Simulation of Multi-Steady States in Low Temperature Gas Discharge

This article presents hydrodynamics simulation of multi-steady states and mode transition by DC-beam-injected gas discharge, and provides a model approach to hysteresis and distinct forms of multi-steady states. The critical transition conditions of the three discharge modes (temperature limited mode, Langmuir mode, and space charge limited mode) are estimated to be dependent on the gas pressure and the filament temperature. Various forms of the multi-steady states in gas discharge can be uniformly explained by the displacement of the mutant positions.The simulation results are in a good agreement with those of the experiments.     

Investigation on the Micro-Discharge Characteristics of Dielectric Barrier Discharge in a Needle-Plate Geometry

In this study, a dielectric barrier discharge device with needle-plate electrodes was used to investigate the characteristics of the micro-discharge in argon at one atmospheric pressure by an optical method. The results show that there are two discharge modes in the dielectric barrier discharge, namely corona mode and filamentary mode. The corona discharge only occurs in the vicinity of the needle tip when the applied voltage is very low. However, the filamentary discharge mode can occur, and micro-discharge bridges the two electrodes when the applied voltage reaches a certain value. The extended area of micro-discharge on the dielectric plate becomes larger with the increase in applied voltage or decrease in gas pressure. The variance of the light emission waveforms is studied as a function of the applied voltage. Results show that very short discharge pulse only appears at the negative half cycle of the applied voltage in the corona discharge mode. However, broad hump (about several microseconds) can be discerned at both the negative half cycle and the positive half cycle for a high voltage in the filamentary mode. Furthermore, the inception voltage decreases and the width of the discharge hump increases with the increase in applied voltage. These experimental phenomena can be explained qualitatively by analyzing the discharge mechanism.     

An Experimental Study on Atmospheric Pressure Glow Discharge in Different Gases

Usually,the electrical breakdown of dielectric barrier discharge(DBD) at atmospheric pressure leads to a filamentary non-homogeneous discharge,However,it is also possible to obtain a diffuse DBD in homogeneous form,called atmospheric pressure glow discharge(APGD).We obtained a uniform APGD in helium and in the mixture of argon with alcohol,and studied the electrical characteristics of helium APGD.It if found that the relationship between discharge current and source frequency is different depending on the difference in gas gap when the applied voltage is kept constant.The discharge current shows an increasing trend with the increased frequency when gas gap is 0.8cm ,but the discharge current tends to decrease with the increased frequency when the gas gap increases.The discharge current always increases with the increased applied voltage when the source frequency is kept constant.We also observed a glow-like discharge in nitrogen at atmospheric pressure.     

Surface Treatment of Polyethylene Terephthalate Film Using Atmospheric Pressure Glow Discharge in Air

Non-thermal plasmas under atmospheric pressure are of great interest in polymer surface processing because of their convenience, effectiveness and low cost. In this paper, the treatment of Polyethylene terephthalate (PET) film surface for improving hydrophilicity using the non-thermal plasma generated by atmospheric pressure glow discharge (APGD) in air is conducted. The discharge characteristics of APGD are shown by measurement of their electrical discharge parameters and observation of light-emission phenomena, and the surface properties of PET before and after the APGD treatment are studied using contact angle measurement, x-ray photoelectron spectroscopy (XPS) and scanning electron microscopy (SEM). It is found that the APGD is homogeneous and stable in the whole gas gap, which differs from the commonly filamentary dielectric barrier discharge (DBD). A short time (several seconds) APGD treatment can modify the surface characteristics of PET film markedly and uniformly. After 10 s APGD treatment, the     

Measurement of the first Townsend's ionization coefficient for atmospheric pressure neon by a dielectric barrier discharge

Fast photography and optical emission spectroscopy are implemented in a 5 mm neon gap dielectric barrier discharge (DBD) at atmospheric pressure with quartz glass used as the dielectric layer. Results show that it starts with a Townsend discharge and ends at a sub-normal glow discharge in neon DBD. Based on the Townsend discharge, the first ionization coefficient of neon is measured. The measurements are consistent with those at low pressure. Optical emission spectroscopy indicates that the spectra are mainly composed of atomic lines of neon, molecular bands and molecular ion bands originating from inevitable gas impurities (mainly nitrogen). Moreover, spectral lines emitted from atomic neon corresponding to the transitions (2p⁵ 3p → 2p⁵ 3s) are predominant. Although the second positive system of N₂(C³Π_u → B³Π_g) is observed, their intensities are too weak compared with neon's spectrum. The molecular nitrogen ion line of 391.4 nm is observed. It reveals that Penning ionization between high energy neon excited states and the inevitable gas impurities plays an important role in the value of the α coefficient.     

Self-Consistent Model for Pulsed Direct-Current N2 Glow Discharge

A self-consistent analysis of a pulsed direct-current (DC) N2 glow discharge is presented. The model is based on a numerical solution of the continuity equations for electron and ions coupled with Poisson‘s equation. The spatial-temporal variations of ionic and electronic densities and electric field are obtained. The electric field structure exhibits all the characteristic regions of a typical glow discharge (the cathode fall, the negative glow, and the positive column). Current-voltage characteristics of the discharge can be obtained from the model. The calculated current-voltage results using a constant secondary electron emission coefficient for the gas pressure 133.32 Pa are in reasonable agreement with experiment.     

Transition from Spark Discharge to Constricted Glow Discharge in Atmospheric Air by Capacitor Coupled Discharge

The transition from a spark discharge to a constricted glow discharge in atmospheric air was studied with a capacitor coupled pin-to-water plasma reactor. The reason of the transition is considered to be of various factors, namely the change of the air gap due to the polarization of water molecules by the electric field, the feedback effect of the capacitors, and the ion trapping mechanism. The effects of the frequency of the power supply, inter-electrode gap, and coupled capacitance on the discharge transition were also investigated.     

Characteristics of a Normal Glow Discharge Excited by DC Voltage in Atmospheric Pressure Air

Atmospheric pressure glow discharges were generated in an air gap between a needle cathode and a water anode. Through changing the ballast resistor and gas gap width between the electrodes, it has been found that the discharges are in normal glow regime judged from the currentvoltage characteristics and visualization of the discharges. Results indicate that the diameter of the positive column increases with increasing discharge current or increasing gap width. Optical emission spectroscopy is used to calculate the electron temperature and vibrational temperature. Both the electron temperature and the vibrational temperature increases with increasing discharge current or increasing gap width. Spatially resolved measurements show that the maxima of electron temperature and vibrational temperature appeared in the vicinity of the needle cathode.     

氢气放电源打靶谱的分析

在以氢气放电源打钆靶为例,分析氢气放电源打靶谱时,发现有以下几类谱线:源谱、靶材料的特征X射线、衍射谱线和一些未知谱线。根据打靶的初级谱可以分辨出源谱;根据靶材料的成分可将特征线区分出来;用改变靶面和入射角、固定测量角的方法及打多晶体靶和非晶体靶的方法可以分辨出X射线衍射谱线;剩下的无法辨识的那些谱线是一种未知谱线,对它的认识还在深入中。     

High Pressure Micro-Slot Hollow Cathode Discharge

A direct current glow discharge source structure operating at high pressure based on the micro-slot hollow cathode is presented in this article. A 100 μm width slot cathode was fabricated of copper, and a stable DC glow discharge with an area of 0.5 mm^2 was produced in noble gases （He, Ne） and air over a wide pressure range （kPa - 10 kPa）. The current-voltage characteristics and the near UV radiation emission of the discharge were studied.     

Discharge Modes Suggested by Emission Spectra of Nitrogen Dielectric Barrier Discharge with Wire-Cylinder Electrodes

In this paper,nitrogen dielectric barrier discharge(DBD) plasma was generated in a quartz tube with coaxial wire-cylinder electrodes at atmospheric pressure.By varying the nitrogen gas flow(FN) in the range of 0-1 m3/h,the plasma optical emission spectra(OES) were measured and studied.The vibration(T_(vib)) and rotation temperature(T_(rot)) of nitrogen were obtained,by fitting the rovibronic bands of N_2(C~3∏_u-B~3∏_g,0-1),and by the Boltzmann plot method for purposes of comparison.T_(vib) increased up to 2481 K with increasing nitrogen flow till0.2 m3/h,and then decreased with further increasing FN,while Trot decreased monotonously and approached to-350 K for FN ≥ 0.6 m~3/h.The intensity of N_2(C~3∏_u-B~3∏_g,0-0,1-0,0-3) and N_2~+(B~2∑_u~+-X~2Σ_g~+,0-0) exhibited similar evolution with increasing FN to those of the T_(vib) and Trot,respectively.The discharge photos revealed that the discharge filaments gradually decreased with increasing FN,and eventually disappeared,which implied that a discharge mode transition emerged with increasing FN.The possible mechanism for the discharge mode transition is studied in detail according to the vibration(T_(vib)) and rotation temperature(T_(rot)) of nitrogen.     

Atmospheric Pressure Radio Frequency Dielectric Barrier Discharges in Nitrogen/Argon

This work reports the experimental results on the characteristics of radio frequency dielectric barrier N2 /Ar discharges.Depending on the nitrogen content in the feed gas and the input power,the discharge can operate in two diferent modes: a homogeneous glow discharge and a constricted discharge.With increasing input power,the number of discharge columns increases.The discharge columns have starlike structures and exhibit symmetric self-organized arrangement.Optical emission spectroscopy was performed to estimate the plasma temperature.Spatially resolved gas temperature measurements,determined from NO emission rotational spectroscopy were taken across the 4.4 mm gap filled by the discharge.Gas temperature in the middle of the gas gap is lower than that close to the electrodes.     

Influence of non-uniform electric field distribution on the atmospheric pressure air dielectric barrier discharge

The dielectric barrier discharge(DBD) in air at atmospheric pressure is not suitable for industrial applications due to its randomly distributed discharge filaments. In this paper, the influence of the electric field distribution on the uniformity of DBD is theoretically analyzed and experimentally verified. It is found that a certain degree of uneven electric field distributions can control the development of electron avalanches and regulate their transition to streamers in the gap. The discharge phenomena and electrical characteristics prove that an enhanced Townsend discharge can be formed in atmospheric-pressure air with a curved-plate electrode. The spectral analysis further confirms that the gas temperature of the plasma produced by the curved-plate electrode is close to room temperature, which is beneficial for industrial applications. This paper presents the relationship between the electron avalanche transition and the formation of a uniform DBD, which can provide some references for the development and applications of the DBD in the future.     

Various concentric-ring patterns formed in a water-anode glow discharge operated at atmospheric pressure

Pattern formation is a very interesting phenomenon formed above a water anode in atmospheric pressure glow discharge. Up to now, concentric-ring patterns only less than four rings have been observed in experiments. In this work, atmospheric pressure glow discharge above a water anode is conducted to produce diversified concentric-ring patterns. Results indicate that as time elapses, the number of concentric rings increases continuously and up to five rings have been found in the concentric-ring patterns. Moreover, the ring number increases continuously with increasing discharge current. The electrical conductivity of the anode plays an important role in the transition of the concentric patterns due to its positive relation with ionic strength. Hence, the electrical conductivity of the water anode is investigated as a function of time and discharge current. From optical emission spectrum, gas temperature and intensity ratio related with density and temperature of electron have been calculated. The various concentric-ring patterns mentioned above have been simulated at last with an autocatalytic reaction model.     

Second Order Fluid Glow Discharge Model Sustained by Different Source Terms

Behavior of charged particles in a DC low pressure glow discharge is studied. The electric properties of the glow discharge in argon, maintained by a constant s...     

Influence of the Transverse Field Component on the Edge Efect in a Short-Gap Discharge

In a general plane-parallel electrode system,the edge of the electrode will undermine the uniformity of the dielectric barrier discharge(DBD)because of the influence of the distorted electrical field.In this paper,the influence of the non-uniform electrical field on the edge efect of DBDs in a short-gap is investigated.We present some of the experimental results of DBDs produced by three kinds of convex-spherical electrodes.The results show that there is a dark area(the homogeneous discharge)in the central region of the electrode and a bright halo(the filamentary discharge)in the outer peripheral region,and the radius of the dark region is determined by the electrode geometry.The calculated results of the transverse(radial)field component distribution on the surface of the electrodes show that the edge efect does not come from the electrode edge,but the transverse field.The discharge has enough space to be fully developed and then format the filamentary discharge in the outer peripheral region because the streamer of the filamentary discharge is driven to move along the direction of the longer path by the transverse field.Thus,the homogeneous discharge(the Townsend DBD or a glow DBD)could not be produced in this area.     

沉积参数对ICF靶丸辉光放电聚合物烧蚀涂层红外特性的影响

采用低压等离子体聚合装置,在溴化钾单晶盐片上制备了气压、功率、反式二丁烯（T₂B）与氢气流量比3个沉积参数系列的辉光放电聚合物（GDP）涂层。对3个系列涂层各自的红外光谱进行比较分析,结合高斯拟合,定量地讨论涂层内部SP³(CH_x)与SP²(CH_x)键的相对含量的变化规律,且探讨了各系列沉积参数对气体分子在等离子体发生区的离解效率和沉积过程活性粒子与涂层新生表面及亚表面相互作用的影响。结果表明,在低气压、较高功率和低流量比参数下,GDP涂层内SP³(CH₃)和氢元素的含量相对较低,SP₂(CH₂)和碳元素的含量相对较高。     

Methane Conversion to C2 Hydrocarbons by Abnormal Glow Discharge at Atmospheric Pressure

Methane conversion to C2 hydrocarbons has been investigated with the addition of hydrogen in a plasma reactor of abnormal glow discharge at atmospheric pressure. The aim of this experiment is to minimize coke formation and improve discharge stability. The typical conditions in the experiment are 300 ml of total feed flux and 400 W of discharge power. The experimental results show that methane conversion is from 91.6% to 35.2% in mol, acetylene selectivity is from 90.2% to 57.6%, and ethylene selectivity is approximately from 7.8% to 3.6%, where the coke increases gradually along with the increase of CH4/H2 from 2 ： 8 to 9 ： 1. A stable discharge for a considerable running time can be obtained only at a lower ratio of CH4/H2 = 2：8 or 3： 7. These phenomena indicate that the coke deposition during methane conversion is obviously reduced by adding a large amount of hydrogen during an abnormal glow discharge. A qualitative interpretation is presented, namely, with abundant hydrogen, the possibility that hydrogen molecules are activated to hydrogen radicals is increased with the help of the abnormal glow discharge. These hydrogen radicals react with carbon radicals to form C2 hydrocarbon products. Therefore, the deposition of coke is restrained.     

Simulation Study on the Self-Sustained Oscillations in DC Driven Glow Discharges at Atmospheric Pressure Under Different Gas Gaps

In this paper,a one-dimensional plasma fluid model is employed to study the selfsustained oscillations in DC-driven helium glow discharges at atmospheric pressure under different gas gaps.Our simulation results indicate that a harmonic current oscillation with tiny amplitude always occur at the onset of instability and transits into a relaxation one as the conductivity of the semiconductor is decreased.It is found that the dynamics of the oscillations are dependent on the gas gaps.The discharge can only exhibit a simple oscillation with unique amplitude and frequency at smaller gas gaps(2 mm) while it can exhibit a more complex oscillation with several different amplitudes and frequencies at larger gas gaps(2 mm).The discharge modes in these current oscillations have also been analyzed.     

The Characteristics of Dielectric Barrier Discharge and its Influence on the Excimer XeCl* Emission

1. IntroductionThere are many reports concerning the dischargemodes at high pressure. The modes of dielectricbarrier discharge (DBD) could be divided mainlyinto two kinds f filament discharge or micro-dischargeand glow discharge or diffused discharge. The fila-ment discharge is a typical characteristic of traditional ozone generator [l], but the characteristics ofDBD in monoatomic gases such as helium, neon andargon at high pressure are'Pfglow-like diffused dis-charge [2]. For air, three co…