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1.
M. Zaatari  J. Siegel 《Indoor air》2014,24(4):350-361
Particles in retail environments can have consequences for the occupational exposures of retail workers and customers, as well as the energy costs associated with ventilation and filtration. Little is known about particle characteristics in retail environments. We measured indoor and outdoor mass concentrations of PM10 and PM2.5, number concentrations of submicron particles (0.02–1 μm), size‐resolved 0.3–10 μm particles, as well as ventilation rates in 14 retail stores during 24 site visits in Pennsylvania and Texas. Overall, the results were generally suggestive of relatively clean environments when compared to investigations of other building types and ambient/occupational regulatory limits. PM10 and PM2.5 concentrations (mean ± s.d.) were 20 ± 14 and 11 ± 10 μg/m3, respectively, with indoor‐to‐outdoor ratios of 1.0 ± 0.7 and 0.88 ± 1.0. Mean submicron particle concentrations were 7220 ± 7500 particles/cm3 with an indoor‐to‐outdoor ratio of 1.18 ± 1.30. The median contribution to PM10 and PM2.5 concentrations from indoor sources (vs. outdoors) was 83% and 53%, respectively. There were no significant correlations between measured ventilation rates and particle concentrations of any size. When examining options to lower PM2.5 concentrations below regulatory limits, the required changes to ventilation and filtration efficiency were site specific and depended on the indoor and outdoor concentration, emission rate, and infiltration level.  相似文献   

2.
Singapore is a tropical country with a high density of day-care facilities whose indoor environments may be adversely affected by outdoor fine particle (PM2.5) air pollution. To reduce this problem requires effective, evidence-based exposure-reduction strategies. Little information is available on the penetration of outdoor PM2.5 into day-care environments. Our study attempted to address the following objectives: to measure indoor infiltration factor (Finf) of PM2.5 from outdoor PM2.5 and to determine the building parameters that modify the indoor PM2.5. We collected indoor/outdoor 1-min PM2.5 from 50 day-care classrooms. We noted mean Finf ± SD of 0.65 ± 0.22 in day-care rooms which are naturally ventilated and lower Finf ± SD values of 0.47 ± 0.18 for those that are air-conditioned: values which are lower than those reported in Singapore residences. The air exchange rates were higher in naturally ventilated rooms (1.47 vs 0.86 h−1). However, fine particle deposition rates were lower for naturally ventilated rooms (0.67 ± 0.43 h−1) compared with air-conditioned ones (1.03 ± 0.55 h−1) presumably due to composite rates linked to the filters within the split unit air-conditioners, higher recirculation rates, and interior surfaces in the latter. Our findings indicate that children remaining indoor in daycares where air-conditioning is used can reduce their PM2.5 exposures during outdoor pollution episodes.  相似文献   

3.
Particle air filters used in central residential forced‐air systems are most commonly evaluated for their size‐resolved removal efficiency for particles 0.3‐10 µm using laboratory tests. Little information exists on the removal efficiency of commercially available residential filters for particles smaller than 0.3 µm or for integral measures of mass‐based aerosol concentrations (eg, PM2.5) or total number concentrations (eg, ultrafine particles, or UFPs) that are commonly used in regulatory monitoring and building measurements. Here, we measure the size‐resolved removal efficiency of 50 new commercially available residential HVAC filters installed in a recirculating central air‐handling unit in an unoccupied apartment unit using alternating upstream/downstream measurements with incense and NaCl as particle sources. Size‐resolved removal efficiencies are then used to estimate integral measures of PM2.5 and total UFP removal efficiency for the filters assuming they are challenged by 201 residential indoor particle size distributions (PSDs) gathered from the literature. Total UFP and PM2.5 removal efficiencies generally increased with manufacturer‐reported filter ratings and with filter thickness, albeit with numerous exceptions. PM2.5 removal efficiencies were more influenced by the assumption for indoor PSD than total UFP removal efficiencies. Filters with the same ratings but from different manufacturers often had different removal efficiencies for PM2.5 and total UFPs.  相似文献   

4.
Q. Zhang  J. Avalos  Y. Zhu 《Indoor air》2014,24(2):190-198
This study characterized fine (PM2.5) and ultrafine particle (UFP, diameter < 100 nm) emissions from microwave popcorn and analyzed influential factors. Each pre‐packed popcorn bag was cooked in a microwave oven enclosed in a stainless steel chamber for 3 min. The number concentration and size distribution of UFPs and PM2.5 mass concentration were measured inside the chamber repeatedly for five different flavors under four increasing power settings using either the foil‐lined original package or a brown paper bag. UFPs and PM2.5 generated by microwaving popcorn were 150–560 and 350–800 times higher than the emissions from microwaving water, respectively. About 90% of the total particles emitted were in the ultrafine size range. The emitted PM concentrations varied significantly with flavor. Replacing the foil‐lined original package with a brown paper bag significantly reduced the peak concentration by 24–87% for total particle number and 36–70% for PM2.5. A positive relationship was observed between both UFP number and PM2.5 mass and power setting. The emission rates of microwave popcorn ranged from 1.9 × 1010 to 8.0 × 1010 No./min for total particle number and from 134 to 249 μg/min for PM2.5.  相似文献   

5.
Correctional centers (prisons) are one of the few non‐residential indoor environments where smoking is still permitted. However, few studies have investigated indoor air quality (IAQ) in these locations. We quantified the level of inmate and staff exposure to secondhand smoke, including particle number (PN) count, and we assessed the impact of the smoking ban on IAQ. We performed measurements of indoor and outdoor PM2.5 and PN concentrations, personal PN exposure levels, volatile organic compounds (VOCs), and nicotine both before and after a complete indoor smoking ban in an Australian maximum security prison. Results show that the indoor 24‐h average PM2.5 concentrations ranged from 6 (±1) μg/m3 to 17 (±3) μg/m3 pre‐ban. The post‐ban levels ranged from 7 (±2) μg/m3 to 71 (±43) μg/m3. While PM2.5 concentrations decreased in one unit post‐ban, they increased in the other two units. Similar post‐ban increases were also observed in levels of PN and VOCs. We describe an unexpected increase of indoor pollutants following a total indoor smoking ban in a prison that was reflected across multiple pollutants that are markers of smoking. We hypothesise that clandestine post‐ban smoking among inmates may have been the predominant cause.  相似文献   

6.
In Paraguay, 49% of the population depends on biomass (wood and charcoal) for cooking. Residential biomass burning is a major source of fine particulate matter (PM2.5) and carbon monoxide (CO) in and around the household environment. In July 2016, cross‐sectional household air pollution sampling was conducted in 80 households in rural Paraguay. Time‐integrated samples (24 hours) of PM2.5 and continuous CO concentrations were measured in kitchens that used wood, charcoal, liquefied petroleum gas (LPG), or electricity to cook. Qualitative and quantitative household‐level variables were captured using questionnaires. The average PM2.5 concentration (μg/m3) was higher in kitchens that burned wood (741.7 ± 546.4) and charcoal (107.0 ± 68.6) than in kitchens where LPG (52.3 ± 18.9) or electricity (52.0 ± 14.8) was used. Likewise, the average CO concentration (ppm) was higher in kitchens that used wood (19.4 ± 12.6) and charcoal (7.6 ± 6.5) than in those that used LPG (0.5 ± 0.6) or electricity (0.4 ± 0.6). Multivariable linear regression was conducted to generate predictive models for indoor PM2.5 and CO concentrations (predicted R2 = 0.837 and 0.822, respectively). This study provides baseline indoor air quality data for Paraguay and presents a multivariate statistical approach that could be used in future research and intervention programs.  相似文献   

7.
In low‐resource settings, there is a need to develop models that can address contributions of household and outdoor sources to population exposures. The aim of the study was to model indoor PM2.5 using household characteristics, activities, and outdoor sources. Households belonging to participants in the Mother and Child in the Environment (MACE) birth cohort, in Durban, South Africa, were randomly selected. A structured walk‐through identified variables likely to generate PM2.5. MiniVol samplers were used to monitor PM2.5 for a period of 24 hours, followed by a post‐activity questionnaire. Factor analysis was used as a variable reduction tool. Levels of PM2.5 in the south were higher than in the north of the city (< .05); crowding and dwelling type, household emissions (incense, candles, cooking), and household smoking practices were factors associated with an increase in PM2.5 levels (P < .05), while room magnitude and natural ventilation factors were associated with a decrease in the PM2.5 levels (P < .05). A reasonably robust PM2.5 predictive model was obtained with model R2 of 50%. Recognizing the challenges in characterizing exposure in environmental epidemiological studies, particularly in resource‐constrained settings, modeling provides an opportunity to reasonably estimate indoor pollutant levels in unmeasured homes.  相似文献   

8.
The objective of this study was to quantify the influence of ventilation systems on indoor particle concentrations in residential buildings. Fifteen occupied, single‐family apartments were selected from three sites. The three sites have three different ventilation systems: unbalanced mechanical ventilation, balanced mechanical ventilation, and natural ventilation. Field measurements were conducted between April and June 2012, when outdoor air temperatures were comfortable. Number concentrations of particles, PM2.5 and CO2, were continuously measured both outdoors and indoors. In the apartments with natural ventilation, I/O ratios of particle number concentrations ranged from 0.56 to 0.72 for submicron particles, and from 0.25 to 0.60 for particles larger than 1.0 μm. The daily average indoor particle concentration decreased to 50% below the outdoor level for submicron particles and 25% below the outdoor level for fine particles, when the apartments were mechanically ventilated. The two mechanical ventilation systems reduced the I/O ratios by 26% for submicron particles and 65% for fine particles compared with the natural ventilation. These results showed that mechanical ventilation can reduce exposure to outdoor particles in residential buildings.  相似文献   

9.
The intensity, frequency, duration, and contribution of distinct PM2.5 sources in Asian households have seldom been assessed; these are evaluated in this work with concurrent personal, indoor, and outdoor PM2.5 and PM1 monitoring using novel low-cost sensing (LCS) devices, AS-LUNG. GRIMM-comparable observations were acquired by the corrected AS-LUNG readings, with R2 up to 0.998. Twenty-six non-smoking healthy adults were recruited in Taiwan in 2018 for 7-day personal, home indoor, and home outdoor PM monitoring. The results showed 5-min PM2.5 and PM1 exposures of 11.2 ± 10.9 and 10.5 ± 9.8 µg/m3, respectively. Cooking occurred most frequently; cooking with and without solid fuel contributed to high PM2.5 increments of 76.5 and 183.8 µg/m3 (1 min), respectively. Incense burning had the highest mean PM2.5 indoor/outdoor (1.44 ± 1.44) ratios at home and on average the highest 5-min PM2.5 increments (15.0 µg/m3) to indoor levels, among all single sources. Certain events accounted for 14.0%-39.6% of subjects’ daily exposures. With the high resolution of AS-LUNG data and detailed time-activity diaries, the impacts of sources and ventilations were assessed in detail.  相似文献   

10.
This work uses an in situ filter test method to measure the size‐resolved removal efficiency of indoor‐generated ultrafine particles (approximately 7–100 nm) for six new commercially available filters installed in a recirculating heating, ventilating, and air‐conditioning (HVAC) system in an unoccupied test house. The fibrous HVAC filters were previously rated by the manufacturers according to ASHRAE Standard 52.2 and ranged from shallow (2.5 cm) fiberglass panel filters (MERV 4) to deep‐bed (12.7 cm) electrostatically charged synthetic media filters (MERV 16). Measured removal efficiency ranged from 0 to 10% for most ultrafine particles (UFP) sizes with the lowest rated filters (MERV 4 and 6) to 60–80% for most UFP sizes with the highest rated filter (MERV 16). The deeper bed filters generally achieved higher removal efficiencies than the panel filters, while maintaining a low pressure drop and higher airflow rate in the operating HVAC system. Assuming constant efficiency, a modeling effort using these measured values for new filters and other inputs from real buildings shows that MERV 13–16 filters could reduce the indoor proportion of outdoor UFPs (in the absence of indoor sources) by as much as a factor of 2–3 in a typical single‐family residence relative to the lowest efficiency filters, depending in part on particle size.  相似文献   

11.
This study evaluated nine ventilation and filtration systems in an unoccupied 2006 house located 250 m downwind of the I‐80 freeway in Sacramento, California. Systems were evaluated for reducing indoor concentrations of outdoor particles in summer and fall/winter, ozone in summer, and particles from stir‐fry cooking. Air exchange rate was measured continuously. Energy use was estimated for year‐round operation in California. Exhaust ventilation without enhanced filtration provided indoor PM2.5 that was 70% lower than outdoors. Supply ventilation with MERV13 filtration provided slightly less protection, whereas supply MERV16 filtration reduced PM2.5 by 97‐98% relative to outdoors. Supply filtration systems used little energy but provided no benefits for indoor‐generated particles. Systems with MERV13‐16 filter in the recirculating heating and cooling unit (FAU) operating continuously or 20 min/h reduced PM2.5 by 93‐98%. Across all systems, removal percentages were higher for ultrafine particles and lower for black carbon, relative to PM2.5. Indoor ozone was 3‐4% of outdoors for all systems except an electronic air cleaner that produced ozone. Filtration via the FAU or portable filtration units lowered PM2.5 by 25‐75% when operated over the hour following cooking. The energy for year‐round operation of FAU filtration with an efficient blower motor was estimated at 600 kWh/year.  相似文献   

12.
We estimated the impact of a smoke‐free workplace bylaw on non‐smoking bar workers' health in Ontario, Canada. We measured bar workers' urine cotinine before (= 99) and after (= 91) a 2004 smoke‐free workplace bylaw. Using pharmacokinetic and epidemiological models, we estimated workers' fine‐particle (PM2.5) air pollution exposure and mortality risks from workplace secondhand smoke (SHS). workers' pre‐law geometric mean cotinine was 10.3 ng/ml; post‐law dose declined 70% to 3.10 ng/ml and reported work hours of exposure by 90%. Pre‐law, 97% of workers' doses exceeded the 90th percentile for Canadians of working age. Pre‐law‐estimated 8‐h average workplace PM2.5 exposure from SHS was 419 μg/m3 or ‘Very Poor’ air quality, while outdoor PM2.5 levels averaged 7 μg/m3, ‘Very Good’ air quality by Canadian Air Quality Standards. We estimated that the bar workers' annual mortality rate from workplace SHS exposure was 102 deaths per 100 000 persons. This was 2.4 times the occupational disease fatality rate for all Ontario workers. We estimated that half to two‐thirds of the 10 620 Ontario bar workers were non‐smokers. Accordingly, Ontario's smoke‐free law saved an estimated 5–7 non‐smoking bar workers' lives annually, valued at CA $50 million to $68 million (US $49 million to $66 million).  相似文献   

13.
Emissions from indoor biomass burning are a major public health concern in developing areas of the world. Less is known about indoor air quality, particularly airborne endotoxin, in homes burning biomass fuel in residential wood stoves in higher income countries. A filter‐based sampler was used to evaluate wintertime indoor coarse particulate matter (PM10‐2.5) and airborne endotoxin (EU/m3, EU/mg) concentrations in 50 homes using wood stoves as their primary source of heat in western Montana. We investigated number of residents, number of pets, dampness (humidity), and frequency of wood stove usage as potential predictors of indoor airborne endotoxin concentrations. Two 48‐h sampling events per home revealed a mean winter PM10‐2.5 concentration (± s.d.) of 12.9 (± 8.6) μg/m3, while PM2.5 concentrations averaged 32.3 (± 32.6) μg/m3. Endotoxin concentrations measured from PM10‐2.5 filter samples were 9.2 (± 12.4) EU/m3 and 1010 (± 1524) EU/mg. PM10‐2.5 and PM2.5 were significantly correlated in wood stove homes (r = 0.36, P < 0.05). The presence of pets in the homes was associated with PM10‐2.5 but not with endotoxin concentrations. Importantly, none of the other measured home characteristics was a strong predictor of airborne endotoxin, including frequency of residential wood stove usage.  相似文献   

14.
Portable air cleaners are increasingly used in polluted areas in an attempt to reduce human exposure; however, there has been limited work characterizing their effectiveness at reducing exposure. With this in mind, we recruited forty-three children with asthma from suburban Shanghai and deployed air cleaners (with HEPA and activated carbon filters) in their bedrooms. During both 2-week filtration and non-filtration periods, low-cost PM2.5 and O3 air monitors were used to measure pollutants indoors, outdoors, and for personal exposure. Indoor PM2.5 concentrations were reduced substantially with the use of air cleaners, from 34 ± 17 to 10 ± 8 µg/m3, with roughly 80% of indoor PM2.5 estimated to come from outdoor sources. Personal exposure to PM2.5 was reduced from 40 ± 17 to 25 ± 14 µg/m3. The more modest reductions in personal exposure and high contribution of outdoor PM2.5 to indoor concentrations highlight the need to reduce outdoor PM2.5 and/or to clean indoor air in multiple locations. Indoor O3 concentrations were generally low (mean = 8±4 ppb), and no significant difference was seen by filtration status. The concentrations of pollutants and the air cleaner effectiveness were highly variable over time and across homes, highlighting the usefulness of real-time air monitors for understanding individual exposure reduction strategies.  相似文献   

15.
There is growing awareness that indoor exposure to particulate matter with diameter ≤ 2.5 μm (PM2.5) is associated with an increased risk of adverse health effects. Cooking is a key indoor source of PM2.5 and an activity conducted daily in most homes. Population scale models can predict occupant exposures to PM2.5, but these predictions are sensitive to the emission rates used. Reported emission rates are highly variable and are typically for the cooking of single ingredients and not full meals. Accordingly, there is a need to assess PM2.5 emissions from the cooking of complete meals. Mean PM2.5 emission rates and source strengths were measured for four complete meals. Temporal PM2.5 concentrations and particle size distributions were recorded using an optical particle counter (OPC), and gravimetric sampling was used to determine calibration factors. Mean emission rates and source strengths varied between 0.54—3.7 mg/min and 15—68 mg, respectively, with 95% confidence. Using a cooker hood (apparent capture efficiency > 90%) and frying in non‐stick pans were found to significantly reduce emissions. OPC calibration factors varied between 1.5 and 5.0 showing that a single value cannot be used for all meals and that gravimetric sampling is necessary when measuring PM2.5 concentrations in kitchens.  相似文献   

16.
A number of studies have estimated population exposure to PM2.5 by examining modeled or measured outdoor PM2.5 levels. However, few have taken into account the mediating effects of building characteristics on the ingress of PM2.5 from outdoor sources and its impact on population exposure in the indoor domestic environment. This study describes how building simulation can be used to determine the indoor concentration of outdoor‐sourced pollution for different housing typologies and how the results can be mapped using building stock models and Geographical Information Systems software to demonstrate the modifying effect of dwellings on occupant exposure to PM2.5 across London. Building archetypes broadly representative of those in the Greater London Authority were simulated for pollution infiltration using EnergyPlus. In addition, the influence of occupant behavior on indoor levels of PM2.5 from outdoor sources was examined using a temperature‐dependent window‐opening scenario. Results demonstrate a range of I/O ratios of PM2.5, with detached and semi‐detached dwellings most vulnerable to high levels of infiltration. When the results are mapped, central London shows lower I/O ratios of PM2.5 compared with outer London, an apparent inversion of exposure most likely caused by the prevalence of flats rather than detached or semi‐detached properties.  相似文献   

17.
Indoor particle number and PM2.5 concentrations were investigated in a radio station surrounded by busy roads. Two extensive field measurement campaigns were conducted to determine the critical parameters affecting indoor air quality. The results indicated that indoor particle number and PM2.5 concentrations were governed by outdoor air, and were significantly affected by the location of air intake and design of HVAC system. Prior to the upgrade of the HVAC system and relocation of the air intake, the indoor median particle number concentration was 7.4×103 particles/cm3 and the median PM2.5 concentration was 7 μg/m3. After the relocation of air intake and the redesign of the HVAC system, the indoor particle number concentration was between 2.3×103 and 3.4×103 particles/cm3, with a median value of 2.7×103 particles/cm3, and the indoor PM2.5 concentration was in the range of 3–5 μg/m3, with a median value of 4 μg/m3. By relocating the air intake of the HVAC, the outdoor particle number and PM2.5 concentrations near the air intake were reduced by 35% and 55%, respectively. In addition, with the relocation of air intake and the redesign of the HVAC system, the particle number penetration rate was reduced from 42% to 14%, and the overall filtration efficiency of the HVAC system (relocation of air intake, pre-filter, AHU and particle losses in the air duct) increased from 58% to 86%. For PM2.5, the penetration rate after the upgrade was approximately 18% and the overall filtration efficiency was 82%. This study demonstrates that by using a comprehensive approach, including the assessment of outdoor conditions and characterisation of ventilation and filtration parameters, satisfactory indoor air quality can be achieved, even for those indoor environments facing challenging outdoor air conditions.  相似文献   

18.
Asian dust storms (ADS) originating from the arid deserts of Mongolia and China are a well-known springtime meteorological phenomenon throughout East Asia. The ventilation systems in office utilize air from outside and therefore it is necessary to understand how these dust storms affect the concentrations of PM2.5 and PM10 in both the indoor and outdoor air. We measured dust storm pollution particles in an office building using a direct-reading instrument (PC-2 Quartz Crystal Microbalance, QCM) that measured particle size and concentration every 10 min for 1 h, three times a day. A three-fold increase in the concentrations of PM2.5 and PM10 in the indoor and outdoor air was recorded during the dust storms. After adjusting for other covariates, autoregression models indicated that PM2.5 and PM10 in the indoor air increased significantly (21.7 μg/m3 and 23.0 μg/m3 respectively) during dust storms. The ventilation systems in high-rise buildings utilize air from outside and therefore the indoor concentrations of fine and coarse particles in the air inside the buildings are significantly affected by outside air pollutants, especially during dust storms.  相似文献   

19.
H. Zhao  B. Stephens 《Indoor air》2016,26(4):571-581
Recent experiments have demonstrated that outdoor ozone reacts with materials inside residential building enclosures, potentially reducing indoor exposures to ozone or altering ozone reaction byproducts. However, test methods to measure ozone penetration factors in residences (P) remain limited. We developed a method to measure ozone penetration factors in residences under infiltration conditions and applied it in an unoccupied apartment unit. Twenty‐four repeated measurements were made, and results were explored to (i) evaluate the accuracy and repeatability of the new procedure using multiple solution methods, (ii) compare results from ‘interference‐free’ and conventional UV absorbance ozone monitors, and (iii) compare results against those from a previously published test method requiring artificial depressurization. The mean (±s.d.) estimate of P was 0.54 ± 0.10 across a wide range of conditions using the new method with an interference‐free monitor; the conventional monitor was unable to yield meaningful results due to relatively high limits of detection. Estimates of P were not clearly influenced by any indoor or outdoor environmental conditions or changes in indoor decay rate constants. This work represents the first known measurements of ozone penetration factors in a residential building operating under natural infiltration conditions and provides a new method for widespread application in buildings.  相似文献   

20.
We report results of analysis of a month‐long measurement of indoor air and environment quality parameters in one gym during sporting activities such as football, basketball, volleyball, badminton, boxing, and fitness. We have determined an average single person's contribution to the increase of temperature, humidity, and dust concentration in the gym air volume of 12500 m3: during 90‐min exercise performed at an average heart rate of 143 ± 10 bpm, a single person evaporated 0.94 kg of water into the air by sweating, contributed 0.03 K to the air temperature rise and added 1.5 μg/m3 and 5 ng/m3 to the indoor concentration of inhalable particles (PM10) and Ca concentration, respectively. As the breathing at the observed exercise intensity was about three times faster with respect to the resting condition and as the exercise‐induced PM10 concentration was about two times larger than outdoors, a sportsman in the gym would receive about a sixfold higher dose of PM10 inside than he/she would have received at rest outside.  相似文献   

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