Evaluation of the characteristics of the neutron reference field using D2O-moderated 252Cf source

The ambient/personal dose equivalent per fluence for D(2)O moderated (252)Cf neutron source was determined by measurement. An appropriate subtraction of the scattered neutrons is required for the accurate measurement of direct neutrons. A cubic shadow object was used for the subtraction of the scattered neutrons from the surroundings. The scattered neutrons to be subtracted vary with the position of the shadow object due to the large volume of the source. Using the Monte Carlo code MCNP-4C, the optimum positions of the shadow object were surveyed for subtracting the scattered neutrons. The energy spectra of direct neutrons were measured in the optimum position. The dosimetric parameters for the D(2)O moderated (252)Cf neutron source were reasonable, taking into account the uncertainties of the parameters.     

Field parameters and dosimetric characteristics of a fast neutron calibration facility: experimental and Monte Carlo evaluations

At the ENEA Institute for Radiation Protection (IRP) the fast neutron calibration facility consists of a remote control device which allows locating different sources (Am–Be, Pu–Li, bare and D₂O moderated ²⁵²Cf) at the reference position, at the desired height from the floor, inside a 10×10×3 m³ irradiation room. Either the ISO reference sources or the Pu–Li source have been characterised in terms of uncollided H^*(10) and neutron fluence according to the ISO calibration procedures. A spectral fluence mapping, carried out with the Monte Carlo Code MCNP^TM, allowed characterising the calibration point, in scattered field conditions, according to the most recent international recommendations. Moreover, the irradiation of personal dosemeters on the ISO water filled slab phantom was simulated to determine the field homogeneity of the calibration area and the variability of the neutron field (including the backscattered component) along the phantom surface. At the ENEA Institute for Radiation Protection the calibration of neutron area monitors as well as personal dosemeters can now be performed according to the international standards, at the same time guaranteeing suitable conditions for research and qualification purposes in the field of neutron dosimetry.     

Radionuclide neutron sources in calibration laboratory--neutron and gamma doses and their changes in time

The calibration laboratory, having standard neutron fields of radionuclide sources, should perform regular measurements of fields' parameters in order to check their stability and to get knowledge of any changes. Usually, accompanying gamma radiation is not of serious concern, but some personal dosemeters, old neutron dose equivalent meters with scintillation detectors and the dose meters of mixed radiation require the determination of this component. In the Laboratory of Radiation Protection Measurements in the Institute of Atomic Energy, Poland, the fields of radionuclide neutron sources (252)Cf, (241)Am-Be and (239)Pu-Be were examined for nearly 20 y. A number of detectors and methods have been applied for the determination of neutron ambient dose equivalent rate and for the determination of neutron and gamma dose components. This paper presents the recent results of measurements of gamma and neutron dose and dose equivalent, compared with the results accumulated in nearly 20 y.     

The clinical practice of 252Cf neutron brachytherapy devices on malignant tumor in China

The 252Cf neutron brachytherapy devices were designed and manufactured after solving those problems: the shield difficulties for 252Cf neutron; the method and facilities for 252Cf neutron source deliver; the dose calculation and measurement for 252Cf neutron. From 1999-2009, more than twenty 252Cf neutron brachytherapy devices had been installed in China. The Chinese radiation oncologists implemented the 252Cf neutron brachytherapy on more than 5 000 different kinds of cancer patients, including cervix cancer; endometrium cancer and achieved ideal results. For special presentation, they had breakthrough on radical treatment for low lying rectal adenocarcinoma with sphincter preservation and melanoma patients after the modification of 252Cf neutron intracavitary applicator and dose calibration.     

Neutron calibration facility with radioactive neutron sources at KRISS

For the purpose of radiation protection, the reference neutron field for calibration of neutron monitors was constructed using radioactive neutron sources-bare-(252)Cf, D(2)O-moderated (252)Cf and (241)Am-Be(alpha,n)-at Korea Research Institute of Standards and Science (KRISS). The well-specified neutron source with its emission rate and the anisotropy was installed at the centre of the neutron irradiation room, which is 6.6 x 7.6 x 6.3 m(3) in size. The neutron spectra of each source was measured using the Bonner sphere spectrometer (KRISS-BSS). Calculations using MCNP5 with realistic geometry and materials in the neutron irradiation room were performed. The calculations and measurements were found to be in good agreement, showing that the neutron calibration facility at KRISS is well established.     

Development of a light-weight portable neutron survey meter

A light-weight portable neutron survey meter was developed using a mixed organic gas counter for dose management at nuclear power plants and accelerator facilities. This survey meter, NSN31041, is ~2 kg in weight and W160×H250×L300 mm(3) in size, which is capable of measuring neutron ambient dose equivalent rate from thermal to 15 MeV neutrons. The neutron energy response of the survey meter is evaluated using continuous energy neutron sources of (252)Cf, (241)Am-Be, thermal neutrons generated from a graphite pile loading a (252)Cf source, concrete-moderated neutrons of (241)Am-Be source and D(2)O-moderated neutrons of (252)Cf source. The measured response data show very good agreement with neutron ambient dose equivalent within a 50 % deviation.     

NIST Calibration of a Neutron Spectrometer ROSPEC

A neutron spectrometer was acquired for use in the measurement of National Institute of Standards and Technology neutron fields. The spectrometer included options for the measurement of low and high energy neutrons, for a total measurement range from 0.01 eV up to 17 MeV. The spectrometer was evaluated in calibration fields and was used to determine the neutron spectrum of an Americium-Beryllium neutron source. The calibration fields used included bare and moderated ²⁵²Cf, monoenergetic neutron fields of 2.5 MeV and 14 MeV, and a thermal-neutron beam. Using the calibration values determined in this exercise, the spectrometer gives a good approximation of the neutron spectrum, and excellent values for neutron fluence, for all NIST calibration fields. The spectrometer also measured an Americium-Beryllium neutron field in a NIST exposure facility and determined the field quite well. The spectrometer measured scattering effects in neutron spectra which previously could be determined only by calculation or integral measurements.     

French comparison exercise with the rotating neutron spectrometer, 'ROSPEC'

The French laboratories in charge of 'neutron' dosimetry using the spectrometer 'ROSPEC', formed a working group in 2001. The participants began to study the behaviour of the instrument with a comparison exercise in broad energy neutron fields recommended by the International Organisation for Standardisation (ISO) and available at the LMDN in Cadarache. The complete version of the ROSPEC is made up of six spherical proportional counters fixed to a rotating platform. These counters cover different energy ranges which overlap each other to provide a link between the detectors, within the energy range from thermal neutrons to 4.5 MeV. The irradiation configurations chosen were ISO standard sources (252Cf, (252Cf+D2O)(/Cd), 241Am-Be) and the SIGMA facility. The results show that the 'thermal and epithermal' neutron fluence was widely overestimated by the spectrometer in all configurations.     

Standardisation of water-moderated 241Am-Be neutron source using De Pangher neutron long counter: experimental and Monte Carlo modelling

A convenient neutron source is made for calibration of neutron survey instruments and personal dosimeters that are used in various nuclear installations such as fuel reprocessing, waste management, fuel fabrication and oil and well logging facilities, etc. This source consists of a bare (241)Am-Be neutron source placed at the centre of a 15-cm radius stainless steel spherical shell filled with distilled water. This paper describes the standardisation of the source at Bhabha Atomic Research Centre, using De Pangher neutron long counter both experimentally and using the Monte Carlo simulation. The ratio of neutron yield of water moderated to the bare (241)Am-Be neutron source was found to be 0.573. From the simulation, the neutron-fluence-weighted average energy of water-moderated (241)Am-Be source (fluence-weighted average energy of 2.25 MeV, dose-weighted average energy of 3.55 MeV) was found to be nearly the same as that of a (252)Cf source (fluence-weighted average energy of 2.1 MeV, dose-weighted average energy of 2.3 MeV). This source can be used for calibration in addition to (252)Cf, to study the variation in response of neutron monitoring instruments.     

Design of a new IRSN thermal neutron field facility using Monte-Carlo simulations

The Institute for Radiological Protection and Nuclear Safety owns a graphite-moderated AmBe neutron field facility, SIGMA, that has to be reconstructed. Monte-Carlo simulations were performed to study the design of a new thermal facility based on IRSN existing facilities. Studies related to an update version of SIGMA concerned the enhancement of the thermal neutrons contribution to the dose equivalent. Calculations were mainly performed for a (252)Cf neutron source distribution located at the centre of a graphite moderator block. A quasi-pure thermal neutron field was obtained with a 2.4 x 2.4 x 2.4-m(3) block of graphite. A second acceptable neutron field was obtained with 3.3-MeV mono-energetic neutrons created by a 400-kV accelerator coupled to a graphite assembly of 1.5 x 1.5 x 1.5 m(3). The characteristics of the studied thermal fields with the requirement for a reference calibration field are compared, and the advantages and drawbacks of the different producing methods are discussed.     

Gamma sensitivity of single-crystal CVD diamond neutron detectors

We have studied the gamma sensitivity of single-crystal CVD diamond neutron detectors using a ²⁵²Cf neutron source placed in a moderator. It has been shown that a major contribution to the count rate of the detectors is made by the gamma rays from the source. We have compared the count rates of a detector with a ¹⁰B boron isotope-based slow-neutron converter and without it. With allowance for the theoretically calculated detection efficiency, the difference between the count rates is consistent with the fraction of slow neutrons measured using a scintillation detector.     

Evaluation of spectrum measurement devices for operational use

Several neutron spectrometers manufactured by Bubble Technology Industries (BTI) were tested and evaluated in a variety of neutron fields. Findings and conclusions are presented for the following BTI instruments: a modification of the Rotational Spectrometer (ROSPEC) that includes a thermal and epithermal capability, the Simple Scintillation Spectrometer that is used in conjunction with the ROSPEC to extend its high-energy range, and the MICROSPEC N-Probe which is capable of providing a crude spectrum over the energy range from thermal to 18 MeV. The main objective of these measurements was to determine the accuracy of both the energy spectrum and dose equivalent information generated by these devices. In addition, the dose response of the Wide-Energy Neutron Detection Instrument (WENDI-II) was measured in all neutron fields relative to a bare ²⁵²Cf calibration. The performance of the WENDI-II rem meter was compared to the dose information generated by the neutron spectrometers. The instruments were irradiated to bare ²⁵²Cf and ²⁴¹AmBe sources, and in a series of moderated ²⁵²Cf fields using a standard D₂O sphere and a set of polyethylene spheres. The measured spectra were benchmarked with a set of detailed Monte Carlo calculations with the same energy bin structure as that of the instruments under test. These calculations allowed an absolute comparison to be made with the measurements on a bin by bin basis. The simulations included the effects of room return and source anisotropy.     

Investigations of shield effect and type of soil on landmine detection

This paper investigates the possibility of optimizing the performance of the neutron backscattering method in landmine detection by designing a suitable shield around a ²⁵²Cf neutron source to reduce the background due to soil and the neutrons emitted from the source that hit the detector directly. A series of Monte Carlo simulations were performed to improve the source shield thickness and to study the elastically backscattered (EBS) ²⁵²Cf neutrons from the buried explosive material TNT in the soil; the optimal configuration was examined against different soil types and source heights. The results obtained in terms of performance of the relative (EBS) neutrons confirmed that the proposed source shield has significantly improved the signal to background ratio. Higher signal-to-background ratio was observed using ²⁵²Cf neutron source as compared to Pu-Be source.     

Arrangement of high-energy neutron irradiation field and shielding experiment using 4 m concrete at KENS

An irradiation field of high-energy neutrons produced in the forward direction from a thick tungsten target bombarded by 500 MeV protons was arranged at the KENS spallation neutron source facility. In this facility, shielding experiment was performed with an ordinary concrete shield of 4 m thickness assembled in the irradiation room, 2.5 m downstream from the target centre. Activation detectors of bismuth, aluminium, indium and gold were inserted into eight slots inside the shield and attenuations of neutron reaction rates were obtained by measurements of gamma-rays from the activation detectors. A MARS14 Monte Carlo simulation was also performed down to thermal energy, and comparisons between the calculations and measurements show agreements within a factor of 3. This neutron field is useful for studies of shielding, activation and radiation damage of materials for high-energy neutrons, and experimental data are useful to check the accuracies of the transmission and activation calculation codes.     

Results of field trials using the NPL simulated reactor neutron field facility

The NPL simulated reactor neutron field facility provides neutron spectra similar to those found in the environs of UK gas-cooled reactors. Neutrons are generated by irradiating a thick lithium-alloy target with monoenergetic protons between 2.5 and 3.5 MeV (depending on the desired spectrum), and then moderated by a 40-cm diameter sphere of heavy water. This represents an extremely soft workplace field, with a mean neutron energy of 25 keV and, more significantly, a mean fluence to ambient dose equivalent conversion coefficient of the order of 20 pSv cm(2), approximately 20 times lower than those of the ISO standard calibration sources (252)Cf and (241)Am-Be. Results of field trials are presented, including readings from neutron spectrometers, personal dosimeters (active and passive) and neutron area survey meters, and issues with beam monitoring are discussed.     

Characteristics of polyethylene-moderated 252Cf neutron sources

Polyethylene-moderated ²⁵²Cf neutron sources were designed to produce neutron reference fields’ spectra that simulate the spectra observed in the workplaces within nuclear reactors and accelerators. The paper describes the neutron sources and fields. Neutron spectra were calculated by the Monte Carlo method and compared with experimental data.     

Status of the cyric neutron TOF facilities upgrade

We describe progress in the Tohoku neutron time-of-flight (TOF) facilities improved to facilitate high resolution measurements for neutrons in the range 10 ≤ E_n ≲ 60 MeV. Efforts have been concentrated on completing the neutron detection system consisting of twelve neutron detectors, in which 23 1 of NE213 liquid scintillator are encapsulated, and a CAMAC-based data acquisition system. A systematic study of the neutron detection efficiency has been performed by Monte Carlo calculation for monochromatic neutrons with E_n ≲ 34 MeV. Results have been tested by counting neutrons from the ⁷Li(p, n)⁷Be reaction and comparing the yield with the absolute neutron fluence determined by activation.     

Two types of multi-moderator neutron spectrometers: Gamma-ray insensitive type and high-efficiency type

Two types of multi-moderator neutron spectrometers were developed; one is a gamma-ray insensitive type, and the other is a high-efficiency type. An indium activation detector is loaded in the former spectrometer, which can measure the photon-dominant pulsed neutron field such as in the primary photon beam of a high-energy medical electron accelerator. The latter, in which a ³He counter is loaded, is so sensitive that it can measure leakage neutrons from a well shielded facility or even the skyshine neutrons. The response functions of the spectrometers were measured by thermal and mono-energetic neutron standard fields, and were also calculated by the one-dimensional discrete ordinates transport code, ANISN. The measured and calculated responses showed generally good agreement. A benchmark measurement of ²⁵²Cf fission neutrons by using these two spectrometers agreed well with the calculated spectrum. The spectrometers were used in the measurements of neutrons produced by a medical electron accelerator and of skyshine neutrons from an intense 14 MeV neutron source facility.     

Experimental and numerical characterization of the neutron field produced in the n@BTF Frascati photo-neutron source

A photo-neutron irradiation facility is going to be established at the Frascati National Laboratories of INFN on the base of the successful results of the n@BTF experiment. The photo-neutron source is obtained by an electron or positron pulsed beam, tuneable in energy, current and in time structure, impinging on an optimized tungsten target located in a polyethylene-lead shielding assembly. The resulting neutron field, through selectable collimated apertures at different angles, is released into a 100 m² irradiation room. The neutron beam, characterized by an evaporation spectrum peaked at about 1 MeV, can be used in nuclear physics, material science, calibration of neutron detectors, studies of neutron hardness, ageing and study of single event effect. The intensity of the neutron beam obtainable with 510 MeV electrons and its fluence energy distribution at a point of reference in the irradiation room were predicted by Monte Carlo simulations and experimentally determined with a Bonner Sphere Spectrometer (BSS). Due to the large photon contribution and the pulsed time structure of the beam, passive photon-insensitive thermal neutron detectors were used as sensitive elements of the BSS. For this purpose, a set of Dy activation foils was used. This paper presents the numerical simulations and the measurements, and compares their results in terms of both neutron spectrum and total neutron fluence.     

High-energy neutron reference fields for the calibration of detectors used in neutron spectrometry

Quasi-monoenergetic reference neutron beams in the energy range between 20 and 100 MeV have been produced and characterized with a proton recoil telescope, a scintillation spectrometer, a ²³⁸U fission chamber and a Bonner sphere spectrometer. The beams are well suited for the calibration of detectors used in neutron spectrometry. A new method is described which reduces the correction for the contribution from low-energy neutrons present in the beams.