Bandgap-assisted surface-plasmon sensing

Surface-plasmon resonance (SPR) is a sensing technique widely used for its label-free feature. However, its sensitivity is contingent on the divergence angle of the excitation beam. The problem becomes pronounced for compact systems when a low-cost LED is used as the light source. When the Kretschmann configuration with a periodically modulated surface is used, a bandgap appears in the surface plasmon dispersion relation. We recognize that the high density of modes on the edge of the surface-plasmon bandgap permits the coupling of a wider range of incidence angles of excitation photons to surface-plasmon polaritons than what is possible in the traditional Kretschmann configuration. Here, the numerical simulation illustrates that the sensitivity, detection limit, and reflectivity minimum of an amplitude-based SPR bandgap-assisted surface-plasmon sensor are almost independent of the divergence angle. Two different bandgap structures are compared with the Kretschmann configuration using the rigorous coupled-wave analysis technique. The results indicate that the bandgap-assisted sensing outperforms traditional SPR sensing when the angular standard deviation of the excitation beam is above 1 degree.     

Excitation of propagating surface plasmons with a scanning tunnelling microscope

Inelastic electron tunnelling excitation of propagating surface plasmon polaritons (SPPs) on a thin gold film is demonstrated. This is done by combining a scanning tunnelling microscope (STM) with an inverted optical microscope. Analysis of the leakage radiation in both the image and Fourier planes unambiguously shows that the majority (up to 99.5%) of the detected photons originate from propagating SPPs with propagation lengths of the order of 10 μm. The remaining photon emission is localized under the STM tip and is attributed to a tip-gold film coupled plasmon resonance as evidenced by the bimodal spectral distribution and enhanced emission intensity observed using a silver STM tip for excitation.     

Subwavelength-scale tailoring of surface phonon polaritons by focused ion-beam implantation

Recent advances in optical nanotechnologies by controlling surface plasmon polaritons in metallic nanostructures demonstrate high potential for subwavelength-scale waveguiding of light, data storage, microscopy or biophotonics. Surprisingly, surface phonon polaritons-infrared counterparts to surface plasmon polaritons-have not been widely explored for nanophotonic applications. As they rely on the infrared or terahertz excitation of lattice vibrations in polar crystals they offer totally different material classes for nanophotonic applications, such as semiconductors and insulators. In an initial step towards nanoscale surface phonon photonics we show evidence that the local properties of surface phonon polaritons can be tailored at a subwavelength-scale by focused ion-beam modification of the crystal structure, even without significant alteration of the surface topography. Such single-step-fabricated, monolithic structures could be used for controlling electromagnetic energy transport by surface phonon polaritons in miniaturized integrated devices operating at infrared or terahertz frequencies. We verify the polaritonic properties of an ion-beam-patterned SiC surface by infrared near-field microscopy. The near-field images also demonstrate nanometre-scale resolved infrared mapping of crystal quality useful in semiconductor processing or crystal growth.     

A surface plasmon study of the optical dielectric function of indium

Abstract

The optical dielectric function of indium is measured by optical excitation of surface plasmon polaritons on an indium-coated silica grating for a range of wavelengths in the visible region of the spectrum. By exciting the surface plasmon polariton at the buried indium-grating interface, the indium surface that supports the surface plasmon polariton is kept free from oxidation. Comparison of angle-dependent reflectivities with a grating modelling theory gives both the real and imaginary parts of the dielectric function of indium. These results are compared with free-electron models to obtain an estimate of the plasma frequency and relaxation time.     

Grating-coupling of surface plasmons onto metallic tips: a nanoconfined light source

We describe and demonstrate a new nanometer-scale broadband light source. It is based on the grating-coupled excitation of surface plasmon polaritons (SPPs) on the shaft of a sharp conical metal taper with a tip radius of few tens of nanometers. Far-field excitation of linear nanoslit gratings results in the resonant generation of SPPs traveling over more than 10 mum to the tip apex and converging to an intense radiative local light spot. Such nanofabricated tips are expected to find various applications in nanospectroscopy, overcoming problems with background illumination in apertureless microscopy.     

Launching propagating surface plasmon polaritons by a single carbon nanotube dipolar emitter

We report on the excitation of propagating surface plasmon polaritons in thin metal films by a single emitter. Upon excitation in the visible regime, individual semiconducting single-walled carbon nanotubes are shown to act as directional near-infrared point dipole sources launching propagating surface plasmons mainly along the direction of the nanotube axis. Plasmon excitation and propagation is monitored in Fourier and real space by leakage radiation microscopy and is modeled by rigorous theoretical calculations. Coupling to plasmons almost completely reshapes the emission of nanotubes both spatially and with respect to polarization as compared to photoluminescence on a dielectric substrate.     

Generation of traveling surface plasmon waves by free-electron impact

The injection of a beam of free 50 keV electrons into an unstructured gold surface creates a highly localized source of traveling surface plasmons with spectra centered below the surface plasmon resonance frequency. The plasmons were detected by a controlled decoupling into light with a grating at a distance from the excitation point. The dominant contribution to the plasmon generation appears to come from the recombination of d-band holes created by the electron beam excitation.     

Compact antenna for efficient and unidirectional launching and decoupling of surface plasmons

Controlling the launching efficiencies and the directionality of surface plasmon polaritons (SPPs) and their decoupling to freely propagating light is a major goal for the development of plasmonic devices and systems. Here, we report on the design and experimental observation of a highly efficient unidirectional surface plasmon launcher composed of eleven subwavelength grooves, each with a distinct depth and width. Our observations show that, under normal illumination by a focused Gaussian beam, unidirectional SPP launching with an efficiency of at least 52% is achieved experimentally with a compact device of total length smaller than 8 μm. Reciprocally, we report that the same device can efficiently convert SPPs into a highly directive light beam emanating perpendicularly to the sample.     

Adiabatic description of superfocusing of femtosecond plasmon polaritons

A surface plasmon polariton is a collective oscillation of free electrons at a metal–dielectric interface. As wave phenomena, surface plasmon polaritons can be focused with the use of an appropriate excitation geometry of metal structures. In the adiabatic approximation, we demonstrate a possibility to control nanoscale short pulse superfocusing based on generation of a radially polarized surface plasmon polariton mode of a conical metal needle in view of wave reflection. The results of numerical simulations of femtosecond pulse propagation along a nanoneedle are discussed. The space–time evolution of a pulse for the near field strongly depends on a linear chirp of an initial laser pulse, which can partially compensate wave dispersion. The field distribution is calculated for different metals, chirp parameters, cone opening angles and propagation distances. The electric field near a sharp tip is described as a field of a fictitious time-dependent electric dipole located at the tip apex.     

Strong resonant coupling of surface plasmon polaritons to radiation modes through a thin metal slab with dielectric gratings

Strong resonant coupling of surface plasmon polaritons to radiation modes by means of a dielectric grating deposited on top of a metal slab is numerically analyzed, and some novel properties of this configuration are discussed. The dielectric grating is not only responsible for coupling of incident light to surface plasmon polaritons but also for outcoupling of the surface plasmon polaritons to radiation modes. A key advantage of the configuration presented is that it is not based on conventional attenuated total reflection using a prism with high refractive index.     

Controlling surface plasmon polaritons in transformed coordinates

Transformational optics allows for a markedly enhanced control of the electromagnetic wave trajectories within metamaterials, with interesting applications ranging from perfect lenses to invisibility cloaks, carpets, concentrators and rotators. Here we present a review of curved anisotropic heterogeneous meta-surfaces designed using the tool of transformational plasmonics, in order to achieve a similar control for surface plasmon polaritons in cylindrical and conical carpets (for the latter we provide some analytical insight), as well as cylindrical cloaks, concentrators and rotators of a non-convex cross-section. Finally, we provide an asymptotic form of the geometric potential for surface plasmon polaritons on such surfaces in the limit of a small curvature.     

Plasmonic Luneburg and Eaton lenses

Plasmonics takes advantage of the properties of surface plasmon polaritons, which are localized or propagating quasiparticles in which photons are coupled to the quasi-free electrons in metals. In particular, plasmonic devices can confine light in regions with dimensions that are smaller than the wavelength of the photons in free space, and this makes it possible to match the different length scales associated with photonics and electronics in a single nanoscale device. Broad applications of plasmonics that have been demonstrated to date include biological sensing, sub-diffraction-limit imaging, focusing and lithography and nano-optical circuitry. Plasmonics-based optical elements such as waveguides, lenses, beamsplitters and reflectors have been implemented by structuring metal surfaces or placing dielectric structures on metals to manipulate the two-dimensional surface plasmon waves. However, the abrupt discontinuities in the material properties or geometries of these elements lead to increased scattering of surface plasmon polaritons, which significantly reduces the efficiency of these components. Transformation optics provides an alternative approach to controlling the propagation of light by spatially varying the optical properties of a material. Here, motivated by this approach, we use grey-scale lithography to adiabatically tailor the topology of a dielectric layer adjacent to a metal surface to demonstrate a plasmonic Luneburg lens that can focus surface plasmon polaritons. We also make a plasmonic Eaton lens that can bend surface plasmon polaritons. Because the optical properties are changed gradually rather than abruptly in these lenses, losses due to scattering can be significantly reduced in comparison with previously reported plasmonic elements.     

Electromagnetic enhancement by a periodic array of nanogrooves in a metallic substrate

We present comprehensive investigations of the electromagnetic enhancement by a periodic array of rectangular nanogrooves in a metallic substrate. The impacts of array parameters and of illumination conditions on the enhanced electric-field intensity are explored using fully vectorial methods. The calculations are performed mainly for gold and for the visible and infrared wavelengths. The fully vectorial results are reproduced and explained by a simple Fabry-Perot model. Compared with the case of a single groove, the electric-field enhancement of the groove array is found to be much higher by almost 1 order of magnitude, which is shown to be related to the excitation of surface plasmon polaritons with the aid of the model. Practical considerations of a finite groove number and of a finite groove length are also provided.     

Quantum statistics of surface plasmon polaritons in metallic stripe waveguides

Heralded single surface plasmon polaritons are excited using photons generated via spontaneous parametric down conversion. The mean excitation rates, intensity correlations, and Fock state populations are studied. The observed dependence of the second-order coherence in our experiment is consistent with a linear uncorrelated Markovian environment in the quantum regime. Our results provide important information about the effect of loss for assessing the potential of plasmonic waveguides for future nanophotonic circuitry in the quantum regime.     

Long-distance indirect excitation of nanoplasmonic resonances

In nanoscopic systems, size, geometry, and arrangement are the crucial determinants of the light-matter interaction and resulting nanoparticles excitation. At optical frequencies, one of the most prominent examples is the excitation of localized surface plasmon polaritons, where the electromagnetic radiation is coupled to the confined charge density oscillations. Here, we show that beyond direct near- and far-field excitation, a long-range, indirect mode of particle excitation is available in nanoplasmonic systems. In particular, in amorphous arrays of plasmonic nanodiscs we find strong collective and coherent influence on each particle from its entire active neighborhood. This dependency of the local field response on excitation conditions at distant areas brings exciting possibilities to engineer enhanced electromagnetic fields through controlled, spatially configured illumination.     

A dual-way directional surface-plasmon-polaritons launcher based on asymmetric slanted nanoslits

We theoretically design a device composed of two asymmetric slanted nanoslits to achieve the directionality of surface plasmon polaritons (SPPs). With proper inclination of the two slits, the desirable relative phase delay can be obtained. When the structure is illuminated by normal incident light, the SPPs can be controlled to deflect the specific direction due to light interference. The SPPs can be altered to the opposite direction when the illuminating light is changed inversely. We develop another way to tailor the relative phase delay by choosing the specific effective index for each slanted slit. In order to acquire higher directional excitation efficiency, our designs have been extended to periodic structures with the pairs of slanting slits. The finite element method is carried on to verify our designs. The simulations show that the best proportion of the SPP field intensity along two opposite directions reaches to around 30.     

Optical control of plasmonic Bloch modes on periodic nanostructures

We study and actively control the coherent properties of surface plasmon polaritons (SPPs) optically excited on a nanohole array. Amplitude and phase of the optical excitation are externally controlled via a digital spatial light modulator (SLM) and SPP interference fringe patterns are designed and observed with high contrast. Our interferometric observations reveal SPPs dressed with the Bloch modes of the periodic nanostructure. The momentum associated with these dressed plasmons (DP) is highly dependent on the grating period and fully matches our theoretical predictions. We show that the momentum of DP waves can, in principle, exceed the SPP momentum. Actively controlling DP waves via programmable phase patterns offers the potential for high field confinement applicable in lithography, surface enhanced Raman scattering, and plasmonic structured illumination microscopy.     

Diffraction Grating Characterization Using Multiple-wavelength Excitation of Surface Plasmon Polaritons

Abstract

In this work we have used the optical excitation of surface plasmon polaritons to characterize the profile of a diffraction grating with a large groove-depth-to-pitch ratio at wavelengths spanning the visible spectrum. This provides us with confirmation of the accuracy of the modelling theory used to predict the optical response of a deep grating. In addition it draws attention to a particular wavelength regime which proves sensitive to the higher harmonics of the grating profile.     

Self-reconstruction property of fractional Bessel beams

We study the self-reconstruction property of a fractional Bessel beam (FBB), where the FBB is described in terms of a Bessel beam of a fractional order for both amplitude and azimuthal phase components. The simulation and experimental results show that the FBB can overcome a block of obstacles and regenerate itself after a characteristic distance. As a comparison, the propagation of a Gaussian beam and an integer-order Bessel beam (IBB) through the same obstacles are also studied.     

Vertical plasmonic resonant nanocavities

We demonstrate plasmonic modes in a vertical nanocavity with an air output window at the top surface and Ag reflectors. The resonances of surface plasmon polaritons are investigated using cathodoluminescence spectroscopy. The resonant modes are determined by comparing experiment and theoretical simulations. The plasmon dispersion relation in the vertical nanocavities shows a strong confinement to the electromagnetic field, and the smallest modal volume is only 0.0014 μm(3). Our work provides insights into the development of nanoscale plasmonic vertical cavity surface-emitting lasers.