A model to predict radon exhalation from walls to indoor air based on the exhalation from building material samples

In recognition of the fact that building materials are an important source of indoor radon, second only to soil, surface radon exhalation fluxes have been extensively measured from the samples of these materials. Based on this flux data, several researchers have attempted to predict the inhalation dose attributable to radon emitted from walls and ceilings made up of these materials. However, an important aspect not considered in this methodology is the enhancement of the radon flux from the wall or the ceiling constructed using the same building material. This enhancement occurs mainly because of the change in the radon diffusion process from the former to the latter configuration. To predict the true radon flux from the wall based on the flux data of building material samples, we now propose a semi-empirical model involving radon diffusion length and the physical dimensions of the samples as well as wall thickness as other input parameters. This model has been established by statistically fitting the ratio of the solution to radon diffusion equations for the cases of three-dimensional cuboidal shaped building materials (such as brick, concrete block) and one dimensional wall system to a simple mathematical function. The model predictions have been validated against the measurements made at a new construction site. This model provides an alternative tool (substitute to conventional 1-D model) to estimate radon flux from a wall without relying on ²²⁶Ra content, radon emanation factor and bulk density of the samples. Moreover, it may be very useful in the context of developing building codes for radon regulation in new buildings.     

Large-scale radon hazard evaluation in the Oslofjord region of Norway utilizing indoor radon concentrations, airborne gamma ray spectrometry and geological mapping

We test whether airborne gamma ray spectrometer measurements can be used to estimate levels of radon hazard in the Oslofjord region of Norway. We compile 43,000 line kilometres of gamma ray spectrometer data from 8 airborne surveys covering 10,000 km² and compare them with 6326 indoor radon measurements. We find a clear spatial correlation between areas with elevated concentrations of uranium daughters in the near surface of the ground and regions with high incidence of elevated radon concentrations in dwellings. This correlation permits cautious use of the airborne data in radon hazard evaluation where direct measurements of indoor radon concentrations are few or absent. In radon hazard evaluation there is a natural synergy between the mapping of radon in indoor air, bedrock and drift geology mapping and airborne gamma ray surveying. We produce radon hazard forecast maps for the Oslofjord region based on a spatial union of hazard indicators from all four of these data sources. Indication of elevated radon hazard in any one of the data sets leads to the classification of a region as having an elevated radon hazard potential. This approach is inclusive in nature and we find that the majority of actual radon hazards lie in the assumed elevated risk regions.     

Radon in indoor air of primary schools: a systematic survey to evaluate factors affecting radon concentration levels and their variability

In order to optimize the design of a national survey aimed to evaluate radon exposure of children in schools in Serbia, a pilot study was carried out in all the 334 primary schools of 13 municipalities of Southern Serbia. Based on data from passive measurements, rooms with annual radon concentration >300 Bq/m³ were found in 5% of schools. The mean annual radon concentration weighted with the number of pupils is 73 Bq/m³, 39% lower than the unweighted 119 Bq/m³ average concentration. The actual average concentration when children are in classrooms could be substantially lower. Variability between schools (CV = 65%), between floors (CV = 24%) and between rooms at the same floor (CV = 21%) was analyzed. The impact of school location, floor, and room usage on radon concentration was also assessed (with similar results) by univariate and multivariate analyses. On average, radon concentration in schools within towns is a factor of 0.60 lower than in villages and at higher floors is a factor of 0.68 lower than ground floor. Results can be useful for other countries with similar soil and building characteristics.     

Radon Risk Mapping using Indoor Monitoring Data - A Case Study of the Lahti Area,Finland

An empirical statistical model is described for the use of indoor radon monitoring data as an indicator of the areal radon risk from soil and bedrock. The percentages of future homes expected to have radon concentrations exceeding the design level of 200 Bq/m³ unless constructed to provide protection against the entry of radon were assessed. The radon prognosis was made for different subareas, soil types and foundation types. This kind of report is used by the health and building authorities. In this study, 2689 indoor radon measurements were made in one of Finland's most radon-prone areas, consisting of eleven municipalities with a total area of 4600 km² and a population of 186,000. Radon concentrations were seasonally adjusted. Data on the location, geology and construction of buildings were determined from maps and questionnaires. The measurements covered different kinds of geological units in the area. The radon risk is highest in the gravel-dominated subarea in an ice-marginal formation and lowest in the northern half of the area in buildings constructed on bedrock. In these two areas, the design level of 200 Bq/m³ would be exceeded in 99% and 39% of new houses with slab-on-grade.     

Coping with radon problem in a private house

In one of the 50 houses in which, during a national radon survey of 1000 homes in Slovenia, indoor radon concentrations exceeded 1000 Bq m⁻³, radon was further investigated. Except in the attic, elevated radon concentrations were found everywhere in the home, ranging from 0.5 to 12 kBq m⁻³. Applying ICRP 65 methodology, an annual effective dose in the range from 9 to 35 mSv was estimated for an inhabitant for different exposure scenarios. The radon problem was successfully mitigated and radon concentration reduced below 200 Bq m⁻³.     

Spatial indoor radon distribution in Mexico City

We present a spatial analysis of residential radon concentrations in the Mexico City Metropolitan Area, which we intend to use to assign radon exposure in an ongoing case-control study. As part of a probabilistic household survey, carried out between May and June 1999, 501 dwellings were selected for indoor placement of solid state nuclear track detectors (LR 115) in a cup array over a period of approximately 90 days. As part of the sampling design, the city was grid partitioned into nine zones and a sample of dwellings was selected in each zone. All zones were simultaneously surveyed. The stratified sampling design allowed us to obtain radon geometric means, adjusted for household characteristics, week of detector placement and number of days of measurement for these zones. Additionally, adjusted geometric means were estimated for the 100 census tracts surveyed and this information was used to obtain a more detailed spatial distribution of residential radon levels through kriging interpolation and surface contouring. Radon levels depended on the room of placement, the floor level and the ventilation habits but not on building materials. Regarding the city zone, the highest adjusted geometric mean was found in the southwest (136 Bqm(-3)), where 46% of the households had an estimated radon level in excess of 200 Bqm(-3). In the rest of the city, the geometric mean concentration ranged between 41 and 98 Bqm(-3). A more detailed spatial distribution showed that, in general, most of the eastern and middle zones of the city had estimated radon geometric means below 74 Bqm(-3), while the western ones had geometric means above this concentration. Very high geometric means, exceeding 111 Bqm(-3) and even reaching 288 Bqm(-3), are estimated for some areas located in the southern and western zones of Mexico City. The obtained spatial distribution shows that the areas with very high estimated residential radon concentrations are close to inactive volcanic mountains. We believe that the geo-statistical techniques, we have used, offer reasonably good estimates of the average spatial residential radon distribution in Mexico City under average ventilation in homes. The use of this indirect approach for radon exposure measurement in epidemiological studies is an inexpensive alternative to direct radon exposure measurement but may be subject to non-differential misclassification error. The effect of such error on the detection of a real increase in lung cancer risk from indoor radon remains to be determined.     

Status of the indoor air chemical pollution in Japanese houses based on the nationwide field survey from 2000 to 2005

This paper describes the present state and the changes in indoor air pollution levels by Volatile Organic Compounds (VOCs) in houses in Japan, as revealed through measurements of indoor VOC concentrations and investigations on the actual conditions in the residential environment by means of a questionnaire survey covering a total of more than 10,000 newly built houses over six years (from 2000 to 2005). The VOCs initially measured were formaldehyde, toluene, xylene, and ethylbenzene, followed by the subsequent inclusion of styrene and acetaldehyde.     

Characterization of indoor air quality in primary schools in Antwerp, Belgium

The indoor air quality of 27 primary schools located in the city centre and suburbs of Antwerp, Belgium, was assessed. The primary aim was to obtain correlations between the various pollutant levels. Indoor:outdoor ratios and the building and classroom characteristics of each school were investigated. This paper presents results on indoor and local outdoor PM2.5 mass concentrations, its elemental composition in terms of K, Ca, Ti, V, Cr, Mn, Fe, Ni, Cu, Zn, Br, Pb, Al, Si, S, and Cl, and its black smoke content. In addition, indoor and local outdoor levels of the gases NO2, SO2, O3, and BTEX (benzene, toluene, ethyl benzene, and xylene isomers) were determined. Black smoke, NO2, SO2 and O3, occurred at indoor:outdoor ratios below unity, indicating their significant outdoor sources. No linear correlation was established between indoor and outdoor levels for PM2.5 mass concentrations and BTEX; their indoor:outdoor ratios exceeded unity except for benzene. Classroom PM2.5 occurred with a different elemental composition than local outdoor PM2.5. The re-suspension of dust because of room occupation is probably the main contributor for the I/O ratios higher than 1 reported for elements typically constituting dust particles. Finally, increased benzene concentrations were reported for classrooms located at the lower levels. PRACTICAL IMPLICATIONS: The elevated indoor PM2.5, and BTEX concentrations in primary school classrooms, exceeding the ambient concentrations, raise concerns about possible adverse health effects on susceptible children. This is aggravated by the presence of carpets and in the case of classrooms at lower levels. Analysis of PM2.5's elemental composition indicated a considerable contribution of soil dust to indoor PM2.5 mass. In order to set adequate threshold values and guidelines, detailed information on the health impact of specific PM2.5 composites is needed. The results suggest that local outdoor air concentrations measurements do not provide an accurate estimation of children's personal exposures to the identified air pollutants inside classrooms.     

Determination of radon exhalation from construction materials using VOC emission test chambers

The inhalation of ²²²Rn (radon) decay products is one of the most important reasons for lung cancer after smoking. Stony building materials are an important source of indoor radon. This article describes the determination of the exhalation rate of stony construction materials by the use of commercially available measuring devices in combination with VOC emission test chambers. Five materials – two types of clay brick, clinker brick, light‐weight concrete brick, and honeycomb brick – generally used for wall constructions were used for the experiments. Their contribution to real room concentrations was estimated by applying room model parameters given in ISO 16000‐9, RP 112, and AgBB. This knowledge can be relevant, if for instance indoor radon concentration is limited by law. The test set‐up used here is well suited for application in test laboratories dealing with VOC emission testing.     

Comparison of Northern Ireland radon maps based on indoor radon measurements and geology with maps derived by predictive modelling of airborne radiometric and ground permeability data

Publicly available information about radon potential in Northern Ireland is currently based on indoor radon results averaged over 1-km grid squares, an approach that does not take into account the geological origin of the radon. This study describes a spatially more accurate estimate of the radon potential of Northern Ireland using an integrated radon potential mapping method based on indoor radon measurements and geology that was originally developed for mapping radon potential in England and Wales. A refinement of this method was also investigated using linear regression analysis of a selection of relevant airborne and soil geochemical parameters from the Tellus Project. The most significant independent variables were found to be eU, a parameter derived from airborne gamma spectrometry measurements of radon decay products in the top layer of soil and exposed bedrock, and the permeability of the ground. The radon potential map generated from the Tellus data agrees in many respects with the map based on indoor radon data and geology but there are several areas where radon potential predicted from the airborne radiometric and permeability data is substantially lower. This under-prediction could be caused by the radon concentration being lower in the top 30 cm of the soil than at greater depth, because of the loss of radon from the surface rocks and soils to air.     

Indoor 222Rn in Tennessee Valley Houses: Seasonal,Building, and Geological Factors

A two-season survey of indoor ²²²Rn concentrations was conducted in 226 occupied houses in Roane County, TN, during 1985 and 1986. A similar survey of 86 houses in Madison County, AL, was conducted in 1988 and 1989. Alpha track detectors were placed in each of the houses for three or more months during the winter heating season. Detectors were placed at the same sampling sites during the following cooling season. In this study, comparisons were made between winter and summer sampling times and between building types. For the data from Madison County, additional comparisons were made among regions of the county that differed in geological characteristics, especially the thickness of overburden above the Chattanooga Shale layer a geological stratum that has high concentrations of ²²⁶Ra and is widely found in the southeastern United States. The geometric means of summer and winter measurements in Roane County were 33 and 54 Bq m^?3, respectively. For Madison County, the summer and winter geometric means were 121 and 88 Bq m^?3, respectively. The winter ²²²Rn concentrations for houses in Roane Coutuy exceeded summer ²²²Rn concentrations, as is generally the case for houses in the US. For houses in Madison County, we found the opposite and atypical situation of higher ²²²Rn concentrations in the summertime. ²²²Rn concentrations differed significantly among groups of houses in distinguishable regions of Madison County. Substructure and other building factors had no observable effect on indoor ²²²Rn concentrations found in this study.     

The impact of indoor thermal conditions,system controls and building types on the building energy demand

It is possible to evaluate the energy demand as well as the parameters related to indoor thermal comfort through building energy simulation tools. Since energy demand for heating and cooling is directly affected by the required level of thermal comfort, the investigation of the mutual relationship between thermal comfort and energy demand (and therefore operating costs) is of the foremost importance both to define the benchmarks for energy service contracts and to calibrate the energy labelling according to European Directive 2002/92/CE. The connection between indoor thermal comfort conditions and energy demand for both heating and cooling has been analyzed in this work with reference to a set of validation tests (office buildings) derived from a European draft standard. Once a range of required acceptable indoor operative temperatures had been fixed in accordance with Fanger's theory (e.g. −0.5 < PMV < −0.5), the effective hourly comfort conditions and the energy consumptions were estimated through dynamic simulations. The same approach was then used to quantify the energy demand when the range of acceptable indoor operative temperatures was fixed in accordance with de Dear's adaptive comfort theory.     

Variation in residential radon levels in new Danish homes

Radon‐222 gas arises from the radioactive decay of radium‐226 and has a half‐life of 3.8 days. This gas percolates up through soil into buildings, and if it is not evacuated, there can be much higher exposure levels indoors than outdoors, which is where human exposure occurs. Radon exposure is classified as a human carcinogen, and new Danish homes must be constructed to ensure indoor radon levels below 100 Bq/m³. Our purpose was to assess how well 200 newly constructed single detached homes perform according to building regulations pertaining to radon and identify the association between indoor radon in these homes and municipality, home age, floor area, floor level, basement, and outer wall and roof construction. Median (5–95 percentile) indoor radon levels were 36.8 (9.0–118) Bq/m³, but indoor radon exceeded 100 Bq/m³ in 14 of these new homes. The investigated variables explained nine percent of the variation in indoor radon levels, and although associations were positive, none of these were statistically significant. In this study, radon levels were generally low, but we found that 14 (7%) of the 200 new homes had indoor radon levels over 100 Bq/m³. More work is needed to determine the determinants of indoor radon.     

Modern indoor climate research in Denmark from 1962 to the early 1990s: an eyewitness report

Modern, holistic indoor climate research started with the formation of an interdisciplinary 'Indoor Climate Research Group' in 1962 at the Institute of Hygiene, University of Aarhus, Denmark. After some years, other groups started similar research in Denmark and Sweden, and later - after the First International Indoor Air Symposium in Copenhagen 1978--this research spread to many countries and today it is carried out globally by probably 2000 scientists. This paper recounts the history of Danish indoor climate research, focusing on the three decades from the early 1960s to the founding of the Indoor Air journal in 1991. The aim of this paper is to summarize what was learned in those earlier years and to call to the attention of researchers in this area the need of multidisciplinary research, mingling epidemiological fact-finding field studies with climate chamber studies and laboratory investigations. PRACTICAL IMPLICATIONS: The review may be of interest to indoor climate researchers who want to know more about the early development of research on this multidisciplinary subject, as it emerged in a small country that undertook pioneering studies.     

A test of radon service providers available on the Internet

With the announcement of the Government of Canada's Radon Guideline and increased public awareness of radon risk, more and more Canadians wish to test their homes for radon. Radon service providers available on the Internet have attracted many homeowners' attention. These services provide an easy and less expensive way for homeowners to test radon levels in their homes. However, a question has frequently been asked, 'How reliable are the radon testing services available on the Internet?' To answer this question, we ordered 36 radon testing kits from 10 service providers on the Internet. The test results showed that online radon testing services could collectively meet the performance requirement. However, the quality of a few service providers needs to be improved. PRACTICAL IMPLICATIONS: Indoor radon tests were performed with detectors ordered from 10 service providers available on the Internet. The results showed that online radon testing services could collectively meet the performance requirement. However, the quality of a few service providers needs to be improved.     

Modelling radon progeny concentration variations in thermal spas

Radon and its short-lived progenies (218Po, 214Pb, 214Bi and 214Po) are well known radioactive indoor pollutants identified as the major radiation burden component of the thermal spa users. Monitoring of short-lived progeny concentration is of great importance for short-term dose estimations both for bathers and working personnel. A prediction model of the short-lived progeny concentration variations was developed and applied on published data of the thermal spas of Lesvos Island. The physical procedures involved were modeled in a set of differential equations describing radon progeny concentration variations on the basis of radon measurements. Published daughter data were fitted on model predictions adjusting non-measured parameters, e.g. attachment and deposition rate constants for attached and unattached progenies. Attachment rate constants were estimated between 50 and 200 h-1 while the deposition rate constants between 0.25 and 5 h-1 for attached progenies and 0.5 and 170 h-1 for the unattached ones. In addition, unattached 218Po, 214Pb and 214Bi progenies were found to be shifted forward in respect to radon approximately 0.001 h, 0.05 h and 0.40 h respectively, while attached 218Po, 214Pb and 214Bi progenies 0.05 h, 0.45 h and 0.65 h respectively.     

Wire-mesh capped deposition sensors: novel passive tool for coarse fraction flux estimation of radon thoron progeny in indoor environments

Deposition-based ²²²Rn and ²²⁰Rn progeny sensors act as unique, passive tools for determining the long time-averaged progeny deposition fluxes in the environment. The use of these deposition sensors as progeny concentration monitors was demonstrated in typical indoor environments as conceptually superior alternatives to gas-based indirect monitoring methods. In the present work, the dependency of these deposition monitors on various environmental parameters is minimized by capping the deposition sensor with a suitable wire mesh. These wire-mesh capped deposition sensors measure the coarse fraction deposition flux, which is less dependent on the change in environmental parameters like ventilation rate and turbulence. The calibration of these wire-mesh capped coarse fraction progeny sensors was carried out by laboratory controlled experiments. These sensors were deployed both in indoor and in occupational environments having widely different ventilation rates. The obtained coarse fraction deposition velocities were fairly constant in these environments, which further confirmed that the signal on the wire-mesh capped sensors show the least dependency on the change in environmental parameters. This technique has the potential to serve as a passive particle sizer in the general context of nanoparticles using progeny species as surrogates. On the whole, there exists a strong case for developing a passive system that responds only to coarse fraction for providing alternative tools for dosimetry and environmental fine particle research.     

Geological factors of the Guadalajara landscapes (Central Spain) and their relevance to landscape studies

The landscapes of a territory are the consequence of its history; overlapped geological, vegetable and cultural histories usually exist on a landscape. At the Mediterranean domain, however, a translucent vegetation exists, and its history is closely related to the geologic and cultural histories, because low-technology agricultural uses on a different hardness rock background control vegetation. Thus, in areas like the Guadalajara province, the geologic composition and the human activities can be considered the primary conditions for landscape configuration. Both condition the typologies, distribution and relative importance of the geotic, biotic and anthropogenic components of landscapes. A complex network of interrelations among all them exists but, in the base of which lie the geology of the territory, included relief, because it has a more independent influence since man cannot modify the geologic factors; such as the colour of the rocks, the size and distribution of rock bodies, the palaeogeographic domains and the tectonic structure all which control landscape development and configuration. Moreover, geology influences conditions and even limit, the presence, typologies and development of the biotic and anthropogenic elements. These factors also have a major relevance for environmental management, educational and economic policy, and, in some cases, for environmental impact assessment.     

Radon Indoors: A Risk-based Approach to Health Protection Criteria

A WHO/EURO working group met in Eilat, Israel, from 28 March to 4 April 1993, to assess the significance of risks to health associated with indoor radon, to develop a unified approach to control radon exposure, and to advise on the communication of associated health risks. A summary of the deliberations of this working group and its conclusions and recommendations are presented in this paper.     

Comparison of the performance of fuzzy controllers for the management of the indoor environment

Fuzzy logic control applied in Indoor Environment Management Systems provides a significant advantage in terms of energy conservation and users’ indoor comfort requirements satisfaction compared with the classical control systems. The aim of the present paper is to compare the performance of five fuzzy controllers (fuzzy P, fuzzy PID, fuzzy PI, fuzzy PD and adaptive fuzzy PD) developed in the framework of the BUILTECH (JOE3-CT97-0044) project which is in part funded by the European Commission JOULE Programme. The performance criteria are the response performance and the energy consumption.