Innovative nuclear technology based on modular multi-purpose lead–bismuth cooled fast reactors

Today's nuclear power is in the state of an intrinsic conflict between economic and safety requirements. This fact makes difficult its sustainable development.

One of the ways of finding the solution to the problem can be the use of modular fast reactors SVBR-75/100 cooled by lead–bismuth coolant that has been mastered in conditions of operating reactors of Russian nuclear submarines.

The inherent self-protection and passive safety properties are peculiar to that reactor due to physical features of small power fast reactors (100 MWe), chemical inertness and high boiling point of lead–bismuth coolant, integral design of the pool type primary circuit equipment.

Due to small power of the reactor, it is possible to fabricate the whole reactor at the factory and to deliver it to the NPP site in practical readiness by using any kind of transport including the railway.

Substantiation of the high level of reactor safety, adaptability of the SVBR-75/100 reactor relative to the fuel type and fuel cycle, issues of non-proliferation of nuclear fissile materials, opportunities of multi-purpose usage of the standard SVBR-75/100 reactors have been viewed in the paper.     

Study on lead–bismuth droplets' generation and their removal by an electrostatic precipitator

The applicability of the electrostatic precipitator for the removal of lead–bismuth droplets generated in the direct-contact boiling lead–bismuth cooled fast reactor is investigated. A small apparatus in which argon gas bubbles through the pool of lead–bismuth and an electrode mounted in the test section is used. The ESP operating voltage was 1000 V. It was found that the removal efficiency of the electrostatic precipitator increases with time up to 96.5%. It appears that the probability of droplet removal is almost independent of the droplet size. There is a small increase in this probability for larger droplets, which is caused likely by the fact that the larger droplets travel at lower velocities. Otherwise the effect of velocity on the removal efficiency is negligible. The electrostatic precipitator current was decreasing during the experiment, which is probably caused by the reduction of the number of droplets in the test section as the electrostatic precipitator was getting more efficient. The electrostatic precipitator current was on the order of 7 μA. The experiment demonstrated the applicability of the electrostatic precipitator for removal of lead–bismuth droplets.     

Modeling and optimization of steam dryer for removal of lead–bismuth droplets

Removal of lead–bismuth droplets from steam flow is a crucial issue in the direct contact boiling lead–bismuth cooled fast reactor. Droplets are generated due to the boiling of water directly in the reactor chimney, where steam for the turbine is generated. The droplets could severely damage the turbine and therefore a steam dryer is used for their removal. This paper presents an optimization of the main steam dryer geometrical parameters and steam inlet velocity. The Lagrangian method is used, in which first the steam flow field is developed using the CFD code FrontFlow/Red and then the particle motion is simulated. It was found that the reduction of the plate spacing can improve the steam dryer performance without a significant increase of pressure drop, the wane pitch has a value after which the steam dryer performance is not significantly improved, the number of wanes of 1.5 was selected at this point, however, a more detailed model is necessary to arrive at the final conclusion. The optimum steam inlet velocity should be found using a detailed economical assessment. Velocities between 2 and 4 m/s seem to be reasonable to achieve good removal efficiency and keep the pressure drop at reasonable values.     

Performance of oxygen sensor in lead–bismuth at high temperature

Performance of yttria-stabilized zirconia solid electrolyte oxygen sensor with a reference electrode of Bi/Bi₂O₃ was investigated. The oxygen sensor was tested in alumina vessel in order to prevent generating of impurities. The oxygen potential in the melt was controlled by injecting steam–hydrogen gas mixture (P_H2/P_H2O) into stagnant LBE. The electromotive force (EMF) of the sensor was compared with the theoretical EMF derived from the Nernst equation at various LBE temperatures (550–700 °C). The influences of various injection gas temperatures (200–500 °C) on the sensor output were also investigated. It was found that the sensor signals of the oxygen potential in LBE have not been affected by the injection gas temperature. The results also showed that the measured EMFs were in good agreement with the theoretical values of the EMF. The material aspects were investigated as well. The SEM (Scanning Electron Microscope) devices were used to analyze the cross-section of oxygen sensors after the exposition to LBE at 700 °C for 1000 h. The SEM micrograph showed that the yttria-stabilized zirconia solid electrolyte had an excellent corrosion resistance to the high temperature LBE as the working fluid and high temperature bismuth as the reference fluid.     

Compatibility of surface-coated steels, refractory metals and ceramics to high temperature lead–bismuth eutectic

Compatibility of cladding material with lead–bismuth eutectic at temperature higher than 650 °C is one of the most crucial issues for feasibility of lead–bismuth-cooled fast reactors with cycle efficiency as high as 40%. In order to search for corrosion-resistant materials with lead–bismuth eutectic at temperature higher than 650 °C, surface-coated steels, some refractory metals and various ceramics were tested by means of stirred-type corrosion test. Lead–bismuth was heated up to 700 °C electrically in an alumina crucible, and oxygen concentration in the lead–bismuth was adequately controlled by injection of argon, steam and hydrogen gas mixture into the lead–bismuth. Specimens of aluminum–iron-alloy-surface-coated steels, refractory metals and ceramics including SiC/SiC composites were immersed in the stirred lead–bismuth for 1000 h. It was found that the surface-coated steels showed good compatibility with the lead–bismuth due to formation of a thin and stable protection layer on the surfaces. Tungsten and molybdenum exhibited high corrosion resistance. On the other hand, niobium is not a reliable material for the high temperature LBE. SiC and Ti₃SiC₂ also exhibited high corrosion resistance. On the other hand, the physical performance of the SiC/SiC composite must be improved especially by minimizing the porosity.     

Design study on reactor structure of Pb–Bi-cooled direct contact boiling water fast reactor (PBWFR)

Pb–Bi-cooled direct contact boiling water small fast reactor (PBWFR) can produce steam by direct contact of feedwater with primary Pb–Bi coolant above the core, and circulate Pb–Bi coolant by means of buoyancy of steam bubbles. The PBWFR is capable of eliminating components of the cooling system such as primary pumps and steam generators, and thereby making the reactor system simple and compact. The specifications of the PBWFR are as follows: the fuel is Pu–U nitride; the core height is 75 cm; the core diameter is 278 cm; the average burnup is 80 GWd/t; the refueling interval is 10 years; the rated electric power is 150 MWe; the rated thermal power is 450 MWt; the core outlet/inlet temperatures are 460 °C/310 °C, respectively; and the operating steam pressure is 7 MPa. The reactor structure design has been formulated, where reactor vessel sizes are 4200 mm (ID) × 19,750 mm (H), the guard vessel is a closed type, the upper structure is made of chimneys, and the core support structure is hung up. An ultrasonic flow meter is installed inside the vessel. The seismic evaluation, design of refueling procedure and cost evaluation have been performed.     

Polonium evaporation and adhesion experiments for the development of polonium filter in lead–bismuth cooled reactors

Fundamental experiments were performed to determine the adhesion characteristics of polonium to different metals and to develop a filter for polonium evaporated from neutron-irradiated LBE. The results of the first experiments suggested that adhesion characteristics are almost the same for stainless steel and nickel metal. The results of the preliminary experiments for a polonium filter suggested that stainless steel mesh with thin wires could effectively collect polonium evaporated from neutron-irradiated LBE. In the experiments, stainless steel wire mesh was used, but from the results of adhesion experiment, it is expected that the same effect can be obtained with wire mesh made of other kinds of metal.     

Safety design of Pb–Bi-cooled direct contact boiling water fast reactor (PBWFR)

In Pb–Bi-cooled direct contact boiling water small fast reactor (PBWFR), steam is generated by direct contact of feedwater with primary Pb–Bi coolant above the core, and Pb–Bi coolant is circulated by steam lift pump in chimneys. Safety design has been developed to show safety features of PBWFR. Negative void reactivity is inserted even if whole of the core and upper plenum are voided hypothetically by steam intrusion from above. The control rod ejection due to coolant pressure is prevented using in-vessel type control rod driving mechanism. At coolant leak from reactor vessel and feedwater pipes, Pb–Bi coolant level in the reactor vessel required for decay heat removal is kept using closed guard vessel. Dual pipes for feedwater are employed to avoid leak of water. Although there is no concern of loss of flow accident due to primary pump trip, feedwater pump trip initiates loss of coolant flow (LOF). Injection of high pressure water slows down the flow coast down of feedwater at the LOF event. The unprotected loss of flow and heat sink (ATWS) has been evaluated, which shows that the fuel temperatures are kept lower than the safety limits.     

Simulation study of steels corrosion phenomenon in liquid lead–bismuth cooled reactors using molecular dynamics methods

Corrosion phenomena of stainless steel in liquid lead–bismuth as a coolant in nuclear fast breeder reactor are a field which is intensively investigated by the researchers in the recent year. We try to study this corrosion phenomena by computer simulation using molecular dynamics methods. The initial positions of the system were taken from the crystal structure data including the cell parameters and the types of the crystal. In this simulation, interatomic potential between Fe–Fe, Pb–Pb, Bi–Bi, Ni–Ni and Cr–Cr was assumed to follow Lennard–Jones potential. The Lennard–Jones potential parameters have been derived by fitting the data available in the literature. Nickel and chromium atoms were substituted into Fe crystal with the percentage of 10% and 16% to construct systems like SS 316. Molecular dynamics simulation has been done by interfacing iron and steel with liquid lead and liquid lead–bismuth in several temperatures. The result of this simulation showed that lead atoms can diffuse into Fe–10%Ni–16%Cr about 1.18 Å at 773 K while in Fe–10%Ni and Fe–16%Cr about 7.25 Å and 11.08 Å, respectively.     

Study on small long-life LBE cooled fast reactor with CANDLE burn-up – Part I: Steady state research

Small long-life reactor is required for some local areas. CANDLE small long-life fast reactor which does not require control rods, mining, enrichment and reprocessing plants can satisfy this demand. In a CANDLE reactor, the shapes of neutron flux, nuclide number densities and power density distributions remain constant and only shift in axial direction.

The core with 1.0 m radius, 2.0 m length can realize CANDLE burn-up with nitride (enriched N-15) natural uranium as fresh fuel. Lead–Bismuth is used as coolant.

From steady state analysis, we obtained the burn-up velocity, output power distribution, core temperature distribution, etc. The burn-up velocity is less than 1.0 cm/year that enables a long-life design easily. The core averaged discharged fuel burn-up is about 40%.     

Thermal-hydraulic analyses of transients in an actinide-burner reactor cooled by forced convection of lead–bismuth

The Idaho National Engineering and Environmental Laboratory (INEEL) and the Massachusetts Institute of Technology (MIT) are investigating the suitability of lead or lead–bismuth cooled fast reactors for producing low-cost electricity as well as for actinide burning. The current analysis evaluated a pool type design that relies on forced circulation of the primary coolant, a conventional steam power conversion system, and a passive decay heat removal system. The ATHENA computer code was used to simulate various transients without reactor scram, including a primary coolant pump trip, a station blackout, and a step reactivity insertion. The reactor design successfully met identified temperature limits for each of the transients analyzed.     

Feasibility neutronic design for the reactor core configurations of a 5 MWth transportable block-type HTR

Small long-life transportable high temperature gas-cooled reactors(HTRs) are interesting because they can safely provide electricity or heat in remote areas or to industrial users in developed or developing countries.This paper presents the neutronic design of the U-Battery,which is a 5 MWth block-type HTR with a fuel lifetime of 5–10 years.Assuming a reactor pressure vessel diameter of less than 3.7 m,some possible reactor core configurations of the 5 MWth U-Battery have been investigated using the TRITON module in SCALE 6.The neutronic analysis shows that Layout 12×2B,a scattering core containing 2 layers of 12 fuel blocks each with 20% enriched235U,reaches a fuel lifetime of 10 effective full power years(EFPYs).When the diameter of the reactor pressure vessel is reduced to 1.8 m,a fuel lifetime of 4 EFPYs will be achieved for the 5 MWth U-Battery with a 25-cm thick graphite side reflector.Layouts 6×3 and 6×4 with a 25-cm thick BeO side reflector achieve a fuel lifetime of 7 and 10 EFPYs,respectively.The comparison of the different core configurations shows that,keeping the number of fuel blocks in the reactor core constant,the annular and scattering core configurations have longer fuel lifetimes and lower fuel cost than the cylindrical ones.Moreover,for the 5 MWth U-Battery,reducing the fuel inventory in the reactor core by decreasing the diameter of fuel kernels and packing fraction of TRISO particles is more effective to lower the fuel cost than decreasing the 235U enrichment.     

Sodium cooled small fast long-life reactor “4S”

CRIEPI and Toshiba Corp. have been exploring to realize a small-sized nuclear reactor for the needs of dispersed energy source and multi-purpose reactor. A conceptual design of 4S (Super-Safe, Small and Simple) reactor is proposed to meet the following design requirements: (1) All temperature feedback reactivity coefficients including whole core sodium void reactivity are negative; (2) The core integrity is secured against all anticipated transient without reactor scram; (3) No emergency power nor active mitigating system is required; (4) The reactivity core lifetime is more than 10 years. The 4S reactor is a metallic fueled sodium cooled fast reactor. A target of an electrical output is 10–50 MW. A remarkable feature of 4S is that its reactivity is not controlled by neutron absorber rods but by neutron reflectors to cope with a long core lifetime and a negative coolant void reactivity.

This study includes a design consideration of 4S. Design discussions are mainly focused on various core designs to meet above requirements. A tall core active height is adopted to gain long core lifetime. An averaged fuel burn-up is tried to be increased up to 100 GWd/ton from a point of economic view. The reference 4S designs are 10 MWe (30 years core lifetime) and 50 MWe (10 years core lifetime).     

Design and safety optimization of ship-based small nuclear power reactors

Design and safety optimization of ship-based nuclear power reactors have been performed. The neutronic and thermo-hydraulic programs of the three-dimensional X–Y–Z geometry have been developed for the analysis of ship-based nuclear power plant. Quasi-static approach is adopted to treat seawater effect and quasi-static approach is also employed to treat neutronic aspect during safety analysis.

The reactors are loop type lead–bismuth-cooled fast reactors with nitride fuel and with relatively large coolant pipe above reactor core, the heat from primary coolant system is directly transferred to water–steam loop through steam generators. The power level is 100–200 MW th and excess reactivity is about 1$. Three types of core were investigated in the optimization process: balance, tall, and pancake with five values of Z–Y size ratio.

As the optimization results, the core outlet temperature distribution is changing with the elevation angle of the reactor system. The pancake core type has larger temperature distribution change as the elevation angle changes due to the sea wave. The natural circulation capability is good for safety. However, large driving head of natural circulation may cause large temperature fluctuation as the elevation angle changes.     

Accident analysis of lead or lead—bismuth cooled small safe long-life fast reactor using metallic or nitride fuel

Safety analysis of a lead or lead—bismuth cooled small safe long-life fast reactor was performed. It is proposed that the reactor be used in relatively isolated areas, and operated to the end of its life without refueling or fuel shuffling. In the present paper the reactor power and lifetime are set at 150 MWt and 12 years respectively. In order to assume its safety performance, the following accidents without scram were simulated with neutronic-thermal-hydraulic analysis: unprotected loss of flow (ULOF), unprotected rod run-out transient over power (UTOP), simultaneous ULOF and UTOP accidents, and simultaneous ULOF, UTOP and unprotected loss of heat sink (ULOHS) accidents. For each type of accident, four types of long-life small reactor (lead cooled metallic fueled, lead cooled nitride fueled, lead-bismuth cooled metallic fueled, and lead—bismuth cooled nitride fueled) were analyzed. It is shown that all the proposed designs can survive these accidents without requiring help from the operator or active devices.     

Natural circulation studies in a lead bismuth eutectic loop

Lead Bismuth Eutectic (LBE) is increasingly getting more attraction as the coolant for advanced reactor systems. It is also the primary coolant of the Compact High Temperature Reactor (CHTR), being designed at BARC. A loop has been set up for thermal hydraulics, instrument development and material related studies relevant to CHTR. Steady state natural circulation experimental studies were carried out for different power levels. Transient studies for start-up of natural circulation in the loop, loss of heat sink and step power change have also been carried out. An 1D code named LeBENC has been developed at BARC to simulate the natural circulation characteristics in closed loops. The salient features of the code include ability to handle non-uniform diameter components, axial thermal conduction in fluid and heat losses from the piping to the environment. This paper deals with the experimental studies carried out in the loop. Detailed validation of the LeBENC code with the experimental data is also discussed in the paper.     

A design study on Pb-208 cooled compact CANDLE burning reactor for future nuclear energy supply

A compact pool-type Pb-208 cooled CANDLE (Constant Axial shape of Neutron flux, nuclide densities and power shape During Life of Energy producing reactor) with a thermal power rating of 125 MWth is considered for the future nuclear energy supply. Natural Pb consists of Pb-204, Pb-206, Pb-207 and Pb-208. Pb-208 has a small capture and inelastic-scattering cross-section, which makes it possible to reduce neutron capture by coolant and to make neutron spectrum harder. In case of Pb-208 coolant instead of natural Pb, the core height and radius are reduced to 1.5 m and 1 m, respectively. The effective multiplication factor of the core, k_eff, could be increased from k_eff = 0.984 of natural Pb up to k_eff = 1.006. For increasing natural circulation head, coolant velocities in each core zone are adjusted by orifice at the core inlet position. The reactor vessel height is equal to that of a typical loop-type demonstration FBR vessel to obtain natural circulation head.     

Natural circulation experiments in a non-uniform diameter lead bismuth loop and validation of LeBENC code

Experimental studies are carried out on natural circulation in a Lead Bismuth Eutectic (LBE) loop. The loop mainly consists of a heated section, air heat exchanger, valves, various tanks and argon gas control system. All the components and piping are made of SS316L. The dissolved oxygen in the LBE is monitored online by an Yttria Stabilised Zirconia (YSZ) oxygen sensor and controlled during the operation of the loop. In this paper the details of the loop and experimental studies carried out with heater power levels varying from 900 W to 5000 W are described. The temperature range of LBE during the experiments was 200 °C–500 °C. The maximum heat loss in the piping is kept less than 20% of the main heater power. Steady state experimental studies are carried out at different power levels and the LBE flow rate was found to be varying from 0.095 kg/s to 0.135 kg/s. The analysis and results of the performance of the heat exchanger with air and water as the secondary coolants are also discussed in the paper. Transient studies were carried out to simulate various events like heat sink loss, step power change and secondary side coolant flow rate change and reported in the paper. In the start up experiments, where the flow is started from stagnant condition of LBE, the time required for starting of natural circulation is found to be 600 s, 400 s and 240 s with power level of 1200 W, 2400 W and 3000 W respectively. The results are compared with available correlation and prediction of computer code LeBENC.     

A numerical investigation of SBLOCA scenario in nuclear heating reactor

Small break loss of coolant accident (SBLOCA) is one of the most important severe accidents in nuclear heating reactor. Nuclear heating reactor designed by Tsinghua University, whose primary loop is integrated layout and designed without main pump. The initial water volume in the reactor vessel is important to determine whether the reactor will be cooled or not as no safety injection system is designed for coolant makeup during the whole scenario. This paper simulates SBLOCA in nuclear heating reactor based on RELAP5. Transient behavior of relevant thermal parameters is specifically analyzed. Moreover, investigation also has been made on SBLOCA scenario based on different residual heat removal correlations and found the long-term residual heat removal capacity is decisive in determining the loss of coolant. The mathematical form of residual heat removal correlation is specifically deducted and can be widely applied to different situations. The envelope line that differentiates the region whether the core is safe or not under different maximum PRHRS capacity is also given.