Picosecond Diode-Pumped Laser System with 9.3-W Average Power and 2.3-mJ Pulse Energy

We describe a diode-pumped Nd:YAG laser that is suitable for micromachining applications and is capable of generating 2.3-mJ pulses at a 4-kHz pulse repetition frequency. The output pulse duration is 20.5 ps. The system is based on a Nd:YAG regenerative amplifier with a novel four-pass postamplifier. The postamplifier incorporates birefringent depolarization compensation and simultaneously prevents parasitic laser oscillation by use of a nonreciprocal beam path. These output pulse energies are achieved without the use of chirped pulse amplification.     

Optical parametric chirped-pulse amplifier as an alternative to Ti:sapphire regenerative amplifiers

We demonstrated a high-pulse energy, femtosecond-pulse source based on optical parametric chirped-pulse amplification. We successfully amplified 1-microm broadband oscillator pulses to 31 mJ and recompressed them to 310-fs pulse duration, at a 10-Hz repetition rate. The gain in our system is 6 x 10(7), achieved by the single passing of only 40 mm of gain material pumped by a commercial Q-switched Nd:YAG laser. This relatively simple system replaces a more complex Ti:sapphire regenerative-amplifier-based chirped-pulse amplification system. Numerous features in design and performance of optical parametric chirped-pulse amplifiers make them a preferred alternative to regenerative amplifiers based on Ti:sapphire in the front end of high-peak-power lasers.     

Evaluation of an ultrabroadband high-gain amplification technique for chirped pulse amplification facilities

Recently, an amplification technique for ultrashort pulses was explored in detail in a theoretical paper by Ross et al. [Opt. Commun. 144, 125 (1997)]. The technique, based on nonlinear optics, is called optical parametric chirped pulse amplification. It has a number of features that, in principle, make it highly attractive. It primarily offers extremely large gains simultaneously with extremely large bandwidths. Additional attractions are virtually no spatial and temporal phase distortion of the amplified pulse, high efficiencies and a low thermal loading, reduced amplified spontaneous emission levels, small optical material lengths, and an inherent simplicity of implementation. We present an evaluation of the technique as a front end amplifier for the ultrashort pulse amplification chain of the Vulcan laser system. Such a device could replace some of the existing amplification in Nd:glass and additionally have a wider effect as a direct replacement of Ti:sapphire regenerative amplifiers on large-scale chirped pulse amplification scale facilities.     

Hollow fiber optics with improved durability for high-peak-power pulses of Q-switched Nd:YAG lasers

To improve the damage threshold of hollow optical waveguides for transmitting Q-switched Nd:YAG laser pulses, we optimize the metallization processes for the inner coating of fibers. For silver-coated hollow fiber as the base, second, and third Nd:YAG lasers, drying silver films at a moderate temperature and with inert gas flow is found to be effective. By using this drying process, the resistance to high-peak-power optical pulse radiation is drastically improved for fibers fabricated with and without the sensitizing process. The maximum peak power transmitted in the fiber is greater than 20 MW. To improve the energy threshold of aluminum-coated hollow fibers for the fourth and fifth harmonics of Nd:YAG lasers, a thin silver film is added between the aluminum film and the glass substrate to increase adhesion of the aluminum coating. By using this primer layer, the power threshold improves to 3 MW for the fourth harmonics of a Q-switched Nd:YAG laser light.     

Pump beam waist-dependent pulse energy generation in Nd:YAG/Cr4+:YAG passively Q-switched microchip laser

Abstract

The incident pump beam waist-dependent pulse energy generation in Nd:YAG/Cr⁴⁺:YAG composite crystal passively Q-switched microchip laser has been investigated experimentally and theoretically by moving the Nd:YAG/Cr⁴⁺:YAG composite crystal along the pump beam direction. Highest pulse energy of 0.4 mJ has been generated when the Nd:YAG/Cr⁴⁺:YAG composite crystal is moved about 6 mm away from the focused pump beam waist. Laser pulses with pulse width of 1.7 ns and peak power of over 235 kW have been achieved. The theoretically calculated effective laser beam area at different positions of Nd:YAG/Cr⁴⁺:YAG composite crystal along the pump beam direction is in good agreement with the experimental results. The highest peak power can be generated by adjusting the pump beam waist incident on the Nd:YAG/Cr⁴⁺:YAG composite crystal to optimize the effective laser beam area in passively Q-switched microchip laser.     

Semiconductor quantum-well saturable absorbers for efficient passive Q switching of a diode-pumped 946 nm Nd:YAG laser

InGaAs quantum wells and a Bragg mirror structure are grown on a GaAs substrate to simultaneously serve as a low-loss saturable absorber and an output coupler for highly efficient Q switching of a diode-pumped Nd:YAG laser operating at 946 nm. With an incident pump power of 9.2 W, the laser produces pulses of 38 ns duration with average pulse energy of as much as 20 microJ at a pulse repetition rate of 55 kHz.     

Hyper-Rayleigh scattering with picosecond pulse trains

We propose a method for measuring hyper-Rayleigh scattering employing pulse trains produced by a Q-switched and mode-locked Nd:YAG laser. The use of the entire pulse train under the Q-switch envelope avoids the need of any device to scan the irradiance, as is usually done with nanosecond and femtosecond single-pulse lasers. To verify the feasibility of the technique, we performed measurements in different solutions of para-nitroaniline and compared the results with those obtained with nanosecond pulses. In both cases, the agreement with the hyperpolarizability values reported in the literature is about the same, but the measurements carried out with pulse trains are at least 20 times faster. Besides the advantage of acquisition speed, the use of pulse trains also allows the instantaneous inspection of slow luminescence contributions arising from multiphoton absorption.     

Broad-spectrum neodymium-doped laser glasses for high-energy chirped-pulse amplification

We have investigated two novel laser glasses in an effort to generate high-energy, broad-spectrum pulses from a chirped-pulse amplification Nd:glass laser. Both glasses have significantly broader spectra (>38 nm FWHM) than currently available Nd:phosphate and Nd:silicate glasses. We present calculations for small signal pulse amplification to simulate spectral gain narrowing. The technique of spectral shaping using mixed-glass architecture with an optical parametric chirped-pulse amplification front end is evaluated. Our modeling shows that amplified pulses with energies exceeding 10 kJ with sufficient bandwidth to achieve 120 fs pulsewidths are achievable with the use of the new laser glasses. With further development of current technologies, a laser system could be scaled to generate one exawatt in peak power.     

Thermal tuning of laser pulse parameters in passively Q-switched Nd:YAG lasers

Modifying the output pulses of a passively Q-switched Nd:YAG laser, operating at 1064 nm, was realized by heating the laser crystal. With the demonstrated laser setups, a 100 K temperature rise led to a more than 50% increase in the pulse energy and a more than 10% decrease in the pulse length. This method offers an effective way to tune the output of the laser without mechanical adjustment or a change of components.     

Comparative study of femtosecond and nanosecond laser-induced breakdown spectroscopy of depleted uranium

We present spectra of depleted uranium metal from laser plasmas generated by nanosecond Nd:YAG (1064 nm) and femtosecond Ti:sapphire (800 nm) laser pulses. The latter pulses produce short-lived and relatively cool plasmas in comparison to the longer pulses, and the spectra of neutral uranium atoms appear immediately after excitation. Evidence for nonequilibrium excitation with femtosecond pulses is found in the dependence of spectral line intensities on the pulse chirp.     

Experimental and theoretical investigation of a multipass, plane mirror, femtosecond dye laser amplifier

Femtosecond pulses of a passive mode-locked Rhodamine-6G dye laser are amplified in a double-stage, three-pass, plane mirror, Sulforhodamine-101 amplifier system. Saturable filters (Schott glass RG645 and Malachite Green) are used to suppress amplified spontaneous emission. Input pulses of 110-fs duration are broadened to 240 fs in the amplifier system and recompressed to 75 fs in a prism-pair compressor. Using a 20-Hz Q-switched Nd:YAG pump laser of 50-mJ second-harmonic output energy, we obtained amplified and recompressed pulses of 180-μJ energy at 625 nm starting with 40-pJ input pulses. The small-signal amplification dynamics is studied numerically. Relevant gain dye and saturable filter parameters are derived. The influence of amplified spontaneous emission is analyzed.     

Pulsed laser energy through fiberoptics for generation of ultrasound

Laser pulses are an effective, noncontacting technique for generating ultrasound in materials. However, for this approach to be practical, a versatile and safe method of delivering the laser pulses must be developed that eliminates exposed beams steered by mirrors and focused by lenses. Investigations by several researchers using fiberoptic delivery systems indicate that fiberoptics may be a viable method for the delivery of laser energy to generate acoustic energy. The main problem experienced with the fiberoptic delivery systems has been the inability to deliver high-energy, short-duration pulses via a fiber for thousands of pulses with no fiber damage and with constant energy output. This paper presents a technique for laser generation of sound using fiberoptics that continuously delivers sustained 20 ns pulses at a pulsing rate of 30 Hz from a doubled, Q-switched Nd:YAG laser operating at 532 nm with output energy from the fiber-optic system up to 26 mJ/pulse. The delivery system is used to excite ultrasound in a molten weld pool as part of a research effort to develop a noncontacting sensing system for real-time weld inspection.     

High-repetition rate 1-J green laser system

A laser-diode-pumped high-repetition-rate zigzag slab Nd:YAG oscillator-amplifier system is developed as the pumping source of a high-average-power and terawatt Ti:sapphire chirped pulse amplification laser system. This system can produce a greater than 2-J high-energy fundamental laser pulse at a repetition rate of 100 Hz. The frequency-doubled energy with a diffusion-bonded KTP crystal is 1 J at a repetition rate of 100 Hz.     

Optical parametric chirped-pulse amplifier and spatiotemporal shaping for a petawatt laser

We present a degenerate noncollinear optical parametric chirped-pulse amplifier pumped by a high-energy, diode-pumped Nd:Glass regenerative amplifier delivering monomode pulses at 527 nm. The spatial mode shaping of the pump pulses is achieved with a diffractive laser cavity element, and temporal pulse shaping makes use of an electro-optic modulator and an arbitrary electrical waveform generator. Amplification at gain saturation achieves tailoring of the signal pulses. Numerical simulations with Miró software are presented and compared with experimental measurements.     

Performance of diode-end-pumped Cr, Nd:YAG self-Q-switched and Nd:YAG/Cr:YAG diffusion bonded lasers

Self-passively Q-switching of a diode-pumped Cr,Nd:YAG, where the Cr⁴⁺ is used as a saturable absorber for the 1064 nm laser emission is reported. The maximum average output power was obtained using an output coupler of R=86%. The self-Q-switched diode pumped laser yielded 1.86-W average output power with low threshold pumping power (≈1.7-W), average slope efficiency of ≈34%, pulse duration of about 14–16 ns, and modulation frequency ranging from 2.4 to 73 kHz, depending on the input pumping power. These results are the highest reported for self-Q-switched lasers. Higher slope efficiency (42%) and shorter Q-switched pulses were obtained for a Q-switched Nd:YAG/Cr⁴⁺:YAG diffusion bonded laser. A comparison of the codoped Cr,Nd:YAG laser performance, with that of a diffusion bonded laser is reported and analyzed.     

Prelase stabilization of the polarization state and frequency of a Q-switched, diode-pumped, Nd:YAG laser

We present an experimental investigation of the energy statistics of the linear polarization components of pulses from a Nd:YAG laser that is repetitively Q-switched with an acousto-optic modulator. Varying the modulator-induced diffraction losses leads to changes in the pulse polarization state and the energy statistics of the polarization components. For conventional Q-switching there is no laser oscillation during the low-Q intervals, and we find that the orthogonal components of the pulses can display large relative energy fluctuations even though the total pulse energy is quite stable. In the prelase mode, a weak continuous-wave background seeds the Q-switched pulses and results in the emission of highly linearly polarized, single-longitudinal-mode pulses with small relative energy fluctuations.     

Seeded femtosecond optical parametric amplification in the mid-infrared spectral region above 3 mum

Femtosecond optical parametric amplification that results in microjoule mid-infrared pulses at wavelengths exceeding 3 mum is demonstrated. Narrow-band quasi-cw seeding at the signal wavelength is applied to ensure the generation of nearly transform-limited femtosecond pulses at the idler wavelength. The broad bandwidth of the parametric amplification provided by pumping with femtosecond pulses from a Ti:sapphire regenerative amplifier at high intensity results in idler pulse durations shorter than the pump pulse length. The potentials of three nonlinear optical crystals that belong to the potassium titanyl phosphate family are comparatively studied. At 1-kHz repetition rate our all-solid-state system produces highly synchronized ~100-fs pulses in the spectral range between 3 and 4 mum.     

A 1319 nm diode-side-pumped Nd:YAG laser Q-switched with graphene oxide

We have demonstrated a diode-side-pumped Q-switched Nd:YAG laser operating at 1319?nm with a saturable absorber of graphene oxide fabricated by the vertical evaporation method. The 1319?nm Q-switched laser pulses were realized with average output power of 820 mW, pulse width of 2?μs and repetition rate of 35?kHz. The pulse energy and peak power were 23.4?μJ and 11.7?W, respectively when the optical pump power was 232?W. The experimental results indicate that graphene oxide is an effective saturable absorber for Q-switched lasers.     

Hollow fibers for delivery of harmonic pulses of Q-switched Nd:YAG lasers

Flexible hollow fibers for delivery of the second, third, and fourth harmonic pulses of Q-switched Nd:YAG lasers are introduced. For the doubled (532-nm) wavelength, we fabricated a hollow fiber with an internal metal and polymer film by using a silver-mirror plating and a liquid-phase-coating method. For tripled (355-nm) and quadrupled (266-nm) Nd:YAG in the ultraviolet region, we fabricated aluminum hollow fibers with or without an internal polymer layer by using the metal-organic chemical-vapor deposition method. Both types of fiber show high stability for the transmission of high-peak power laser pulses with low transmission losses.     

Diode-pumped passively Q-switched Nd:YVO4 green laser with a periodically poled KTP and Cr4+:YAG saturable absorber

A diode-pumped passively Q-switched Nd:YVO4 green laser with a periodically poled KTP and Cr4+:YAG saturable absorber is realized. The dependences of pulse repetition rate, pulse energy, pulse width, and peak power on incident pump power are measured for the generated green-light pulses. A rate-equation model is introduced to theoretically analyze the results obtained in the experiment, in which the spatial distribution of the intracavity photon density is taken into account. The numerical solutions of the rate equations agree with the experimental results.