Effects of thoron on a radon detector of pulse-ionization chamber type

A radon detector of pulse-ionization chamber (PIC) type could have some sensitivity for thoron. Thus, the presence of thoron could interfere with precise measurement of radon. In the present study, effects of thoron on the most common type of PIC detector (commercial name AlphaGUARD) were investigated using an exposure chamber. The AlphaGUARD was exposed to a mixture of radon and thoron, together with a radon/thoron discriminative monitor that employs a silicon solid-state detector. The thoron sensitivity of the PIC detector was estimated by comparing the two detectors. As a result, the thoron sensitivity was about 10% compared with the radon sensitivity. In other words, the radon concentration (Bq m(-3)) measured with the PIC detector was approximately the sum of the actual radon concentration (Bq m(-3)) and 10% of the thoron concentration (Bq m(-3)). The sensitivity to thoron should be considered in measurements in thoron-enhanced areas.     

Effective dose assessment for workers in caves in the Czech Republic: experiments with passive radon detectors

The new RAMARN system for radon volume activity measurement was developed in 2003 and has been in use since then. RAMARN system consists of a plastic chamber that is conically cylindrical in shape and about 0.5 l in volume; a bare Kodak LR 115 is located on the bottom of this diffusion chamber. The size was chosen to avoid the influence of deposited decay products of radon. Kodak has a spectrometric character-the tracks are visualized only for alphas with energies between 1 and 3 MeV that touch the foil; thus the effective volume has a lens shape. The response therefore corresponds to diffused radon and half of (218)Po born by radon gas decay. The experiments described below were conducted as one part of a routine methodology control, focused on classifying worker irradiation from natural ionizing radiation sources in show caves and in caves used for speleotherapy.     

A new passive radon-thoron discriminative measurement system

A new passive radon-thoron discriminative measurement system has been developed for monitoring radon and thoron individually. It consists of a 'couple' of passive integrating devices with a CR39 nuclear track detector (NTD). The experimental prototype is based on the application of a new concept of NTD instrument developed at ENEA, named Alpha-PREM, acronym of piston radon exposure meter, which allows controlling the detector exposure with a patented sampling technique (Int. Eu. Pat. and US Pat.). The 'twin diffusion chambers system' was based on two A-PREM devices consisting of the standard device, named NTD-Rn, and a modified version, named NTD-Rn/Tn, which was set up to improve thoron sampling efficiency of the diffusion chamber, without changing the geometry and the start/stop function of the NTD-Rn device. Coupling devices fitted on each device allowed getting a system, which works as a double-chamber structure when deployed at the monitoring position. In this paper both technical and physical aspects are considered.     

Study of gel materials as radioactive 222Rn gas detectors

Commercial hair gel material (polyvinyl pyrolydone triethanolamine carbopol in water) and bacteriological agar (phycocolloid extracted from a group of red-purple algae, usually Gelidium sp.) have been studied as radioactive radon gas detectors. The detection method is based on the diffusion of the radioactive gas in the gel material, and the subsequent measurement of trapped products of the natural decay of radon by gamma spectrometry. From the several radon daughters with gamma radiation emission (214Pb, 214Bi, 214Po, 210Pb, 210Po), two elements, 214Pb (0.352 MeV) and 214Bi (0.609 MeV), were chosen for the analysis in this work; in order to determine the best sensitivity, corrections were made for the short half-life of the analysed isotopes. For the gamma spectrometry analysis, a hyperpure germanium solid state detector was used, associated with a PC multichannel analyser card with Maestro and Microsoft Excel software. The results show the viability of the method: a linear response in a wide radon concentration range (450-10,000 Bq m(-3)), reproducibility of data, easy handling and low cost of the gel material. This detection methodology opens new possibilities for measurements of radon and other radioactive gases.     

Detection properties of a measuring system for a continuous soil radon concentrations monitoring.

The continual soil-gas radon concentration measurements are absolutely crucial for a reliable assessment of radon entry characteristics into the indoor building environment. For this purpose, a new detection system (a continuous monitor RM-3) was developed and tested. The detection principle of the monitoring device is based on an airflow ionisation chamber operating in a current mode. A comprehensive series of testing and calibration experiments have been carried out in a laboratory environment. An output signal of the device caused by the radon concentration in a sensitive detection volume significantly depends on a detector ventilation rate, the gas flow rate through the ionisation chamber. A set of calibration experiments was accomplished with the artificial radon source application and close circuit experimental arrangements. The system detection properties including applied experimental conditions and key results of pilot in situ measurements are reported in detail.     

A self-calibrating radon monitor with statistical discrimination

A radon monitor, able to perform the measurement of the radon and its progeny volumic activity, in a gamma-ray or natural radiation background field, was developed. The instrument consists of a 10 l ionization chamber, a high voltage source, an integrating preamplifier, a data acquisition system and a personal computer. A new method for self-calibration of Radon volumic activity measurements, based on the alpha counting with an ionization chamber is also presented.     

Towards the use of small amounts of activated charcoal along with well-type NaI(Tl) detector for indoor radon measurements

The feasibility of using small quantities of activated charcoal and a 7.6 cm x 7.6 cm NaI(Tl) well-type detector was investigated for indoor radon measurements. Vials, filled with 10 g of charcoal, were exposed for different indoor radon concentration levels typical of Kuwait dwellings. After exposure, the vials were sealed and kept for 3 h to allow radon to come into radioactive equilibrium with its progenies and were then analysed by gamma-ray spectrometry using the well-type NaI(Tl) detector. The variation of radon absorption by the vials filled with charcoal with exposure time was also studied. A comparative study of the present technique with the standard technique of using 70 g charcoal canisters and flat NaI detector was also performed. After establishing the suitability of the technique, the charcoal vials were then used to investigate the effect of air-ventilation on the concentration levels of the indoor radon. Results show that there is a reduction in the radon concentration level (up to 25%) when the air-ventilation system was switched on. The paper presents the results of the study on the feasibility of combining small amounts of activated charcoal with a well-type NaI(Tl) detector in the measurement of indoor radon concentrations.     

Development of a new thoron progeny detector based on SSNTD and the collection by an electric field

The importance of (220)Rn (thoron) progeny for human exposure has been widely recognised in the past decades. Since no stable equilibrium factor was found between indoor thoron and its progeny, and the concentration of thoron progeny varies with time, it is necessary to develop detectors for long-term measurement that directly sample and detect thoron progeny. However, power supply of this kind of detectors has always been a problem. In this study, a set of device that is suitable for long-term measurement is introduced. A high-voltage electric field was formed for the collection of charged aerosols attached by (222)Rn (radon) and thoron progenies on solid-state nuclear track detector. Impact from radon progeny could be eliminated with a shield of Al foil of appropriate thickness. Tests were made both in an experimental house and in a thoron chamber in Helmholtz Zentrum München to determine the parameters and to verify the universality under different conditions.     

Radon progeny in Egyptian underground phosphate mines

In addition to the workers in uranium mines, the staff of other underground mines, such as workers in underground phosphate mines, can be exposed to 222Rn and its progeny. In this study the individual radon progeny concentrations were measured in three Egyptian underground phosphate mines to estimate the occupational exposure of the workers at those sites. A filter method was used to measure individual radon progeny concentrations (218Po, 214Pb and 214Po). The reported mean values of radon progeny concentrations exceed the action levels which are recommended by ICRP 65 (1993). Based on the measured individual radon progeny concentrations (218Po, 214Pb and 214Po) in these mines, the annual effective dose for the workers has been calculated using the lung dose model of ICRP 66 (1994). According to the obtained results, some countermeasures were recommended in this study to minimise these exposure levels.     

Simultaneous measurements of indoor radon, radon-thoron progeny and high-resolution gamma spectrometry in Greek dwellings

Simultaneous indoor radon, radon-thoron progeny and high-resolution in situ gamma spectrometry measurements, with portable high-purity Ge detector were performed in 26 dwellings of Thessaloniki, the second largest town of Greece, during March 2003-January 2005. The radon gas was measured with an AlphaGUARD ionisation chamber (in each of the 26 dwellings) every 10 min, for a time period between 7 and 10 d. Most of the values of radon gas concentration are between 20 and 30 Bq m(-3), with an arithmetic mean of 34 Bq m(-3). The maximum measured value of radon gas concentration is 516 Bq m(-3). The comparison between the radon gas measurements, performed with AlphaGUARD and short-term electret ionisation chamber, shows very good agreement, taking into account the relative short time period of the measurement and the relative low radon gas concentration. Radon and thoron progeny were measured with a SILENA (model 4s) instrument. From the radon and radon progeny measurements, the equilibrium factor F could be deduced. Most of the measurements of the equilibrium factor are within the range 0.4-0.5. The mean value of the equilibrium factor F is 0.49 +/- 0.10, i.e. close to the typical value of 0.4 adopted by UNSCEAR. The mean equilibrium equivalent thoron concentration measured in the 26 dwellings is EEC(thoron) = 1.38 +/- 0.79 Bq m(-3). The mean equilibrium equivalent thoron to radon ratio concentration, measured in the 26 dwellings, is 0.1 +/- 0.06. The mean total absorbed dose rate in air, owing to gamma radiation, is 58 +/- 12 nGy h(-1). The contribution of the different radionuclides to the total indoor gamma dose rate in air is 38% due to 40K, 36% due to thorium series and 26% due to uranium series. The annual effective dose, due to the different source terms (radon, thoron and external gamma radiation), is 1.05, 0.39 and 0.28 mSv, respectively.     

Fraction of the positive 218Po and 214Pb clusters in indoor air

The fraction of the positively charged unattached radon decay products, 218Po and 214Pb in indoor air was determined by model calculations. The results of the calculations were confirmed by measurements in a test chamber (volume: 8 m3). The fraction of both radionuclides depends on the attachment parameter (S(1)) and the neutralisation rate (nu) in room air. The total removal parameter S1 = lambda1 + v + q(f) + X = lambda1 C1f/C0 considers the attachment rate to aerosol particles (X), plate-out rate to room surfaces (q(f)) and the ventilation rate (nu) (lambda1: decay constant of 218Po). The S1-value of room can be determined by measurement of the concentration of the unattached 218Po clusters (C1f) and radon (C0). The neutralisation rate (nu) in environmental air depends mainly on the ion production rate. The influence of the relative humidity in the range 30-95% (temperature: 20 degrees C) is negligible. In addition, equal neutralisation rates for 218Po and 214Pb could be derived. In room air with ion production rates between 5 and 500 nC kg(-1) h(-1) mainly generated by the alpha emitters of radon, thoron and their short-lived decay products, the fractions for positive 218Po clusters vary between 55 and 17% and for 214Pb clusters between 53 and 14%. For a typical average concentration of radon (50 Bq m(-3)) and thoron (10 Bq m(-3)) in homes, 48% of 218Po clusters and 45% of 214Pb clusters are positively charged.     

Field comparison of two different passive radon detectors

The present paper describes field performance of two different passive radon monitor devices formed, respectively, by a CR-39 track detector enclosed in a diffusion chamber and a cellulose nitrate detector (LR-115) in a heat-sealed polyethylene bag. The most important scope of these investigations was to study the performance of these detectors directly in the field. To this end, two different types of radon monitors mentioned above have been exposed simultaneously in 100 school rooms within the Italian region Friuli Venezia Giulia. Finally, the accuracy of their responses has been evaluated by exposing them under extreme humidity conditions and/or together with other radon measurement instruments.     

氡析出率测量中的218Po非平衡修正

通过对传统的累积法测量氡析出率模型实验验证,发现得到的氡析出率明显偏低。对测氡仪器的工作原理与集氡罩中氡的浓度变化规律进行分析,发现是由于被测介质表面析出的氡不断进入集氡罩,218Po与氡没有平衡,造成测量的氡浓度明显偏低。通过非平衡修正得到了修正后的氡析出率测量理论模型。利用修正后的该模型得到的介质表面氡析出率与参考值符合得较好,误差小于7%。此外比较优值函数的取值也可发现:修正后的理论模型优值函数的取值小于传统模型,这表明修正后的理论模型更符合实际,该理论模型可应用于氡析出率仪的研制与改进。     

Uncertainty in radon measurements with CR39 detector due to unknown deposition of Po

Uncertainty in radon measurements using the CR39 solid-state nuclear track detector in chambers is introduced by the unknown fraction f₁ of ²¹⁸Po that deposited onto the inner chamber walls. This uncertainty was estimated for cylindrical chambers with different size in the present study. It was found that the uncertainty increased with the chamber height and radius. For short chambers with a height H=2 cm the uncertainty was less than 5%, while in tall chambers with H=7 cm it could be up to 17%. The radial track density on the CR39 detector inside the diffusion chamber was also found to be dependent on the fraction f₁. In this work, some examples of this dependence are shown.     

Development and management of a radon assessment strategy suitable for underground railway tunnelling projects

The construction of underground tunnels through radon-bearing rock poses a radiation health risk to tunnelling workers from exposure to radon gas and its radioactive decay products. This paper presents the development and practical application of a radon assessment strategy suitable for the measurement of radon in tunnelling work environments in Hong Kong. The assessment strategy was successfully evaluated on a number of underground railway tunnelling projects over a 3 y period. Radon measurements were undertaken using a combination of portable radon measurement equipment and track etch detectors (TEDs) deployed throughout the tunnels. The radon gas monitoring results were used to confirm that ventilation rates were adequate or identified, at an early stage, when further action to reduce radon levels was required. Exposure dose estimates based on the TED results showed that the exposure of tunnel workers to radon did not exceed 3 mSv per annum for the duration of each project.     

Radon in soil gas--investigation and data standardisation at radon reference sites, Czech Republic

Radon risk mapping at building sites in the Czech Republic indicate an advisable level of protection of buildings against the penetration of radon from the geological basement. Various techniques and instruments are used for the measurement of radon in soil gas. A national radon chamber and three radon reference sites in Central Bohemia enable radon data standardisation. Tests of field radon measurements and the reported radon activity concentration in soil gas at the reference sites are based on comparisons with other organisations and with a database of reference site measurements. The radon reference sites have been used for various investigations of radon in soil gas during the period 2000-07.     

Experimental determination of the absorption rate of unattached radon progeny from respiratory tract to blood

An exposure methodology was developed for the determination of the absorption rate of unattached radon progeny deposited in the human respiratory tract to blood. Twenty-one volunteers were exposed in a radon chamber during well-controlled aerosol and radon progeny conditions, with predominantly unattached radon daughters. Special efforts were made to restrict the dose to the volunteers to an absolute maximum of 0.08 mSv. Measurements of radon gas and radon progeny in blood samples of these volunteers indicated absorption half times of 20 min to 60 min. Former determinations, mainly performed with much larger aerosol particles of diameters between 100 nm and 1,000 nm, implied absorption half times around 10 h. This indicates that the absorption of radon decay products from ciliated airways into blood is dependent upon particle size and particle composition.     

氡测量仪检定/校准装置的研制

为建立氡测量的计量标准,研制以多功能的标准氡室为核心的氡测量仪检定/校准装置。采用氡浓度动态稳定技术以实现氡浓度的自动调控;设计用夹胶钢化玻璃制作氡室以减少箱体对氡的吸附,并具有良好的保温效果;设计制作温湿度调控系统和气溶胶发生与采集装置,实现氡子体放射性气溶胶的检测功能。装置氡室体积为4m3,氡浓度测量范围为370～20000Bq/m3,氡浓度值测量结果的相对扩展不确定度不超过5.8%,可用于测氡仪器的检定校准和氡子体放射性气溶胶的实验研究。     

A chamber to test the response of radon detectors to changing environmental conditions

Radon risk assessment is carried out by means of accurate measurements with active or passive instrumentation. All radon detectors must be calibrated and tested using a radon chamber containing a known concentration of radon produced by specific sources of (226)Ra. Some chambers can also be used to test the response of detectors as a function of environmental conditions. In this case, a calibration curve can be inferred with respect to change in one of the considered parameters. For this aim, a new radon chamber was designed and realised to perform calibration and to study the detector response in a large range of variation of the environmental parameters (pressure, 700-1100 mbar; temperature, 5-50°C; humidity, 10-90 %). The first experiments conducted to study the influence of environmental parameters on the detector response have shown flexibility and ease of use of the chamber.     

The NIST Primary Radon-222 Measurement System

Within the United States, the national standard for radon measurements is embodied in a primary radon measurement system that has been maintained for over 50 years to accurately measure radon (²²²Rn) against international and national radium (²²⁶Ra) standards. In turn, all of the radon measurements made at the National Institute of Standards and Technology (NIST) and the radon transfer calibration standards and calibration services provided by NIST are directly related to this national radon standard. This primary radon measurement system consists of pulse ionization chambers and ancillary gas handling and gas purification equipment. The system is currently undergoing a significant upgrading and expansion which will replace the extant outdated system.