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1.
The U.S. Environmental Protection Agency (EPA) has promulgated new national ambient air quality standards for PM10 (particles smaller than 10 μm aerodynamic diameter). Samplers used to collect PM10 must be subjected to wind tunnel tests before they can be approved as part of a designated reference or equivalent method. Monodisperse liquid and solid particles are used over a range of particle sizes and windspeeds to characterize the sampling effectiveness and 50 percent cutpoint of candidate samplers. This paper describes an EPA wind tunnel test facility, sampler test procedures, and the results of selected sampler tests with liquid and solid test particles. The agreement between wind tunnel results and observations from field measurements of ambient particulate matter is also discussed.  相似文献   

2.
This article uses numerical simulation to investigate the effect of sampler bluntness, particle size, and sampler orientation on aspiration efficiency in calm air. The procedure is to first numerically solve the velocity field around the sampler in calm air and then to trace the particle trajectories and calculate the the aspiration efficiency. Two samplers are studied: a two-dimensional parallel plate and a two-dimensional blunt cylinder. The variation of aspiration efficiency with particle size shows two minima between two asymptotic values. When the samplers are facing upward, the asymptotic values are 1 for very small particles and the ratio of particle settling velocity to suction velocity for very large particles. At other orientations, the horizontal-facing and the downward-facing, the asymptotic value for large particles is 0. The sampler bluntness has an important effect in the region of particle size where there is competition between the particle inertia and the fluid drag force (i.e., 5 μm < d > 100 μm in our case). A blunt sampler always has higher aspiration efficiency than does a sharp-edged sampler in this region of particle sizes. For very small particles and very large particles, the aspiration efficiencies approach asymptotic values and the sampler bluntness has little effect. The results also show that the sampler orientation affects the predicted aspiration efficiency  相似文献   

3.
Massive-flow air samplers are being deployed around the world to collect aerosol samples for analysis of radioactivity as a result of nuclear tests and nuclear accidents. An aerosol wind tunnel capable of an 1100 m3 min?1 flow rate was built at Lovelace Respiratory Research Institute (LRRI) to test the sampling efficiency of these samplers. This aerosol wind tunnel uses a stationary air blender to enhance mixing, and therefore it achieves the required uniform distribution of wind speed and aerosol concentration in the test section. The test section of the wind tunnel has a cross section that is 4.3 m × 3.7 m. The aerosol wind tunnel was tested for performance in terms of distribution of wind speed, turbulent intensity, SF6 tracer gas concentration, and aerosol concentration. Test criteria consistent with U.S. Environmental Protection Agency (EPA) and American National Standards Institute (ANSI) standards were adopted as the guidelines for the aerosol wind tunnel. Additional criteria for aerosol wind tunnel were also recommended. Initial test of the aerosol wind tunnel showed that the wind tunnel could be operated in a wind speed range of 2 to 24 km h?1. Within this range, the distribution of wind speed SF6 trace gas concentration and aerosol concentration in two-thirds of the central area of the test section showed coefficient of variances (COVs) of less than 10% for the range of wind speeds. This met the stringent guidelines for aerosol wind tunnel performance set by EPA and ANSI standards.

The LRRI wind tunnel was used to evaluate the collection efficiency of the sampling head of massive-volume air samplers, including the Snow White sampler. The sampler was tested in this aerosol wind tunnel for particles between 2 and 20 μm. The sampling flow rates were 500 and 700 m3 h?1 for the tested wind speeds of 2.2 and 6.6 m S?1, respectively. The results showed that sampling efficiency was influenced by both sampling flow rate and wind speed. The sampling efficiency decreased with an increase in particle size of between 2 and 20 μm. The sampling efficiency also decreased as the wind speed was increased from 2.2 to 6.6 m S?1.  相似文献   

4.

The purpose of this study was to numerically simulate the performance of an aerosol sampler with a curved, blunt, multi-orificed inlet in order to understand the sampling characteristics of the first prototype of the button personal inhalable aerosol sampler ("button sampler"). Because the button sampler inlet design is too complicated to apply a three-dimensional model, an axisymmetric two-dimensional model was created to be similar in geometry and to simulate the major features of the airflow through the sampler when facing the wind. Particle trajectories were calculated in a variety of wind velocities and were categorized into 5 groups based on their interactions with the curved surface of the sampling plane. Empirical sampling efficiencies of the button sampler for 3 particle sizes were used to adjust the calculated sampling efficiencies in an attempt to improve the accuracy of the two-dimensional axisymmetric model in accounting for interactions between particles and the surface of the inlet of the button sampler. Sampling efficiencies for other particle sizes were then predicted. The results showed that sampling efficiency decreased with increasing particle size up to approximately 40 w m and then remained virtually unchanged at about 35% up to 100 w m. Although the efficiencies were lower than the American Conference of Governmental Industrial Hygienists' (ACGIH) inhalability curve for larger particles, the pattern of the predicted sampling efficiency was quite similar to the ACGIH inhalability curve. Sampling efficiencies for liquid aerosol particles larger than 15 w m were predicted to be noticeably lower than those for solid particles. The results also showed that the multi-orificed curved surface played an important role in establishing a pressure drop with desired flow alignment inside the sampler, thus greatly reducing the wind effect and significantly improving the uniformity of particle deposition on the filter. The less uniform deposition found at high wind velocity can be improved by increasing the sampling flow rate.  相似文献   

5.
Experimental filtration data were collected in an effort to validate an impaction model previously developed and presented. Using a sampler with a 9.5 μm pore diameter Nuclepore filter, collection efficiencies were measured for both liquid and solid aerosols over a size range of 2–9 μm. Data for the liquid aerosol showed good agreement with the impaction model; however, data for the solid aerosol indicated an appreciably lower collection efficiency than predicted by the model. The liquid aerosol data validate the impaction model. The solid aerosol data indicate particle bounce or reintrainment subsequent to impact and underscore particle capture as a problem to be dealt with if the Nuclepore surface is to be used as a size selective filter.  相似文献   

6.
Particle capture experiments conducted in turbulent cross flow with various aerosols involving liquid and/or solid particulates have resulted in collection efficiencies which are in excess of the values predicted by the various known models of particle capture, i.e., inertial impaction, interception and Brownian diffusion. In one type of experiment the turbulent air stream, carrying submicron dust particles, is flowing past a cylindrical collector (such as a piece of wire) with its axis orientated perpendicular to the direction of flow. Collecting efficiencies ranging up to about 20% have been found under conditions where the conventional models of particle capture predict practically zero collection efficiencies. In another type of experiment involving injecting a fog (2–80 μm diameter water droplets) into the dusty gas stream carrying submicron size dust particles which subsequently enters a slow turning fan. While passing through the fan, the fog agglomerates into raindrops while scavenging most of the dust particles. For example, a 0.8 μm median particle size aluminum silicate pigment was collected with 97–99.5% efficiency, the exact value depending on the operating conditions. Theoretical analysis of these phenomena may be based on the idea of synergism involving inertial impaction and eddy diffusion: the smaller dust particles/drops are captured by the larger drops in the fan and the dust particles are captured by the wires because (a) there is a significant relative velocity between them and (b) because the particles undergo eddy diffusion.  相似文献   

7.
We recently developed an electrostatic collector for bioaerosols that electrostatically deposits biological particles onto a 3.2 mm electrode covered by a superhydrophobic substance. The deposited biological particles are removed and collected by rolling water droplets (20 or 40 microliter) which results in high concentration rates. The collector has been improved further by integrating it with an electrical charger. Here, we describe the development and optimization of the charger and collection chamber, while maximizing collection efficiency and minimizing particle loss. The resulting sampler is made of static dissipative material (e.g., Delrin), is shaped as a closed half cylinder, and is integrated with a charger. The sampler's round top section contains eight carbon fiber brushes (ion sources to charge particles), while its flat bottom section holds a rectangular collection electrode (254 × 3.2 mm) made of pressed carbon fiber and coated with a superhydrophobic material.

The optimized configuration of the EPSS Mark II had a collection efficiency of up to 84% when sampling airborne Escherichia coli at 10 L/min and for 10 min. The bacteria were accumulated in rolling water droplets as small as 20 microliters, and the sampler achieved sample concentration rates of up to 4.2 × 105/min. When the sampler was operated for a longer time period (60 min), its collection efficiency was 72%. The efficiency decrease was most likely due to a reduced particle removal from the electrode, but the difference was not statistically significant. Since the EPSS Mark II shows satisfactory collection efficiency and high sample concentration rate, it could serve as a basis for developing a field-deployable version of the sampler.

Copyright 2015 American Association for Aerosol Research  相似文献   

8.
ABSTRACT

A new principle for collecting airborne particles, including microorganisms, has been introduced by injecting the particles into a swirling airflow from where they are removed onto a collection surface. A dry surface, a surface coated with an adhesive substance or a surface wetted by a liquid swirled onto the collection surface from a reservoir below can be used in the new collection method. The swirling air motion and aerosol injection into it are achieved by drawing the airborne particles through nozzles that are directed at an angle toward the collection surface. This principle has been incorporated into a new sampler that has been named “Swirling Aerosol Collector” (SAC; commercially available as the “BioSampler” from SKC Inc., Eighty Four, PA). The physical performance of the SAC has been evaluated against the widely used AGI-30 impinger by measuring the particle concentrations upstream and downstream of each sampler with an aerodynamic particle sizer. Tests with monodisperse polystyrene latex (PSL) particles ranging from 0.3 to 2.0 μm have shown that the SAC has better collection efficiency than the AGI-30 when the same collection liquid is used. A conventional impinger maintains constant collection efficiency for a relatively short sampling period, as the liquid evaporates quickly due to the violent bubbling of the liquid. In contrast to conventional impingers, the SAC can be used with nonevaporating liquids that are considerably more viscous than the liquids used in the impingers. Thus, the SAC can sample over any period of time. The new aerosol sampler produces minimal or no reaerosolization of particles collected in the liquid in contrast to significant reaerosolization in a conventional impinger. Since the SAC projects the aerosol particles toward the collection surface where they are removed from the swirling flow, it avoids or significantly reduces particle bounce from the collection surface even when the surface is dry.  相似文献   

9.
The design of a new aerosol sampler, called the blunt-body aerosol sampler (BASE), to sample interstitial particles inside clouds while avoiding the problem of cloud droplet shatter artifacts is introduced. The primary design feature of the inlet is a blunt body that houses an aerosol inlet toward its aft end. The housing is designed to be blunt enough to deflect large cloud particles traveling around the body while being streamlined enough to maintain an attached boundary layer under aircraft flow conditions. The attached flow requirement ensures that shatter particles formed from the impaction of cloud droplets on the blunt body are retained close to the surface of the body. A region of large particle shadow is, thus, created in the aft of the blunt-body housing, where an aerosol inlet can sample interstitial particles in the absence of cloud particles. Computational fluid dynamics (CFD) simulations are used to optimize the shape of the blunt body, and the final sampler design is predicted to sample particles smaller than 2 μm from the freestream while being uninfluenced by cloud droplet shatter particles of the same size. Wind tunnel tests were performed on a prototype model to confirm the attached nature of the boundary layer flow around the blunt body and to establish the size-dependent behavior of shatter particles in the vicinity of the housing. While the experiments provide initial validation of the interstitial inlet design concept, some discrepancies were observed between the wind tunnel tests and CFD predictions, suggesting a need for improvements in simulations, inlet design, and/or test methodology. Initial analyses of field data obtained from the first aircraft deployment of BASE confirm that sampling of shatter-free interstitial aerosol is possible with the inlet, but full performance characterization of BASE will require significant additional aircraft-based experiments under a range of cloud conditions.

Copyright 2013 American Association for Aerosol Research  相似文献   

10.
A method and test system have been developed for the laboratory evaluation of the performance of bioaerosol samplers. The method differentiates between the overall physical sampling efficiency (which reflects the inlet and collection efficiencies) and the biological sampling efficiency (which reflects the survival of the test microorganisms during the sampling process). The number concentrations of laboratory-generated bioaerosol particles are measured with an aerosol size spectrometer up- and downstream of the bioaerosol sampler being tested. In a bioaerosol impactor, which was specially designed for testing microbiological aspects of bioaerosol sampling, the inlet and collection efficiencies are differentiated by measuring downstream of the collection surface location with and without the collection surface in place. The number of recovered particles is counted as microcolonies with a microscope after sampling the bioaerosol particles into agar and culturing them. The total recovery of these bioaerosol particles is determined as a ratio of the number of viable microorganisms recovered to the number of bioaerosol particles present in the air sampling volume upstream from the sampler. This total recovery is a measure of the ratio of culturable to non-culturable bacteria present in the air. By measuring physical and microbiological aspects simultaneously, information is gained on aspects of bioaerosol sampling that cannot be determined by either of these branches of science alone. This is exemplified by tests on the influence of relative humidity and desiccation time on colony count.

The newly-developed system can be used to test any bioaerosol sampler. A special single-stage impactor was designed, built and used to study how different sampling and analysis variables affect the total recovery of bioaerosol particles. The designed impactor was calibrated using PSL particles. Its inlet sampling efficiency was found to be within the range of 96–99.5%, depending on the sampling conditions and particle size, if the latter is less than 8 μm (this range represents single bacteria, bacterial agglomerates, and fungi). The collection efficiency was found to be about 100% when collecting PSL particles larger than 0.7 μm in diameter at 201 min−1 or higher air flows.

The total recovery of microorganisms measured under these conditions is characterized only by the “survivability” of microorganisms during their sampling. It was found that relative humidity had a pronounced effect on total Pseudomonas fluorescens recovery. Experimental data also showed that the sampling time may be limited due to bacterial desiccation and subsequent loss in viability of collected microorganisms.  相似文献   


11.
《Journal of aerosol science》2003,34(11):1493-1504
Electret filters are composed of permanently charged electret fibers and are widely used in applications requiring high collection efficiency and low-pressure drop. We tested electret filter media used in manufacturing cabin air filters by applying two different charging states to the test particles. These charging states were achieved by spray electrification through the atomization process and by bipolar ionization with an aerosol neutralizer, respectively. Polydisperse solid NaCl particles with 0.1%, and 1% solutions or liquid dicotyl sebacate (DOS) particles were generated from an atomizer, and they were loaded on the filter media. The amount of charge, the mean particle size, and the particle material significantly affected the collection performance of the electret filter media for submicron particles. The collection efficiency of the electret filter media degraded as more particles were loaded, and showed minimum efficiency at steady state. The electret filter media captured the highly charged particles more efficiently during the transient state. At steady state, the filter media loaded with smaller NaCl particles showed lower collection efficiency. The filter media loaded with liquid DOS particles showed collection efficiency much lower than those loaded with solid NaCl particles.  相似文献   

12.
Conventional gravitational wet scrubbers, which generally perform removal of fine particles with low efficiency, cannot meet new standards for pollution emissions. One way of improving the collection efficiency of fine particles is to impose additional electrostatic forces upon particles by means of particle‐charging, or droplet‐charging, or even opposite‐charging of particles and droplets. A Monte Carlo method for population balance modeling is presented to describe the particle removal processes of gravitational wet scrubbers with electrostatic enhancement, in such a way that the grade collection efficiency and particle size distribution are calculated quantitatively. Numerical results show that, the grade collection efficiency of submicron particles is only ca. 5 % in conventional wet scrubbers. However, it reaches ca. 25 % in particle‐charging wet scrubbers, ca. 70 % in droplet‐charging wet scrubbers, and even above 99 % in opposite‐charging wet scrubbers. Furthermore, population balance modeling is used to optimize the operational parameters of the droplet‐charging wet scrubbers by means of the quantitative comparison of the grade collection efficiency. It is found that the operational parameters that are beneficial to the high‐efficiency removal of fine particles are faster gas velocity, slower droplet velocity, larger liquid‐to‐gas flow ratio, larger charge‐to‐mass ratio of droplets, smaller geometric mean diameter and smaller geometric standard deviation of droplets.  相似文献   

13.
A thermophoretic sampler is designed for the collection of particles smaller than 10 nm. The sampler is composed of heated and cooled surfaces separated by a gap of 0.1 mm; a bypass flow is introduced in the design to minimize the diffusional loss of nanoparticles in the upstream flow channel. Particles may be directly deposited on a 3 mm diameter TEM grid for chemical analysis or on other substrates for other purposes. Calculations show that at an inlet flow rate of 1.5 lpm and thermal gradient of 5 × 105 K/m, a maximum collection efficiency of 41% can be achieved for a particle diameter of 1 nm. Ag particles with median size of 6 nm are used to characterize the thermophoretic sampler collection efficiency. The TEM images show that a sizeable number of particles less than 10 nm in diameter are collected, although they are not uniformly distributed on the grid, and the collection efficiency deduced from these deposited particles is much less than the theoretical estimation. Despite this, the efficiency is orders of magnitude higher than previous designs and it is easier to build.  相似文献   

14.
The proof of concept of a novel in-line real impactor (IRI) for preseparation of large particles in ambient inlets was demonstrated with a 1,250 L/min design. Numerical simulations predicted a cutpoint Stokes number 0.3 for a ratio of jet-to-plate spacing to jet width (S/W) of 2.0 and 0.5 for a ratio of 4.0. This variation in cutpoint Stokes number allows minor adjustments in cutpoint for a given device size. Experimental benchmark tests support the prediction of a shift in cutpoint with S/W. Inlet systems with flow rates of 100 and 400 L/min were designed by Stokes scaling of the 1,250 L/min IRI and integrating the lower flow devices with an existing inlet aspiration section and an insect screen. Experiments with the inlet system were conducted in a wind tunnel with particles from 3 to 20 μm aerodynamic diameter (AD) and wind speeds of 2, 8, and 24 km/h. A nominal cutpoint of approximately 11 μm AD was selected to accommodate bioaerosol sampling needs, and the wind tunnel results showed the average cutpoints of the 100 and 400 L/min inlet systems at the three wind speeds were 11.2 and 11.6 μm AD, respectively. Stand-alone tests with the 100 and 400 L/min IRIs were conducted where dry dusts (Arizona road dust/fine and coarse) were impacted on three types of collection surfaces (dry, grease-coated, and oil-soaked porous surfaces) to characterize solid particle carryover. The oil-soaked porous media allowed the least carryover of large solid particles.  相似文献   

15.
Exposure to fungal aerosols is of concern in indoor environments. However, sampling limitations have previously made it difficult to assess exposures accurately, especially long-term exposures. A prototype personal aerosol sampler, based on cyclone principles and using a 1.5 ml microcentrifuge tube as a particle collection receptacle has been designed and fabricated. Collection efficiency for aerosol particles in the size range of fungal spores has been evaluated for different types of microcentrifuge tubes, together with the effect of a polyethylene glycol coating on the inside of the tube and the effect of adding water to the tube. Monodisperse, fluorescently tagged polymer microspheres with median diameters of 0.5, 1, 2, 3, 6, 11, and 16 μm were used to evaluate sampler performance with particle diameter. The microcentrifuge-tube sampler was tested at flow rates of 2 and 4 liters per minute (l/min). Experimental results indicate that the microcentrifuge-tube sampler has an aspiration efficiency of 100% in calm air for particles up to 16 μm. At 4 l/min, the microcentrifuge-tube sampler is able to collect nearly 100% of particles greater than 3 μm and > 90% of particles between 2.5 and 3 μm. The 50% cutoff size is 1.5 μm. The performance of the sampler did not vary with the different brands of tubes tested or with the presence or absence of a coating on the tube surface. Furthermore, the addition of water to the tube resulted in a slight increase in collection efficiency. A sampling time of 5 h was feasible at 45–50% relative humidity before evaporation led to significant water loss.

The cutoff size of 1.5 μm is comparable to many commercially available bioaerosol samplers. Besides being easy to use, simple to fabricate, and inexpensive, this novel sampler has several advantages over conventional samplers: long-term samples are possible (the limitation of impaction methods); there is no sample transfer loss since the transfer step has been eliminated (the limitation of filter cassettes); laboratory analyses are not dependent solely upon a single analysis method (the limitation of impaction methods), and there is no sampler adherence loss (the limitation of trying to wash microorganisms from filters). In addition, use of the sampler would be applicable in a variety of occupational settings from low bioaerosol concentrations (i.e., indoor environments) to high bioaerosol concentrations (i.e., agricultural setting) by varying sampling time periods and using sensitive analytical methods.  相似文献   

16.
The inlet sampling characteristics of several commercial bioaerosol samplers operating in indoor and outdoor environments have been analyzed by use of available and newly developed equations for sampling efficiency. With a focus on the physical aspects of sampling efficiency, the aspiration and transmission efficiencies have been calculated for the bioaerosol particle size range 1–30 μm, which represents single bacteria, bacteria aggregates, bacteria carrying particles, fungal spores, yeast, and pollen. Under certain sampling conditions, the bioaerosol concentration was found to be significantly over- or underestimated. At wind velocities between 0 and 500 cm s−1, calculations show that the AGI-30 would sample 1–10 μm particles with an inlet sampling efficiency of 20–100%. The entrance efficiency of the 6-stage Andersen viable sampler is 90–150% when sampling isoaxially with respect to horizontal aerosol flows, and 8–100% when oriented vertically at a right angle to the horizontal aerosol flow. For the Burkard portable air sampler, an even wider range of deviation may occur. The bioaerosol samplers used for large particles such as pollen are even less accurate: e.g. 10 times the ambient concentration of Lycopodium spores has been calculated to be aspirated by the Lanzoni sampler when operated at 0.5 1 min−1 facing the wind at wind velocity of about 500 cm s−1.

The actual bioaerosol concentration can be calculated from the measured data by use of the indicated procedures. The sampling efficiency graphs presented can be used to bracket the sampling conditions that enable the investigator to avoid or minimize significant sampling biases for each sampler. The findings can also be used for the design of new samplers or for improving commercially available samplers.  相似文献   


17.
Here, we present a concept of a personal electrostatic bioaerosol sampler (PEBS), which is an open channel collector consisting of a novel wire-to-wire particle charger and a collection section housing a double-sided and removable metal collection plate and two quarter-cylinder ground electrodes. The charger consists of a tungsten wire (25.4 mm long and 0.076 mm in diameter) connected to high voltage and positioned in the center of the charging section (a cylinder 50.8 mm long and 25.4 mm in diameter); a ring of stainless steel wire 0.381 mm in diameter surrounds the hot electrode at its midpoint and is grounded. The newly designed wire-to-wire charger produces lower ozone concentrations compared to traditional wire-to-plate or wire-to-cylinder charger designs. The particles captured on the collection plate are easily eluted using water or other fluids. The sampler was iteratively optimized for optimum charging and collection voltages, and collection electrode geometry. When tested with polystyrene latex particles ranging from 0.026 µm to 3.1 µm in diameter and 10 L/min collection flow rate, the sampler's collection efficiency was approximately 70%–80% at charging and collection voltages of +5.5 kV and ?7 kV, respectively. The PEBS showed this collection efficiency at sampling times ranging from 10 min to 4 h. Preliminary tests with Bacillus atrophaeus bacterial cells and fungal spores of Penicillium chrysogenum showed similar collection efficiency. The use of a unique wire-to-wire charger resulted in ozone production below 10 ppb. Due to low ozone emissions, this sampler will allow maintaining desirable physiological characteristics of the collected bioaerosols, leading to a more accurate sample analysis.

© 2017 American Association for Aerosol Research  相似文献   

18.
The physical sampling efficiency of three commonly used samplers for bioaerosols has been determined under controlled conditions in a wind tunnel. Non-biological, monodisperse test aerosols of aerodynamic diameters up to 23 μm were used in a range of wind speeds up to 5 m s−1. The performance of each sampler type was different. For the Andersen Microbial Sampler and the Casella Slit Sampler, sampling efficiency dropped both with increasing wind speed and particle size, while for the Aerojet General Glass Cyclone, performance was generally independent of windspeed and particle size. This work is part of a larger study to determine both the physical and the biological sampling efficiencies of currently used samplers for bioaerosols. The results highlight the importance of understanding the performance of aerosol monitoring equipment, if results obtained in the field are to be interpreted correctly.  相似文献   

19.
Methods are presented for the use of liquid particles to measure sampling efficiencies and wall losses in size-selective samplers and for the use of solid particles to assess bounce and reentrainment. By testing a dichotomous sampler, it is demonstrated that the liquid particle methods are accurate; solid particle methods are less accurate and are still under development. Two methods are presented; in the first, particles are produced by spray-drying droplets from the vibrating orifice generator. Aerodynamic diameters are determined directly with a new Laser Settling Velocimeter or, indirectly, based on optical microscopy and the properties of the vibrating orifice generator. Alternatively, solid particles, such as pre-sized glass beads, are produced from bulk materials by a novel Sonic Fluidized Bed. The solid particle techniques are illustrated by testing the Size-Selective Inlet.  相似文献   

20.
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