共查询到18条相似文献,搜索用时 51 毫秒
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利用溶胶-凝胶法制备了Zn掺杂改性TiO_2催化剂。通过X射线衍射仪、扫描电子显微镜对制备的光催化剂进行表征,考察了该催化剂对亚甲基蓝废水的光催化降解性能。结果表明,Zn成功掺入TiO_2中,Zn掺杂改性TiO_2和纯TiO_2均属于锐钛矿TiO_2晶型。在催化剂投入量为1.5g/L、亚甲基蓝质量浓度为10mg/L、降解时间为0~2h条件下,Zn掺杂改性TiO_2催化剂对亚甲基蓝溶液的降解率超过60%,明显高于纯TiO_2的降解率。 相似文献
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采用溶胶-凝胶法制备了Er-Ce共掺杂的TiO2纳米粉体,并以亚甲基蓝溶液为目标降解物研究了掺杂纳米TiO2粉体在紫外光作用下的光吸收和光催化性能。采用TG-DTA、XRD和TEM等测试技术对样品的晶型、形貌和粒径尺寸进行了表征。结果表明,Er-Ce共掺杂的TiO2粉体最佳热处理温度为550℃,结晶完整、主晶相为锐钛矿型,平均粒径约为20nm;掺杂可使TiO2吸收带发生红移,光催化性能增强;共掺杂体系的最佳量为n(Er):n(TiO2)=0.1%,n(Ce):n(TiO2)=0.05%。此掺杂量的TiO2粉体对亚甲基蓝有良好的降解效果,反应2h降解效果达到92.37%,优于同等条件下制备的未掺杂的纯TiO2粉体。掺杂复合光催化剂对亚甲基蓝的降解遵循一级动力学方程。 相似文献
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讨论采用改良的溶胶-凝胶法,以钛酸丁酯为前驱体,以冰醋酸为鳌合剂,通过水解缩聚作用制备纳米TiO2,掺杂稀土金属进行改性,进行CO2光催化还原制甲醇研究;利用X射线衍射(XRD)、高分辨透射电镜(HRTEM)、BET比表面积、光致发光光谱(PL)技术来分析制得的光催化材料结构、吸光性能、化学吸附等特性,期待能弄清楚纳米TiO2结构与催化效果之间的关系,从而确定主导CO2光催化还原反应效率的因素。 相似文献
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纳米TiO2光催化剂的结构调控及其光催化活性研究 总被引:7,自引:1,他引:7
以酞酸丁酯和冰醋酸分别为前驱物和酸催化剂,采用溶胶 凝胶法制备了纳米 TiO2 粉体, 并且通过改变水体溶液中酞酸丁酯,醋酸和水的摩尔比来调控纳米TiO2 粉体的大小以及光催化活性;探讨在溶胶 凝胶法制备过程中在水溶液中添加表面活性剂十二烷基苯磺酸钠 ( DBS ) 和共溶剂无水乙醇(CH3CH2OH)来调控TiO2 粉体以及光催化活性。用X射线衍射和透射电子显微镜等手段对不同条件制备的纳米粉体的微观结构进行了表征,并且以甲基橙染料的降解为模型反应,考察了不同制备条件下的催化剂的光催化活性,而且对纳米粉体结构和光催化性能之间的关系进行了讨论。 相似文献
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采用溶胶-凝胶法制备了掺Ag复合改性的纳米TiO2复合材料,以提高纳米TiO2在日光下的催化活性。采用差热-热重分析法、X射线衍射、透射电子显微镜、分光光度计等测试技术分析和研究了Ag-TiO2复合材料的微观结构、组织和性能,并探讨了影响Ag-TiO2复合材料光催化性能的各种因素。研究结果表明,利用溶胶-凝胶法可以获得纳米级二氧化钛,单晶尺寸10~30nm。Ag的掺杂会降低锐钛矿相向金红石相的转变温度,掺杂最佳值为Ag/Ti(摩尔比)=0.03;在550℃下热处理1h的Ag-TiO2的光催化性能最高,日光下光照3h对甲基橙的分解率可达97%。 相似文献
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TiO2 nanoparticles modified with nitrogen and sulfur were prepared from titania nanotubes by a facile wet chemistry method. The samples synthesized with different thiourea/TiO2 ratios showed a uniform nanoparticle size distribution centred at approximately 10 nm with a developed specific surface area of 246 m2 g-1. These modified nanosized photocatalysts exhibited higher photocatalytic activity for the degradation of gaseous isopropanol than unmodified titania nanotubes under visible illumination. This could be attributed to the synergistic effects of a large specific surface area, strong absorption in the visible region, a redshift in the adsorption edge, and surface adsorption modification induced by nitrogen and sulfur compounds. 相似文献
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AbstractTiO2 nanoparticles modified with nitrogen and sulfur were prepared from titania nanotubes by a facile wet chemistry method. The samples synthesized with different thiourea/TiO2 ratios showed a uniform nanoparticle size distribution centred at approximately 10 nm with a developed specific surface area of 246 m2 g-1. These modified nanosized photocatalysts exhibited higher photocatalytic activity for the degradation of gaseous isopropanol than unmodified titania nanotubes under visible illumination. This could be attributed to the synergistic effects of a large specific surface area, strong absorption in the visible region, a redshift in the adsorption edge, and surface adsorption modification induced by nitrogen and sulfur compounds. 相似文献
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合成温度对二氧化钛纳米管的影响 总被引:3,自引:0,他引:3
以P25纳米粉体和NaOH为原料,采用水热合成法,在不同的合成温度下制备TiO2纳米管.用XRD、TEM、BET、TG-DSC、Uv-vis等方法对TiO2纳米管的形貌、成分和性能进行了表征.结果表明,合成温度对产物有显著影响:随着反应温度的升高,纳米管的比表面积逐渐增大,长度逐渐增长,而管径基本不变,纳米管的产率也有增加的趋势.150℃反应制得粉体的比表面积为641.855m2/g,管外径为8nm.160℃反应制得的粉体经560℃处理后降解亚甲基蓝的能力要远优于市售的P25纳米粉体.鉴于以前水热处理温度对纳米管形成方面的影响研究报道较少,系统的研究了温度对纳米管形成的影响. 相似文献
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Antibacterial properties of silver-doped titania 总被引:1,自引:0,他引:1
Thiel J Pakstis L Buzby S Raffi M Ni C Pochan DJ Shah SI 《Small (Weinheim an der Bergstrasse, Germany)》2007,3(5):799-803
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Preparation and sintering behaviour of nanostructured alumina/titania composite powders modified with nano-dopants 总被引:2,自引:0,他引:2
Yong Yang You Wang Zheng Wang Gang Liu Wei Tian 《Materials Science and Engineering: A》2008,490(1-2):457-464
Nanostructured alumina/titania composite powders were prepared by doping with small amounts of nanosized zirconia and ceria. The nanosized raw materials powders were reconstituted into nanostructured particles by ball milling, spray drying and heat treating. Then, the nanostructured reconstituted powders were cool-isostatic pressed and pressureless-sintered into bulk ceramics. The phase composition and microstructures of reconstituted powders and as-prepared ceramic composites were characterized by using X-ray diffractometer (XRD), scanning electron microscope (SEM) and energy-dispersive spectrometer (EDS). The sintering behaviour of the nanostructured ceramic composite powders and the effects of nano-dopants and sintering temperatures on the microstructures of the ceramic composites were investigated and discussed. It was found that nano-dopants could lower the sintering temperature and accelerate densification of ceramic composites. 相似文献