3He Spin Filter for Neutrons

The strongly spin-dependent absorption of neutrons in nuclear spin-polarized ³He opens up the possibility of polarizing neutrons from reactors and spallation sources over the full kinematical range of cold, thermal and hot neutrons. This paper gives a report on the neutron spin filter (NSF) development program at Mainz. The polarization technique is based on direct optical pumping of metastable ³He atoms combined with a polarization preserving mechanical compression of the gas up to a pressure of several bar, necessary to run a NSF. The concept of a remote type of operation using detachable NSF cells is presented which requires long nuclear spin relaxation times of order 100 hours. A short survey of their use under experimental conditions, e.g. large solid-angle polarization analysis, is given. In neutron particle physics NSFs are used in precision measurements to test fundamental symmetry concepts.     

Compressing Spin-Polarized 3He With a Modified Diaphragm Pump

Nuclear spin-polarized ³He gas at pressures on the order of 100 kPa (1 bar) are required for several applications, such as neutron spin filters and magnetic resonance imaging. The metastability-exchange optical pumping (MEOP) method for polarizing ³He gas can rapidly produce highly polarized gas, but the best results are obtained at much lower pressure (~0.1 kPa). We describe a compact compression apparatus for polarized gas that is based on a modified commercial diaphragm pump. The gas is polarized by MEOP at a typical pressure of 0.25 kPa (2.5 mbar), and compressed into a storage cell at a typical pressure of 100 kPa. In the storage cell, we have obtained 20 % to 35 % ³He polarization using pure ³He gas and 35 % to 50 % ³He polarization using ³He-⁴He mixtures. By maintaining the storage cell at liquid nitrogen temperature during compression, the density has been increased by a factor of four.     

A New Method for Precision Cold Neutron Polarimetry Using a 3He Spin Filter

We present a new method for precision measurement of the capture flux polarization of a polychromatic (white), continuous cold neutron beam, polarized by a ³He spin filter. This method allows an in situ measurement and does not require knowledge of the neutron beam wavelength distribution. We show that a polarimetry precision of 0.1 % is possible.     

Test of He-based neutron polarizers at NIST

Neutron spin filters based on polarized ³He are useful over a wide neutron energy range and have a large angular acceptance among other advantages. Two optical pumping methods, spin-exchange and metastability-exchange, can produce the volume of highly polarized ³He gas required for such neutron spin filters. We report a test of polarizers based on each of these two methods on a new cold, monochromatic neutron beam line at the NIST Center for Neutron Research.     

Precision Neutron Polarimetry for Neutron Beta Decay

The abBA collaboration is developing a new type of field-expansion spectrometer for a measurement of the three correlation coefficients a, A, and B and the shape parameter b. The measurement of A and B requires precision neutron polarimetry. We will polarize a pulsed cold neutron beam from the SNS using a ³He neutron spin filter. The well-known polarizing cross section for n-³He has a 1/v dependence, where v is the neutron velocity, which is used to determine the absolute beam polarization through a time-of-flight (TOF) measurement. We show that by measuring the TOF dependence of A and B, the coefficients and the neutron polarization can be determined with a small loss of the statistical precision and with negligible systematic error. We conclude that it is possible to determine the neutron polarization averaged over a long run in the neutron beta decay experiment with a statistical error less than 10⁻⁴. We discuss various sources of systematic uncertainty in the measurement of A and B and conclude that the fractional systematic errors are less than 2 × 10⁻⁴.     

Packed Powder as Superleak for Spin Pump Experiments in Superfluid 3He A1

Experimental exploration of highly spin-polarized states of liquid ³He by applying external magnetic field is limited by the availability of static magnetic field. In the “ferromagnetic” superfluid A₁ phase of liquid ³He there is an alternate method for boosting spin-polarization by the process of spin pumping without requiring such high magnetic field. The spin pumping in the A₁ phase takes advantage of a superleak (SL) acting simultaneously as a filter for both entropy and spin. The spin pump technique that uses the SL-spin filter and a mechanical actuator enables us to directly boost polarization of ³He. The amount of enhancement of spin polarization has been limited so far. We are now developing a new type of SL filter made of packed aluminum oxide powder (referred as PAP-SL), in order to achieve greater enhancement of spin polarization. Several kinds of the PAP-SL filter were constructed by pressing aluminum oxide powders into a cylinder holder. The packed structures were carefully characterized by a flow-rate-measurement, X-ray tomography, and mercury intrusion porosimetry. The preliminary result shows that the PAP-SL works as SL filter for the superfluid ³He.     

Observation of the 3He(n,tp) Reaction by Detection of Far-Ultraviolet Radiation

We have detected Lyman alpha radiation, 121.6 nm light produced from the n = 2 to n = 1 transition in atomic hydrogen, as a product of the ³He(n, tp) nuclear reaction occurring in a cell of ³He gas. The predominant source of this radiation appears to be decay of the 2p state of tritium produced by charge transfer and excitation collisions with the background ³He gas. Under the experimental conditions reported here we find yields of tens of Lyman alpha photons for every neutron reaction. These results suggest a method of cold neutron detection that is complementary to existing technologies that use proportional counters. In particular, this approach may provide single neutron sensitivity with wide dynamic range capability, and a class of neutron detectors that are compact and operate at relatively low voltages.     

Recent Experiments on Spin Polarized Liquid 3He

The importance of spin fluctuations on the physical properties of liquid ³ He can be probed by studying the polarization dependence of its magnetic susceptibility and viscosity. We discuss the present state of two such experiments. Using the rapid melting technique, to strongly polarize liquid ³ He, we have measured the viscosity enhancement induced by the polarization up to unprecedented large polarizations at a low temperature (80 mK). At a polarization of 60 %, the enhancement reaches a factor 2.5, comparable to that of the inverse susceptibility at the same polarization. Now at Oxford Instruments Research Instruments     

He and BF3 neutron detector pressure effect and model comparison

Radiation detection systems for homeland security applications must possess the capability of detecting both gamma rays and neutrons. The radiation portal monitor systems that are currently deployed use a plastic scintillator for detecting gamma rays and ³He gas-filled proportional counters for detecting neutrons. Proportional counters filled with ³He are the preferred neutron detectors for use in radiation portal monitor systems because ³He has a large neutron cross-section, is relatively insensitive to gamma-rays, is neither toxic nor corrosive, can withstand extreme environments, and can be operated at a lower voltage than some of the alternative proportional counters. The amount of ³He required for homeland security and science applications has depleted the world supply and there is no longer enough available to fill the demand. Thus, alternative neutron detectors are being explored.Two possible temporary solutions that could be utilized while a more permanent solution is being identified are reducing the ³He pressure in the proportional counters and using boron trifluoride gas-filled proportional counters. Reducing the amount of ³He required in each of the proportional counters would decrease the rate at which ³He is being used; not enough to solve the shortage, but perhaps enough to increase the amount of time available to find a working replacement. Boron trifluoride is not appropriate for all situations as these detectors are less sensitive than ³He, boron trifluoride gas is corrosive, and a much higher voltage is required than what is used with ³He detectors. Measurements of the neutron detection efficiency of ³He and boron trifluoride as a function of tube pressure were made. The experimental results were also used to validate models of the radiation portal monitor systems.     

Heat conduction in spin-polarized gaseous3He at low temperature

A dilute gas of³He exhibits an interesting dependence of its transport properties on the nuclear spin polarization, resulting from the indistinguishability of the fermions during binary collisions. This article reports experimental results on the heat conductivity of gaseous³He in the 1.2–4.2 K range, the gas being polarized by laser optical pumping. The heat conductivity is found to change with the nuclear polarization. Compared to preliminary data already reported, the present work has been carried out with more care to control all the heat fluxes reaching the measurement cell, and the temperature range has been extended. The results are compared to recently improved calculations. The temperature dependence of the effect is now found to be in satisfactory agreement with theory.     

Radio frequency-induced polarization of ultra-cold neutrons or how to pump a two-level system

The well-known technique of optical pumping can be used to polarize a neutron beam in a transient way. In our experiment we demonstrate that an unpolarized beam of ultra-cold neutrons (UCN), interacting solely with a set of magnetic fields can become polarized without losing the “wrong” spin component.     

Brute Force Polarization of 129Xe

Hyperpolarized ¹²⁹Xe has numerous applications in Nuclear magnetic resonance (NMR) and magnetic resonance imaging(MRI). As an alternative to the laser optical pumping method of production of hyperpolarized ¹²⁹Xe gas, we have investigated the brute force technique which uses a very high magnetic field and millikelvin temperatures. One obstacle to this technique is the extremely long spin lattice relaxation times of nuclei in solids at very low temperature. We exploit the fact that liquid ³He can be used as an effective relaxant to enable ¹²⁹Xe to be spin polarized on a high surface area substrate in a few hours. We are able to identify the contributions of different atomic layers to the magnetization by analyzing the ¹²⁹Xe NMR spectrum. Furthermore, the addition of ⁴He allows us to turn off the relaxation mechanism, thereby preserving the polarization. The technique could be applied to nuclei other than ¹²⁹Xe.     

Enhanced variant designs and characteristics of the microstructured solid-state neutron detector

Silicon diodes with large aspect ratio perforated microstructures backfilled with ⁶LiF show a dramatic increase in neutron detection efficiency beyond that of conventional thin-film coated planar devices. Described in this work are advancements in the technology with increased microstructure depths and detector stacking methods to increase thermal neutron detection efficiency. The highest efficiency devices thus far have delivered over 37% intrinsic thermal neutron detection efficiency by device-coupling stacking methods. The detectors operate as conformally diffused pn junction diodes with 1 cm² square-area. Two individual devices were mounted back-to-back with counting electronics coupling the detectors together into a single dual-detector device. The solid-state silicon device operated at 3 V and utilized simple signal amplification and counting electronic components. The intrinsic detection efficiency for normal-incident 0.0253 eV neutrons was found by calibrating against a ³He proportional counter and a ⁶LiF thin-film planar semiconductor device. This work is a part of on-going research to develop solid-state semiconductor neutron detectors with high detection efficiencies and uniform angular responses.     

Superfluid 3He in Presence of Spin-Polarized Scattering Centers

The influence of spin-exchange scattering centers on triplet Cooper pairing is considered by exploring the behavior of superfluid ³He in high porosity aerogel, containing ³He atoms localized on the surface of silica strands. The homogeneously distributed isotropic scattering system of spin-polarized impurity centers is adopted as a simple model to investigate the contribution of the spin-exchange scattering channel for quasiparticles to the formation of non-unitary superfluid A₁-phase in the aerogel environment. It is demonstrated that an interference between the potential and exchange parts of quasiparticle scattering from spin-polarized impurity centers can change considerably the temperature width and the spin structure of the A₁-phase in aerogel. PACS numbers: 05.70 Ln, 05.70 Jk, 64.     

A multipurpose He refrigerator

We introduce a mini ³He refrigerator, operating at ∼300 mK starting from 4.2 K without pumping on the main ⁴He bath. The innovative idea is that the present one is suitable for a very fast operation; for its use, it is sufficient a storage ⁴He Dewar. In this way we drastically reduce the time required to cool it down, because there is no need for a classic cryostat. This prototype is particularly aimed for all those operations in which it is necessary to test a large number of samples that do not require long duration measurements at low temperature.     

The effect of the demagnetizing field on coherent spin precession in a normal fermi liquid

We consider an effect of the demagnetizing field, produced by the magnetic moments of nuclei of³He, on coherent precession of spin in liquid spin polarized³He or in spin polarized solutions of³He in⁴He. Formulae for the shape of the precessing domain wall and for the relaxation rate of the coherently precessing structure are rederived taking into account the demagnetizing field. For pure³He and concentrated solutions of³He in⁴He the width of the domain wall increases and the relaxation rare decreases with polarization. Measurement of the relaxation rate of the precessing structure can be used as an alternative method for the determination of the spin diffusion coefficient in Fermi liquids.     

Bulk nuclear polarization of solid3He

Measurements are given on the bulk nuclear spin polarization in a liquid-solid³He mixture cooled by compressional cooling to below 5 mK in a magnetic field of 54.5 kG. Owing to the low Pauli spin susceptibility of liquid³He, the observed polarization is primarily due to solid³He. A maximum average nuclear polarization of 47% was observed, although the corresponding solid³He polarization is believed to be higher. Our novel detection system, using a dual directional coupler for cw NMR, is a simple and versatile means of working in the awkward frequency range around 180 MHz. We also report transient heating measurements in the³He system which indicate that the internal thermal equilibrium time in bulk solid³He on the³He melting curve appears to be quite short (less than 5 min) at these temperatures. One type of transient measurement is complicated by the dramatic effect of the contribution of the³He nuclear magnetization to the total local magnetic field. This contribution is considered via a simple model.This work has been supported by the U.S. Atomic Energy Commission under Contract No. AT(04-3)-34, P.A. 143.     

Neutron detection gamma ray sensitivity criteria

The shortage of ³He has triggered the search for effective alternative neutron detection technologies for national security and safeguards applications. Any new detection technology must satisfy two basic criteria: (1) it must meet a neutron detection efficiency requirement, and (2) it must be insensitive to gamma-ray interference at a prescribed level, while still meeting the neutron detection requirement. It is the purpose of this paper to define measureable gamma ray sensitivity criteria for neutron detectors. Quantitative requirements are specified for: intrinsic gamma ray detection efficiency and gamma ray absolute rejection. The gamma absolute rejection ratio for neutrons (GARRn) is defined, and it is proposed that the requirement for neutron detection be 0.9<GARRn<1.1 at a 10 mR/h exposure rate. An example of the results from a ³He based neutron detector is provided showing that this technology can meet the stated requirements. Results from tests of some alternative technologies are also reported.     

Liquid4He as a cryogenic coating for gaseous spin polarized3He

Nuclear spin polarization can be produced by optical pumping of³He gas in sealed samples at a temperature below 1 K. The wall relaxation can be minimized by covering the container walls with a⁴He film, and relaxation timesT ₁ longer than 1000 sec have been observed. A study of the residual relaxation is reported here. Spin relaxation appears to take place near the helium-substrate boundary. This situation is characterized by an adsorption energy very different from the known binding energies of³He quasiparticles on and in bulk liquid⁴He. Models are presented which reproduce the observedT ₁ variations on temperature and on other experimental parameters.Laboratoire associé au Centre National de la Recherche Scientifique et à l'Université Paris VI.     

On Polarization-Induced Zero Temperature Spin Wave Damping in Dilute 3He

We have observed spin waves in dilute ³ He, spin polarized by a ⁴ He circulating dilution refrigerator. The maximum polarization is a factor 5 higher than the equilibrium polarization in the magnetic field of 10.54 T at temperatures between 10 and 20 mK. The measured spin wave damping is about a factor 4 lower than the damping expected from previous spin echo experiments in ³ He- ⁴ He mixtures, which confirmed the prediction of polarization-induced spin wave damping at zero temperature in Fermi liquids. Our experiment shows that the existence of polarization-induced spin wave damping remains an open question.