Field quantization,photons and non-Hermitean modes

Field quantization in unstable optical systems is treated by expanding the vector potential in terms of non-Hermitean (Fox-Li) modes. We define non-Hermitean modes and their adjoints in both the cavity and external regions and make use of the important bi-orthogonality relationships that exist within each mode set. We employ a standard canonical quantization procedure involving the introduction of generalized coordinates and momenta for the electromagnetic (EM) field. Three-dimensional systems are treated, making use of the paraxial and monochromaticity approximations for the cavity non-Hermitean modes. We show that the quantum EM field is equivalent to a set of quantum harmonic oscillators (QHOs), associated with either the cavity or the external region non-Hermitean modes, and thus confirming the validity of the photon model in unstable optical systems. Unlike in the conventional (Hermitean mode) case, the annihilation and creation operators we define for each QHO are not Hermitean adjoints. It is shown that the quantum Hamiltonian for the EM field is the sum of non-commuting cavity and external region contributions, each of which can be expressed as a sum of independent QHO Hamiltonians for each non-Hermitean mode, except that the external field Hamiltonian also includes a coupling term responsible for external non-Hermitean mode photon exchange processes. The non-commutativity of certain cavity and external region annihilation and creation operators is associated with cavity energy gain and loss processes, and may be described in terms of surface integrals involving cavity and external region non-Hermitean mode functions on the cavity-external region boundary. Using the essential states approach and the rotating wave approximation, our results are applied to the spontaneous decay of a two-level atom inside an unstable cavity. We find that atomic transitions leading to cavity non-Hermitean mode photon absorption are associated with a different coupling constant to that for transitions leading to photon emission, a feature consequent on the use of non-Hermitean mode functions. We show that under certain conditions the spontaneous decay rate is enhanced by the Petermann factor.     

Macroscopic canonical quantization in quantum optics: Properties of quasi mode annihilation and creation operators

Abstract

Macroscopic canonical quantization of the EM field and radiative atom systems occurring in quantum optics experiments involving linear classical optics devices can be carried out via expansion of the vector potential either in terms of true mode functions for the optical device or in terms of approximate or quasi mode functions. The relationship between the true mode and quasi mode annihilation, creation operators is determined and shown to involve a Bogolubov transformation. Analytic properties are also examined and it is found that the annihilation, creation operators times the square root of the angular frequency are analytic functions of the variables specifying the modes.     

Generalized quasi mode theory of macroscopic canonical quantization in cavity quantum electrodynamics and quantum optics. II. Application to reflection and refraction at a dielecric interface

Abstract

The generalization of the quasi mode theory of macroscopic quantization in quantum optics and cavity QED presented in the previous paper, is applied to provide a fully quantum theoretic derivation of the laws of reflection and refraction at a boundary. The quasi mode picture of this process involves the annihilation of a photon travelling in the incident region quasi mode, and the subsequent creation of a photon in either the incident region or transmitted region quasi modes. The derivation of the laws of reflection and refraction is achieved through the dual application of the quasi mode theory and a quantum scattering theory based on the Heisenberg picture. Formal expressions from scattering theory are given for the reflection and transmission coefficients. The behaviour of the intensity for a localized one photon wave packet coming in at time minus infinity from the incident direction is examined and it is shown that at time plus infinity, the light intensity is only significant where the classical laws of reflection and refraction predict. The occurrence of both refraction and reflection is dependent upon the quasi mode theory coupling constants between incident and transmitted region quasi modes being nonzero, and it is seen that the contributions to such coupling constants come from the overlap of the mode functions in the boundary layer region, as might be expected from a microscopic theory.     

Generalized quasi mode theory of macroscopic canonical quantization in cavity quantum electrodynamics and quantum optics I. Theory

Abstract

The quasi mode theory of macroscopic quantization in quantum optics and cavity QED developed by Dalton, Barnett and Knight is generalized. This generalization allows for cases in which two or more quasi permittivities, along with their associated mode functions, are needed to describe the classical optics device. It brings problems such as reflection and refraction at a dielectric boundary, the linear coupler, and the coupling of two optical cavities within the scope of the theory. For the most part, the results that are obtained here are simple generalizations of those obtained in previous work. However the coupling constants, which are of great importance in applications of the theory, are shown to contain significant additional terms which cannot be ‘guessed’ from the simpler forms. The expressions for the coupling constants suggest that the critical factor in determining the strength of coupling between a pair of quasi modes is their degree of spatial overlap. In an accompanying paper a fully quantum theoretic derivation of the laws of reflection and refraction at a boundary is given as an illustration of the generalized theory. The quasi mode picture of this process involves the annihilation of a photon travelling in the incident region quasi mode, and the subsequent creation of a photon in either the incident region or transmitted region quasi modes.     

The standard model in cavity quantum electrodynamics. II. Coupling constants and atom field interaction

Abstract

Specific forms of the travelling and trapped vector mode functions for a three-dimensional Fabry-Perot cavity are developed from the general results of the preceding paper, with parameters describing the output cavity mirror chosen for a typical high Q cavity case. Cavity and external quasi-mode functions associated with the quasi-mode theory of macroscopic canonical quantization are then obtained via an idealized choice of output mirror parameters. The coupling constants describing photon exchange processes between the single cavity quasi-mode associated with each Fabry-Perot resonance and various external quasi-modes are calculated, and their slow dependence on the external quasi-mode frequency shows that the conditions for irreversible Markovian damping of the cavity quasi-mode are satisfied. For radiative atoms placed in the cavity the coupling constants for energy exchange processes with sideways travelling external quasi-modes also vary slowely, so that Markovian spontaneous emission damping occurs for the radiative atoms. However, their coupling with the isolated cavity quasi-modes is associated with reversible photon exchanges as represented via one photon Rabi frequencies. The standard model in cavity quantum electrodynamics, in which the basic processes are described by a cavity damping rate, a radiative atom spontaneous decay rate and an atom-cavity mode coupling constant has now been justified in terms of the quasi-mode theory of macroscopic canonical quantization.     

The standard model in cavity quantum electrodynamics. I. General features of mode functions for a Fabry-Perot cavity

Abstract

In the present and the accompanying paper a justification of the standard model of cavity quantum electrodynamics is given in terms of a quasi-mode theory of macroscopic canonical quantization. The coupling of the cavity quasi-mode to external quasi-modes is treated for the representative case of the three-dimensional Fabry-Perot cavity. The general form of the travelling and trapped mode functions for this cavity are derived in this paper and the mode-mode coupling constants are calculated in the accompanying paper. The slow dependence of the coupling constants with the mode frequency difference demonstrates that the conditions for Markovian damping of the cavity quasimode are satisfied. As also discussed in the accompanying paper, the interaction of radiative atoms with cavity quasi-modes is associated with reversible energy exchanges between atom and cavity and represented by Rabi coupling constants. The interaction of radiative atoms located within the cavity with sideways travelling external quasi-modes involves slowly varying coupling constants and is associated with irreversible spontaneous emission dampling. The basic processes represented in the standard cavity quantum electrodynamics model and the associated coupling constant and decay rates thereby follow from the quasi-mode theory.     

Quasimode theory of quantum optical processes in photonic band gap materials

This paper deals with atomic systems coupled to a structured reservoir of quantum EM field modes, with particular relevance to atoms interacting with the field in photonic band gap materials. The case of high Q cavities has been treated elsewhere using Fano diagonalization based on a quasimode approach, showing that the cavity quasimodes are responsible for pseudomodes introduced to treat non-Markovian behaviour. The paper considers a simple model of a photonic band gap case, where the spatially dependent permittivity consists of a constant term plus a small spatially periodic term that leads to a narrow band gap in the spectrum of mode frequencies. Most treatments of photonic band gap materials are based on the true modes, obtained numerically by solving the Helmholtz equation for the actual spatially periodic permittivity. Here the field modes are first treated in terms of a simpler quasimode approach, in which the quasimodes are plane waves associated with the constant permittivity term. Couplings between the quasimodes occur owing to the small periodic term in the permittivity, with selection rules for the coupled modes being related to the reciprocal lattice vectors. This produces a field Hamiltonian in quasimode form. A matrix diagonalization method may be applied to relate true mode annihilation operators to those for quasimodes. The atomic transitions are coupled to all the quasimodes, and the true mode atom-EM field coupling constants (one-photon Rabi frequencies) are related to those for the quasimodes and also expressions are obtained for the true mode density. The results for the one-photon Rabi frequencies differ from those assumed in other work. Expressions for atomic decay rates are obtained using the Fermi Golden rule, although these are valid only well away from the band gaps.     

Determining the state of a single cavity mode from photon statistics

Abstract

We present various schemes for measuring the quantum state of a single mode of the electromagnetic field. These involve measuring the photon statistics for the mode before and after an interaction with either one or two two-level atoms. The photon statistics conditioned on the final state of the atoms, for two choices of the initial set of atomic states, along with the initial photon statistics, may be used to calculate the complete quantum state in a simple manner. Alternatively, when one atom is used, two unconditioned sets of photon statistics, each after interaction with a single atom in different initial states, along with the initial photon statistics may be used to calculate the initial state in a simple manner. When the cavity is allowed to interact with just one atom, only pure cavity states which do not contain zeros in the photon distribution may be reconstructed. When two atoms are used we may reconstruct pure states which do not contain adjacent zeros in the photon distribution. Coherent states and number states are among those that may be measured with one-atom interaction, and squeezed states and ?Schrödinger cats‘ are among those that may be measured with a two-atom interaction.     

Quantum Dynamics of a Hyper-Raman Coupled Model Interacting with Two Quantized Cavity Fields

The quantum dynamics of a hyper-Raman coupled model interacting with two modes of the quantized cavity field is described. The model consists of a four-level atom in a v configuration where transitions between the ground and excited states occur through the absorption (emission) of two photons from one mode and the emission (absorption) of one photon from the other and where two intermediate states are taken to be far off-resonance and are adiabatically removed. This is a multiphoton extension of the Jaynes-Cummings model and is exactly solvable. We study the atomic inversion and investigate the production of non-classical light exhibiting antibunching, violations of the Cauchy-Schwartz inequality, and squeezing.     

Photon coincidence spectroscopy for two-atom cavity quantum electrodynamics

We show that photon coincidence spectroscopy can provide an unambiguous signature of two atoms simultaneously interacting with a quantized cavity field mode. We also show that the single-atom Jaynes—Cummings model can be probed effectively via photon coincidence spectroscopy, even with deleterious contributions to the signal from two-atom events. In addition, we have explicitly solved the eigenvectors and eigenvalues of two two-level atoms coupled to a quantized cavity mode for differing coupling strengths.     

Highly directional emission and photon beaming from nanocrystal quantum dots embedded in metallic nanoslit arrays

We demonstrate a directional beaming of photons emitted from nanocrystal quantum dots that are embedded in a subwavelength metallic nanoslit array with a divergence angle of less than 4°. We show that the eigenmodes of the structure result in localized electromagnetic field enhancements at the Bragg cavity resonances, which could be controlled and engineered in both real and momentum space. The photon beaming is achieved using the enhanced resonant coupling of the quantum dots to these Bragg cavity modes, which dominates the emission properties of the quantum dots. We show that the emission probability of a quantum dot into the narrow angular mode is 20 times larger than the emission probability to all other modes. Engineering nanocrystal quantum dots with subwavelength metallic nanostructures is a promising way for a range of new types of active optical devices, where spatial control of the optical properties of nanoemitters is essential, on both the single and many photons level.     

Influence of Kerr-like medium on the dynamics of a two-mode Raman coupled model

Abstract

We study the quantum dynamics of an effective two-level atom interacting with two modes via Raman process inside an ideal cavity in the presence of Kerr non-linearity. The cavity modes interact both with the atom as well as the Kerr-like medium. The unitary transformation method presented here, not only solves the time-dependent problem, but also provides the eigensolutions of the interacting Hamiltonian at the same time. We study the atomic-population dynamics and the dynamics of the photon statistics in the two cavity modes. The influence of the Kerr-like medium on the statistics of the field is explored and it is observed that Kerr medium introduces antibunching in mode 1 and this effect is enhanced by a stronger interaction with the non-linear medium. In the high non-linear coupling regime anticorrelated beam become correlated. Kerr medium also introduces non-classical correlation between the two modes.     

Ordered systems of site-controlled pyramidal quantum dots incorporated in photonic crystal cavities

The coupling of a prescribed number of site-controlled pyramidal quantum dots (QDs) with photonic crystal (PhC) cavities was studied by polarization and power-dependent photoluminescence measurements. The energy of the cavity mode could be readily tuned, making use of the high spectral uniformity of the QDs and designing PhC cavities with different hole radii. Efficient coupling of the PhC cavity modes both to the ground state and to the excited state transitions of the QDs was observed, whereas no evidence for far off-resonant coupling was found.     

Spontaneous and Induced Atomic Decay in Photonic Band Structures

Abstract

We present a comprehensive quantum electrodynamical analysis of the interaction between a continuum with photonic band gaps (PBGs) or frequency cut-off and an excited two-level atom, which can be either ‘bare’ or ‘dressed’ by coupling to a near-resonant field mode. A diversity of novel features in the atom and field dynamics is shown to arise from the non-Markovian character of radiative decay into such a continuum of modes. Firstly the excited atom is shown to evolve, by spontaneous decay, into a superposition of non-decaying single-photon dressed states, each having an energy in a different PBG, and a decaying component. This superposition is determined by the atomic resonance shift, induced by the spontaneously emitted photon, into or out of a PBG. The main novel feature exhibited by the decaying excited-state component is the occurrence of beats between the shifted atomic resonance frequency and the PBG cut-off frequencies, corresponding to a non-Lorentzian emission spectrum. Secondly the induced decay of a resonantly driven atom into such a continuum exhibits a cascade of transitions down the ladder of dressed states, which are labelled by decreasing photon numbers of the driving mode. Remarkably, this cascade is terminated at the dressed-state doublet, from which all subsequent transitions to lower doublets are forbidden because they fall within the PBG. This doublet then becomes an attractor state for the populations of higher-lying doublets. As a result, the photon-number distribution of the driving mode becomes strongly sub-Poissonian.     

Retrodiction as a tool for micromaser field measurements

We use retrodictive quantum theory to describe cavity field measurements by successive atomic detections in the micromaser. We calculate the state of the micromaser cavity field prior to detection of sequences of atoms in either the excited or ground state, for atoms that are initially prepared in the excited state. This provides the POM elements, which describe such sequences of measurements.     

Field-dipole orientation mechanism and higher order modes in atom guides

Abstract

In cavity quantum electrodynamics (CQED), cavity size, dipole position and dipole orientation are the main factors controlling cavity effects, for example, suppression and enhancement of spontaneous emission. However, the dynamical effects of dipole orientation in CQED have, to date, remained largely unexplored, with most treatments simply concentrating on two (or three) orthogonal directions to illustrate the variations of CQED effects with dipole orientation. No mechanism which determines the evolution of the dipole orientation has been put forward to describe typical situations where atoms move in the field of an excited cavity mode. We emphasize here that in the presence of a cavity mode, the average dipole orientation is automatically determined at every point to be parallel to the direction of the electric field vector of the cavity mode. Besides giving rise to a single value for the spontaneous emission rate, this mechanism is shown to have important consequences for the dynamics of atoms in atom guides. In particular, it determines the average trapping potential distributions and the average radiation forces which guide the atoms along a cylindrical cavity. The effects of the field-dipole orientation mechanism are illustrated with reference to typical situations involving sodium atoms in sub-micron cylindrical guides. The role of a higher order cavity mode of the cylinder in the dynamics is highlighted in terms of its influence on the rotational and vibrational motions in such guides.     

Implementation of three-qubit Toffoli gates via the Heisenberg XY model in coupled cavities

We propose a distributed quantum architecture (three atoms trapped in three coupled cavities) to construct an asymmetric spin 1/2 Heisenberg XY model. The effective atom–atom coupling is obtained with the cavity modes and the atomic excited states being virtually populated. We then demonstrate that the model can be used for implementing a three-qubit Toffoli gate with high fidelity. The feasibility and effectiveness of our scheme as well as the influences of decoherence effects (the atomic spontaneous emission and the cavity decay) on the gate fidelity are finally discussed. The scheme can be generalized for distributed quantum computation with the Heisenberg XY model.     

Quantum effects in the transient dynamics of a many mode Jaynes-Cummings model

Abstract

Phenomenology and mechanisms of energy exchange, due to induced atomic processes of absorption and emission, are investigated in the evolution of a two-mode Jaynes-Cummings model. One field mode is initially in a highly coherent populated state and the other one is initially empty. The field mode exchanges energy with the atom by two mechanisms, related to very different atomic dynamics, which operate in complementary phases of the system evolution. One mechanism determines the energy exchanges which involve only the populated mode and the atom. The other is responsible for mode-mode photon exchanges and becomes relevant when the first mechanism is quenched. Thus there is no competition between the atomic emission in the empty mode and processes involving the atom and the highly populated mode. Quantum features related to entanglement of atom and field states are discussed. Cooperative effects between the two field modes and their incompatibility with the predictions of neo-classical theory are evidenced.     

A scheme for a conditional quantum phase gate using a bimodal cavity and a ladder-type three-level atom

A scheme is proposed to implement a two-qubit conditional quantum phase gate for the intracavity field using a single ladder-type three-level atom driven by two modes in a high-Q cavity. The quantum information is encoded on the Fock states of a bimodal cavity. The averaged fidelity of the gate can be expected to reach 99.86%.     

Spin-resolved Purcell effect in a quantum dot microcavity system

We demonstrate the spin selective coupling of the exciton state with cavity mode in a single quantum dot (QD)-micropillar cavity system. By tuning an external magnetic field, each spin polarized exciton state can be selectively coupled with the cavity mode due to the Zeeman effect. A significant enhancement of spontaneous emission rate of each spin state is achieved, giving rise to a tunable circular polarization degree from -90% to 93%. A four-level rate equation model is developed, and it agrees well with our experimental data. In addition, the coupling between photon mode and each exciton spin state is also achieved by varying temperature, demonstrating the full manipulation over the spin states in the QD-cavity system. Our results pave the way for the realization of future quantum light sources and the quantum information processing applications.