A New Turbulent-Burst-Based Model for Particle Resuspension from Rough Surfaces in Turbulent Flow

Particle resuspension could affect human exposure to particulate matter (PM) and serves as a potential route for infection transmission in indoor environments. A new resuspension model incorporating the effects of turbulent bursts, depletion of resuspendable particles, adhesion force distribution, and environmental relative humidity (RH) is proposed. In the proposed model, Monte Carlo simulation is used to model the occurrence of turbulent bursts and the depletion of resuspendable particles on surfaces. The adhesion force distribution and RH effects were included by employing the recently proposed adhesion force distribution model. Model validation is conducted by comparing model predictions against reported experimental data found in the literature. The effects of RH and particle size on resuspension are investigated using the proposed model. The threshold free stream velocity increases by two and three times when the RH increases from 36% to 61% and 67%, respectively. The threshold friction velocity decreases by five times when the particle size increases from 30.1 μm to 111 μm. The proposed model provides a physically reasonable framework for describing particle resuspension under turbulent flow. The capability of predicting the effect of RH greatly enhances the practical application of current resuspension models.

Copyright 2014 American Association for Aerosol Research     

Model Experiments of the Resuspension Caused by Road Traffic

In the literature field experiments were performed in which factors affecting the resuspension of particulate material by road traffic were investigated. The factors involved were in most cases the particle size and the speed of the car. In some cases even the size of the car was varied (medium-sized car or truck). The present experiments were made to obtain a better understanding of the influence of the aerodynamic effects (not the tire effects) affecting resuspension by road traffic. In the experiments a model was used to investigate the influence of its shape, its velocity, and its distance to the surface. The experiments also included the size of the particles and the kind of surface from which the particles were resuspended. These experiments were performed in order to make possible a better interpretation of the field tests     

Effects of relative humidity and particle and surface properties on particle resuspension rates

Wind tunnel experiments examined the coupled effects of relative humidity (RH) and surface and particle properties on aerodynamically induced resuspension. Hydrophilic glass spheres and hydrophobic polyethylene spheres ～20 μm in diameter, with nanoscale surface features, were resuspended from hydrophilic glass, hydrophobic chemical agent resistant coating (CARC), and gold surfaces. Roughness of the glass and gold surfaces was on the nanoscale, whereas CARC surfaces had microscale roughness. Different particle–surface combinations yielded van der Waals interactions that varied by a factor of 4, but these differences had a relatively minor effect on resuspension. Wind tunnel RH was varied between 7% and 78%. Overall, RH affected the resuspension of hydrophilic particles on hydrophilic surfaces most strongly and that of hydrophobic particles on hydrophobic surfaces the least. For each particle–surface combination there was a threshold RH value below which resuspension rates were essentially constant and in good agreement with a dimensionless model of particle resuspension.

Copyright © 2016 American Association for Aerosol Research     

A Particle Resuspension Model in Ventilation Ducts

A turbulent burst model is used and evaluated for particle resuspension in ventilation ducts in this study. The model is a prolongation of the turbulent burst model developed by Cleaver and Yates with an approach to the critical jump-start air velocity for particle resuspension. This critical jump-start air velocity is introduced to estimate the fraction of particles resuspended under the turbulent burst. The model results were compared with experimental data that is available in literature. Both the model results and experiments show that resuspension rate increased with the increase of particle diameter and air speed in ducts. However, the model results did not show a significant decay of particle resuspension rate over time, which was shown in the experiments. Limitations of the model are discussed to explain the discrepancy between the model and the experimental results.

Copyright 2012 American Association for Aerosol Research     

Impact of Airflow Characteristics on Particle Resuspension from Indoor Surfaces

Resuspension is an important source of indoor particles. We measured the resuspension of 1 to 20 μm particles on common indoor materials and explored the importance of turbulence to the resuspension process. Experimental variables included materials (linoleum, carpet, and galvanized sheet metal) and bulk air velocity (5, 10, 15, 20, and 25 m/s). At each of these conditions the turbulence intensity in the boundary layer was varied between a low, medium, and high state and ranged from 9 to 34% at the surface. For comparison of resuspension from the considered surfaces and at different flow conditions, we use the relative resuspension, which quantifies resuspension without requiring knowledge of the number of particles initially seeded on the surface. The relative resuspension compares the fraction of particles resuspended at the experimental conditions to the maximum achieved with a controlled impinging jet. In general, the results show that for the ranges considered, increasing velocity caused the largest increase in resuspension, followed by increasing turbulence intensity and then increasing particle diameter. All three material types showed consistent patterns with carpet having the largest resuspension for a given set of conditions, followed by linoleum and then by galvanized sheet metal. High turbulence and high velocity conditions minimized the differences between materials. An understanding of the relative magnitudes of these effects allows for better analysis and mitigation of indoor resuspension.     

Resuspension of Particulate Matter from Carpet Due to Human Activity

This work investigated the resuspension and subsequent translocation of particulate matter (PM) from carpeted flooring surfaces due to walking. In addition, the effect of HVAC systems and ceiling fans on mixing and/or translocation of resuspended PM was studied. Testing took place both in a residence with a well-worn, soiled carpet and in an environmental test chamber. Prescribed walking occurred with PM measurements taken at multiple sampling heights. Scanning electron microscopy (SEM) of carpet fibers was used to determine the fraction of dust available for resuspension. These data, in conjunction with resuspended mass concentrations from this study, were used to generate emission factors by particle size for walking on both new and worn carpet.

Carpet loading does not affect the emission factor, indicating that the amount of resuspended PM is directly proportional to the available PM in the carpet. While relative humidity (RH) plays an important role in resuspension from new carpets, with high RH enhancing resuspension, it has the opposite affect with old carpets, with increased RH decreasing resuspension. With the HVAC system on, translocated particles 1.2 m horizontally from the source had number concentrations of approximately 20–40% of those at the source. With a ceiling fan on, extensive mixing was noted with little difference seen in particle resuspension by height. With the ceiling fan off, there was very little mixing present and particle size varied substantially by height.     

Modelling of particle resuspension by a turbulent airflow and the role of particle size,surface roughness and electric charge

A resuspension model based on the Lennard–Jones intermolecular potential is applied to a monolayer deposit of spherical particles. The model considers the interactions between a particle and a surface under the influence of an external turbulent airflow. The particle–surface interaction was modelled with and without particle deformation due to elastic flattening. The resuspension rate was calculated by a kinetic force-balance approach whereby particle detachment occurs when the instantaneous joint contribution of the lift and drag forces exceeds the total adhesive force of the particle–surface system. Enhanced aerodynamic particle removal driven by the moment of the lift and drag forces was determined. Model predictions suggest that inclusion of the moment of the aerodynamic forces provides a suitable model for particle detachment (initiated by rolling). The importance of elastic deformation was found to depend on adhesive forces, characteristics of the substrate surface (surface roughness) and particle size. The model was applied to a number of laboratory experiments. For one set of experiments, we identified two resuspension regimes depending on whether small non-deformable or large deformable (equivalently, strongly or weakly bound) particles resuspended at high or low friction velocities. A modified model incorporating the effect of particle charge is also presented. Results indicate that particle resuspension is possible even when electrostatic forces are present, but the resuspension rate decreases considerably, depending on particle size, particle charge and surface roughness.     

Resuspension of Dust Particles in a Chamber and Associated Environmental Factors

Experiments investigating particle resuspension from human activities were conducted in a full-scale experimental chamber. The experiments tested three types of flooring (vinyl tiles, new and old level-loop carpets) and two ventilation configurations (ceiling and side wall supply systems). The floorings were seeded with 0.1–10 μ m test particles. The airborne particle concentration was measured by an array of optical particle counters (OPCs) in the chamber. Resuspension rates were estimated in size ranges of 0.8–1, 1.0–2.0, 2.0–5.0, and 5.0–10 μm ranging from 10^?5–10^?2 hr^?1, with higher resuspension rates associated with larger particles. Resuspension via walking activity varied from experiment to experiment. “Heavy and fast” walking was associated with higher resuspension rates than less active walking, most likely due to a combination of increased pace, increased air swirl velocity, and electrostatic field effects established by the walking. The type of floorings also influenced the particle resuspension. Given the same size and mass distribution of test particles per unit floor area, resuspension rates for the seeded new level-loop carpet were significantly higher than those for the vinyl tile flooring for larger particles (1.0–10 μ m) under the ceiling air supply system.     

Modelling of the resuspension of particle clusters from multilayer aerosol deposits with variable porosity

A model for the resuspension of multilayer aerosol deposits has been developed taking into account the dependence of resuspension rates on the deposit structure, as well as the fact that particles are typically resuspended in clusters. The model is based on three main concepts: Constructing artificial, irregular particle deposits with variable bed porosity; identifying resuspendable clusters on the surface of these deposits by means of a sufficiently simple topological criterion; and assigning resuspension probabilites per unit time to resuspendable clusters based on a balance between forces of adhesion and turbulent bursts. The model accounts at least qualitatively for several experimental observations not predicted so far by any previous resuspension model. A similarity analysis of the model leads to the identification of non-dimensional groups that could possibly be used in empirical correlations.     

Triboelectric charging of fungal spores during resuspension and rebound

The triboelectric charging of fungal spores was experimentally characterized during rebound and resuspension. A fungal spore source strength tester (FSSST) was used as a primary aerosol generator for spores of three fungal species and two powders (silicon carbide and silver). The critical velocity of rebound was determined using a variable nozzle area impactor (VNAI), and the charging state of particles after resuspension and rebound was measured using the FSSST, different impactor setups, electrometers, and optical particle counters. In the impactor setups and the FSSST, five different surface materials relevant for indoor environments were used (steel, glass, polystyrene, paper, and polytetrafluoroethylene). The critical velocity of rebound was determined to be 0.57 m/s for fungal spores, which is relatively low compared to silicon carbide and previous results for micron-sized aerosol particles. Based on the rebound impactor measurements, we were able to define the crucial parameters of charge transfer for different particle–surface material pairs. A contact charge parameter, which describes the triboelectric charging during rebound, was found to have a negative correlation with the charging state of the particles after the resuspension from an impactor. This connects the triboelectric charging during rebound and resuspension to each other. Based on the contact charge parameter values, quantified triboelectric series could be formed. The results of this work show that fungal spores can be charged both positively and negatively during rebound and resuspension depending on the fungal species and surface material.

Copyright © 2016 American Association for Aerosol Research     

Effects of air temperature and humidity on particle deposition

Particle deposition in a fully developed turbulent duct flow was studied. The random walk model of Lagrangian approach was used to predict the trajectories of 3000 particles with a density of 900 kg/m³. The effects of thermophoretic force and air humidity were also considered. The results were compared with the previous studies with a particle size range of 0.01–50 μm and air flow velocity of 5 m/s. The profile of dimensionless deposition velocity with relaxation time presents a V-shaped curve and the results are in good agreement with the previous studies.The effects of air temperature and humidity on particle deposition with a particle size of 1 μm were also investigated. The results show that thermophoretic force accelerates particle deposition onto the duct walls with increasing temperature difference between air flow and the duct wall surface. Meanwhile, it was found that particle deposition velocity increases with air humidity.     

高湿黏性颗粒在聚四氟乙烯微孔膜滤料表面沉积特性的数值模拟

基于聚四氟乙烯(PTFE)微孔膜滤料扫描电镜(SEM)图像,建立PTFE微孔膜滤料微观结构模型,采用计算流体力学和离散单元法(CFD?DEM)耦合的方法对黏性颗粒在微孔膜滤料表面沉积特性进行模拟,引入液桥力模型,忽略范德华力的作用,统计计算域内颗粒的受力情况,分析了不同表面能条件下3~6 ?m粒径颗粒在微孔膜滤料表面的沉积特性,将模拟结果与黏附效率的经验公式进行对比。结果表明,黏附效率与经验值、颗粒受力与液桥力模型的相对误差均在6%以内,CFD?DEM耦合计算方法可用于模拟不同环境湿度条件下的颗粒沉积;过滤风速、粒径与黏性是影响沉积形态的重要因素,提高过滤风速及增大颗粒粒径与黏性,颗粒更易在滤料表面形成稳定的树突结构,黏附效率及含尘压降增加。环境相对湿度影响两物体间液桥体积,接触力影响颗粒沉积,当增加表面能与液桥体积时,接触力及液桥力均相应增加,根据受力平衡原理,环境相对湿度对颗粒沉积影响很大。     

A Stochastic Model for Particle Deposition and Bounceoff

A new model for particle deposition and bounceoff that combines current knowledge of turbulent bursts with the stochastic properties of turbulent fluctuations is presented. The model predictions for deposition velocities agree with experimental results in the literature for dimensionless particle relaxation time τ_p ⁺ > 2. For τ_p ⁺ > 10, most of the particles delivered to the edge of the viscous sublayer are able to deposit onto the surface due to their inertia; the deposition velocity approaches an asymptotic value because the process becomes limited by the rate of turbulent delivery to the viscous sublayer. Because of the penetration of turbulent fluctuations into the viscous sublayer, the minimum values of vertical velocities needed for particles to deposit onto the surface are smaller than those predicted by the free flight model. Most of the deposition occurs from those turbulent fluctuations at the upper tail of the distribution of the vertical component of air velocity.

In addition to the deposition velocity, the model is able to provide the distribution of particle velocities on reaching the surface which is used to compute the fraction of particle bounceoff. The model predictions for the fractions of rebound agree reasonably with the measured results from a wind tunnel experiment for τ_p ⁺ > 2. However, both the deposition velocity and the fraction of rebound are underestimated by the model for τ_p ⁺ < 2. Other mechanisms such as Brownian diffusion must be included in further revisions to this model in order to obtain satisfactory predictions for smaller values of τ_p ⁺.     

Experimental study of aerodynamic resuspension of RDX residue

Residues of hazardous substances, such as chemical compounds with low vapor pressure, radioactive particles, or biological contamination can remain on surfaces for a prolonged period of time. The fate of these particles partially depends on the aerodynamic resuspension rates from the surfaces that are a function of particle and surface properties as well as the environmental conditions. The aerodynamic resuspension can be used for non-contact surface sampling. The removal rates of microscopic explosive trimethylenetrinitramine (RDX) particles from smooth glass surfaces in a controlled flow environment are investigated in this paper. The shear stress in the flow cell is calculated using computational fluid dynamics as a function of velocity. The RDX particle samples are prepared by dry transfer. Particle sizes and morphologies are measured by 3D scanning electron microscopy (SEM) and optical profilometry. The resuspension rates are calculated based on the changes in the total coverage area before and after exposure to aerodynamic forces. These rates are correlated with wall shear stresses, particle size, and morphology. For non-spherical particles, the removal rates are proportional to the particle shape factor defined as a ratio of particle height to the projected equivalent diameter.

Copyright © 2019 American Association for Aerosol Research     

一种新型受热面飞灰颗粒的沉积特性

以一种余热锅炉中新型的受热面为研究对象,采用实验研究和数值模拟的方法研究其飞灰沉积特性。建立了菱形受热面飞灰颗粒的沉积模型,对飞灰颗粒的反弹、黏附及脱落过程进行预测,并与叉排管束和顺排管束的含灰烟气流的速度场、温度场和飞灰颗粒沉积率进行比较。结果表明,菱形受热面在换热和飞灰沉积方面优势明显。沉积主要集中于受热面左上部,颗粒由于惯性碰撞在迎风侧沉积。相同速度下,随颗粒粒径增加沉积率先增大后减小,在3 m·s^-1的烟气流速下颗粒直径为5 μm时飞灰颗粒沉积率最高,为9.49%。保持粒径不变,随速度增大沉积率逐渐降低。     

Experimental Study of Impulse Resuspension with Laser Doppler Vibrometry

Particle resuspension due to mechanical impulse was studied for spherical polymethylmethacrylate (pmma) particles ranging from 1.7 to 14.4 μm in diameter on titanium dioxide (TiO₂) and silicon dioxide (SiO₂) wafers. Dry powders were dispersed, electrostatically neutralized, and allowed to deposit under the influence of gravity. Contaminated surfaces were then mechanically excited with a 5 MHz piezoelectric transducer where surface accelerations (～10⁶ m/s²) and resuspension ratios were quantified with laser Doppler vibrometry (LDV) and digital microscopy, respectively. For TiO₂, experiments were performed over a broad range of relative humidity (25 to 95%) to assess the effects of capillary condensation. Resuspension was a monotonically decreasing function of relative humidity. Existing theories were used to separate data into two adhesion regimes based on capillary bridge formation: van der Waals (vdW) and capillary dominated adhesion. For relative humidity above 60%, resuspension forces were nondimensionalized by the theoretical capillary force. Resuspension data for all particle sizes and relative humidity were described by a single sigmoid function dependent on the dimensionless resuspension force. Below 60% relative humidity, resuspension forces were nondimensionalized by the vdW force calculated with Johnson–Kendall–Roberts adhesion theory. The experimental work of adhesion (pmma-TiO₂) was optimized such that the dimensionless resuspension curves, for capillary and vdW forces, had equivalent dimensionless resuspension forces at 50% resuspension. The calculated value, 0.047 J/m², was within the range of values expected from other published works. Resuspension was not observed for particles on SiO₂ substrates. This result was attributed to electrostatic surface charge patches where particle charge and surface resistivities were measured to analyze the relative influence of electrostatic adhesion forces.

Copyright 2012 American Association for Aerosol Research     

Multilayer Resuspension of Small Identical Particles by Turbulent Flow

ABSTRACT

A model for the resuspension of a multilayer deposit by turbulent flow is developed. The resuspension rate is obtained by solving a set of coupled, first-order kinetic equations. The multilayer resuspension rate depends explicitly on single-particle resuspension rates that are determined from a modified energy-transfer model. The surface-particle and particle-particle interaction potentials are calculated by a microscopic approach based on the integration of the Lennard-Jones intermolecular interaction potential. The effect of the surface roughness, which leads to a distribution of the adhesive forces, is considered, as well as the energy transfer from the fluctuating part of the turbulent flow to the particle. It is shown that for a geometrical arrangement of deposited particles with a co-ordination number of two (particles stacked on top of each other) particles from the top layers resuspend at lower friction velocities than particles adjacent to the surface. The predicted long-term resuspension rate decays algebraically with exposure time. Calculations are presented for a two-layer deposit of either SnO₂ and Al₂O₃ particles on a stainless steel surface.     

Effects of particle concentration and size on the dissipation rate and turbulent kinetic energy of oil

The presence of particles in oil can change the quasi-sequence structure of the turbulent flow of the oil, and it is extremely important to explore the turbulent energy dissipation rate of the particulate-containing oil and ensure the safe and stable operation of the oil-using equipment. Thus, the flow field of the oil containing particles in the pipeline was experimentally studied by a particle image velocimeter (PIV); the turbulent kinetic energy of the oil was calculated using the transient velocity vector field measured by the PIV; and the dissipation rate distribution was calculated using the large eddy PIV method. The influence of different particle sizes and particle concentrations on the normal distribution of the turbulent kinetic energy and dissipation rate was analyzed. The results show that the distribution of the turbulent kinetic energy in the normal direction is non-unidirectional and in a parabolic shape. The 25 μm particle size has a great influence on the turbulence kinetic energy and the dissipation rate of the oil; with increasing particle concentration, the flow field distribution of the turbulent kinetic energy increases in the region near the wall, and gradually decreases in the central region. The turbulent kinetic energy distribution of the oil is in the shape of a quasi-cosine; the flow field of the dissipation rate is larger in the near-wall region and the central region and shows an inverted ‘W’ shape. This provides a theoretical basis for improving the efficiency of oil transportation, discussing the monitoring of particulate matter in oil, and reducing oil pollution.     

Wind tunnel study and numerical simulation of dust particle resuspension from indoor surfaces in turbulent flows

Particle resuspension from flooring is an important source of air pollution in the indoor environment. In this work, resuspension of monolayer, polydisperse, irregularly shaped dust particles from various types of floorings was studied via a series of wind tunnel experiments. The range of free-stream velocity needed for resuspension of dust particles was evaluated as a function of particle size and material of particles and surfaces. In addition, a Monte Carlo simulation for predicting the resuspension of dust particles was developed. The resuspension model took into account the effects of particle irregularity, particle surface roughness, and flow characteristics. The dust particle resuspension from different floorings for several particle sizes was evaluated. The model predictions for resuspension fractions were compared with the experimental data and good agreement was observed. The study provided information on the role of airflow velocity on irregular dust particle resuspension from common floorings.     

Aerosol Particle Removal and Re-entrainment in Turbulent Channel Flows - A Direct Numerical Simulation Approach

Aerosol particle removal and re-entrainment in turbulent channel flows are studied. The instantaneous fluid velocity field is generated by the direct numerical simulation (DNS) of the Navier - Stokes equation via a pseudospectral method. Particle removal mechanisms in turbulent channel flows are examined and the effects of hydrodynamic forces, torques and the near-wall coherent vorticity are discussed. The particle resuspension rates are evaluated, and the results are compared with the model of Reeks. The particle equation of motion used includes the hydrodynamic, the Brownian, the shearinduced lift and the gravitational forces. An ensemble of 8192 particles is used for particle resuspension and the subsequent trajectory analyses. It is found that large-size particles move away roughly perpendicular to the wall due to the action of the lift force. Small particles, however, follow the upward flows formed by the near-wall eddies in the low-speed streak regions. Thus, turbulent near-wall vortical structures play an important role in small particle resuspension, while the lift is an important factor for reentrainment of large particles. The simulation results suggests that small particles (with τ_p⁺ ≤ 0.023) primarily move away from the wall in the low-speed streaks, while larger particles (with τ_p⁺ ≥ 780) are mostly removed in the high-speed streaks.