Study of a Greek area with enhanced indoor radon concentrations

In this paper the focus is on Arnea Chalkidikis, an area in Greece with granitic geological background and indications of possible elevated radon concentration indoors. Data are reported of indoor radon measurements with etched track detectors and those are used for dosimetric estimations. Moreover, data are reported on soil gas and soil radon concentrations in Arnea, as well as radon and uranium concentrations in water samples. From the measured radon concentrations in water samples the contribution to the overall dose has been calculated. For a period of 1 month, indoor radon and progeny activity has also been monitored in the dwelling that has the maximum indoor radon concentration in Greece. This dwelling is in Arnea and the dose delivered to the inhabitants has been calculated. The mean annual effective dose due to indoor radon was 4.5 mSv and about 11% of this was due to the use of water. Mean soil gas concentration and soil radon concentration were (90 +/- 30) kBq m(-3) (p<0.05) and (30 +/- 5) kBq m(-3) (p<0.05) respectively. Mean uranium concentration of the water samples was (98 +/- 13) mBq l(-1) (p<0.05).     

Indoor exposure of population to radon in the FYR of Macedonia

The authors present the results of a year-long survey of the indoor radon concentration levels in the FYR of Macedonia. A total number of 437 dwellings in eight statistical regions were subject to radon concentration measurements by using CR-39 track detectors. The annual mean indoor radon concentration in each measuring site was estimated from the four individual measurements with 3 months duration. The measuring period was from December 2008 to December 2009. The distribution of the results was nearly log-normal. The arithmetic and geometric mean values of the annual mean value of radon concentration were estimated to be 105 ± 84 and 84*/1.9 Bq m(-3), respectively. The annual effective dose due to indoor exposure to radon in the dwellings was estimated to be 2.1*/1.9 mSv y(-1).     

Simultaneous measurements of indoor radon, radon-thoron progeny and high-resolution gamma spectrometry in Greek dwellings

Simultaneous indoor radon, radon-thoron progeny and high-resolution in situ gamma spectrometry measurements, with portable high-purity Ge detector were performed in 26 dwellings of Thessaloniki, the second largest town of Greece, during March 2003-January 2005. The radon gas was measured with an AlphaGUARD ionisation chamber (in each of the 26 dwellings) every 10 min, for a time period between 7 and 10 d. Most of the values of radon gas concentration are between 20 and 30 Bq m(-3), with an arithmetic mean of 34 Bq m(-3). The maximum measured value of radon gas concentration is 516 Bq m(-3). The comparison between the radon gas measurements, performed with AlphaGUARD and short-term electret ionisation chamber, shows very good agreement, taking into account the relative short time period of the measurement and the relative low radon gas concentration. Radon and thoron progeny were measured with a SILENA (model 4s) instrument. From the radon and radon progeny measurements, the equilibrium factor F could be deduced. Most of the measurements of the equilibrium factor are within the range 0.4-0.5. The mean value of the equilibrium factor F is 0.49 +/- 0.10, i.e. close to the typical value of 0.4 adopted by UNSCEAR. The mean equilibrium equivalent thoron concentration measured in the 26 dwellings is EEC(thoron) = 1.38 +/- 0.79 Bq m(-3). The mean equilibrium equivalent thoron to radon ratio concentration, measured in the 26 dwellings, is 0.1 +/- 0.06. The mean total absorbed dose rate in air, owing to gamma radiation, is 58 +/- 12 nGy h(-1). The contribution of the different radionuclides to the total indoor gamma dose rate in air is 38% due to 40K, 36% due to thorium series and 26% due to uranium series. The annual effective dose, due to the different source terms (radon, thoron and external gamma radiation), is 1.05, 0.39 and 0.28 mSv, respectively.     

Radiological characterisation of Artvin and Ardahan provinces of Turkey

Indoor radon concentration measurements were carried out and corresponding annual effective doses due to exposure to indoor radon were determined in Artvin and Ardahan provinces located in the eastern part of Turkey. The measurements were performed for four seasons in order to determine the seasonal fluctuations mostly observed in indoor environments. Indoor radon concentration values were observed to range from 21 to 321 Bq m?3 for the Artvin province and from 53 to 736 Bq m?3 for the Ardahan province. It was observed that minimum indoor radon concentration values were obtained in summer, while the highest ones were observed in winter. Indoor radon concentration values of the current study were compared with those of other provinces in Turkey. As elevated indoor radon concentrations are mostly correlated with high 23?U activity concentrations in soil, a total of 57 and 33 soil samples were collected from the Artvin and Ardahan provinces, respectively, to determine 23?U activity concentration as well as the concentration of 232Th and ??K--naturally occurring radionuclides. It was also observed that soil samples collected from the study areas contained 13?Cs as an artificial radionuclide.     

MCP-N (LiF:Mg,Cu,P) TLDs for radon measurements with charcoal canisters

A method of measurement of radon concentration in air was developed, based on high-sensitivity LiF:Mg,Cu,P (MCP-N, TLD Poland) thermoluminescent detectors installed in charcoal canisters. The canisters were exposed typically for 72 h in a calibration chamber with a radon concentration ranging from 100 Bq x m(-3) to 87 kBq x m(-3). It was found that in these conditions the signal registered by the TL detectors was proportional to the 222Rn concentration and the lowest limit of detection (LLD) was at a level of 100 Bq x m(-3). The proposed method can be used in large-scale, multi-site surveys aimed at screening for high levels of indoor radon concentration or for measuring ground radon exhalation rates.     

Seasonal variation of indoor radon concentration in dwellings of Alexandria city, Egypt

Inhalation of radon ((222)Rn) and daughter products are a major source of natural radiation exposure. Keeping this in view, seasonal indoor radon measurement studies have been carried out in 68 dwellings belonging to 17 residential areas in Alexandria city, Egypt. LR-115 Type 2 films were exposed for four seasons of 3 months each covering a period of 1 y for the measurement of indoor radon levels. Assuming an indoor occupancy factor of 0.8 and a factor of 0.4 for the equilibrium factor of radon indoors, it was found that the estimated annual average indoor radon concentration in the houses surveyed ranged from 45 ± 8 to 90 ± 13 Bq m(-3) with an overall average value of 65 ± 10 Bq m(-3). The observed annual average values are greater than the world average of 40 Bq m(-3). Seasonal variation of indoor radon shows that maximum radon concentrations were observed in the winter season, whereas minimum levels were observed in the summer season. The season/annual ratios for different type of dwellings varied from 1.54 to 2.50. The mean annual estimated effective dose received by the residents of the studied area was estimated to be 1.10 mSv. The annual estimated effective dose is less than the recommended action level (3-10 mSv y(-1)).     

Soil radon measurements in the Canadian cities

Radon has been identified as the second leading cause of lung cancer after tobacco smoking. Information on indoor radon concentrations is required to assess the lung cancer burden due to radon exposure. Since radon in soil is believed to be the main source of radon in homes, measurements of soil gas radon concentrations can be used to estimate variations in radon potential of indoor environments. This study reports surveys of natural background variation in soil radon levels in four cities, Montreal, Gatineau, Kingston and the largest Canadian city of Toronto. A total of 212 sites were surveyed. The average soil gas radon concentrations varied significantly from site to site, and ranged from below detection limit to 157 kBq m(-3). For each site, the soil radon potential (SRP) index was determined with the average soil radon concentration and average soil permeability measured. The average SRP indexes are 20±16, 12±11, 8±9 and 12±10 for Montreal, Gatineau, Kingston and Toronto, respectively. The results provide additional data for the validation of an association between indoor and soil radon potentials and for the development of radon potential map of Canada.     

Exposures to 222Rn from consumption of underground municipal water supplies in Pakistan

This paper presents the results of radon ((222)Rn) concentration measurements in municipal supply drinking water in metropolitan Lahore city of Pakistan and evaluation of consequent radiological effects. In this respect, water samples were collected in all nine municipal towns of Lahore city and analysed employing a high-resolution gamma spectrometric system. Radon concentration varied from 2.0 +/- 0.3 to 7.9 +/- 2.1 Bq l(-1). Mean value of annual effective dose for an individual consumer was assessed to be 16.5 +/- 12.8 microSv y(-1). (222)Rn mean concentration measured in this study is comparable with the reported values for drinking water determined worldwide and found to be less than the limit of 100 Bq l(-1) recommended by the World Health Organisation for public water supplies. The results of this study may be helpful in establishing background levels of radon in drinking water that could be used not only to distinguish additional contributions when a contamination event occurs but also to implement water quality standards by the concerned authorities to maintain radioactive contamination free drinking water supplies for the population.     

An update on thoron exposure in Canada with simultaneous ²²²Rn and ²²⁰Rn measurements in Fredericton and Halifax

Naturally occurring isotopes of radon in indoor air are identified as the second leading cause of lung cancer after tobacco smoking. Radon-222 (radon gas) and radon-220 (thoron gas) are the most common isotopes of radon. While extensive radon surveys have been conducted, indoor thoron data are very limited. To better assess thoron exposure in Canada, radon/thoron discriminating detectors were deployed in 45 homes in Fredericton and 65 homes in Halifax for a period of 3 months. In this study, radon concentrations ranged from 16 to 1374 Bq m(-3) with a geometric mean (GM) of 82 Bq m(-3) and a geometric standard deviation (GSD) of 2.56 in Fredericton, and from 4 to 2341 Bq m(-3) with a GM of 107 Bq m(-3) and a GSD of 3.67 in Halifax. It is estimated that 18 % of Fredericton homes and 32 % of Halifax homes could have radon concentrations above the Canadian indoor radon guideline of 200 Bq m(-3). This conclusion is significantly higher than the previous estimates made 30 y ago with short-term radon measurements. Thoron concentrations were below the detection limit in 62 % of homes in both cities. Among the homes with detectable thoron concentrations, the values varied from 12 to 1977 Bq m(-3) in Fredericton and from 6 to 206 Bq m(-3) in Halifax. The GM and GSD were 86 Bq m(-3) and 3.19 for Fredericton, and 35 Bq m(-3) and 2.35 for Halifax, respectively. On the basis of these results, together with previous measurements in Ottawa, Winnipeg and the Mont-Laurier region of Quebec, it is estimated that thoron contributes ～8 % of the radiation dose due to indoor radon exposure in Canada.     

A combination study of indoor radon and in situ gamma spectrometry measurements in Greek dwellings

The aim of the present study was to investigate of a possible correlation between indoor radon and indoor gamma dose rates deduced by in situ gamma spectrometry measurements by using a portable HPGe detector. Indoor radon and high resolution in situ gamma spectrometry measurements were performed in 60 apartments in Thessaloniki, the second largest city of Greece. Geometric mean radon concentration is 52 Bq m(-3). The mean total absorbed dose rate in air due to gamma radiation is 56 +/- 9 nGy h(-1). The contribution of the different radionuclides to the total indoor gamma dose rate in air is 41% due to 40K, 36% due to the thorium series and 23% due to the uranium series. No correlation was found between indoor gamma dose rate due to the uranium series and indoor radon for ground and first floor apartments. For upper floor apartments (above the second floor) a weak correlation is observed. The mean annual effective dose due to radon is 1.15 mSv, i.e., more than four times higher compared to the effective dose due to gamma radiation (0.27 mSv).     

Indoor radon concentration in the rural dwellings of Chhattisgarh state (India)

Inhalation of radon and its daughter products is the major contributor to the total exposure of the population to natural radiation. An indoor radon survey has been carried out in the state of Chhattisgarh (80.26 degrees N to 84.41 degrees N and 17.8 degrees E to 24.1 degrees E), India under the national coordinated radon project of the Department of Atomic Energy. In the frame of this project indoor radon concentration has been measured in 105 dwellings situated in different villages of Chhattisgarh state. Houses were selected for measurements to cover the most common type of houses generally existing in the rural areas. Measurements have been done on quarterly integrating cycle for one full year in each dwelling using radon cup dosemeter employing LR-115, type-II (pelliculable), solid-state nuclear track detectors. The gamma radiation level was also checked in each dwelling using a gamma survey meter. It was found that the annual average indoor radon concentration in these dwellings varies from 9.91 to 87.84 Bq m(-3) with overall mean value of 26.48 Bq m(-3). Gamma level in these rural dwellings varies from 14.84 to 26.56 microR h(-1) with mean value of 18.68 microR h(-1). We observed that the radon concentration is relatively higher in the houses where the floor is bare but relatively lower in those houses where the floor is tiled or cemented.     

Indoor radon survey in dwellings of nine cities in the Eastern and the Western provinces of Saudi Arabia

The results of a first phase of an indoor radon survey in a total of 1610 dwellings distributed in nine cities of the Eastern and the Western provinces of Saudi Arabia are presented. The objective of this radon survey was to obtain representative indoor radon data for seven cities in the Eastern province. Khafji, Hafr Al-Batin, Abqaiq, Qatif, Al-Ahsa, Dammam and Khobar and to compare this with two cities in the Western province, Madina and Taif. So far, detailed radon data is not available for Saudi Arabia: therefore, this radon survey provides a base line for Saudi Arabia in the Radon World Atlas. On average, 200 indoor radon dosemeters were distributed in each city and placed for a period of one year starting from May 2001 to May 2002. The total number of collected dosemeters was 847. A total of 724 houses and 98 schools were covered in this survey. The results of the survey in the cities showed that the overall minimum, maximum and average radon concentrations were 1, 137 and 22 Bq m(-3), respectively. Geometric mean and geometric standard deviations of the radon distribution were found to be 18 and 1.92, respectively. In one of the dwellings in Qatif city, radon concentration, measured by a passive system and then confirmed by an active system, was found to be 535 +/- 23 and 523 +/- 22 Bq m(-3), respectively. The result of a radon survey in 98 schools showed that the minimum, maximum and average radon concentrations were 1, 70 and 19 Bq m(-3), respectively. The average radon concentration for each city was also determined. The lowest average radon concentration (8 Bq m(-3)) was found in Al-Ahsa while the highest average concentration (40 Bq m(-3)) was found in Khafji.     

Long-term measurements of thoron, its airborne progeny and radon in 205 dwellings in Ireland

Long-term (circa 3 months) simultaneous measurements of indoor concentrations of thoron gas, airborne thoron progeny and radon were made using passive alpha track detectors in 205 dwellings in Ireland during the period 2007-09. Thoron progeny concentrations were measured using passive deposition monitors designed at the National Institute of Radiological Sciences (NIRS), Japan, whereas thoron gas concentrations were measured using Raduet detectors (Radosys, Budapest). Radon concentrations were measured in these dwellings by means of NRPB/SSI type alpha track radon detectors as normally used by the Radiological Protection Institute of Ireland (RPII). The concentration of thoron gas ranged from <1 to 174 Bq m(-3) with an arithmetic mean (AM) of 22 Bq m(-3). The concentration of radon gas ranged from 4 to 767 Bq m(-3) with an AM of 75 Bq m(-3). For radon, the estimated annual doses were 0.1 (min), 19.2 (max) and 1.9 (AM) mSv y(-1). The concentration of thoron progeny ranged from <0.1 to 3.8 Bq m(-3) [equilibrium equivalent thoron concentration (EETC)] with an AM of 0.47 Bq m(-3) (EETC). The corresponding estimated annual doses were 2.9 (max) and 0.35 (mean) mSv y(-1). In 14 or 7% of the dwellings, the estimated doses from thoron progeny exceeded those from radon.     

Indoor radon in rural dwellings of the South-Pannonian region

The results of indoor radon survey in the South-Pannonian Province Vojvodina (Serbia and Montenegro) are presented. The sampling strategy was oriented towards suburban and urban regions in the Province. For the dwellings typical for such regions the geometric mean annual radon activity concentration of 76.1 Bq m(-3) is measured (1000 measurements). This result leads to the annual dose estimate of 4.3 mSv y(-1), which is above the recommended action limit of ICRP. For urban dwellings in Novi Sad (the Province capital), the annual mean value of 54 Bq m(-3) (220 measurements) is obtained. By comparison of these two results it is concluded that radon surveys based on measurements in urban environment may seriously underestimate the radon-related health risk. The elevated radon levels could not be explained by elevated uranium levels of surface soil.     

Evaluation of radon concentration in well and tap waters in Bursa, Turkey

(222)Rn measurements in water samples collected from 27 wells and 19 taps that were supplied from the investigated wells were conducted using the AlphaGUARD PQ 2000PRO radon gas analyser at sites across several geologic formations within the city of Bursa, Turkey. The measured radon concentrations ranged from 1.46 to 53.64 Bq l(-1) for well water and from 0.91 to 12.58 Bq l(-1) for tap water. Of the 27 sites sampled, only 7 had radon levels above the safe limit of 11.1 Bq l(-1) recommended by the USEPA. In general, all determined concentrations were well below the 100 Bq l(-1) revised reference level proposed by the European Union. These values of radon concentrations in water samples are compared with those reported from other countries. Doses resulting from the consumption of these waters were calculated. The minimum and the maximum annual mean effective doses due to (222)Rn intake through water consumption were 0.02 μSv a(-1) and 1.11 μSv a(-1), respectively.     

Pilot study of indoor radon in Greek workplaces

Radon and gamma dose rate measurements have been performed in 561 workplaces in 19 prefectures of Greece. The distribution of radon concentration can be well described by a log-normal distribution. Most of the radon concentrations are between 50 and 200 Bq m(-3) with an arithmetic mean of 123 Bq m(-3). The maximum measured value of radon gas concentration is 695 Bq m(-3). About 10% of the workplaces exceed 200 Bq m(-3). Only a small fraction ( approximately 1%) of workplaces exceed the European Commission action level (400 Bq m(-3)). Despite the relative small fraction of workplaces which exceed the value of 400 Bq m(-3), it is clear from the results of the present work that for certain prefectures, further and more extensive research is needed.     

Exposure to 222Rn in ten underground mines in Iran

Concentrations of 222Rn were measured in ten non-uranium underground mines in Iran, including three metal mines and seven coal mines. Two active techniques were applied for these measurements (1) activated charcoal and (2) scintillation cell. A maximum mean concentration of 1.33 kBq.m(-3) was found in the Robat-Karim manganese mine with a hot spot of 12 kBq.M(-3), while the concentration in the Venarge-Qom manganese mine was less than 10 Bq.m(-3), leading to annual effective dose equivalents of 8.3 mSv and (0.06 mSv respectively. The mean concentration levels of 222Rn in coal mines were found to be almost 500 Bq.m(-3), leading to annual effective dose equivalent of 3 mSv.     

Radon concentration measurements in the Amasra coal mine, Turkey

In this study, the results of atmospheric radon measurements that were performed for the Amasra underground coal mine in Zonguldak bituminous coal basin (Turkey) are presented. The radon measurements were performed for 40 days between November 2004 and December 2004 using passive nuclear etched track detectors. The radon concentrations vary from a minimum value 49 Bq m(-3) in a site located at +40 m to a maximum value 223 Bq m(-3) in a site located at -100 m. Mean concentration is 117 (Bq m(-3)). This value is well below the action level of 500-1,500 Bq m(-3) recommended by the International Commission on Radiological Protection (ICRP) (1993). The mean effective dose value for workers of this mine of 3.4 microSv per day was obtained. This result shows that protection against radiological hazards would not be necessary for workers of this mine((2)).     

Indoor radon concentration and its possible dependence on ventilation rate and flooring type

The results of radon concentration measurements carried out in dwellings with natural ventilation for 1 y in Bangalore are reported. Measurements, covering three sessions of the day (morning, afternoon, night) were performed two times in a month for 1 y at a fixed place of each dwelling at a height of 1 m above the ground surface in selected dwellings. The low-level radon detection system (LLRDS), an active method, was used for the estimation of radon concentration. The measurements were aimed to understand the diurnal variation and the effect of ventilation rate and flooring type on indoor radon concentration. The geometric mean (± geometric standard deviation) of indoor radon concentration from about 500 measurements carried out in 20 dwellings is found to be 25.4 ± 1.54 Bq m?3. The morning, afternoon and night averages were found to be 42.6 ± 2.05, 15.3 ± 2.18 and 28.5 ± 2.2 Bq m?3, respectively. The approximate natural ventilation rates of the dwellings were calculated using the PHPAIDA--the on-line natural ventilation, mixed mode and air infiltration rate calculation algorithm and their effects on indoor radon concentrations were studied. The inhalation dose and the lung cancer risk due to indoor radon exposure were found to be 0.66 mSv y?1 and 11.9 per 10? persons, respectively. The gamma exposure rate was also measured in all the dwellings and its correlation with the inhalation dose rate was studied.     

Background gamma terrestrial dose rate in Nigerian functional coal mines

Measurements of the background terrestrial gamma radiation dose rates at different indoor and outdoor locations on the surfaces of Okpara underground and Okaba open cast mines in Nigeria were made. Two duly calibrated low-level gamma survey metres were held 1 m above the ground surface for these measurements. Measurements were also made at various locations inside the mine tunnel at the Okpara mine. Results indicate that the indoor background gamma radiation is comparable for both mining environments. The mean outdoor gamma dose rate determined for the Okaba mining environment is 10.4 nGy h(-1) as against 11.7 nGy h(-1) for Okpara. The ranges are 8.5-16.5 nGy h(-1) for the Okpara measurements and 7.5-14.0 nGy h(-1) for Okaba. Thus, the outdoor gamma dose rates appear to be generally lower at the Okaba open cast mine than at Okpara. The indoor dose rate values range from 11.0 to 17.0 nGy h(-1) in both environments. These indoor measurements have nearly the same mean values 14.4 and 14.5 nGy h(-1) for Okpara and Okaba environments, respectively. The indoor to outdoor dose rate ratio is 1.2 for Okpara and 1.4 for Okaba. These values are in consonance with the corresponding ratio given in literature. Dose rate measurements inside the mine tunnel at the Okpara mine are higher than the surface indoor measurements ranging from 13.5 to 20.5 nGy h(-1) with a mean of 16.5 nGy h(-1). The higher dose rate values measured in the mine tunnel are attributable to the concentration of radon in the 'closed' environment of the mine tunnel.