近场光镊与AFM探针复合的光阱力分析

本文针对纳米材料的纳米操作,提出了一种复合激光近场光镊与AFM探针进行纳米操作的方法,并基于动量守恒原理,采用三维时域有限差分方法建立了该方案中激光近场对纳米微粒的作用力模型,分析了各轴向光阱力的分布情况,讨论了两探针间距离、针尖材料的电导率、入射平面光场的偏振方向、入射角和波长等参数对近场光阱力的影响.结果表明:位于...     

同轴纳米柱对亚波长金属牛眼结构EOT的调控

牛眼结构是一种典型的纳米光学结构。本文设计了一种带有同轴纳米柱的牛眼结构,利用时域有限差分法(FDTD)研究了该结构的增强透射效应。研究发现,柱的半径和高度对透射特性具有显著的影响,恰当选择柱的半径和高度会得到最大的透射强度。另外,牛眼结构对环境折射率有较高的灵敏度。理论分析表明,该种结构的透射增强效应是由局域表面等离激元与表面极化等离激元相互作用产生。这为纳米光学元件的研发与应用提供一个新的思路。     

时域有限差分法及其在室内声场模拟中的应用

时域有限差分法将声波基本方程表示为一个时间和空间的迭代方程组,实现对室内声场中低频段的模拟计算。在介绍时域肯限差分法基本原理的基础上,着重探讨采用时域有限差分法模拟室内声场时边界条件的处理方法及该方法在室内声场模拟中的应用。分析了该方法存在的一些问题及其应用前景。     

利用直达波和海面反射波到达时延反演深海声速剖面

研究了利用直达波与海面反射波到达时延反演深海声速剖面的方法,采用最严经验模态方法组织利用历史水文数据并进行反演,并利用 2016年南海中南部冬季调查的实验数据进行了验证。反演结果与实测声速剖面在深度小于 710 m处的平均绝对误差的最大值为 2.15 m·s^-1,反演结果与实测值基本相符。     

Influence of Surfactant Bilayers on the Refractive Index Sensitivity and Catalytic Properties of Anisotropic Gold Nanoparticles

Shape‐controlled synthesis of gold nanoparticles generally involves the use of surfactants, typically cetyltrimethylammonium (CTAX, X = Cl^?, Br^?), to regulate the nucleation growth process and to obtain colloidally stable nanoparticles. The surfactants adsorb on the nanoparticle surface making further functionalization difficult and therefore limit their use in many applications. Herein, the influence of CTAX on nanoparticle sensitivity to local dielectric environment changes is reported. It is shown, both experimentally and theoretically, that the CTAX bilayer significantly reduces the refractive index (RI) sensitivity of anisotropic gold nanoparticles such as nanocubes and concave nanocubes, nanorods, and nanoprisms. The RI sensitivity can be increased by up to 40% by removing the surfactant layer from nanoparticles immobilized on a solid substrate using oxygen plasma treatment. This increase compensates for the otherwise problematic decrease in RI sensitivity caused by the substrate effect. Moreover, the removal of the surfactants both facilitates nanoparticle biofunctionalization and significantly improves their catalytic properties. The strategy presented herein is a simple yet effective universal method for enhancing the RI sensitivity of CTAX‐stabilized gold nanoparticles and increasing their potential as transducers in nanoplasmonic sensors, as well as in catalytic and biomedical applications.