RF-pumped infrared laser using transverse gas flow

A transverse gas flow configuration has been developed utilizing RF discharge waveguide technology for several infrared lasers. Two potential applications have been identified: pulsed chemical laser and CW CO2laser. In the 3.8 μm DF laser, the flowing gas device provides rapid gas replenishment to maintain high electrical efficiency at high repetition rates. An average power of 0.6 W was achieved at 1 kHz. An order of magnitude power improvement can potentially be developed in a closed cycle system. In the CW CO2laser, the flowing gas provides efficient cooling so that high output power per unit gain length can be achieved. A 16 W output in a 20 cm gain length device, corresponding to a record 0.8 W/cm output has been demonstrated. This system can be developed into a 20-60 W laser with a 20-50 cm gain length.     

Effects of gas flow on gain of 10.6 micron CO2laser amplifiers

Small-signal gain of flowing gas CO2laser amplifiers at 10.6 microns has been optimized for media including pure CO2CO2: N2, CO2: He, CO2: CO, CO2: O2, CO2: N2: He, CO2: CO : He, and CO2: CO : N2. Optimum gain of all flowing gas systems studied increases monotonically with increasing gas flow rate. In the low CO2flow rate region, 10 < RCO2: < 50 cm³/min, gas flow enhances the gain most for systems containing N2. Results provide strong evidence that the rapid increase in gain with flow rate in CO2: N2mixtures is due to removal by convection of the dissociated product CO. For 50 < RCO2< 200 cm³/min, a slow linear increase in gain of all gas mixtures with increasing flow rate occurs and is attributed to the cooling of gas temprature by convection. A stronger dependence of gainGon amplifier boreD, viz.,G propto I/D, was obtained for flowing gas media relative to that previously observed for nonflowing gas mixtures which is consistent with the proposed mechanism of gas cooling by convection. Highest gain values obtained were 7.8 and 6.2 dB/m with the flowing gas mixtures CO2: N2: He and CO2: CO : He, respectively, in a 12 mm bore water-cooled amplifier tube. Similarities between CO2: N2and CO2: CO systems suggest that pumping of the CO2laser by resonant transfer from CO* (upsilon = 1) can be significant.     

Gain measurement in the CO2laser discharge

In order to examine the CO2laser oscillation mechanism, a measurement was made of the unsaturated gain of CO2laser radiation in an active medium of gas discharge containing CO2, N2, and He. A two-beam optical balance method was used to measure the gain in an amplifier; the accuracy of the measurement was approximately 10 percent. The output of a CO2-N2-He laser was used as the radiation source. The absolute power of the probing beam, which has a diameter of approximately 5 mm, was maintained at approximately 15 mW. Saturation was not observed at probing signal levels up to 80 mW. Amplifier tubes with diameters of 55, 34, 12, and 5 mm were used. The dependence of the amplifier gain on the current density, pressure, composition of the gas mixture, and tube diameter was measured. Comparison was also made of the calculated and measured values for the laser population inversion.     

Gain characteristics of CO2laser amplifiers at 10.6 microns

Single-pass gain at 10.6 microns has been studied parametrically in nonflowing CO2or buffered CO2amplifying media. The gain profile across the amplifier diameter and integrated gain both were determined. Parameters varied included buffer gas type, mixture ratio, gas pressure, amplifier bore, discharge current, and wall temperature. Tube bores of 12, 22, and 34 mm and buffer gases of H2, He, Ne, A, and N2were studied. Optimum gain is relatively independent of current density, but decreases with increasing wall temperature. The pressure-diameter relationshipP_{CO_{2}} cdot D sim 4torr-cm was found to hold for CO2, CO2:He, and CO2:N2amplifying media at optimum gain. The gain depends strongly on the CO2partial pressure and is relatively insensitive to the buffer gas pressure except for the case of H2. The maximum gain decreased slowly with increasing amplifier diameter. The highest gain, 1.7 dB/meter, was achieved with a helium buffer gas in amplifiers with a diameter of 22 mm or less. No gain saturation was detected for a 30-dB range of input signal power, from a milliwatt to a few watts. Spectrograms showed that the principal spontaneous emission from CO2:He amplifiers in the 2000-7000-Å range consisted of CO bands; no CO2bands or He line spectra were observed.     

Large aperture CO2laser discharges

Large aperture high-pressure gas laser discharges are a prerequisite for the development of high-energy gas lasers of sufficient power for the production of plasmas of thermonuclear interest. Of the several approaches being followed toward the attainment of such discharges, one utilizing weak volumetric preionization of the active gas region produced by UV radiation is described. The use of this technique has resulted in the successful generation of atmospheric-pressure CO2laser discharges between electrodes separated by 30 cm, having total cross sections of ∼600 cm². With input energies of ∼200 J/1 small signal gain values of 4-5 percent cm^-1were measured in 1 : 1 : 3 gas mixtures of CO2, N2, and He, respectively. It is thus concluded that this excitation technique could be incorporated into the fabrication of large volume gas laser amplifiers having beam cross sections in excess of 10³cm²and total output-energy capabilities ofsim 10^{4}J.     

Long-term operation of a sealed CO2laser

The life expectancy of a sealed CO2laser tube depends, to a great extent, on the interaction of the molecules existing in the discharge at the cathode. The data reported here indicates that after operation of a sealed laser, only CO and O2are formed in concentrations comparable to the initial fill gases of CO2, N2, and He. The CO, CO2, and O2, in particular, were found to be completely adsorbed at the Ni cathode within several hundred hours of tube operation. A loss of 10.6 μm power output accompanied this adsorption. As expected, the process was reversible to a degree since the laser resumed operation at the initial power level after the cathode region had been heated to 300°C. This process of adsorption-desorption was repeated several times up to an accumulated operating time of 705 hours. During this time, the power output remained at a substantially constant value. However, the loss of CO2by carbon deposits ultimately means an end to tube life.     

New techniques for determining vibrational temperatures, dissociation, and gain limitations in CW CO2lasers

We have developed an accurate method of determining vibrational temperatures and populations in CO2laser discharges. Our technique involves the use of both the regular 00 ° 1 and sequence 00 ° 2 laser transitions as probes of a CO2laser amplifier. We have been able to separately investigate the quantitative effects of gas heating, dissociation, and ν3mode excitation efficiency on the small-signal gain in typical CW CO2lasers. In general we find that the maximum gain attained in a typical flowing gas CW CO2laser is limited by dissociation of CO2at high discharge currents. To investigate the more fundamental limitations on the gain, we used a short discharge tube with fast flow rates. Contrary to many previous results, we find that thermal effects play a somewhat secondary role in the discharge dynamics, and that the lower laser level populations are small under all discharge conditions. Our results show that the chief limitation on gain in CW CO2lasers is the "saturation" of the ν3mode vibrational temperature T3at high discharge currents. This saturation effect is observed for a wide range of gas mixtures and pressures, and has been studied in detail. Gain coefficients as high as 3.3 percent/cm have been obtained in a conventional 1-cm bore CW discharge tube. We also report preliminary results of an experiment which uses a tunable diode laser to measure gain on a large variety of transitions in a CO2discharge. The diode laser measurements give a striking confirmation of the results described above, and provide the first direct experimental evidence that a Boltzmann distribution exists in the vibrational modes of discharge excited CO2.     

Gain characteristics of an atmospheric sealed CW CO2laser

Experimental and analytical investigations have been made on unsaturated gain g0of a CO2electric-discharge convection laser, in which discharge current flow, gas flow, and the optical axis are mutually perpendicular. Stable glow discharges in sealed gas mixtures of CO2, CO, N2, and He were maintained at pressures up to 780 torr with an input power density of about 90 W/cm³. The ratio of electric field to neutral particle densityE/Nwas1.7 times 10^{-16}V . cm²and was independent of the total gas pressureP. The electron density in a positive column of the glow discharge was about4 times 10^{10}cm^-3. Detailed spatial distributions of g0at a wavelength near 10.6 μm were measured in the pressure range from 100 to 780 torr. Measurements were also made on the current dependence of g0and on the change in gowith discharge time. The g0distributions along the gas flow direction were found to agree with those calculated from the electron density distribution and the relaxation rate constant of the upper laser level on the basis of continuity equations for a two-level model. The integrated value of g0along the flow direction was proportional to P^-0.8whenE/N, electron density, and gas temperature were held constant. A maximum value of the g0distribution, which was proportional to P^-0.3, was 0.14 percent/cm at 780 torr.     

A radiatively pumped CW CO2laser

A proof of principle experiment to demonstrate the physics of a radiatively pumped laser has been carried out. For the first time, a blackbody cavity has optically pumped a CW CO2laser. Results are presented from a series of experiments using mixtures of CO2, He, and Ar in which maximum output power was obtained with a 20 percent CO2- 15 percent He-65 percent AR mixture. The dependence of the output power on the blackbody temperature and the cooling gas flow rate is also discussed. By appropriately varying these parameters, continuous output powers of 8-10 mW have been achieved.     

Waveguide CO2laser gain: Dependence on gas kinetic and discharge properties

Using a simple rate equation approach we examine the gas kinetic and discharge properties of waveguide CO2lasers. We calculate the dependence of the population inversion and laser small-signal gain on gas pressure, gas mixture, pumping rate (discharge current), tube bore diameter, and wall temperature. The results indicate, for example, that at a pressure of 50 torr and a tube-bore diameter of 0.125 cm, the gain is optimized with a gas mixture in the ratio CO2:N2:He of 1:0.75: 1.5. At higher pressures the gain is optimized by using more helium-rich mixtures. We also calculate the dependence of laser tunability on the gas kinetic properties and cavity losses. We find that for low-loss cavities the laser tunability may substantially exceed the molecular full width at half-maximum. Furthermore, the more helium-rich gas mixtures give greater tunability when cavity losses are small, and less tunability when cavity losses are large. The roles of the various gases in the waveguide CO2laser are the same as those in conventional devices. By contrast with conventional lasers, however, the waveguide laser transition is homogeneously broadened. Thus the dependence of gain on gas pressure and other kinetic properties differs substantially from that predicted by scaling results from conventional low-pressure lasers.     

An electro-aerodynamic CO2scan laser

An electro-aerodynamic CO2scan laser with a vanadium dioxide control reflector has been demonstrated. Gas flow, electrical discharge, and optical path are coaxial. A gain coefficient of 0.015 cm^-1has been achieved in a tapered discharge tube with 3.175 cm limiting aperture. Scanning speed near 10⁵directions per second can be utilized over3.7 times 10_{4}resolvable directions in space. Scanning output power up to 9 W was shown.     

Comparison of computer simulation and experimental results for a 16 µm HBr/CO2laser

An improved version of a computer model simulates 16μm laser output from an optically pumped HBr/CO2/Ar laser cavity. A rate equation approach is used to examine the time history of vibrational and rotational excitation and subsequent lasing from the HBr/ CO2gas mixture. Rotational nonequilibdum phenomena in HBr and CO2are included. The effect of bleaching a particular vibrational-rotational transition with optical saturation is modeled in detail. The results of the computer simulation are compared to the laboratory observations from two separate experiments. The model predicts accurately the effect of changing partial pressures of the constituent gases on 16μm power and energy. The model reveals the important kinetic mechanisms yielding these trends. Finally, the model is modified to simulate optical pumping by an HF laser of an HF/CO2/Ar gas mixture. A case by case comparison with the results of the HBr model prediction show significantly lower 9.4 μm powers and energies for any given HF pressure and no evidence of 16μm laser output from the HF/CO2gas mixture.     

Small-signal gain and time-resolved spectroscopy of the D2-F2/CO2pulsed chemical transfer laser system

Measurements made of the small-signal gain and time-resolved spectral output of a flash-initiated D2-F2/CO2chemical transfer laser system are reported. Small-signal gain measurements indicate a possible lack of rotational equilibration among the rotational levels of the CO2during the DF-CO2V-V energy transfer process. Time-resolved spectral output of this system, operated as a laser oscillator, is presented as verification of the small-signal gain results.     

Gain and fluorescence characteristics of flowing CO2laser systems

Single-pass gain has been measured for flowing CO2, CO2-N2, CO2-He, CO2-N2-He, and CO2-N2-H2mixes. The gain for CO2-N2mixes varies as d^-0.9, wheredis the tube diameter. The diameter dependence of the gain is less pronounced for CO2- N2-He mixes; a peak gain of 4.7 dB/m was obtained in a 1/2 in diam tube. Fluorescence data indicate that the upper laser level population is saturated at 100 mA in all cases. The addition of He, H2, or O2depopulates the lower laser level; helium further increases the population of the upper laser level. The addition of CO increases the population of the upper laser level, probably by resonant transfer from the excited vibrational states of CO.     

管板式横流10kWCO_2激光器的实验研究

本文叙述一台具有重复脉冲辅助放电的横向流动连续CO_2激光器。实验研究了放电特性,并给出激光器增益和输出功率的实验和计算结果。激光器最大输出功率12600W。在输出功率10200W条件下一次充气连续运行超过8h,功率不稳定度±1.5％。     

Performance of a compact sealed 200-W CO2laser

The performance characteristics of a compact (3-ft³) TEM00-mode single-wavelength CO2laser are described. The optic axis, gas flow velocity, and glow discharge are mutually orthogonal in the sealed-off laser head. The laser produces up to 300 W of TEM00- mode 10.6-μm power.     

A sealed high-repetition-rate TEA CO2laser

A compact atmospheric pressure CO2laser utilizing a double-discharge technique has been constructed and operated at repetition rates to 100 pulses/s. With the addition of small amounts of hydrogen and carbon monoxide to give a gas mixture of He:N2: CO2:CO:H2= 69.3:11:15:4:0.7, sealed operational lifetimes exceeding2 times 10^{6}pulses have been obtained. Operating in this mode, the output energy density is about 8-9 J/l at repetition frequencies of 30-40 pulses/s for input energy densities of 60-70 J/l. The operation of the sealed laser has been studied by means of mass spectroscopic measurements of the gas mixture. It has been determined that sealed operation is possible as long as the oxygen concentration is kept below 1-2 percent. It has also been found that the addition of small amounts of H2and CO will keep the oxygen concentration below 2 percent by reducing the CO2decomposition, allowing sealed operation. The experimental results are compared to the predictions of a theoretical model in which neutral and negative-ion processes have been included. The calculations indicate that when small amounts of oxygen or water are present in the discharge the negative-ion population is significantly increased and the ratio of negative-ions to electronsN_{n}/N_{e}can approach values near unity. These are the conditions under which discharge arcing was found to occur. The model also predicts that the dissociation equilibrium of the CO2can be controlled by the addition of the above concentrations of hydrogen and CO.     

Amplification at 10.6 µ in the negative glow of a hollow-cathode discharge in a CO2-He mixture

An amplifier for 10.6-μ radiation of a CO2laser has been constructed using the negative glow of a hollow-cathode discharge. The single-pass gain of 10 percent per meter reported here from such a discharge in a CO2-He mixture is less than that realizable in the positive column of a glow discharge used for CO2lasers under comparable conditions. The addition of N2, CO, or O2was not found to increase the gain.     

Radio-frequency preionization in a supersonic transverse electrical discharge laser

Preionization produced by a radio-frequency (RF) discharge near the cathode of a transverse flow electrical-discharge laser is used to initiate spatially diffuse discharge pulses in a Mach 3 flow of CO2-N2-He gas at pressures up to 160 torr. Main discharge uniformity and laser output performance have been determined as a function of pressure and RF discharge characteristics.     

Gas-chromatographic studies of the products in a sealed TE CO2laser discharge

In this investigation the degraded gas mixture in a sealed TE CO2laser discharge was analyzed gas-chromatographically, which enabled us to determine the concentration of CO accurately, even in the presence of large quantities of N2. According to the reversible decomposition reaction 2CO2rightleftharpoons2CO + O2, [CO]/2[O2], which should be unity, was found to be noticeably more than unity. The deviation of the O2concentration from that needed to satisfy the CO2decomposition equation was more than 26 percent. No oxides of nitrogen were detected and the missing oxygen was recovered when the degraded gas mixture was heated to the dissociation temperature of ozone.