Subcooled boiling incipience on a highly smooth microheater

Subcooled boiling incipience on a highly smooth microscale heater (270 μm × 270 μm) submerged in FC-72 liquid is investigated. Using high-speed imaging and a transient heat flux measurement technique, the mechanics of homogeneous nucleation on the heater are elucidated. Bubble incipience on the microheater was observed to be an explosive process. It is found that the superheat limit of boiling liquid is required for bubble incipience. It is concluded that boiling incipience on the microheater is a homogeneous liquid–vapor phase change process. This is in contrast to recent observations of low-superheat heterogeneous nucleation on metallic surfaces of rms roughness ranging from 4 to 28 nm [T.G. Theofanous, J.P. Tu, A.T. Dinh, T.N. Dinh, The boiling crisis phenomenon part I: nucleation and nucleate boiling heat transfer, Exp. Therm. Fluid Sci. 26 (2002) 775–792; Y. Qi, J.F. Klausner, Comparison of gas nucleation and pool boiling site densities, J. Heat Transfer 128 (2005) 13–20; Y. Qi, J.F. Klausner, Heterogeneous nucleation with artificial cavities, J. Heat Transfer 127 (2005) 1189–1196]. Following the explosive bubble incipience, the boiling process on the microheater can be maintained at much lower superheats. This is mainly due to the necking during bubble departure that leaves an embryo from which the next-generation bubbles grow.     

Dynamic characteristics of transient boiling on a square platinum microheater under millisecond pulsed heating

A series of experimental investigations of boiling incipience and bubble dynamics of water under pulsed heating conditions for various pulse durations ranging from 1 ms to 100 ms were conducted. Using a very smooth square platinum microheater, 100 μm on a side, and a high-speed digital camera, the boiling incipience was observed and investigated as a function of the bulk temperature of the microheater, pulse power level, and pulse duration. Given a specific pulse duration, for low pulse power levels, there would be no bubble nucleation or bubble mergence, for moderate pulse power levels, individual bubbles generated on the heater merged to form a single large bubble, while for high pulse power levels, the rapid growth of the individual bubbles and subsequent bubble interaction, resulted in a reduction in bubble coalescence into a single larger bubble, referred to as bubble splash. The transient heat flux range at which bubble coalescence occurs was identified experimentally, along with the temporal variations of bubble size, bubble interface velocity and interface acceleration.     

Effect of pulse heating parameters on the microscale bubble dynamics at a microheater surface

We study the effects of pulse heating parameters on the micro bubble behavior of a platinum microheater (100 μm×20 μm) immersed in a methanol pool. The experiment covers the heat fluxes of 10–37 MW/m² and pulse frequencies of 25–500 Hz. The boiling incipience is initiated at the superheat limit of methanol, corresponding to the homogeneous nucleation. Three types of micro boiling patterns are identified. The first type is named as the bubble explosion and regrowth, consisting of a violent explosive boiling and shrinking, followed by a slower bubble regrowth and subsequent shrinking, occurring at lower heat fluxes. The second type, named as the bubble breakup and attraction, consists of the violent explosive boiling, bubble breakup and emission, bubble attraction and coalescence process, occurring at higher heat fluxes than those of the first type. The third type, named as the bubble size oscillation and large bubble formation, involves the initial explosive boiling, followed by a short periodic bubble growth and shrinking. Then the bubble continues to increase its size, until a constant bubble size is reached which is larger than the microheater length.     

Saturated flow boiling heat transfer and associated bubble characteristics of FC-72 on a heated micro-pin-finned silicon chip

An experiment is carried out here to investigate flow boiling heat transfer and associated bubble characteristics of FC-72 on a heated micro-pin-finned silicon chip flush-mounted in the bottom of a horizontal rectangular channel. Besides, three different micro-structures of the chip surface are examined, namely, the smooth, pin-finned 200 and pin-finned 100 surfaces. The pin-finned 200 and 100 surfaces, respectively, contain micro-pin-fins of size 200 μm × 200 μm × 70 μm (width × length × height) and 100 μm × 100 μm × 70 μm. The pitch of the fins is equal to the fin width for both surfaces. The effects of the FC-72 mass flux, imposed heat flux, and surface micro-structures of the silicon chip on the FC-72 saturated flow boiling characteristics are examined in detail. The experimental data show that an increase in the FC-72 mass flux causes a delay in the boiling incipience. However, the flow boiling heat transfer coefficient is not affected by the coolant mass flux. But adding the micro-pin-fin structures to the chip surfaces can effectively enhance the single-phase convection and flow boiling heat transfer. Moreover, the mean bubble departure diameter and active nucleation site density are reduced for a rise in the FC-72 mass flux. A higher coolant mass flux results in a higher mean bubble departure frequency. Furthermore, larger bubble departure diameter, higher bubble departure frequency, and higher active nucleation site density are observed at a higher imposed heat flux. We also note that adding the micro-pin-fins to the chips decrease the bubble departure diameter and increase the bubble departure frequency. However, the departing bubbles are larger for the pin-finned 100 surface than the pin-finned 200 surface but the bubble departure frequency exhibits an opposite trend. Finally, empirical equations to correlate the present data for the FC-72 single-phase liquid convection and saturated flow boiling heat transfer coefficients and for the bubble characteristics are provided.     

Effects of electric field on microbubble growth in a microchannel under pulse heating

Effects of imposed DC electric fields on microbubble growth generated from a rectangular Pt micro-heater (140 × 100 μm) fabricated on one wall of the microchannel under pulse heating are investigated experimentally in this paper. Bubble dynamics and surface temperature response of the microheater during pulse heating are observed and recorded using a high speed CCD and data acquisition system. Measurements of nucleation time and nucleation temperature and heat flux at boiling inception are taken at a fixed flow rate of 0.6 ml/min and pulse width of 1 ms, and with the electric field strength gradually increasing from zero. With increasing electric field strength, it is found that heat flux required for boiling inception is increased, boiling nucleation time is delayed, and nucleation temperature is reduced. Bubble growth is suppressed by the inward dielectrophoresis force acting at the vapor/water interface which is induced by the electric field. As a result, the diameter of the bubble becomes smaller, and the interface instability is suppressed during the bubble growth period. In addition, it is found that multiple nucleate sites appear on the surface of the micro-heater at high heat flux when the electric field is increased to a sufficiently high strength. A map showing regimes of single and multi nucleate sites in a plot of heat flux versus electric field strength is obtained.     

Microscale heterogeneous boiling on smooth surfaces—from bubble nucleation to bubble dynamics

In this investigation, boiling incipience and bubble dynamics on a microheater with a geometry of 100 μm × 100 μm fabricated with MEMS technology are evaluated using a high-speed digital camera. For the purpose of comparison with conventional boiling heat transfer, boiling incipience and bubble dynamics are also studied on a carefully selected microheater with a fabricated defect (i.e., a microcavity on the heater surface). Of industrial interest are the effects of dissolved gases on boiling incipience and bubble dynamics, which are also discussed in detail. The possible nucleation temperature (or incipience temperature) is analyzed and discussed from the perspective of the measured bulk temperature of the microheater and a 3D heat conduction numerical model. The time-resolved bubble dynamics (i.e., the bubble size evolution, interface velocity and interface acceleration) are all presented along with high-speed digital images. Based upon this investigation, it is clear that explosive boiling can take place on a smooth surface no matter how slow the heating rate, and dissolved gases have a significant influence on the incipience temperature and bubble behavior. Furthermore, this study illustrates that the classical kinetics of boiling can explain the explosive boiling occurring on a smooth surface in principle and can provide a useful guide for the design of microscale heat transfer and/or MEMS devices. Although unexpected, due to the gravitational effects, Marangoni flow on the vapor–liquid interface induced by the temperature gradient was also observed.     

A four-zone model for saturated flow boiling in a microchannel of rectangular cross-section

A four-zone flow boiling model is presented to describe saturated flow boiling heat transfer mechanisms in a microchannel of rectangular cross-section. The boiling process in the microchannel is assumed to be a cyclic passage of four zones: (i) liquid-slug zone, (ii) elongated bubble zone, (iii) partially-dryout zone, and (iv) fully-dryout zone. The existence of the partially-dryout zone in this model is proposed to take into consideration of corner effects on boiling heat transfer in the microchannel. To verify this new model, an experimental study was carried out to investigate flow boiling heat transfer of water in a microchannel having a rectangular cross-section with a hydraulic diameter of 137 μm (202 μm in width and 104 μm in depth) with a length of 30 mm under three-side heating condition. The data for bubble nucleation frequency was correlated in terms of the Boiling number, which was used to determine the heat transfer coefficient. It is found that the present four-zone flow boiling model successfully predicts trends of boiling heat transfer data in a microchannel with a rectangular cross-section, having a sharp peak at low vapor quality depending on the mass flow rate. The predictions of flow boiling heat transfer coefficient in the microchannel are found in good agreement with experimental data with a MAE of 13.9%.     

Subcooled flow boiling heat transfer and associated bubble characteristics of FC-72 on a heated micro-pin-finned silicon chip

Experiments are conducted here to investigate subcooled flow boiling heat transfer and associated bubble characteristics of FC-72 on a heated micro-pin-finned silicon chip flush-mounted on the bottom of a horizontal rectangular channel. In the experiments the mass flux is varied from 287 to 431 kg/m² s, coolant inlet subcooling from 2.3 to 4.3 °C, and imposed heat flux from 1 to 10 W/cm². Besides, the silicon chips contain three different geometries of micro-structures, namely, the smooth, pin-finned 200 and pin-finned 100 surfaces. The pin-finned 200 and 100 surfaces, respectively, contain micro-pin-fins of size 200 μm × 200 μm × 70 μm (width × length × height) and 100 μm × 100 μm × 70 μm. The measured data show that the subcooled flow boiling heat transfer coefficient is reduced at increasing inlet liquid subcooling but is little affected by the coolant mass flux. Besides, adding the micro-pin-fin structures to the chip surface can effectively raise the single-phase convection and flow boiling heat transfer coefficients. Moreover, the mean bubble departure diameter and active nucleation site density are reduced for rises in the FC-72 mass flux and inlet liquid subcooling. Increasing coolant mass flux or reducing inlet liquid subcooling results in a higher mean bubble departure frequency. Furthermore, larger bubble departure diameter, higher bubble departure frequency, and higher active nucleation site density are observed as the imposed heat flux is increased. Finally, empirical correlations for the present data for the heat transfer and bubble characteristics in the FC-72 subcooled flow boiling are proposed.     

Nucleation site interaction between artificial cavities during nucleate pool boiling on silicon with integrated micro-heater and temperature micro-sensors

Nucleate boiling is commonly characterised as a very complex and elusive process. Many involved mechanisms are still not fully understood and more detailed consideration is needed. In this study, bubble growth from micro-fabricated artificial cavities with varied spacing on a horizontal 380 μm thick silicon wafer was investigated. The horizontally oriented boiling surface was heated by a thin resistance heater integrated on the rear of the silicon test section. The temperature was measured using 16 integrated micro-sensors situated on the boiling surface, each with an artificial cavity located in its geometrical centre. Experiments with three different spacings 1.5, 1.2 and 0.84 mm in between cavities with a nominal mouth diameter of 10 μm and a depth of 80 μm were undertaken. To conduct pool boiling experiments, the test section was mounted inside a closed stainless steel boiling chamber with optical access and completely immersed in degassed fluorinert FC-72. Bubble nucleation, growth and detachment at 0.5 and 1 bar absolute pressure were investigated using high-speed imaging. The effect of decreasing inter-site distance on bubble nucleation frequency, bubble departure frequency and diameter with increasing wall superheat is presented. Furthermore, the frequency of horizontal bubble coalescence was determined. The regions of influence on the measured frequencies and bubble departure diameter were compared with recently published findings.     

On the eruptive boiling in silicon-based microchannels

This study investigates experimentally eruptive boiling in a silicon-based rectangular microchannel with a hydraulic diameter of 33.7 μm, a width of 99.8 μm and a depth-to-width ratio of 0.203. The microchannel is made of SOI wafer and prepared using bulk micro-machining and anodic bonding. The surface roughness for both the bottom and the side walls was measured using an atomic force microscope. The evolution of the eruptive boiling of water in the smooth microchannel was clearly observed using an ultra high-speed video camera (up to 50,000 frames/s) at mass fluxes of 417 and 625 kg/m² s and a heat flux from 14.9 to 372 kW/m². It is confirmed that eruptive boiling is a form of rapid bubble nucleation after which the bubble merges with a slug bubble downstream in a short distance or evolve to a slug bubble. The bubble frequency in all of the cases studied is provided. Eruptive boiling may be predicted classically with nano-sized cavities that are consistent with the measured surface roughness.     

An experimental study of heater size effect on micro bubble generation

An experimental study of the heater size effect on micro boiling is reported in detail. Using a 1.66-ms-wide heating pulse, boiling in subcooled water was investigated on a series of micron/submicron thin film Pt heaters with various feature sizes ranging from 0.5 μm to 70 μm. It was found that there existed a critical heater size (10 μm): single spherical bubble generation with heater’s feature size less than 10 μm; oblate vapor blanket on the heater surface with the size larger than 10 μm. The bubble dynamics was studied by the visualization of the bubble nucleation process with a high-speed CCD. The onset bubble nucleation temperature was measured by using each Pt heater as a resistive temperature sensor. The formation of the oblate vapor blanket was attributed to the condensation effect of the vapor outside the superheated zone. The analysis was further validated by generating spherical bubble on heater with size larger than 10 μm with a longer heating pulse.     

Bubble growth and horizontal coalescence in saturated pool boiling on a titanium foil,investigated by high-speed IR thermography

Growth of an isolated bubble and horizontal coalescence events between bubbles of dissimilar size were examined during pool nucleate boiling of water on a horizontal, electrically-heated titanium foil 25 μm thick. Wall temperature measurements on the back of the foil by high-speed IR camera, synchronized with high-speed video camera recordings of the bubble motion, improved the temporal and spatial resolution of previous observations by high-speed liquid crystal thermography to 1 ms and 40 μm, respectively, leading to better detailed maps of the transient distributions of wall heat flux. The observations revealed complex behaviour that disagreed with some other observations and current modelling assumptions for the mechanisms of heat transfer over the wall contact areas of bubbles and interactions between bubbles. Heat transfer occurred from the entire contact area and was not confined to a narrow peripheral triple-contact zone. There was evidence of an asymmetrical interaction between bubbles before coalescence. It was hypothesised that a fast-growing bubble pushed superheated liquid under a slow-growing bubble. Contact of this liquid with regions of the wall that had been pre-cooled during bubble growth caused local reductions in the wall heat flux. During coalescence, movement of liquid under both bubbles caused further changes in the wall heat flux that also depended on pre-cooling. Contraction of the contact area caused a peripheral reduction in the heat flux and there was no evidence of a large increase in heat flux during detachment. Boiling on very thin foils imposes special conditions. Sensitivity to the thermal history of the wall must be taken into account when applying the observations and hypotheses to other conditions.     

Local measurement of flow boiling in structured surface microchannels

Experiments were conducted to investigate flow boiling in 200 μm × 253 μm parallel microchannels with structured reentrant cavities. Flow morphologies, boiling inceptions, heat transfer coefficients, and critical heat fluxes were obtained and studied for mass velocities ranging from G = 83 kg/m² s to G = 303 kg/m² s and heat fluxes up to 643 W/cm². Comparisons of the performance of the enhanced and plain-wall microchannels were performed. The microchannels with reentrant cavities were shown to promote nucleation of bubbles and to support significantly better reproducibility and uniformity of bubble generation. The structured surface was also shown to significantly reduce the boiling inception and to enhance the critical heat flux.     

Lateral coalescence of bubbles in the presence of a DC electric field

In this work, the influence of electrohydrodynamic forces on lateral bubble coalescence during nucleate pool boiling is investigated. An experimental pool boiling test facility was used with n-pentane as the working fluid. Boiling took place atop a polished copper surface on which two artificial nucleation sites were fabricated. The nucleation sites were 180 μm in diameter and 500 μm deep with a centre-to-centre spacing of 660 μm. Two diametrically opposed windows allowed for illumination and high speed videography of the bubble growth process from the two nucleation sites. For the saturated boiling tests considered here, bubbles only formed at the two artificial nucleation sites allowing their coalescence behaviour to be scrutinized. A screen electrode above the boiling surface and a high voltage DC power supply facilitated the establishment of the electric field which was varied between 0 and 34.5 kVcm^− 1. Observation of the high speed videos has revealed that bubble coalescence is influenced in such a way that it is delayed in the presence of the electric field to such an extent that, at the highest electric field strength tested, it is avoided all together. To help explain the observed results, a simple numerical model is solved showing that bubbles in close proximity to one another create an electric field distribution with high intensity between them. The overall result is net polarization forces that push the bubbles apart, and the closer they are together the larger this repulsive force becomes.     

On the rise paths of single vapor bubbles after the departure from nucleation sites in subcooled upflow boiling

A photographic study was carried out for the subcooled flow boiling of water to elucidate the rise characteristics of single vapor bubbles after the departure from nucleation sites. The test section was a transparent glass tube of 20 mm in inside diameter and the flow direction was vertical upward; liquid subcooling was parametrically changed within 0–16 K keeping system pressure and liquid velocity at 120 kPa and 1 m/s, respectively. The bubble rise paths were analyzed from the video images that were obtained at the heat flux slightly higher than the minimum heat flux for the onset of nucleate boiling. In the present experiments, all the bubbles departed from their nucleation sites immediately after the inception. In low subcooling experiments, bubbles slid upward and consequently were not detached from the vertical heated wall; the bubble size was increased monotonously with time in this case. In moderate and high subcooling experiments, bubbles were detached from the wall after sliding for several millimeters and migrated towards the subcooled bulk liquid. The bubbles then reversed the direction of lateral migration and were reattached to the wall at moderate subcooling while they collapsed due to the condensation at high subcooling. It was hence considered that the mechanisms of the heat transfer from heated wall and the axial growth of vapor volume were influenced by the difference in bubble rise path. It was observed after the inception that bubbles were varied from flattened to more rounded shape. This observation suggested that the bubble detachment is mainly caused by the change in bubble shape due to the surface tension force.     

Effects of surfactant additive on flow boiling over a microheater under pulse heating

An experimental investigation has been carried out to study effects of surfactant additive on microscale boiling under pulse heating over a Pt microheater (140 × 100 μm²) fabricated in a trapezoidal microchannel (600 μm in width and 150 μm in depth). Experiments are carried out for six different surfactant concentrations of Triton X-100 ranging from 47 ppm to 2103 ppm, for mass flux in the range from 45 kg/m² s to 225 kg/m² s, pulse width in the range from 50 μs to 2 ms, and heat flux in the range from 3 MW/m² to 65 MW/m². As in existing work on pool boiling under steady heating, it is found that nucleate boiling becomes more vigorous and heat transfer is enhanced greatly with the addition of surfactant with maximum boiling heat transfer occurs at the critical micelle concentration (cmc). Furthermore, these maximum values of boiling heat transfer coefficient increase with decreasing pulse width. When concentration is below cmc, the heat flux needed for nucleation increases with increasing concentration and the nucleation temperature is reduced. When concentration is higher than cmc, the boiling heat transfer coefficient decreases and nucleation temperature is higher than that of pure water.     

Nanofluid stabilizes and enhances convective boiling heat transfer in a single microchannel

The flow boiling heat transfer in a single microchannel was investigated with pure water and nanofluid as the working fluids. The microchannel had a size of 7500 × 100 × 250 μm, which was formed by two pyrex glasses and a silicon wafer. A platinum film with a length of 3500 μm and a width of 80 μm was deposited at the bottom channel surface, acting as the heater and temperature sensor. The nanofluid had a low weight concentration of 0.2%, consisting of de-ionized water and 40 nm Al₂O₃ nanoparticles. The nanoparticle deposition phenomenon was not observed. The boiling flow displays chaotic behavior due to the random bubble coalescence and breakup in the milliseconds timescale at moderate heat fluxes for pure water. The flow instability with large oscillation amplitudes and long cycle periods was observed with further increases in heat fluxes. The flow patterns are switched between the elongated bubbles and isolated miniature bubbles in the timescale of 100 s. It is found that nanofluid significantly mitigate the flow instability without nanoparticle deposition effect. The boiling flow is always stable or quasi-stable with significantly reduced pressure drop and enhanced heat transfer. Miniature bubbles are the major flow pattern in the microchannel. Elongated bubbles temporarily appear in the milliseconds timescale but isolated miniature bubbles will occupy the channel shortly. The decreased surface tension force acting on the bubble accounts for the smaller bubble size before the bubble departure. The inhibition of the dry patch development by the structural disjoining pressure, and the enlarged percentage of liquid film evaporation heat transfer region with nanoparticles, may account for the heat transfer enhancement compared to pure water.     

Effects of heater size and working fluids on nucleate boiling heat transfer

The present study is an experimental investigation of nucleate boiling heat transfer mechanism in pool boiling from wire heaters immersed in saturated FC-72 coolant and water. The vapor volume flow rate departing from a wire during nucleate boiling was determined by measuring the volume of bubbles from the wire utilizing the consecutive-photo method. The effects of the wire size on heat transfer mechanism during a nucleate boiling were investigated, varying 25 μm, 75 μm, and 390 μm, by measuring vapor volume flow rate and the frequency of bubbles departing from a wire immersed in saturated FC-72. One wire diameter of 390 μm was selected and tested in saturated water to investigate the fluid effect on the nucleate boiling heat transfer mechanism. Results of the study showed that an increase in nucleate boiling heat transfer coefficients with reductions in wire diameter was related to the decreased latent heat contribution. The latent heat contribution of boiling heat transfer for the water test was found to be higher than that of FC-72. The frequency of departing bubbles was correlated as a function of bubble diameters.     

Lower limit of homogeneous nucleation boiling explosion for water

In this paper, the lower limit for the occurrence of homogeneous nucleation boiling explosion during water heating at atmospheric pressure has been determined by applying a new theoretical model proposed by the authors. Two different cases of water heating have been considered for the study of homogeneous nucleation boiling explosion. In one case, the liquid on the surface is linearly heated at a rate of 10 K/s to 10⁹ K/s. In another case, the liquid suddenly contacts with a high temperature surface such as in case of quenching with impinging jet or droplet. With the assumption of liquid boiling without any cavity or surface effect, the liquid temperature limit at which homogeneous boiling explosion occurs essentially corresponds to a value of 302 °C even though the surface is heated very slowly. On the other hand, during water contact with hot surfaces, the occurrence of the homogeneous boiling explosion within a characteristic time period of 1 ms is obtained at a maximum liquid temperature of 303 °C for a limiting steady state boundary temperature of about 304 °C. From the definition of the steady-state interface boundary temperature of two 1-D semi-infinite body contact problem, the lower limiting surface temperatures for the occurrence of the homogeneous nucleation boiling explosion have been determined for water contact with various solid surfaces at different initial liquid temperatures ranging from 0 °C to 100 °C. The effects of the parametric variation in the boundary heating conditions on various characteristics of the homogeneous boiling explosion such as liquid temperature and time of boiling explosion, heat-flux across the liquid–vapor interface at the boiling explosion, etc. are determined and compared with other results reported in the literature.