The standard model in cavity quantum electrodynamics. II. Coupling constants and atom field interaction

Abstract

Specific forms of the travelling and trapped vector mode functions for a three-dimensional Fabry-Perot cavity are developed from the general results of the preceding paper, with parameters describing the output cavity mirror chosen for a typical high Q cavity case. Cavity and external quasi-mode functions associated with the quasi-mode theory of macroscopic canonical quantization are then obtained via an idealized choice of output mirror parameters. The coupling constants describing photon exchange processes between the single cavity quasi-mode associated with each Fabry-Perot resonance and various external quasi-modes are calculated, and their slow dependence on the external quasi-mode frequency shows that the conditions for irreversible Markovian damping of the cavity quasi-mode are satisfied. For radiative atoms placed in the cavity the coupling constants for energy exchange processes with sideways travelling external quasi-modes also vary slowely, so that Markovian spontaneous emission damping occurs for the radiative atoms. However, their coupling with the isolated cavity quasi-modes is associated with reversible photon exchanges as represented via one photon Rabi frequencies. The standard model in cavity quantum electrodynamics, in which the basic processes are described by a cavity damping rate, a radiative atom spontaneous decay rate and an atom-cavity mode coupling constant has now been justified in terms of the quasi-mode theory of macroscopic canonical quantization.     

Quasi mode theory of macroscopic canonical quantization in quantum optics and cavity quantum electrodynamics

Abstract

A macroscopic, canonical quantization of the EM field and radiating atom system in quantum optics and cavity QED involving classical, linear optical devices, based on expanding the vector potential in terms of quasi mode functions is presented. The quasi mode functions approximate the true mode functions for the device, and are obtained by solving the Helmholtz equation for an idealized spatially dependent electric permittivity function describing the device. The Hamiltonian for the EM field and radiating atom system is obtained in multipolar form and the quantum EM field is found to be equivalent to a set of quantum harmonic oscillators, one oscillator per quasi mode. However, unlike true mode theory where the quantum harmonic oscillators are uncoupled, in the quasi mode theory they are coupled and photon exchange processes can occur. Explicit expressions for the coupling constants are obtained. The interaction energy between the radiative atoms and the quantum EM field depends on the amplitudes of the quasi mode functions at the positions of the radiating atoms, similar to that for the true mode approach. The simpler forms for the quasi mode functions enable the atom-field interaction energy to be written in a form in which the atoms are only coupled to certain types of modes—for example cavity quasi modes, which are large inside the optical cavity. In such cases the escape of energy from excited atoms in the cavity can be pictured in quasi mode theory as a two step process—the atom de-excites and creates a photon in a cavity quasi mode, the photon in the cavity quasi mode is then lost and appears as a photon in an external quasi mode. In this process the first step occurs via the atom-cavity quasi mode interaction, the second through coupling between cavity and external quasi modes. This may be contrasted with the true mode approach, where the excited atom loses its energy and the photon is created in one of the true modes. As all true modes have non-zero amplitudes outside as well as inside the cavity, the escape of energy from excited atoms in the cavity is seen as a one step process. An application of the quasi mode theory to the quantum theory of the beam splitter is outlined. The unitary operator used to describe this device is a scattering operator, relating initial and long time values of annihilation, creation operators for pairs of incident and reflected modes, interpreted here as quasi modes.     

Generalized quasi mode theory of macroscopic canonical quantization in cavity quantum electrodynamics and quantum optics I. Theory

Abstract

The quasi mode theory of macroscopic quantization in quantum optics and cavity QED developed by Dalton, Barnett and Knight is generalized. This generalization allows for cases in which two or more quasi permittivities, along with their associated mode functions, are needed to describe the classical optics device. It brings problems such as reflection and refraction at a dielectric boundary, the linear coupler, and the coupling of two optical cavities within the scope of the theory. For the most part, the results that are obtained here are simple generalizations of those obtained in previous work. However the coupling constants, which are of great importance in applications of the theory, are shown to contain significant additional terms which cannot be ‘guessed’ from the simpler forms. The expressions for the coupling constants suggest that the critical factor in determining the strength of coupling between a pair of quasi modes is their degree of spatial overlap. In an accompanying paper a fully quantum theoretic derivation of the laws of reflection and refraction at a boundary is given as an illustration of the generalized theory. The quasi mode picture of this process involves the annihilation of a photon travelling in the incident region quasi mode, and the subsequent creation of a photon in either the incident region or transmitted region quasi modes.     

Generalized quasi mode theory of macroscopic canonical quantization in cavity quantum electrodynamics and quantum optics. II. Application to reflection and refraction at a dielecric interface

Abstract

The generalization of the quasi mode theory of macroscopic quantization in quantum optics and cavity QED presented in the previous paper, is applied to provide a fully quantum theoretic derivation of the laws of reflection and refraction at a boundary. The quasi mode picture of this process involves the annihilation of a photon travelling in the incident region quasi mode, and the subsequent creation of a photon in either the incident region or transmitted region quasi modes. The derivation of the laws of reflection and refraction is achieved through the dual application of the quasi mode theory and a quantum scattering theory based on the Heisenberg picture. Formal expressions from scattering theory are given for the reflection and transmission coefficients. The behaviour of the intensity for a localized one photon wave packet coming in at time minus infinity from the incident direction is examined and it is shown that at time plus infinity, the light intensity is only significant where the classical laws of reflection and refraction predict. The occurrence of both refraction and reflection is dependent upon the quasi mode theory coupling constants between incident and transmitted region quasi modes being nonzero, and it is seen that the contributions to such coupling constants come from the overlap of the mode functions in the boundary layer region, as might be expected from a microscopic theory.     

Photon filters in a microwave cavity

Abstract

In an earlier paper we concluded that time-dependent parameters in the atom-mode interaction can be utilized to modify the quantum field in a cavity. When an atom shoots through the cavity field, it is expected to experience a trigonometric time dependence of its coupling constant. We investigate the possibilities this offers to modify the field. As a point of comparison we use the solvable Rosen-Zener model, which has parameter dependences roughly similar to the ones expected in a real cavity. We do confirm that by repeatedly sending atoms through the cavity, we can obtain filters on the photon states. Highly non-classical states can be obtained. We find that the Rosen-Zener model is more sensitive to the detuning than the case of a trigonometric coupling.     

Determining the state of a single cavity mode from photon statistics

Abstract

We present various schemes for measuring the quantum state of a single mode of the electromagnetic field. These involve measuring the photon statistics for the mode before and after an interaction with either one or two two-level atoms. The photon statistics conditioned on the final state of the atoms, for two choices of the initial set of atomic states, along with the initial photon statistics, may be used to calculate the complete quantum state in a simple manner. Alternatively, when one atom is used, two unconditioned sets of photon statistics, each after interaction with a single atom in different initial states, along with the initial photon statistics may be used to calculate the initial state in a simple manner. When the cavity is allowed to interact with just one atom, only pure cavity states which do not contain zeros in the photon distribution may be reconstructed. When two atoms are used we may reconstruct pure states which do not contain adjacent zeros in the photon distribution. Coherent states and number states are among those that may be measured with one-atom interaction, and squeezed states and ?Schrödinger cats‘ are among those that may be measured with a two-atom interaction.     

Controlling decoherence of a two-level atom in a lossy cavity

Abstract

By use of external periodic driving sources, we demonstrate the possibility of controlling the coherent as well as the decoherent dynamics of a two-level atom placed in a lossy cavity. The control of the coherent dynamics is elucidated for the phenomenon of coherent destruction of tunnelling (CDT), i.e. the coherent dynamics of a driven two-level atom in a quantum superposition state can be brought practically to a complete standstill. We study this phenomenon for different initial preparations of the two-level atom. We then proceed to investigate the decoherence originating from the interaction of the two-level atom with a lossy cavity mode. The loss mechanism is described in terms of a microscopic model that couples the cavity mode to a bath of harmonic field modes. A suitably tuned external cw-laser field applied to the two-level atom slows down considerably the decoherence of the atom. We demonstrate the suppression of decoherence for two opposite initial preparations of the atomic state: a quantum superposition state as well as the ground state. These findings can be used to decrease the influence of decoherence in qubit manipulation processes.     

Meeting Report

Abstract

The cooperative dynamics of a microlaser consisting of two threelevel atoms interacting with a pump field and two quantized cavity modes forming a radiative cascade are studied. Adiabatic elimination of one mode leads to a strong dynamical entanglement between the internal states of the atoms which allows us to study the effects of a cavity-mediated dipole-dipole interaction. We show that the coherent dynamics of the two-atom system will preferentially couple symmetrical linear combinations of internal states. If this coupling dominates the dynamics, the two-atom system will behave like a single atom with correspondingly larger dipole moment, that is a superradiant two-atom system. Even very small spontaneous decay causes transitions from symmetrical to antisymmetrical states and conversely. The hopping between two subsets of the state space can give rise to intriguing phenomena such as bistability of the laser mode intensity. By a randomization of the two coupling phases we recover the standard independent-atom laser theory.     

Field-dipole orientation mechanism and higher order modes in atom guides

Abstract

In cavity quantum electrodynamics (CQED), cavity size, dipole position and dipole orientation are the main factors controlling cavity effects, for example, suppression and enhancement of spontaneous emission. However, the dynamical effects of dipole orientation in CQED have, to date, remained largely unexplored, with most treatments simply concentrating on two (or three) orthogonal directions to illustrate the variations of CQED effects with dipole orientation. No mechanism which determines the evolution of the dipole orientation has been put forward to describe typical situations where atoms move in the field of an excited cavity mode. We emphasize here that in the presence of a cavity mode, the average dipole orientation is automatically determined at every point to be parallel to the direction of the electric field vector of the cavity mode. Besides giving rise to a single value for the spontaneous emission rate, this mechanism is shown to have important consequences for the dynamics of atoms in atom guides. In particular, it determines the average trapping potential distributions and the average radiation forces which guide the atoms along a cylindrical cavity. The effects of the field-dipole orientation mechanism are illustrated with reference to typical situations involving sodium atoms in sub-micron cylindrical guides. The role of a higher order cavity mode of the cylinder in the dynamics is highlighted in terms of its influence on the rotational and vibrational motions in such guides.     

The non-degenerate optical parametric oscillator in the strong-coupling regime

Abstract

A fully quantum treatment of the non-degenerate optical parametric oscillator in the extreme quantum limit of small photon numbers and very high nonlinear coupling strength is presented. When the nonlinear coupling constant becomes comparable with the cavity decay rate, the sharp threshold that is usually encountered disappears, a situation reminiscent of microlasers. Furthermore the output light exhibits unusual statistical properties such as strong super-Poissonian behaviour of the pump mode for (very) large coupling constants.     

Two-level atom and multichromatic waves in a lossless cavity

Abstract

In this paper, we shall examine a generalized version of the Jaynes-Cummings model in which a two-level atom moves in a lossless cavity and is coupled to multichromatic waves with general frequencies and coupling constants. We shall show that both the motion of the atom and the photon conversion between multichromatic waves are dynamically correlated. Using the semiclassical approximations introduced in a previous paper, we obtain the equations which describe the dynamics of this quantum system and discuss the solutions in several special cases. In particular, we point out that the motion of the atom may be controlled by the electromagnetic modes, and vice versa, that is the amplitudes and phases of the electromagnetic fields in the cavity may also be determined by the position of the atom.     

On the possibility of preparing decoherence-free states in a cavity

The effect of decoherence in a quantum system can be viewed as a consequence of the interaction with the environment. As has been pointed out first by Dicke, in a system of N two-level atoms where each of the atoms is individually dipole coupled to the environment, there are collective subradiant states that have no dipole coupling to photon modes, and therefore they are expected to decay more slowly. We have recently proposed a scheme which is intended to create such states in a detuned cavity. We shall examine here the conditions under which our scheme can be used and compare them with the experimental possibilities. The analysis shows that our proposal can be implemented with present-day techniques achieved in atom—cavity interaction experiments.     

Entanglement-induced population trapping by Schrödinger's cat

Abstract

We propose an experiment that is a variation of the Schrödinger's cat ′paradox' wherein the entanglement between a microscopic system and a macroscopic system is of primary interest. The experiment involves tunable entanglement and serves as a model for controllable decoherence in the context of cavity quantum electrodynamics where atoms interact dispersively with a cavity field initially in a coherent state. The interaction produces an entanglement between the atom and the field, and the degree of entanglement can be probed by subjecting the atom to resonant classical radiation after it leaves the cavity. The amplitude of the resulting Rabi oscillations reflects the degree of the entanglement, there being no Rabi oscillations when the entanglement is maximum. We show that the cavity damping does not affect the experiment.     

Quantum non-demolition measurements using cold atoms in an optical cavity

Abstract

In this paper we present a theoretical analysis of a recent quantum non-demolition experiment in optics using cold atoms in a magneto-optical trap as a nonlinear medium. A signal beam and a meter beam from two independent lasers are coupled within a A-type three-level scheme in the D1 line of ⁸⁷Rb atoms. The experimental results for the relevant quantum correlations of the fields represent up to now the best achievement for a single back-action evading measurement. Moreover, they are found to be in remarkably good agreement with the theoretical predictions from a fully quantum model for three-level atoms in a doubly resonant cavity.     

Probing the radiative transition of single molecules with a tunable microresonator

Using a tunable optical microresonator with subwavelength spacing, we demonstrate controlled modulation of the radiative transition rate of a single molecule, which is measured by monitoring its fluorescence lifetime. Variation of the cavity length changes the local mode structure of the electromagnetic field, which modifies the radiative coupling of an emitting molecule to that field. By comparing the experimental data with a theoretical model, we extract both the pure radiative transition rate as well as the quantum yield of individual molecules. We observe a broad scattering of quantum yield values from molecule to molecule, which reflects the strong variation of the local interaction of the observed molecules with their host environment.     

Field quantization,photons and non-Hermitean modes

Field quantization in unstable optical systems is treated by expanding the vector potential in terms of non-Hermitean (Fox-Li) modes. We define non-Hermitean modes and their adjoints in both the cavity and external regions and make use of the important bi-orthogonality relationships that exist within each mode set. We employ a standard canonical quantization procedure involving the introduction of generalized coordinates and momenta for the electromagnetic (EM) field. Three-dimensional systems are treated, making use of the paraxial and monochromaticity approximations for the cavity non-Hermitean modes. We show that the quantum EM field is equivalent to a set of quantum harmonic oscillators (QHOs), associated with either the cavity or the external region non-Hermitean modes, and thus confirming the validity of the photon model in unstable optical systems. Unlike in the conventional (Hermitean mode) case, the annihilation and creation operators we define for each QHO are not Hermitean adjoints. It is shown that the quantum Hamiltonian for the EM field is the sum of non-commuting cavity and external region contributions, each of which can be expressed as a sum of independent QHO Hamiltonians for each non-Hermitean mode, except that the external field Hamiltonian also includes a coupling term responsible for external non-Hermitean mode photon exchange processes. The non-commutativity of certain cavity and external region annihilation and creation operators is associated with cavity energy gain and loss processes, and may be described in terms of surface integrals involving cavity and external region non-Hermitean mode functions on the cavity-external region boundary. Using the essential states approach and the rotating wave approximation, our results are applied to the spontaneous decay of a two-level atom inside an unstable cavity. We find that atomic transitions leading to cavity non-Hermitean mode photon absorption are associated with a different coupling constant to that for transitions leading to photon emission, a feature consequent on the use of non-Hermitean mode functions. We show that under certain conditions the spontaneous decay rate is enhanced by the Petermann factor.     

Generation of photon number states on demand

Abstract

Experiments with single atoms have become routine. In this paper two groups of these experiments will be reviewed with special emphasis on applications to study quantum phenomena in the atom-radiation interaction. The first one deals with the one-atom maser and the second one with another cavity quantum electrodynamic device on the basis of trapped ions. The latter device has interesting applications in quantum computing and quantum information.     

Simple quantum information algorithms in cavity QED

Abstract

Cavity quantum electrodynamics has already proven to be a system capable of demonstrating basic tools in quantum information theory. By combining these tools, we show how simple quantum information protocols could be implemented. We will focus on the examples of the Grover search algorithm and quantum cloning.     

Photon coincidence spectroscopy for two-atom cavity quantum electrodynamics

We show that photon coincidence spectroscopy can provide an unambiguous signature of two atoms simultaneously interacting with a quantized cavity field mode. We also show that the single-atom Jaynes—Cummings model can be probed effectively via photon coincidence spectroscopy, even with deleterious contributions to the signal from two-atom events. In addition, we have explicitly solved the eigenvectors and eigenvalues of two two-level atoms coupled to a quantized cavity mode for differing coupling strengths.