Kerr nonlinearity and optical multi-stability in a four-level Y-type atomic system

The nonlinear response to applied fields of a four-level Y-type atomic system is investigated. The effect of laser intensity and quantum interference induced by spontaneous emission on optical bistability, optical multi-stability and Kerr nonlinearity is then discussed. It is found that the threshold of the optical bistability can substantially be reduced by the quantum interference. So, an enhanced Kerr nonlinearity with reduced absorption can be achieved.     

Controllable nonlinear effects in a hybrid optomechanical semiconductor microcavity containing a quantum dot and Kerr medium

We theoretically investigate the nonlinear effects in a hybrid quantum optomechanical system consisting of two optically coupled semiconductor microcavities containing a quantum dot and a Kerr nonlinear substrate.The steady-state behaviour of the mean intracavity optical field demonstrates that the system can be used as an all optical switch. We further investigate the spectrum of small fluctuations in the mechanical displacement of the movable distributed Bragg reflectors and observe that normal mode splitting takes place for high Kerr nonlinearity and pump power. In addition, we have shown that steady state of the system exhibits two possible bipartite entanglements by proper tuning of the system parameters. The entanglement results suggest that the proposed system has the potential to be used in quantum communication platform. Our work demonstrates that the Kerr-nonlinearity can effectively control the optical properties of the hybrid system, which can be used to design efficient optical devices.     

Optical switching and normal mode splitting in hybrid semiconductor microcavity containing quantum well and Kerr medium driven by amplitude-modulated field

ABSTRACT

We theoretically investigate optical bistability/multistability for all optical switching signature in a hybrid semiconductor microcavity system comprising a quantum well and a Kerr nonlinear substrate. The system is essentially two optically coupled microcavities with one of the microcavity being driven by an external amplitude-modulated pump laser. We show that the switching between bistable and multistable behaviour is influenced by the modulated pump laser, Kerr nonlinearity and the optical coupling between the two microcavities. We further investigate the intracavity spectrum of quantum fluctuations which exhibit the well-known normal mode splitting (NMS). The NMS behaviour is also found to be influenced by the system parameters. These results demonstrate that the present hybrid nonlinear system can be used in designing sensitive optical devices.     

Free-space communication through turbulence: a comparison of plane-wave and orbital-angular-momentum encodings

Abstract

Free-space communication allows one to use spatial mode encoding, which is susceptible to the effects of diffraction and turbulence. Here, we discuss the optimum communication modes of a system while taking such effects into account. We construct a free-space communication system that encodes information onto the plane-wave (PW) modes of light. We study the performance of this system in the presence of atmospheric turbulence, and compare it with previous results for a system employing orbital-angular-momentum (OAM) encoding. We are able to show that the PW basis is the preferred basis set for communication through atmospheric turbulence for a system with a large Fresnel number product. This study has important implications for high-dimensional quantum key distribution systems.     

Controllable optical bistability and Fano line shape in a hybrid optomechanical system assisted by kerr medium: possibility of all optical switching

We theoretically analyse the optical and optomechanical nonlinearity present in a hybrid system consisting of a quantum dot(QD) coupled to an optomechanical cavity in the presence of a nonlinear Kerr medium, and show that this hybrid system can be used as an all optical switch. A high degree of control and tunability via the QD-cavity coupling strength, the Kerr and the optomechanical nonlinearity over the bistable behaviour shown by the mean intracavity optical field and the power transmission of the weak probe field can be achieved.The results obtained in this investigation has the potential to be used for designing efficient all-optical switch and high sensitive sensors for use in Telecom systems.     

Hot‐Electron‐Assisted Femtosecond All‐Optical Modulation in Plasmonics

The optical Kerr nonlinearity of plasmonic metals provides enticing prospects for developing reconfigurable and ultracompact all‐optical modulators. In nanostructured metals, the coherent coupling of light energy to plasmon resonances creates a nonequilibrium electron distribution at an elevated electron temperature that gives rise to significant Kerr optical nonlinearities. Although enhanced nonlinear responses of metals facilitate the realization of efficient modulation devices, the intrinsically slow relaxation dynamics of the photoexcited carriers, primarily governed by electron–phonon interactions, impedes ultrafast all‐optical modulation. Here, femtosecond (≈190 fs) all‐optical modulation in plasmonic systems via the activation of relaxation pathways for hot electrons at the interface of metals and electron acceptor materials, following an on‐resonance excitation of subradiant lattice plasmon modes, is demonstrated. Both the relaxation kinetics and the optical nonlinearity can be actively tuned by leveraging the spectral response of the plasmonic design in the linear regime. The findings offer an opportunity to exploit hot‐electron‐induced nonlinearities for design of self‐contained, ultrafast, and low‐power all‐optical modulators based on plasmonic platforms.     

Designed ultrafast optical nonlinearity in a plasmonic nanorod metamaterial enhanced by nonlocality

All-optical signal processing enables modulation and transmission speeds not achievable using electronics alone. However, its practical applications are limited by the inherently weak nonlinear effects that govern photon-photon interactions in conventional materials, particularly at high switching rates. Here, we show that the recently discovered nonlocal optical behaviour of plasmonic nanorod metamaterials enables an enhanced, ultrafast, nonlinear optical response. We observe a large (80%) change of transmission through a subwavelength thick slab of metamaterial subjected to a low control light fluence of 7 mJ cm(-2), with switching frequencies in the terahertz range. We show that both the response time and the nonlinearity can be engineered by appropriate design of the metamaterial nanostructure. The use of nonlocality to enhance the nonlinear optical response of metamaterials, demonstrated here in plasmonic nanorod composites, could lead to ultrafast, low-power all-optical information processing in subwavelength-scale devices.     

Performance enhancement of GaN-based light-emitting diodes by surface plasmon coupling and scattering grating

Using the analysis of the evanescent surface plasmon polariton (SPP) mode at the GaN/Ag interface as basis, we propose a light-emitting diode (LED) structure with a plasmonic Ag nanostructure and sapphire grating to enhance external quantum efficiency. The 2D finite-difference time-domain method is used to study the spectral properties of the hybrid structure and the effects of structural parameters on light emission enhancement. The plasmonic Ag nanostructure couples recombination energy to the SPP modes at the GaN/Ag interface, whereas the sapphire grating scatters photons out of the LED chips with high extraction efficiency. Under optimal parameters, external quantum efficiency enhancement increases to approximately eighteen times the original value at a relatively long wavelength.     

Nonlinear quantum optical computing via measurement

Abstract

We show how the measurement induced model of quantum computation proposed by Raussendorf and Briegel (2001, Phys. Rev. Letts., 86, 5188) can be adapted to a nonlinear optical interaction. This optical implementation requires a Kerr nonlinearity, a single photon source, a single photon detector and fast feed forward. Although nondeterministic optical quantum information proposals such as that suggested by KLM (2001, Nature, 409, 46) do not require a Kerr nonlinearity they do require complex reconfigurable optical networks. The proposal in this paper has the benefit of a single static optical layout with fixed device parameters, where the algorithm is defined by the final measurement procedure.     

Nanoantenna-enhanced gas sensing in a single tailored nanofocus

Metallic nanostructures possess plasmonic resonances that spatially confine light on the nanometre scale. In the ultimate limit of a single nanostructure, the electromagnetic field can be strongly concentrated in a volume of only a few hundred nm(3) or less. This optical nanofocus is ideal for plasmonic sensing. Any object that is brought into this single spot will influence the optical nanostructure resonance with its dielectric properties. Here, we demonstrate antenna-enhanced hydrogen sensing at the single-particle level. We place a single palladium nanoparticle near the tip region of a gold nanoantenna and detect the changing optical properties of the system on hydrogen exposure by dark-field microscopy. Our method avoids any inhomogeneous broadening and statistical effects that would occur in sensors based on nanoparticle ensembles. Our concept paves the road towards the observation of single catalytic processes in nanoreactors and biosensing on the single-molecule level.     

Induced chirality through electromagnetic coupling between chiral molecular layers and plasmonic nanostructures

We report a new approach for creating chiral plasmonic nanomaterials. A previously unconsidered, far-field mechanism is utilized which enables chirality to be conveyed from a surrounding chiral molecular material to a plasmonic resonance of an achiral metallic nanostructure. Our observations break a currently held preconception that optical properties of plasmonic particles can most effectively be manipulated by molecular materials through near-field effects. We show that far-field electromagnetic coupling between a localized plasmon of a nonchiral nanostructure and a surrounding chiral molecular layer can induce plasmonic chirality much more effectively (by a factor of 10(3)) than previously reported near-field phenomena. We gain insight into the mechanism by comparing our experimental results to a simple electromagnetic model which incorporates a plasmonic object coupled with a chiral molecular medium. Our work offers a new direction for the creation of hybrid molecular plasmonic nanomaterials that display significant chiroptical properties in the visible spectral region.     

Quantum correlation in dephasing decay and its effect on interference in three-level systems

The quantum correlation in dephasing decay can be realized, when the energy fluctuations of transition frequencies are synchronized. The correlation in the three-level atom systems will enhance the interference in the absorption and change the nature of the interference, from destructive to constructive in cascade low-driving three-level atom and from constructive to destructive in V-type three-level atom. The quantum correlation is observed by properly introducing the collision or time-dependent magnetic field through the increase or decrease of the resonant absorption.     

Phase control of Kerr nonlinearity in V-type system with spontaneously generated coherence

We study phase control of linear and nonlinear optical responses in a three-level atomic system in V-configuration exhibiting spontaneously generated coherence (SGC). Because of the SGC effect, the strength of Kerr nonlinearity strongly depends upon the relative phase between the probe and control fields as well as the absorptions. By controlling the relative phase appropriately, large Kerr nonlinearity can be achieved with canceled linear and nonlinear absorptions. Combining with the phase modulation, the strict decay condition of spontaneous decay rates is not needed.     

Coherent molecular resonances in quantum dot-metallic nanoparticle systems: coherent self-renormalization and structural effects

It is known that surface-plasmon resonances of metallic nanoparticles can significantly enhance the field experienced by semiconductor quantum dots. In this paper we show that, when quantum dots are in the vicinity of metallic nanoparticles and interact with coherent light sources (laser fields), coherent exciton-plasmon coupling (quantum coherence effects) can increase the amount of the plasmonic field enhancement significantly. We also study how the coherent molecular resonances generated by such a coupling process are influenced by the self-renormalization of the plasmonic fields and the structural parameters of the systems, particularly the size and shape of the metallic nanoparticle. The renormalization process happens via mutual impacts of the radiative decay rate of excitons and the coherent exciton-plasmon coupling on each other. Our results highlight the conditions where the molecular resonances become very sharp, offering optical switching processes with high extinction ratio and wide ranging device applications.     

All-optical control of a single plasmonic nanoantenna-ITO hybrid

We demonstrate experimentally picosecond all-optical control of a single plasmonic nanoantenna embedded in indium tin oxide (ITO). We identify a picosecond response of the antenna-ITO hybrid system, which is distinctly different from transient bleaching observed for gold antennas on a nonconducting SiO(2) substrate. Our experimental results can be explained by the large free-carrier nonlinearity of ITO, which is enhanced by plasmon-induced hot-electron injection from the gold nanoantenna into the conductive oxide. The combination of tunable antenna-ITO hybrids with nanoscale plasmonic energy transfer mechanisms, as demonstrated here, opens a path for new ultrafast devices to produce nanoplasmonic switching and control.     

Evolution of Coherent States in a Dispersionless Fibre with Saturable Nonlinearity and the Generation of Macroscopic Quantum-superposition States

Abstract

We study the evolution of a initially coherent state of an electromagnetic field propagating in a Kerr medium with saturable nonlinearity. By using the quantum phase distribution formalism, we analyse the dependence of the output signal phase configuration upon input field amplitude. We observe that the saturation of the nonlinear contribution of the refractive index of the propagation medium introduces interference effects that compromise the observation of macroscopically well distinguishable components of the output state. For input amplitudes much larger than a characteristic saturation amplitude the final state differs from the input state only by an overall phase shift. Possible relevance of the present results in the experimental search of Schrödinger cat-like states using semiconductor-doped glass optical fibres is discussed.     

Quantum plexcitonics: strongly interacting plasmons and excitons

We present a fully quantum mechanical approach to describe the coupling between plasmons and excitonic systems such as molecules or quantum dots. The formalism relies on Zubarev's Green functions, which allow us to go beyond the perturbative regime within the internal evolution of a plasmonic nanostructure and to fully account for quantum aspects of the optical response and Fano resonances in plasmon-excition (plexcitonic) systems. We illustrate this method with two examples consisting of an exciton-supporting quantum emitter placed either in the vicinity of a single metal nanoparticle or in the gap of a nanoparticle dimer. The optical absorption of the combined emitter-dimer structure is shown to undergo dramatic changes when the emitter excitation level is tuned across the gap-plasmon resonance. Our work opens a new avenue to deal with strongly interacting plasmon-excition hybrid systems.     

Non-Fermi Behavior of the Itinerant-Electron Ferromagnet near the Quantum Phase Transition Point

We used the Renormalization Group (RG) method in the Hertz–Millis version to study the quantum phase transition of the itinerant-electron ferromagnet. Near the quantum phase transition point the system present a non-Fermi behavior in agreement with the experimental results. The importance of long-range interactions considered by Belitz–Kirkpatrick–Vojta was taken into consideration, showing the importance of the marginal parameters.     

Fano-like interference in self-assembled plasmonic quadrumer clusters

Assemblies of strongly interacting metallic nanoparticles are the basis for plasmonic nanostructure engineering. We demonstrate that clusters of four identical spherical particles self-assembled into a close-packed asymmetric quadrumer support strong Fano-like interference. This feature is highly sensitive to the polarization of the incident electric field due to orientation-dependent coupling between particles in the cluster. This structure demonstrates how careful design of self-assembled colloidal systems can lead to the creation of new plasmonic modes and the enabling of interference effects in plasmonic systems.     

Gain without inversion in hybrid quantum dot-metallic nanoparticle systems

We study the generation of tunable gain without inversion in semiconductor quantum dots using plasmonic effects. For this we investigate the impact of localized surface plasmons on coherent nonlinear exciton effects in a quantum dot when it is located in the vicinity of a metallic nanoparticle. It is shown that when such a system is exposed to a laser field and the distance between the quantum dot and the metallic nanoparticle is reduced the initial impact of plasmons is enhancement of the ac-Stark shift in the quantum dot. When this distance is reduced beyond a critical value, the results show abrupt formation of a significant of amount of gain without inversion in the quantum dot. We show that such a 'molecular' gain is associated with the plasmonic metaresonance (PMR) formed via combined effects of laser-induced coherence in the quantum dot and plasmons.