共查询到19条相似文献,搜索用时 62 毫秒
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酚类污染物是常见的有机污染物之一,含酚废水处理难度大、毒性强,对自然环境与人类健康具有严重危害。催化湿式过氧化氢氧化技术(CWPO)以H2O2为氧化剂,利用催化剂催化产生·OH强氧化性自由基,可去除水中难降解有机污染物。介绍了CWPO非负载与负载型催化剂在含酚废水中的应用情况,负载型催化剂更具应用前景。利用密度泛函理论(DFT)分析了苯酚、间甲酚污染物主要降解途径,降解含酚废水是通过体系中·OH逐步改变苯环稳定结构形成苯醌类中间体,该中间体C-C断裂开环形成短链羧酸,最终完全矿化为CO2和H2O。未来可从制备稳定环保催化剂、分析实际废水降解机制方面展开研究,以发挥CWPO在含酚废水中的应用潜力。 相似文献
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混合型表面活性剂液膜法处理含酚废水研究 总被引:24,自引:1,他引:24
研究了兰-113B=Span-80--煤油NaOH液膜体系处理苯酚废水的最佳操作工用于对高浓度含酚废水进行处理,实验结果表明,混合型表面活性剂各项指标均较好,除酚效率可达99%以上,对内相NaOH的最佳浓度的确定给出了估算方法。 相似文献
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电极材料对含酚废水处理效果的影响 总被引:1,自引:0,他引:1
含酚废水是难降解有机废水,电化学方法处理工业废水具有高效、快速、无二次污染及适应性强的特点.该法是基于电极上的直接氧化和产生的自由基的间接氧化除去废水中的污染物.电极材料是电化学处理方法的核心,在很大程度上决定了废水处理效率.着重概述了不同电极材料对酚类降解效果的影响,认为该方法处理含酚废水应选择高过电位、性能稳定、活性高、成本低的电极材料. 相似文献
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含钛高炉渣光催化降解邻硝基酚的实验研究 总被引:5,自引:0,他引:5
研究了用处理过的含钛高炉渣作为光催化材料光催化降解邻硝基酚溶液,并探讨了影响其光催化性的多种影响因素,以寻求含钛高炉渣综合利用的新途径.实验结果表明:含钛高炉渣作为光催化材料对邻硝基酚溶液有降解作用;邻硝基酚溶液的浓度越低,降解率越高.本实验中,用负载于玻璃片的含钛高炉渣降解邻硝基酚溶液时,最佳溶液浓度为15mg/L;邻硝基酚溶液的pH值为3.0时降解率最大;对邻硝基酚溶液施加电压可提高光催化效率,降解率随电压的增大而增大. 相似文献
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采用微波两步法合成了1-辛基-3-甲基咪唑六氟磷酸([Omim]PF6)离子液体,采用多种方法表征了离子液体的结构。研究了[Omim]PF6对模拟焦化含酚废水(苯酚、甲酚、二甲酚)的萃取,考察了反应体系相比、反应时间、温度、体系pH值、微波辅助反应时长对萃取效果的影响。结果表明:在体系相比为V离子液体∶V含酚溶液=1∶1.5,反应时间为10min,反应温度为20℃,体系pH值为6,微波辅助反应时间40s的条件下,对含酚溶液的萃取率可达99.86%,并且[Omim]PF6具有良好的再生性能。 相似文献
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天然有机高分子及其改性产品在污水处理中的应用 总被引:4,自引:0,他引:4
天然有机高分子及其改性产品以其来源广、价廉、残留毒性小的独特优势在污水处理中广泛用作絮凝剂、重金属吸附剂。文章着重介绍了近年来研究较多的淀粉类、甲壳素 /壳聚糖类在污水处理中的应用 ,同时还介绍了其他天然有机高分子及其改性产品在该行业中的应用。 相似文献
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本文以聚二甲基硅氧烷(PDMS)为膜材料,乙烯基三乙氧基硅烷(VTES)为交联剂,在聚偏氟乙烯(PVDF)中空纤维支撑膜表面通过交联反应制备出PDMS/PVDF中空纤维渗透汽化复合膜。采用扫描电子显微镜和全反射傅里叶红外光谱仪表征复合膜的形貌和结构变化。研究了膜对正丁醇-水、异丙醇-水及丙酮-水三种模拟含盐有机废水的分离效果,并考察了温度对膜性能的影响。结果表明:PDMS/PVDF中空纤维膜对这三种模拟含盐有机废水有较好的分离效果,操作温度为40 oC时,膜的渗透通量分别为275.95 g/(m2.h)、322.16 g/(m2.h)、489.76 g/(m2.h),分离因子为37.82、12.60、33.12。 相似文献
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Inhibitory effects of toxic compounds on nitrification process for cokes wastewater treatment 总被引:8,自引:0,他引:8
Cokes wastewater is one of the most toxic industrial effluents since it contains high concentrations of toxic compounds such as phenols, cyanides and thiocyanate. Although activated sludge process has been adapted to treat this wastewater, nitrification process has been occasionally upset by serious inhibitory effects of toxic compounds. In this study, therefore, we examined inhibitory effects of ammonia, thiocyanate, free cyanide, ferric cyanide, phenol and p-cresol on nitrification in an activated sludge system, and then correlated their threshold concentrations with the full-scale pre-denitrification process for treating cokes wastewater. Ammonia below 350 mg/L did not cause substrate inhibition for nitrifying bacteria. Thiocyanate above 200mg/L seemed to inhibit nitrification, but it was due to the increased loading of ammonia produced from its biodegradation. Free cyanide above 0.2mg/L seriously inhibited nitrification, but ferric cyanide below 100mg/L did not. Phenol and p-cresol significantly inhibited nitrification above 200 mg/L and 100mg/L, respectively. Meantime, activated carbon was added to reduce inhibitory effects of phenol and free cyanide. 相似文献
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《Advanced Powder Technology》2020,31(8):3236-3245
In this study, the adsorption of fluoride ion (F-) from synthetic wastewater was performed using activated carbon/Fe3O4 nanocomposite in a batch system. To prepare activated carbon (AC), oak shell was used. Also, several analyses such as BET, SEM, EDX, FTIR, XRD, VSM and DLS analyzes were used to study the structure and morphology of the AC/Fe3O4 nanocomposite. BET analysis indicated that the specific surface area of Fe3O4 and AC/Fe3O4 were 65.44 and 226.78 m2/g, respectively, which shows the surface area of the AC/Fe3O4 composite was significantly increased compared to Fe3O4. Also, the particle size of the AC/Fe3O4 composite was obtained 75 nm by the DLS analysis. The sorption tests indicated that the highest sorption efficiency of fluoride ion using the Fe3O4/AC nanocomposite was obtained 97.4%. Moreover, the experimental results were well fitted with the Freundlich model. The maximum monolayer uptake capacity using the AC/Fe3O4 was obtained as 454.54 mg/g and showed a remarkable adsorption capacity, whichever achieved for fluoride ion sorption. Also, zero-point charge of pH (pHzpc) was obtained 5. Furthermore, the kinetic data were described by the quasi-second-order model. Besides, the thermodynamic parameters showed that the uptake of fluoride ion with the AC/Fe3O4 nanocomposite was spontaneous, practical, and endothermic. The outcomes suggest that AC/Fe3O4 nanocomposite can be effectively applied for the F- ion removal from synthetic wastewater. 相似文献
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Ahmad Hamad Ahmed Aidan Mohammed Fayed Mehrab Mehrvar 《Clean Technologies and Environmental Policy》2005,7(3):177-181
Experimental investigation shows that UV/hydrogen peroxide (H2O2) oxidation of a more concentrated phenolic wastewater can lead to economical savings. The savings can be achieved by the
lower amount of H2O2 required and time needed to treat the wastewater. Phenolic wastewater can be concentrated by treating the bulk wastewater
with activated carbon. The concentrated wastewater that is generated from activated carbon regeneration (assumed to be fully
regenerated by steam) can then be treated with UV/H2O2. Experimental results show that H2O2 concentration goes through an optimum value where adding any more H2O2 will result in less effective removal of contaminants. Conductivity of treated wastewater increases sharply then drops down.
This could be attributed to the presence of high molecular compounds, inorganic acids, and OH radicals. 相似文献