共查询到20条相似文献,搜索用时 15 毫秒
1.
Munki Kim 《Combustion and Flame》2009,156(12):2252-2263
This study examines the effect of acoustic excitation using forced coaxial air on the flame characteristics of turbulent hydrogen non-premixed flames. A resonance frequency was selected to acoustically excite the coaxial air jet due to its ability to effectively amplify the acoustic amplitude and reduce flame length and NOx emissions. Acoustic excitation causes the flame length to decrease by 15% and consequently, a 25% reduction in EINOx is achieved, compared to coaxial air flames without acoustic excitation at the same coaxial air to fuel velocity ratio. Moreover, acoustic excitation induces periodical fluctuation of the coaxial air velocity, thus resulting in slight fluctuation of the fuel velocity. From phase-lock PIV and OH PLIF measurement, the local flow properties at the flame surface were investigated under acoustic forcing. During flame-vortex interaction in the near field region, the entrainment velocity and the flame surface area increased locally near the vortex. This increase in flame surface area and entrainment velocity is believed to be a crucial factor in reducing flame length and NOx emission in coaxial jet flames with acoustic excitation. Local flame extinction occurred frequently when subjected to an excessive strain rate, indicating that intense mass transfer of fuel and air occurs radially inward at the flame surface. 相似文献
2.
Jeongseog Oh Pilwon Heo Youngbin Yoon 《International Journal of Hydrogen Energy》2009,34(18):7851-7861
The effects of acoustic excitation on the reduction in nitric oxidant (NOx) emission were experimentally investigated in non-premixed lifted hydrogen jet flames with coaxial air. The purpose of the present work was to analyze the acoustic forcing effect on the flow field, the reaction zone, and NOx emission, and to study the mechanisms of NOx reduction and flame stabilization. To analyze of the flow field, a PIV method was used that incorporated two Nd-YAG lasers and a CCD camera. The reaction zone was visualized by taking OH* chemiluminescence images with a 307.1 ± 5 nm narrow band pass filter and an ICCD camera. A flow condition was carefully selected at uF = 150, 200, 250 m/s and uA = 12, 16, 20 m/s, which was sustainable for acoustic excitation in a lifted flame region. The frequency was swept from 150 to 1000 Hz in 5 Hz steps. From the measurements of the flow field, the reaction zone, and NOx emission, we concluded that NOx emission was reduced and minimized at the resonance frequency. The vortex that was generated by acoustic forcing promoted air entrainment and enhanced the fuel-air mixing rate. This premixing effect resulted in a lower flame temperature, and thus lower NOx emissions. In addition, the liftoff height periodically fluctuated due to the stretch effect as the vortex interacted with the flame base. 相似文献
3.
Han S. Kim Vaibhav K. ArghodeMartin B. Linck Ashwani K. Gupta 《International Journal of Hydrogen Energy》2009
The effect of hydrogen addition in methane-air premixed flames has been examined from a swirl-stabilized combustor under confined conditions. The effect of hydrogen addition in methane-air flame has been examined over a range of conditions using a laboratory-scale premixed combustor operated at 5.81 kW. Different swirlers have been investigated to identify the role of swirl strength to the incoming mixture. The flame stability was examined for the effect of amount of hydrogen addition, combustion air flow rates and swirl strengths. This was carried out by comparing adiabatic flame temperatures at the lean flame limit. The combustion characteristics of hydrogen-enriched methane flames at constant heat load but different swirl strengths have been examined using particle image velocimetry (PIV), micro-thermocouples and OH chemiluminescence diagnostics that provided information on velocity, thermal field, and combustion generated OH species concentration in the flame, respectively. Gas analyzer was used to obtain NOx and CO concentration at the combustor exit. The results show that the lean stability limit is extended by hydrogen addition. The stability limit can reduce at higher swirl intensity to the fuel-air mixture operating at lower adiabatic flame temperatures. The addition of hydrogen increases the NOx emission; however, this effect can be reduced by increasing either the excess air or swirl intensity. The emissions of NOx and CO from the premixed flame were also compared with a diffusion flame type combustor. The NOx emissions of hydrogen-enriched methane premixed flame were found to be lower than the corresponding diffusion flame under same operating conditions for the fuel-lean case. 相似文献
4.
NOx emission indices were experimentally measured for partially premixed laminar flames of five different H2/CO/CO2 fuels over a wide range of equivalence ratios. Through those fuels, the effects of H2/CO ratio and CO2 concentration on NOx emissions, flame appearance, visible flame height and flame temperature are presented. EINOx values increase when 1.0 ≤ Φ ≤ 1.6, then remain near the highest value, before decreasing slowly when 3.85 ≤ Φ ≤ ∞. The increase of the CO2 concentration reduces the EINOx for the whole range of equivalence ratios, while the increase in the H2/CO ratio reduces the EINOx when Φ ≤ 2.0 and is inconsequential for richer mixtures. The variation in flame temperatures approximates EINOx trends. The variation of flame color from blue to orange when the H2/CO ratio is increased might be explained by higher CO levels in by-product combustion. 相似文献
5.
Active control of a bluff-body stabilized methane/air jet flame issued from a coaxial nozzle is made by using miniature magnetic flap actuators attached to the outer nozzle. CH radical chemiluminescence, and CO and NOx emissions are measured to assess the flame characteristics. By changing the flapping Strouhal number, the flame stability and CO emission are drastically improved under different equivalence ratio (?) conditions. At ? = 0.72, the optimum Strouhal number for stable combustion is unity, since methane/air mixing is enhanced by large-scale vortices synchronized with the flap motion. On the other hand, at a lower equivalence ratio of ? = 0.48, the optimum Strouhal number is much larger than unity; with small-scale vortices, the premixed combustion is stabilized by stratified mixing. In addition to acetone and OH-PLIF, a new two-line OH-PLIF is employed for flame temperature measurement. The longitudinal flame temperature distribution is obtained from conditional-averaged OH fluorescence intensities at the OH front taken with two different excitation lines. CO and NOx emission characteristics of the controlled flame are discussed on the basis of the local fuel and OH distributions and the flame temperature. 相似文献
6.
H.S. Zhen C.W. Leung C.S. Cheung 《International Journal of Heat and Mass Transfer》2010,53(5-6):902-909
The thermal and emission characteristics of a swirl-stabilized turbulent inverse diffusion flame (IDF) burning liquefied petroleum gas (LPG) were studied experimentally and the results of visible flame lengths, flame temperatures, in-flame gaseous species concentrations and global pollutant emissions were reported.The flame shape and length of the swirling IDF and a non-swirling IDF were compared. The swirling IDF is featured by a large internal recirculation zone (IRZ), which plays an important role in stabilizing and shortening the flame. Compared with the non-swirling IDF, the swirling IDF is shorter, wider and more stable. For the swirling IDF, both temperature and species distributions are uniform in the IRZ. Comparison of the radial NOx/temperature distributions indicates that the thermal NO mechanism plays a leading role in NOx formation, since the high-temperature IRZ favors thermal NO production. The effects of air jet Reynolds number (Re) and overall equivalence ratio (Ф) on centerline temperature and emission index were examined. The main finding is that the IRZ which is large in size and high in temperature dominates the thermal and emission characteristics of the swirling flame.Efforts were made to compare the global NOx and CO emissions of the swirling and non-swirling IDFs. It was found that strong swirl and lean combustion are two key factors for reducing NOx emission. However, the decreasing NOx emission is compromised by increasing CO. Under stoichiometric and rich conditions, EINOx of the swirling IDFs is slightly higher, but the EICO is significantly lower. Further comparison of EINOx with other studies indicates that the swirling IDF can achieve low NOx emission. 相似文献
7.
The overall pollutants emission from impinging swirling and non-swirling inverse diffusion flames (IDFs) was evaluated quantitatively by the ‘hood’ method. The results of in-flame volumetric concentrations of CO and NOx and overall pollutants emission of CO and NOx in terms of emission index were reported. The in-flame volumetric concentrations of CO and NOx were measured through a small hole drilled on the impingement plate. In comparison with the corresponding open flame, the CO and NOx concentrations for the impinging swirling IDF are greatly lowered due to the entrainment of much more ambient air which is related to the increased flame surface area. For the swirling and non-swirling IDFs, the EINOx increases as the nozzle-to-plate distance (H) increases because more space is available for the development of the high-temperature zone in the free jet portion of the impinging flame, which favors the thermal NO formation. The variation of EICO with H is different for the impinging swirling and non-swirling IDFs because they have different flame structures. For both flames, the EICO is high when their main reaction zone or inner reaction cone is impinged and quenched by the copper plate. The parameters of air jet Reynolds number, overall equivalence ratio and nozzle-to-plate distance have significant influence on the overall pollutants emission of the impinging swirling and non-swirling IDFs and the comparison shows that the swirling IDF emits less NOx and CO under most of the experimental conditions tested. Furthermore, it is found that compared with the open flames, the impinging flames emit lower level of NOx and higher level of CO. 相似文献
8.
《International Journal of Hydrogen Energy》2022,47(60):25404-25417
The impact of pilot flame operation on the combustion of pure methane and hydrogen-enriched methane (H2/CH4: 50/50 in vol%) fuels was investigated in a gas turbine model combustor under atmospheric conditions. The burner assembly was designed to mimic the geometry of an industrial burner, the Siemens DLE Burner, in which a concentric annular ring equipped with pilot flame burners is implemented in the dome of the combustor. Two pilot burner configurations have been investigated: a non-premixed and a partially premixed pilot arrangement. The performance of the pilot burners was evaluated for varying Reynolds number (Re) and H2 enrichment. High-speed OH1 chemiluminescence imaging, as well as simultaneous planar laser-induced fluorescence measurements of the OH radicals and formaldehyde (CH2O) were used for evaluating the dynamics and structures of the flames for different conditions. Furthermore, emission measurements were carried out to determine the influence of hydrogen dilution on the NOx and CO emission levels. The main findings are (a) the effect of the pilot flame is sensitive to the Reynolds number of the main flame and the type of the pilot flame, (b) the stability range becomes narrower with increasing hydrogen ratio, due to the tendency to flashback, (c) non-premixed pilot flames lower the NOx and increase the CO emissions, albeit rather small differences in the emissions have been detected, and (d) the NOx and CO emissions become significantly lower with increasing hydrogen ratio. 相似文献
9.
Parag Rajpara Rupesh Shah Jyotirmay Banerjee 《International Journal of Hydrogen Energy》2018,43(36):17505-17519
The present research aims to assess the potential of hydrogen in the form of a supplementary fuel to accelerate combustion chemistry and reduce CO emissions of methane fuelled upward swirl gas turbine combustor. Effects of hydrogen enrichment on flame characteristics and chemical kinetics are analysed using Large Eddy Simulations (LES). Flame visualization is performed and measurements of temperature and emissions at the exit of combustor are reported. For the same energy input, flames are relatively broader and shorter at higher hydrogen concentrations. Augmentation of hydrogen is advantageous in terms of flame velocity, temperature, rate of chemical reactions and CO emissions. Higher flame temperature favours NOx emissions at higher hydrogen content. At a constant volumetric fuel flow, reduction in carbon-generated species is attributed to hydrocarbon substitution and chemical kinetic effects are less. Hydrogen addition increases flame temperature, decreases flame dimensions and reduces CO emissions with marginal increase in NOx emissions. 相似文献
10.
The effects of bluff-body lip thickness on the several physical parameters like flame length, radiant fraction, gas temperature and NOx emissions in liquefied petroleum gas (LPG)–H2 jet diffusion flame are investigated experimentally. Results indicate that the flame length reduces with the addition of hydrogen in the bluff-body stabilized flame, which can be attributed to the enhanced reactivity and residence time of the mixture gases. Moreover, with increasing lip thickness of the bluff body, the flame length also gets reduced. The soot free length fraction (SFLF) is observed to be enhanced with H2 addition to the fuel stream. In contrast, the SFLF gets reduced with increasing lip thickness repetition, which is due to the reduced induction period of soot formation. The emission index of NOx (EINOx) is found to be attenuated in coaxial burner with hydrogen addition. In contrast it is observed to be enhanced in bluff-body stabilized flame. The former is due to the reduction in residence time of gas mixture, whereas the latter can be explained on the basis of increased flame temperature. Besides this, NOx emission level is also found to be enhanced with increasing lip thickness due to enhanced residence time. 相似文献
11.
《International Journal of Hydrogen Energy》2017,42(32):20809-20823
The present study numerically investigated the effect of oxygen enrichment on the precise structure and NOx formation characteristics of turbulent syngas non-premixed flames. The turbulence-chemistry interactions were represented by a Lagrangian flamelet model. In context with the Lagrangian flamelet model, the NO concentration was obtained directly from the flamelet calculation based on full NOx chemistry, with radiative heat loss being accounted for through the flamelet energy equation. Computations were performed for three different syngas compositions with a designated nitrogen dilution level. Numerical results indicated that, for the CO-rich composition with the lowest LHV yielding the highest scalar dissipation rate and shortest flight time, the flame structure was dominantly influenced by turbulence-chemistry interactions. On the other hand, with regard to the H2-rich composition with the highest LHV yielding the lowest injection velocity and longest flight time, the flame structure was strongly influenced by radiative cooling. The peak NO level was remarkably elevated by increased oxygen level due to the elevated temperature of the oxygen-enriched flame. In the enhanced oxygen level (30%), the H2-rich case produced the highest NO level due to a higher temperature and longer residence time within the hot flame zone, while the CO-rich case yielded the lowest NO level due to a lower temperature and shorter residence time. It was also found that, by enhancing the oxygen level, contributions of NNH and N2O to total NO emission rapidly decreased while the contributions of the thermal NO path were progressively dominant for all cases. 相似文献
12.
By using OH-PLIF technique, experiments were conducted for laminar Bunsen flame of premixed CO/H2/air mixtures with equivalence ratio ranging from 0.5 to 1.8. Reynolds number was varied from 800 to 2200, XH2 = H2/(H2+CO) in the mixture was varied from 20% to 100% to study the effects of both preferential diffusion and flame curvature on flame structures and laminar flame burning velocities. Results showed that the combined effects of preferential diffusion and curvature gave an interesting phenomenon of the flame OH radical distributions on high hydrogen content flames. Furthermore, with the increase of H2 fraction in fuel mixture, the effects of both preferential diffusion and flame curvature were increased. Interpretation of flame stretch effect on laminar burning velocity is also provided in this paper. 相似文献
13.
Jeong Park Dong Jin Hwang June Sung Park Jeong Soo Kim Sang In Keel Han Chang Cho Dong Soon Noh Tae Kwon Kim 《国际能源研究杂志》2007,31(5):472-485
Hydrogen-blending effects in flame structure and NO emission behaviour are numerically studied with detailed chemistry in methane–air counterflow diffusion flames. The composition of fuel is systematically changed from pure methane to the blending fuel of methane–hydrogen through H2 molar addition up to 30%. Flame structure, which can be described representatively as a fuel consumption layer and a H2–CO consumption layer, is shown to be changed considerably in hydrogen-blending methane flames, compared to pure methane flames. The differences are displayed through maximum flame temperature, the overlap of fuel and oxygen, and the behaviours of the production rates of major species. Hydrogen-blending into hydrocarbon fuel can be a promising technology to reduce both the CO and CO2 emissions supposing that NOx emission should be reduced through some technologies in industrial burners. These drastic changes of flame structure affect NO emission behaviour considerably. The changes of thermal NO and prompt NO are also provided according to hydrogen-blending. Importantly contributing reaction steps to prompt NO are addressed in pure methane and hydrogen-blending methane flames. Copyright © 2006 John Wiley & Sons, Ltd. 相似文献
14.
R.W. Schefer W.D. Kulatilaka B.D. Patterson T.B. Settersten 《Combustion and Flame》2009,156(6):1234-1241
The common misconception that hydrogen flames are not visible is examined. Examples are presented of clearly visible emissions from typical hydrogen flames. It is shown that while visible emissions from these flames are considerably weaker than those from comparable hydrocarbon flames, they are indeed visible, albeit at reduced light levels in most cases. Detailed flame spectra are presented to characterize flame emission bands in the ultraviolet, visible and infrared regions of the spectrum that result in a visible hydrogen flame. The visible blue emission is emphasized, and recorded spectra indicate that fine spectral structure is superimposed on a broadband continuum extending from the ultraviolet into the visible region. Tests were performed to show that this emission does not arise from carbon or nitrogen chemistry resulting from carbon-containing impurities (hydrocarbons) in the hydrogen fuel or from CO2 or N2 entrainment from the surrounding air. The spectral structure, however, is also observed in methane flames. The magnitude of the broadband emission increases with flame temperature in a highly nonlinear manner while the finer spectral structure is insensitive to temperature. A comparison of diffusion and premixed H2 flames shows that the fine scale structure is comparable in both flames. 相似文献
15.
Experiments were performed to add hydrogen to liquefied petroleum gas (LPG) and methane (CH4) to compare the emission and impingement heat transfer behaviors of the resultant LPG–H2–air and CH4–H2–air flames. Results show that as the mole fraction of hydrogen in the fuel mixture was increased from 0% to 50% at equivalence ratio of 1 and Reynolds number of 1500 for both flames, there is an increase in the laminar burning speed, flame temperature and NOx emission as well as a decrease in the CO emission. Also, as a result of the hydrogen addition and increased flame temperature, impingement heat transfer is enhanced. Comparison shows a more significant change in the laminar burning speed, temperature and CO/NOx emissions in the CH4 flames, indicating a stronger effect of hydrogen addition on a lighter hydrocarbon fuel. Comparison also shows that the CH4 flame at α = 0% has even better heat transfer than the LPG flame at α = 50%, because the longer CH4 flame configures a wider wall jet layer, which significantly increases the integrated heat transfer rate. 相似文献
16.
17.
This study is concerned with the response of conical flames to acoustic modulations. It deals with the dynamics of the velocity field in the fresh gases feeding the flame. Experiments are carried out to determine the gain and phase shift between the excitation signal and the axial velocity signal. This information, combined with PIV data, is used to identify the propagation mode in the fresh stream. Experiments indicate that three ranges can be defined based on a Strouhal number St involving the burner diameter and the upstream flow velocity. When this number is sufficiently low (St?1), the response consists in a convective wave featuring a phase velocity close to that of the mean flow. As St is augmented (1?St?Stc), where Stc depends on the flame geometry, the phase difference between the velocity oscillation and the imposed signal nearly vanishes in a finite region adjacent to the burner exhaust indicating that the perturbation propagates at the speed of sound. Further away from the burner, velocity perturbations exhibit convective features again. In the third frequency range, corresponding to higher modulation frequencies (St?Stc), velocity perturbations are dominated by acoustics in most of the experimental domain. It is shown that this behavior results from the upstream influence of the flame wrinkling. The region of influence may be deduced by considering the velocity potential associated with the flame motion. When this perturbation potential takes large values, the flow is dominated by the convective wave. This suitably reproduces experimental observations. 相似文献
18.
Non-premixed acoustically perturbed swirling flame dynamics 总被引:1,自引:0,他引:1
Uyi Idahosa 《Combustion and Flame》2010,157(9):1800-1814
An investigation into the response of non-premixed swirling flames to acoustic perturbations at various frequencies (fp = 0-315 Hz) and swirl intensities (S = 0.09 and 0.34) is carried out. Perturbations are generated using a loudspeaker at the base of an atmospheric co-flow burner with resulting velocity oscillation amplitudes |u′/Uavg| in the 0.03-0.30 range. The dependence of flame dynamics on the relative richness of the flame is investigated by studying various constant fuel flow rate flame configurations. Flame heat release rate is quantitatively measured using a photomultiplier with a 430 nm bandpass filter for observing CH∗ chemiluminescence which is simultaneously imaged with a phase-locked CCD camera. The flame response is observed to exhibit a low-pass filter characteristic with minimal flame response beyond pulsing frequencies of 200 Hz. Flames at lower fuel flow rates are observed to remain attached to the central fuel pipe at all acoustic pulsing frequencies. PIV imaging of the associated isothermal fields show the amplification in flame aspect ratio is caused by the narrowing of the inner recirculation zone (IRZ). Good correlation is observed between the estimated flame surface area and the heat release rate signature at higher swirl intensity flame configurations. A flame response index analogous to the Rayleigh criterion in non-forced flames is used to assess the potential for a strong flame response at specific perturbation configurations and is found to be a good predictor of highly responsive modes. Phase conditioned analysis of the flame dynamics yield additional criteria in highly responsive modes to include the effective amplitude of velocity oscillations induced by the acoustic pulsing. In addition, highly responsive modes were characterized by velocity to heat release rate phase differences in the ±π/2 range. A final observed characteristic in highly responsive flames is a Strouhal number between 1 and 3.5 based on the burner co-flow annulus diameter (St = fpUavg/dm). Finally, wavelet analyses of heat release rate perturbations indicate highly responsive modes are characterized by sustained low frequency oscillations which accompany the high amplitude velocity perturbations at these modes. Higher intensity low frequency heat release rate oscillations are observed for lean flame/low pulsing frequency conditions. 相似文献
19.
Seungro LeeOh Chae Kwon 《International Journal of Hydrogen Energy》2011,36(16):10117-10128
The potential of partial ammonia substitution to improve the safety of hydrogen use was evaluated computationally, using counterflow nonpremixed ammonia/hydrogen/air flames at normal temperature and pressure. The ammonia-substituted hydrogen/air flames were considered using a recent kinetic mechanism and a statistical narrow-band radiation model for a wide range of flame strain rates and the extent of ammonia substitution. The effects of ammonia substitution on the extinction limits and structure, including nitrogen oxide (NOx) and nitrous oxide (N2O) emissions, of nonpremixed hydrogen/air flames were investigated. Results show reduction of the high-stretch extinction (i.e., blow-off) limits, the maximum flame temperature and the concentration of light radicals (e.g., H and OH) with ammonia substitution in hydrogen/air flames, supporting the potential of ammonia as a carbon-free, clean additive for improving the safety of hydrogen use in nonpremixed hydrogen/air flames. For high-stretched flames, however, NOx and N2O emissions substantially increase with ammonia substitution even though ammonia substitution reduces flame temperature, implying that chemical effects (rather than thermal effects) of ammonia substitution on flame structure are dominant. Radiation effects on the extinction limits and flame structure are not remarkable particularly for high-stretched flames. 相似文献
20.
《International Journal of Hydrogen Energy》2020,45(39):20426-20435
This paper investigated the hydrogen enriched methane/air flames diluted with CO2. The turbulent premixed flame was stabilized on a Bunsen type burner and the two dimensional instantaneous OH profile was measured by Planar Laser Induced Fluorescence (PLIF). The flame front structure characteristics were obtained by extracting the flame front from OH-PLIF images. And the turbulence-flame interaction was analyzed through the statistic parameters. The role of hydrogen addition as well as CO2 dilution on the features of turbulent flame were revealed by those parameters. In this work, hydrogen fractions of 0, 0.2 and CO2 dilution ratios of 0, 0.05 and 0.1 were studied. Results showed that hydrogen addition can enhance turbulent burning velocity ST/SL through decreasing the scale of the finer structure of the wrinkled flame front, caused by the smaller flame instability scale. In contrast, CO2 dilution decreased turbulent burning velocity ST/SL due to its inactive response to turbulence perturbation and larger flame wrinkles. For all flames, the probability density function (PDF) profile of the local curvature radius R shows a bias to positive value, resulted from the flame intrinsic instability. The PDF profile of R decreases with CO2 dilution, while the value of local curvature radius corresponding to the peak PDF is larger. This indicates that larger wrinkles structure was generated due to CO2 dilution, which leads to the decrease in ST/SL as a consequence. Hydrogen addition increases the flame volume and results in more intense combustion. CO2 dilution has a decrease effect on flame volume for both XH2 = 0 and XH2 = 0.2 while the decrease is obvious at XH2 = 0.2, ZCO2 = 0.1. In all, hydrogen enrichment improves the combustion while CO2 can moderate combustion. Therefore, adding hydrogen and CO2 in natural gas can be a potential method for adjusting the combustion intensity in combustion chamber during the combustor design. 相似文献