?x ‐based structures are studied to compare the effect of femtosecond laser and hot‐electron pulses. It is demonstrated that a single femtosecond hot‐electron pulse causes deterministic magnetization reversal in either Gd‐rich and FeCo‐rich alloys similarly to a femtosecond laser pulse. In addition, it is shown that the limiting factor of such manipulation for perpendicular magnetized films arises from the formation of a multidomain state due to dipolar interactions. By performing time‐resolved measurements under various magnetic fields, it is demonstrated that the same magnetization dynamics are observed for both light and hot‐electron excitation, and that the full magnetization reversal takes place within 40 ps. The efficiency of the ultrafast current‐induced magnetization manipulation is enhanced due to the ballistic transport of hot electrons before reaching the GdFeCo magnetic layer. 相似文献
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Mohammad Taghinejad Hossein Taghinejad Zihao Xu Yawei Liu Sean P. Rodrigues Kyu‐Tae Lee Tianquan Lian Ali Adibi Wenshan Cai 《Advanced materials (Deerfield Beach, Fla.)》2018,30(9)
The optical Kerr nonlinearity of plasmonic metals provides enticing prospects for developing reconfigurable and ultracompact all‐optical modulators. In nanostructured metals, the coherent coupling of light energy to plasmon resonances creates a nonequilibrium electron distribution at an elevated electron temperature that gives rise to significant Kerr optical nonlinearities. Although enhanced nonlinear responses of metals facilitate the realization of efficient modulation devices, the intrinsically slow relaxation dynamics of the photoexcited carriers, primarily governed by electron–phonon interactions, impedes ultrafast all‐optical modulation. Here, femtosecond (≈190 fs) all‐optical modulation in plasmonic systems via the activation of relaxation pathways for hot electrons at the interface of metals and electron acceptor materials, following an on‐resonance excitation of subradiant lattice plasmon modes, is demonstrated. Both the relaxation kinetics and the optical nonlinearity can be actively tuned by leveraging the spectral response of the plasmonic design in the linear regime. The findings offer an opportunity to exploit hot‐electron‐induced nonlinearities for design of self‐contained, ultrafast, and low‐power all‐optical modulators based on plasmonic platforms. 相似文献
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Song Han Longqing Cong Yogesh Kumar Srivastava Bo Qiang Mikhail V. Rybin Abhishek Kumar Ravikumar Jain Wen Xiang Lim Venu Gopal Achanta Shriganesh S. Prabhu Qi Jie Wang Yuri S. Kivshar Ranjan Singh 《Advanced materials (Deerfield Beach, Fla.)》2019,31(37)
The remarkable emergence of all‐dielectric meta‐photonics governed by the physics of high‐index dielectric materials offers a low‐loss platform for efficient manipulation and subwavelength control of electromagnetic waves from microwaves to visible frequencies. Dielectric metasurfaces can focus electromagnetic waves, generate structured beams and vortices, enhance local fields for advanced sensing, and provide novel functionalities for classical and quantum technologies. Recent advances in meta‐photonics are associated with the exploration of exotic electromagnetic modes called the bound states in the continuum (BICs), which offer a simple interference mechanism to achieve large quality factors (Q) through excitation of supercavity modes in dielectric nanostructures and resonant metasurfaces. Here, a BIC‐driven terahertz metasurface with dynamic control of high‐Q silicon supercavities that are reconfigurable at a nanosecond timescale is experimentally demonstrated. It is revealed that such supercavities enable low‐power, optically induced terahertz switching and modulation of sharp resonances for potential applications in lasing, mode multiplexing, and biosensing. 相似文献
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Artemios Karvounis Behrad Gholipour Kevin F. MacDonald Nikolay I. Zheludev 《Advanced materials (Deerfield Beach, Fla.)》2019,31(1)
Electrostriction is a property of all naturally occurring dielectrics whereby they are mechanically deformed under the application of an electric field. It is demonstrated here that an artificial metamaterial nanostructure comprising arrays of dielectric nanowires, made of silicon and indium tin oxide, is reversibly structurally deformed under the application of an electric field, and that this reconfiguration is accompanied by substantial changes in optical transmission and reflection, thus providing a strong electro‐optic effect. Such metamaterials can be used as the functional elements of electro‐optic modulators in the visible to near‐infrared part of the spectrum. A modulator operating at 1550 nm with effective electrostriction and electro‐optic coefficients of order 10?13 m2 V?2 and 10?6 m V?1, respectively, is demonstrated. Transmission changes of up to 3.5% are obtained with a 500 mV control signal at a modulation frequency of ≈6.5 MHz. With a resonant optical response that can be spectrally tuned by design, modulators based on the artificial electrostrictive effect may be used for laser Q‐switching and mode‐locking among other applications that require modulation at megahertz frequencies. 相似文献
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Rebecca L. Gieseking Chad Risko Seth R. Marder Jean‐Luc Brédas 《Advanced materials (Deerfield Beach, Fla.)》2014,26(1):68-84
All‐optical switching—controlling light with light—has the potential to meet the ever‐increasing demand for data transmission bandwidth. The development of organic π‐conjugated molecular materials with the requisite properties for all‐optical switching applications has long proven to be a significant challenge. However, recent advances demonstrate that polymethine dyes have the potential to meet the necessary requirements. In this review, we explore the theoretical underpinnings that guide the design of π‐conjugated materials for all‐optical switching applications. We underline, from a computational chemistry standpoint, the relationships among chemical structure, electronic structure, and optical properties that make polymethines such promising materials. 相似文献
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Park H Shin D Kang G Baek S Kim K Padilla WJ 《Advanced materials (Deerfield Beach, Fla.)》2011,23(48):5796-5800
Based on conventional colloidal nanosphere lithography, we experimentally demonstrate novel graded-index nanostructures for broadband optical antireflection enhancement including the near-ultraviolet (NUV) region by integrating residual polystyrene antireflective (AR) nanoislands coating arrays with silicon nano-conical-frustum arrays. This is a feasible optimized integration method of two major approaches for antireflective surfaces: quarter-wavelength AR coating and biomimetic moth's eye structure. 相似文献
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Manukumara Manjappa Ankur Solanki Abhishek Kumar Tze Chien Sum Ranjan Singh 《Advanced materials (Deerfield Beach, Fla.)》2019,31(32)
Solution‐processed lead iodide (PbI2) governs the charge transport characteristics in the hybrid metal halide perovskites. Besides being a precursor in enhancing the performance of perovskite solar cells, PbI2 alone offers remarkable optical and ultrasensitive photoresponsive properties that remain largely unexplored. Here, the photophysics and the ultrafast carrier dynamics of the solution processed PbI2 thin film is probed experimentally. A PbI2 integrated metamaterial photonic device with switchable picosecond time response at extremely low photoexcitation fluences is demonstrated. Further, findings show strongly confined terahertz field induced tailoring of sensitivity and switching time of the metamaterial resonances for different thicknesses of PbI2 thin film. The approach has two far reaching consequences: the first lead‐iodide‐based ultrafast photonic device and resonantly confined electromagnetic field tailored transient nonequilibrium dynamics of PbI2 which could also be applied to a broad range of semiconductors for designing on‐chip, ultrafast, all‐optical switchable photonic devices. 相似文献
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Xiangling Tian Hongyu Luo Rongfei Wei Chunhui Zhu Qianyi Guo Dandan Yang Fengqiu Wang Jianfeng Li Jianrong Qiu 《Advanced materials (Deerfield Beach, Fla.)》2018,30(31)
Pulsed lasers operating in the mid‐infrared (3–25 µm) are increasingly becoming the light source of choice for a wide range of industrial and scientific applications such as spectroscopy, biomedical research, sensing, imaging, and communication. Up to now, one of the factors limiting the mid‐infrared pulsed lasers is the lack of optical switch with a capability of pulse generation, especially for those with wideband response. Here, a semiconductor material of bismuth oxyselenide (Bi2O2Se) with a facile processibility, constituting an ultrabroadband saturable absorber for the mid‐infrared (actually from the near‐infrared to mid‐infrared: 0.8–5.0 µm) is exhibited. Significantly, it is found that the optical response is associated with a strong nonlinear character, showing picosecond response time and response amplitude up to ≈330.1% at 5.0 µm. Combined with facile processibility and low cost, these solution‐processed Bi2O2Se materials may offer a scalable and printable mid‐infrared optical switch to open up the long‐sought parameter space which is crucial for the exploitation of compact and high‐performance mid‐infrared pulsed laser sources. 相似文献
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Pulsed Lasers: An Ultrabroadband Mid‐Infrared Pulsed Optical Switch Employing Solution‐Processed Bismuth Oxyselenide (Adv. Mater. 31/2018)
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Xiangling Tian Hongyu Luo Rongfei Wei Chunhui Zhu Qianyi Guo Dandan Yang Fengqiu Wang Jianfeng Li Jianrong Qiu 《Advanced materials (Deerfield Beach, Fla.)》2018,30(31)
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Prakash Pitchappa Abhishek Kumar Saurav Prakash Hariom Jani Thirumalai Venkatesan Ranjan Singh 《Advanced materials (Deerfield Beach, Fla.)》2019,31(12)
The strikingly contrasting optical properties of various phases of chalcogenide phase change materials (PCM) has recently led to the development of novel photonic devices such as all‐optical non‐von Neumann memory, nanopixel displays, color rendering, and reconfigurable nanoplasmonics. However, the exploration of chalcogenide photonics is currently limited to optical and infrared frequencies. Here, a phase change material integrated terahertz metamaterial for multilevel nonvolatile resonance switching with spatial and temporal selectivity is demonstrated. By controlling the crystalline proportion of the PCM film, multilevel, non‐volatile, terahertz resonance switching states with long retention time at zero hold power are realized. Spatially selective reconfiguration at sub‐metamaterial scale is shown by delivering electrical stimulus locally through designer interconnect architecture. The PCM metamaterial also features ultrafast optical modulation of terahertz resonances with tunable switching speed based on the crystalline order of the PCM film. The multilevel nonvolatile, spatially selective, and temporally tunable PCM metamaterial will provide a pathway toward development of novel and disruptive terahertz technologies including spatio‐temporal terahertz modulators for high speed wireless communication, neuromorphic photonics, and machine‐learning metamaterials. 相似文献
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使用多次超声离心分散法将单壁碳纳米管(SWNTs)溶入聚(3-辛基)噻吩(P3OTH)溶液中制得P3OTH/SWNTs复合液(溶剂为四氢呋喃)。研究了该复合液在不同功率及调制频率控制光(532nm)作用下的全光开关特性。实验发现,在7mW、258Hz的控制光调制下,该复合液较P3OTH单体溶液的全光开关调制深度提高了2倍;控制光功率为7mW时,复合液样品在25Hz的控制频率下调制深度可达84%。在此基础上增加控制频率到432.5Hz,该样品的开关响应时间达到1ms,并且可维持40%以上的调制深度;在140Hz时,将控制光功率降低,该复合液样品的调制深度增大,当控制光功率降低到3.6mW时,达到最大值62%。结果表明样品具有良好的全光开关特性,具有潜在的研究及应用价值。 相似文献
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James A. Dolan Raphael Dehmel Angela Demetriadou Yibei Gu Ulrich Wiesner Timothy D. Wilkinson Ilja Gunkel Ortwin Hess Jeremy J. Baumberg Ullrich Steiner Matthias Saba Bodo D. Wilts 《Advanced materials (Deerfield Beach, Fla.)》2019,31(2)
Optical metamaterials offer the tantalizing possibility of creating extraordinary optical properties through the careful design and arrangement of subwavelength structural units. Gyroid‐structured optical metamaterials possess a chiral, cubic, and triply periodic bulk morphology that exhibits a redshifted effective plasma frequency. They also exhibit a strong linear dichroism, the origin of which is not yet understood. Here, the interaction of light with gold gyroid optical metamaterials is studied and a strong correlation between the surface morphology and its linear dichroism is found. The termination of the gyroid surface breaks the cubic symmetry of the bulk lattice and gives rise to the observed wavelength‐ and polarization‐dependent reflection. The results show that light couples into both localized and propagating plasmon modes associated with anisotropic surface protrusions and the gaps between such protrusions. The localized surface modes give rise to the anisotropic optical response, creating the linear dichroism. Simulated reflection spectra are highly sensitive to minute details of these surface terminations, down to the nanometer level, and can be understood with analogy to the optical properties of a 2D anisotropic metasurface atop a 3D isotropic metamaterial. This pronounced sensitivity to the subwavelength surface morphology has significant consequences for both the design and application of optical metamaterials. 相似文献
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Qiangbing Guo Yudong Cui Yunhua Yao Yuting Ye Yue Yang Xueming Liu Shian Zhang Xiaofeng Liu Jianrong Qiu Hideo Hosono 《Advanced materials (Deerfield Beach, Fla.)》2017,29(27)
All the optical properties of materials are derived from dielectric function. In spectral region where the dielectric permittivity approaches zero, known as epsilon‐near‐zero (ENZ) region, the propagating light within the material attains a very high phase velocity, and meanwhile the material exhibits strong optical nonlinearity. The interplay between the linear and nonlinear optical response in these materials thus offers unprecedented pathways for all‐optical control and device design. Here the authors demonstrate ultrafast all‐optical modulation based on a typical ENZ material of indium tin oxide (ITO) nanocrystals (NCs), accessed by a wet‐chemistry route. In the ENZ region, the authors find that the optical response in these ITO NCs is associated with a strong nonlinear character, exhibiting sub‐picosecond response time (corresponding to frequencies over 2 THz) and modulation depth up to ≈160%. This large optical nonlinearity benefits from the highly confined geometry in addition to the ENZ enhancement effect of the ITO NCs. Based on these ENZ NCs, the authors successfully demonstrate a fiber optical switch that allows switching of continuous laser wave into femtosecond laser pulses. Combined with facile processibility and tunable optical properties, these solution‐processed ENZ NCs may offer a scalable and printable material solution for dynamic photonic and optoelectronic devices. 相似文献