Generation and propagation of a resonant CARS signal from biomolecules: Application to dipicolinic acid

Abstract

We develop a theoretical approach and perform simulations of coherent anti-Stokes Raman scattering (CARS) with ultrashort laser pulses. The signal is generated by biomolecules having subpicosecond dephasing times, from femtosecond pulses on exact resonance with the molecular transitions. All propagation effects are explicitly accounted for, including pump depletion, Raman amplification, parametric generation and pulse reshaping. Our model predicts that a measurable CARS signal can be generated by the dipicolinic acid biomolecule under realistic conditions.     

Tungsten tri-oxide (WO3) film absorber for generating Q-switched pulses in erbium laser

ABSTRACT

This paper reports a new type of passive saturable absorber (SA) made of transition metal oxide (TMO) embedded in polyvinyl alcohol (PVA). The Tungsten trioxide (WO₃)-PVA SA is placed in an erbium-doped fibre laser cavity to produce Q-switched pulses operating at 1562.82?nm. The pulse laser starts to manifest at the threshold pump power of 40?mW and continues to exist until the maximum pump power of 195?mW. Within that pump power range, its pulse energy, repetition rate and pulse width vary from 98 to 142.85?nJ, 29.86 to 56.7?kHz and 5.032 to 1.85?µs, respectively. The pulse train is stable with a signal to noise ratio of 70?dB. This is the first demonstration of a Q-switched laser using such a SA.     

Pump beam waist-dependent pulse energy generation in Nd:YAG/Cr4+:YAG passively Q-switched microchip laser

Abstract

The incident pump beam waist-dependent pulse energy generation in Nd:YAG/Cr⁴⁺:YAG composite crystal passively Q-switched microchip laser has been investigated experimentally and theoretically by moving the Nd:YAG/Cr⁴⁺:YAG composite crystal along the pump beam direction. Highest pulse energy of 0.4 mJ has been generated when the Nd:YAG/Cr⁴⁺:YAG composite crystal is moved about 6 mm away from the focused pump beam waist. Laser pulses with pulse width of 1.7 ns and peak power of over 235 kW have been achieved. The theoretically calculated effective laser beam area at different positions of Nd:YAG/Cr⁴⁺:YAG composite crystal along the pump beam direction is in good agreement with the experimental results. The highest peak power can be generated by adjusting the pump beam waist incident on the Nd:YAG/Cr⁴⁺:YAG composite crystal to optimize the effective laser beam area in passively Q-switched microchip laser.     

Ti: Sapphire Pumped Femtosecond Optical Parametric Oscillator Exhibiting Soliton Formation

Abstract

The configuration and operation of a singly resonant Ti: sapphire pumped optical parametric oscillator (OPO) based on KTP is discussed. Cavity arrangements with and without dispersion compensation are described and the generation of sub-40 fs transform-limited pulses is highlighted. Evidence for soliton pulse formation in the OPO is presented and good quantitative agreement with existing theory is implied. Results of amplitude and phase noise measurements of the OPO are given and compared with those of the pump laser. Generation of pulses at several visible wavelengths by non-phase-matched processes is also briefly discussed.     

500 Hz ultraviolet dye laser with pulse energy 1.7 mJ and potential for PLIF imaging

ABSTRACT

This paper describes a high-pulse-energy frequency-doubled ultraviolet dye laser operating at a repetition rate of 500?Hz. The pump source is a laser-diode side-pumped Q-switched Nd:YAG laser with a pulse energy of 29?mJ at 532?nm. A master oscillator power amplifier is employed to amplify the output pulse of the dye laser to 8.1?mJ at 566?nm, and by frequency doubling with BBO crystal a pulse energy of 1.7?mJ at 283?nm is achieved with a pulse width of 8?ns. This is more than four times the largest reported pulse energies generated by other fixed-frequency dye lasers when operating at repetition rates of more than 1?kHz. The conversion efficiency and stability of dye laser are discussed, which show the potential for high-speed laser diagnostics in the fields of combustion and turbulent flow detection.     

Generation of carrier-envelope phase-controlled isolated attosecond pulses using chirped femtosecond excitation lasers

ABSTRACT

We present an efficient approach for producing a carrier-envelope phase controlled isolated attosecond pulse by an optimized intense driving laser pulse. High-order harmonics are produced by numerically solving the time-dependent Schrödinger equation for the one-dimensional hydrogen atom in an ultrashort laser pulse. We define an efficient cost function to optimize the laser pulse by a genetic algorithm scheme. Our approach produces single attosecond pulses with desired properties, including the carrier-envelope phase, central frequency, and duration. Also, we analyze the time–frequency profiles of the attosecond emissions to gain a deeper insight into the underlying physical mechanism.     

Frequency Spectral Measurements of a Pulsed,TE CO2

Abstract

Experimental measurements of the intra-pulse chirp and temporal coherence from a Joule class TE CO₂ laser incorporating LAWS transmitter design features are presented. Digitized quadrature data (I and Q) from our ground-based coherent Doppler lidar system utilizing return signals off a hard target in the telescope far field are processed using fast Fourier transform and pulse pair techniques to obtain laser pulse frequency spectral components (offset frequency and spectral width) and high-resolution (～ 50 ns/sample) frequency chirp profiles. Less than 300 kHz of frequency chirp is observed in the first 3·5 μs of the laser pulse which contains approximately 90% of the pulse energy. Spectral width of the laser pulse, including both chirp and transform limited components, are measured to be less than 300 kHz full width at half maximum.     

Femtosecond laser pulse propagation in a uniaxial crystal

Abstract

The wave equation describing the vector propagation of a femtosecond laser pulse of a few optical cycles in a uniaxial crystal is solved numerically by the method of unidirectional waves. Propagation of the pulse in the direction normal to the optical axis is studied, taking into account both second- and third-order nonlinearities of the crystal. Conversion efficiency as a function of crystal length, pump intensity and pulse duration is studied. As an example, the propagation of femtosecond laser pulse of τ = 10 fs duration at λ = 810 nm in a LiNbO₃ crystal 12 μm thick is studied numerically.     

High Repetition Rate,High Average Power Er:YAG Laser at 2·94 μm

Abstract

A simple kinetic model is presented which describes the temporal behaviour of an Er:YAG laser pulse and predicts c.w. operation. The use of transfer dye to selectively pump the erbium ions, and suitable optimisation of laser cavity parameters has allowed operation up to 40Hz with 4W average power. 10W at 100Hz is predicted.     

MEH-PPV organic material as saturable absorber for Q-switching and mode-locking applications

ABSTRACT

Q-switched and mode-locked pulse generation in Erbium-doped fiber lasers (EDFLs) are demonstrated using Poly [2-methoxy-5-(2-ethylhexyloxy)-1,4-phenylenevinylene] (MEH-PPV) organic semiconductor material as a saturable absorber (SA) for the first time. The MEH-PPV was prepared in the form of a thin film having a modulation depth of 12% and saturation intensity of 40?MW/cm². The SA was placed in a laser cavity to produce a stable Q-switched operating at 1564.0?nm. The maximum repetition rate of 78.62?kHz, minimum pulse width of 3.54?µs and maximum pulse energy of 59.45?nJ were attained at 125.2?mW pump power. On the other hand, by incorporating an additional 100?m long single mode fiber, the mode locked EDFL self-started as the pump power was raised above 125.2?mW. The soliton pulse was obtained due to the enhancement of the nonlinearity in the cavity. The mode-locked laser operated at 1568.5?nm with a fixed repetition rate of 1.859?MHz and pulse width of 2.97?ps.     

Diode-pumped passively mode-locked Nd:GYSGG laser at 1061 nm with periodically poled LiNbO3 nonlinear mirror

ABSTRACT

We report a nonlinear-mirror mode-locked diode-pumped solid-state Nd:GYSGG laser operating at 1061?nm. The nonlinear mirror comprises a periodically poled LiNbO₃(PPLN) crystal and a dichroic mirror. Continuous-wave mode-locked laser with an output power of 450?mw is obtained under a diode pump power of 5.5?W at 808?nm. The repetition rate of the mode-locked laser is 97.1?MHz and the bandwidth of spectral is 1.3?nm. Considering the group velocity mismatch (GVM) of PPLN, we estimate the minimum pulse width is about 9?ps.     

Pulsed Laser Written Diffraction Gratings in Liquid Crystal Polymers

Abstract

In this work the writing of diffraction gratings in liquid crystal polymer films is studied, where the exposure mechanism is thermal and takes the material from an opaque to a transparent state. A pulsed ruby laser is used to write gratings and the evolution of diffraction is monitored using a continuous wave laser. The resulting diffraction efficiency is compared with an analytic theory for a range of laser pulse energies and grating spacings. Results from the comparison are very good, and final efficiencies of around 5% are obtained, which is near the theoretical maximum for the material used.     

Passively Q-switched Nd:YVO4 waveguide laser using graphene as a saturable absorber

We report on passively Q-switched lasers in femtosecond laser written waveguide in Nd:YVO₄ crystal. Using graphene as a saturable absorber, passively Q-switched waveguide laser operations are achieved along both TE and TM polarizations with single modal profiles. Furthermore, all-angle linear light pump was utilized to investigate the thorough information of the polarization effects of the laser, showing that the optimum polarization for laser generation is TE. The maximum average output power is estimated to be 129 mW with 12.2% slope efficiency, corresponding to single-pulse energy of 8.1 nJ, pulse duration of 25.0 ns and repetition rate of 16.3 MHz.     

Laser-diode-pumped passively Q-switched Nd:YVO4 green laser with periodically poled KTP and GaAs saturable absorber

A laser-diode-pumped passively Q-switched Nd:YVO₄ green laser with periodically poled KTP (PPKTP) and GaAs saturable absorber has been realized. The dependences of pulse repetition rate, pulse energy, pulse width and peak power on incident pump power for the generated-green-light pulses are measured. At the maximum incident pump power of 4.1 W, the maximum average output power of 113 mW is obtained, corresponding to an optical conversion efficiency of 2.8%. At the same pump power, stable green laser pulses of duration of 44.6 ns and energy of 0.28 µJ are generated at a repetition rate of 403.4 kHz. The coupling wave rate equations for a passively Q-switched laser are also given and the numerical solutions agree with the experimental results.     

Dynamics of Gain-switched and Mode-locked Semiconductor Lasers

Abstract

The two processes of gain switching and mode-locking in a semiconductor laser are studied within a single theoretical framework. It is shown that the pulse profiles generated for each process are governed by essentially the same equations, and that the difference between the two cases lies merely in the value of a timescale. The results are supported by computer simulations in which the dependence of the system dynamics on parameters such as the bias current, the modulation depth, the modulation frequency, and the level of spontaneous emission is explored.     

Amplification of Picosecond Pulses in Neodymium-doped Single-mode Optical Fibres

Abstract

The picosecond pulses from the output of a fibre-grating pair compressed mode-locked c.w. pumped Nd : YAG laser have been amplified in a neodymium-doped single mode optical fibre using a counter propagating c.w. pump geometry. Gains of up to times ten were measured in a 2·5 m fibre length for input signal energies of up to 0·2 pJ per pulse.     

Influence of heating of the active region in InGaAsP/InP injection lasers on their spectral characteristics

Spectral and spatial characteristics of the output of InGaAsP/InP separate-confinement double heterostructure laser are investigated. The measurements are performed in quasicontinuous and continuous pumping regimes at room temperature. These lasers are shown to be spatially single-mode over the entire working range of currents. The broadening of the longitudinal modes under quasicontinuous pumping is attributed to heating of the active region of the lasers. The pump pulse duration at which heating of the active region of the lasers can be neglected is estimated. Pis’ma Zh. Tekh. Fiz. 25, 88–94 (April 26, 1999)     

The Laser Amplifier with a Stimulated Scattering Mirror

Abstract

A laser scheme with scattered volume employed as a cavity mirror is considered. The laser threshold and the output pulse characteristics are calculated.     

A History of the Photographic Lens

Abstract

We investigate the transient and the steady-state behaviour of the photon statistics of a single-atom laser, consisting of a three-level Λ system, driven by an incoherent external pump field and strongly coupled to a single mode of an optical cavity. For several limiting cases we are able to obtain analytical results. A comparison with standard multi-atom laser theory reveals a surprisingly good agreement down to very small intracavity photon numbers. Under appropriate operating conditions a calculation of the second-order intensity correlation function yields sub-Poissonian statistics as well as strong antibunching induced by the nonlinear dynamics of the atom.     

A generation of 2 μm Q-switched thulium-doped fibre laser based on anatase titanium(IV) oxide film saturable absorber

We demonstrate a Q-switched thulium-doped fibre laser operating at approximately 1935 nm wavelength using anatase titanium(IV) oxide (TiO₂) embedded in polyvinyl alcohol as the passive newly saturable absorber (SA). The film has absorption loss of 3.5 dB and modulation depth of 33%. It is sandwiched between two fibre ferrules in a ring laser cavity to produce self-started pulse train with a repetition rate that is tuned from 30.12 to 36.96 kHz as the 1552-nm pump power is increased from 289 to 485 mW. At maximum pump power, the laser produced a Q-switching pulse train with pulse duration, output power, pulse energy and peak power of 1.91 μs, 11 mW, 0.3 μJ and 146 mW, respectively. These results show that the TiO₂ is a new potential SA material for pulsed laser applications.