Prediction analysis of dose equivalent responses of neutron dosemeters used at a MOX fuel facility

To predict how accurately neutron dosemeters can measure the neutron dose equivalent (rate) in MOX fuel fabrication facility work environments, the dose equivalent responses of neutron dosemeters were calculated by the spectral folding method. The dosemeters selected included two types of personal dosemeter, namely a thermoluminescent albedo neutron dosemeter and an electronic neutron dosemeter, three moderator-based neutron survey meters, and one special instrument called an H(p)(10) monitor. The calculations revealed the energy dependences of the responses expected within the entire range of neutron spectral variations observed in neutron fields at workplaces.     

Bonner sphere neutron spectrometry at spent fuel casks

For transport and interim storage of spent fuel elements from power reactors and vitrified highly active waste (HAW) from reprocessing, various types of casks are used. The radiation exposure of the personnel during transportation and storage of these casks is caused by mixed photon–neutron fields and, frequently, the neutron dose is predominant. In operational radiation protection, survey meters and even personal dosemeters with imperfect energy dependence of the dose-equivalent response are used, i.e. the fluence response of the devices does not match the fluence-to-dose equivalent conversion function. In order to achieve more accurate dosimetric information and to investigate the performance of dosemeters, spectrometric investigations of the neutron fields are necessary. Therefore, fluence spectra and dose rates were measured by means of a simple portable Bonner multisphere spectrometer (BSS). The paper describes briefly the experimental set-up and evaluation procedure. Measured spectra for different locations, types of casks and inventory are discussed. The spectra provide a basis to determine dose rates and other integral quantities with higher accuracy and for choosing suitable area monitors, respectively, to establish correction factors applied to the dosemeter reading.     

Determination of personal dose equivalents in accelerator radiation fields

Values for the dose equivalent are required for radiation protection purposes, but determination of such values can be quite difficult for high energy radiations. The accurate determination of personal dose equivalents in accelerator radiation fields requires the propel use of appropriate radiological quantities and units, knowledge of the dose equivalent response of the personal dosemeters used, measurement or calculation of the fluence spectrum in the workplace and the fluence spectrum of the reference radiation used to calibrate the dosemeters, in addition to knowledge of the appropriate fluence-to-dose equivalent conversion coefficients. This information can then be used to select the appropriate dosemeters, set up the optimum calibration conditions, or to establish correction factors that account for differences in the calibration and workplace fluence spectra. High energy neutrons account for a significant fraction of the dose equivalent received by workers at accelerator facilities, and this work discusses the procedures and methods needed to determine dose equivalent produced by neutrons in the vicinity of high energy particle accclerators.     

Personal neutron dosimetry in nuclear power plants using etched track and albedo thermoluminescence dosemeters

Measurement of the personal dose equivalent rates for neutrons is a difficult task because available dosemeters do not provide the required energy response and sensitivity. Furthermore, the available wide calibration spectra recommended by the International Standard Organisation does not reproduce adequately the spectra encountered in practical situations of the nuclear industry. There is a real necessity to characterise the radiation field, in which workers can be exposed, and to calibrate personal dosemeters in order to determine the dose equivalent in these installations. For this reason, we measure the neutron spectrum with our Bonner sphere system and we fold this spectrum with energy-dependent fluence-to-dose conversion coefficients to obtain the reference dose equivalent rate. This reference value is then compared with the personal dosemeter reading to determine a field-specific correction factor. In this paper, we present the values of this field-specific correction factor for etched track and albedo thermoluminescence dosemeters at three measurement locations inside the containment building of the Vandellòs II nuclear power plant. We have found that assigning to each personal dosemeter the mean value of the field-specific correction factors of the three measurement locations, allows the evaluation of neutron personal dose equivalent rate with a relative uncertainty of approximately 25 and 15% for the PADC and albedo dosemeters, respectively.     

Electronic personal neutron dosemeters for high energies: measurements, new developments and further needs

The results of measurements with neutron energies up to 60 MeV are shown for the personal neutron dosemeters Thermo Electron EPD-N2, ALOKA PDM-313 and the PTB prototype dosemeter DOS-2002. All dosemeters show dose equivalent responses that are about a factor of 10, too high at 60 MeV. A new prototype dosemeter-called DOS-2005-consisting of a detector with a thin effective layer of 6 microm has been set up at PTB. The dose equivalent response of this dosemeter and that of the newly developed dosemeter SAPHYDOSE-N was measured up to 19 MeV. Both dosemeters indicate a more flat response at high neutron energies. Further needs-optimisations, measurements and calculations-for use at high-energy accelerators and in space are discussed.     

Radionuclide neutron sources in calibration laboratory--neutron and gamma doses and their changes in time

The calibration laboratory, having standard neutron fields of radionuclide sources, should perform regular measurements of fields' parameters in order to check their stability and to get knowledge of any changes. Usually, accompanying gamma radiation is not of serious concern, but some personal dosemeters, old neutron dose equivalent meters with scintillation detectors and the dose meters of mixed radiation require the determination of this component. In the Laboratory of Radiation Protection Measurements in the Institute of Atomic Energy, Poland, the fields of radionuclide neutron sources (252)Cf, (241)Am-Be and (239)Pu-Be were examined for nearly 20 y. A number of detectors and methods have been applied for the determination of neutron ambient dose equivalent rate and for the determination of neutron and gamma dose components. This paper presents the recent results of measurements of gamma and neutron dose and dose equivalent, compared with the results accumulated in nearly 20 y.     

On the interpretation and use of neutron calibration coefficients

Calibration laboratories provide measurement services that include determining the calibration coefficients for neutron survey meters and personal dosemeters. While there are numerous documents dealing with the procedures for calibration of neutron measuring devices, the purpose of this paper is to clarify the use of the particular dose equivalent conversion coefficients used at the National Institute of Standards and Technology and the Pacific Northwest National Laboratory for these calibrations.     

Compliance of electronic personal neutron dosemeters with the new International Standard IEC 61526

The recommendations and test requests for the dose equivalent response of personal neutron dosemeters formulated by the new International Standard IEC 61526 are summarised. In particular, IEC 61526 allows the use of broad fields if dosemeters do not fulfil the hard requirements using monoenergetic neutrons. Some broad fields which can work as a replacement field using ISO sources ((252)Cf, (252)Cf (D(2)O mod.), (241)Am-Be) and simulated workplace fields (CANEL and SIGMA) are described. This work shows the results of recent measurements of the personal dose equivalent response for the dosemeters Thermo Electron EPD-N2, Aloka PDM-313 and the prototype dosemeter PTB DOS-2002, and discusses their compliance with respect to the new IEC 61526 standard.     

Intercomparison on measurements of the quantity personal dose equivalent Hp(10) in photon fields in the African region

An intercomparison was arranged by the International Atomic Energy Agency for the African region for personal dose equivalent. This was arranged with a view to helping member states to comply with dose limitation requirements and to harmonise the use of internationally agreed quantities and recommended assessment methods. The scope of the intercomparison was aimed at passive dosemeters, which determine the personal dose equivalent in photon radiation fields. The comparison protocol is presented together with the results.     

The use of passive personal neutron dosemeters to determine the neutron dose equivalent component of radiation fields in spacecraft

For the altitude range and inclination of the International Space Station (ISS), secondary neutrons can be a major contributor to dose equivalent inside a spacecraft. The exact proportion is very dependent on the amount of shielding of the primary galactic cosmic radiation and trapped particles, but is likely to lie in the range of 10-50%. Personal neutron dosemeters of simple design, processed using simple techniques developed for personal dosimetry, may be used to estimate this neutron component.     

Development of a neutron personal dose equivalent detector

A new neutron-measuring instrument that is intended to measure a neutron personal dose equivalent, H(p)(10) was developed. This instrument is composed of two parts: (1) a conventional moderator-based neutron dose equivalent meter and (2) a neutron shield made of borated polyethylene, which covers a backward hemisphere to adjust the angular dependence. The whole design was determined on the basis of MCNP calculations so as to have response characteristics that would generally match both the energy and angular dependencies of H(p)(10). This new instrument will be a great help in assessing the reference values of neutron H(p)(10) during field testing of personal neutron dosemeters in workplaces and also in interpreting their readings.     

Electronic personal dosemeters: the solution to problems of individual monitoring in mixed neutron/photon fields?

An overview is given showing the main principles of the present-day electronic neutron dosemeters. The radiological performance of the devices is described in a comparative way. This includes chiefly the personal dose equivalent Hp(10) response for monoenergetic neutrons and in practical fields with broad energy distributions and estimations of the low dose limit for neutrons.     

Calibration of personal dosemeters in mixed neutron-photon fields: some problems and their solution

In neutron reference radiation fields, the conventional true value of the personal dose equivalent, H(p)(10), is derived from the spectral neutron fluence and recommended conversion coefficients. This procedure requires the phantom on which the personal dosemeter is mounted to be irradiated with a broad and parallel beam. In many practical situations, the change of the neutron fluence and/or the energy distribution over the surface of the phantom may not be neglected. For a selection of typical irradiation conditions in neutron reference radiation fields, the influence of this effect has been analysed using numerical methods. A further problem, which is of relevance for the calibration of dosemeters measuring both the neutron and the photon component of mixed fields, is the 'double counting' of the dose equivalent due to neutron-induced photons. The relevance of this conceptual problem for calibrations in mixed-field dosimetry was analysed.     

A comparison of different neutron spectroscopy systems at the reactor facility VENUS

The VENUS facility is a zero-power research reactor mainly devoted to studies on LWR fuels. Localised high-neutron rates were found around the reactor, with a neutron/gamma dose equivalent rate ratio as high as three. Therefore, a study of the neutron dosimetry around the reactor was started some years ago. During this study, several methods of neutron spectroscopy were employed and a study of individual and ambient dosemeters was performed.A first spectrometric measurement was done with the IPSN multisphere spectrometer in three positions around the reactor. Secondly, the ROSPEC spectrometer from the Fraunhofer Institut was used. The spectra were also measured with the bubble interactive neutron spectrometer. These measurements were compared with a numerical simulation of the neutron field made with the code TRIPOLI-3. Dosimetric measurements were made with three types of personal neutron dosemeters: an albedo type, a track etch detector and a bubble detector.     

Electronic neutron personal dosimetry with superheated drop detectors

The prototype of an electronic personal neutron dosemeter based on superheated drop detectors is presented. This battery operated device comprises a neutron sensor, bubble-counting electronics and a temperature controller ensuring an optimal dose equivalent response. The neutron sensor is a 12 ml detector vial containing an emulsion of about 50,000 halocarbon-12 droplets of 100 microns diameter. The temperature controller is a low-power, solid-state device stabilising the emulsion at 31.5 degrees C by means of an etched foil heater. The microprocessor controlled counting electronics relies on a double piezo-electric transducer configuration to record bubble formation acoustically via a comparative pulse-shape analysis of ambient noise and detector signals. The performance of the dosemeter was analysed in terms of the requirements presently developed for neutron personal dosemeters. The detection threshold is about 1 microSv, while the personal dose equivalent response to neutrons in the thermal to 62 MeV range falls within a factor 1.6 of 13 bubbles per microSv.     

Evaluation of individual monitoring in mixed neutron/photon fields: mid-term results from the EVIDOS project

EVIDOS is an EC sponsored project that aims at an evaluation and improvement of radiation protection dosimetry in mixed neutron/photon fields. This is performed through spectrometric and dosimetric investigations during different measurement campaigns in representative workplaces of the nuclear industry. The performance of routine and, in particular, novel personal dosemeters and survey instruments is tested in selected workplace fields. Reference values for the dose equivalent quantities, H(*)(10) and H(p)(10) and the effective dose E, are determined using different spectrometers that provide the energy distribution of the neutron fluence and using newly developed devices that determine the energy and directional distribution of the neutron fluence. The EVIDOS project has passed the mid-term, and three measurement campaigns have been performed. This paper will give an overview and some new results from the third campaign that was held in Mol (Belgium), around the research reactor VENUS and in the MOX producing plant of Belgonucléaire.     

Comparison of neutron dose quantities and instrument and dosemeter readings at representative locations in an MOX fuel fabrication plant

The relationships between operational and protection quantities, and values of personal dosemeter and instrument readings have been determined for a recently designed MOX fuel fabrication plant. The relationships between the quantities, and the readings of personal dosemeters are sensitive to both the energy and direction distribution of neutron fluence. The energy distributions were calculated using the Monte Carlo code MCBEND. The direction distribution was addressed by calculating independently, spectral components for which the direction distribution could be reasonably assumed. At representative locations, and for assumed worker orientations, the radiation field is analysed as having, in general, three components—a direct, unidirectional component from the nearest identified discrete source, which is considered incident A-P, several unidirectional components from other such sources which are treated as a rotational component and a scattered isotropic component. The calculated spectra were folded with conversion coefficients for personal dose equivalent, H_p(10)_slab (A-P, ROT and ISO), effective dose, E, (A-P, ROT and ISO), ambient dose equivalent, H^*(10), personal dosemeter (AP, ROT and ISO) and survey instrument response characteristics.     

Measured and calculated angular responses of panasonic UD-809 thermoluminescence dosemeters to neutrons

Multi-element thermoluminescence dosemeters (TLD), such as the Panasonic UD-809, are used in personal dosimetry. The Panasonic UD-809 dosemeter consists of one gamma sensitive and three neutron sensitive TLD elements with different filter materials. In this work, the neutron energy responses (the number of (n,alpha) reactions per neutron) of the neutron-sensitive TLD elements of the Panasonic UD-809 dosemeter were calculated using the MCNP Monte Carlo transport code. Experiments were performed in a calibration geometry with an unmoderated 252Cf neutron source. These measurements were made with the dosemeter placed on the centre front face of a polymethylmethacrylate (PMMA) slab phantom. The phantom was rotated in the horizontal plane from -90 to +90 degrees, in 15 degree increments. Good agreement between calculated and measured element responses was observed. The angular dependency of personal dose equivalent was also calculated for parallel beams of 252Cf neutrons and compared to the TLD element angular responses.     

Response of Harshaw neutron thermoluminescence dosemeters in terms of the revised ICRP/ICRU recommendations

To monitor workers for external neutron radiation dose, the Y-12 National Security Complex utilises the thermoluminescence dosemeters (TLDs) manufactured by Harshaw. At Y-12, the majority of external dose to workers is due to low-energy photon and/or beta particles emitted from uranium and its progeny. However, some neutron dose is expected since neutrons are produced from (alpha,n) reactions in various compounds found at the plant, including UF4 and UF6. Neutron sources, such as 252Cf, are also used throughout the complex. The Harshaw neutron dosemeter consists of two gamma-sensitive elements (7Li) and two neutron-sensitive elements enriched in 6Li with various shielding/filter materials placed around each of them. In this work, the energy response of the dosemeter to neutrons has been calculated using the Monte Carlo transport code MCNP Version 4-C and, these results are compared with the measured response of the dosemeter to unmoderated and D2O-moderated 252Cf neutrons. The response of the dosemeter has also been determined in terms of the personal absorbed dose and personal dose equivalent as a function of neutron energy based on the recommendations of the ICRP Publication 60 and ICRU Report 49. The energy response of the dosemeter characteristics can be used to generate spectral conversion coefficients for routine neutron absorbed dose and dose equivalent calculations.     

Evaluation of two personal dosemeters in polyenergetic mono- and multi-directional neutron fields

The neutron dose-equivalent response of two commercially available electronic personal neutron dosemeters was studied in several laboratory-produced broad-spectrum neutron fields. Fluence-weighted mean energies ranged from 200 keV to 4 MeV; personal dose-equivalent rates ranged from 75 to 10 mSv h(-1); and angles of incidence were multidirectional, 0 degrees, 30 degrees and 60 degrees. Three of these fields have been shown previously to resemble ones found in CANDU (Canadian Deuterium Uranium is a registered trademark of the Atomic Energy of Canada Limited) power plant workplaces. Both dosemeters were found to perform reasonably well across the range of energy spectra and angles of incidence. One type of dosemeter displayed values of the personal dose equivalent that were, at worst, within a factor of approximately 2 of the reference values and, at best, within a few per cent of the reference values. The other type displayed values of the personal dose equivalent that were consistently within unity and 20% of the reference values. Although the radiological performance of one was found to be more accurate, this device was also found to be the less rugged of the two. Some of the data acquired in this work were compared with results previously published by others. There was consistency between these sets of data.