Comparison of Northern Ireland radon maps based on indoor radon measurements and geology with maps derived by predictive modelling of airborne radiometric and ground permeability data

Publicly available information about radon potential in Northern Ireland is currently based on indoor radon results averaged over 1-km grid squares, an approach that does not take into account the geological origin of the radon. This study describes a spatially more accurate estimate of the radon potential of Northern Ireland using an integrated radon potential mapping method based on indoor radon measurements and geology that was originally developed for mapping radon potential in England and Wales. A refinement of this method was also investigated using linear regression analysis of a selection of relevant airborne and soil geochemical parameters from the Tellus Project. The most significant independent variables were found to be eU, a parameter derived from airborne gamma spectrometry measurements of radon decay products in the top layer of soil and exposed bedrock, and the permeability of the ground. The radon potential map generated from the Tellus data agrees in many respects with the map based on indoor radon data and geology but there are several areas where radon potential predicted from the airborne radiometric and permeability data is substantially lower. This under-prediction could be caused by the radon concentration being lower in the top 30 cm of the soil than at greater depth, because of the loss of radon from the surface rocks and soils to air.     

地下空间氡的产生机理及通风控制

本文建立了土壤和建材的氡析出模型,在充分考虑各个影响因素的前提下,推导出了土壤和建材的表面析氡率公式,并依据此公式,进而推导出了室内氡浓度与通风换气效率的关系式。应用以上公式,对一典型的地下空间模型进行了计算,结果表明:地下空间氡的主要来源是土壤氡气的逸出,约占总析氡量的70豫～90豫;在较高的氡浓度状态下,室内氡浓度对通风十分敏感,增大地下空间的通风换气率,会使空气氡浓度大幅度的降低。因此,若按照地下空间的标准新风量进行设计,控制室内氡水平在400Bq/m3以内是很容易的,但是若要控制室内氡水平在200Bq/m3以内,则至少需要25.2m3/h的人均新风量,考虑新风不能得到完全利用,所需引入的室外新风量至少为31.5m3/h(以地下商场为例)。     

Radon and radon daughter evaluation in a natural radioactivity survey indoors

An indoor survey in order to estimate the population exposure in five towns of an Italian Region is presented. A particular methodology for the campaign was planned and is being applied. Gamma spectrometry of building materials, exposure rate measurements indoors and outdoors and radon concentration measurements indoors were taken with different techniques. A correlation was found between mean gamma exposure rate and mean radon concentration in the houses investigated. An evaluation of mean effective dose equivalents for the inhabitants of the five towns is reported.     

In situ gamma spectroscopy to characterize building materials as radon and thoron sources

In situ gamma spectroscopy is widely utilized to determine the outdoor gamma dose rate from the soil and to calculate the natural and artificial radionuclide concentration and their contribution to the dose rate. The application of in situ gamma spectroscopy in indoor environments can not supply quantitative information about activity concentration of radionuclides in building materials, but this technique can provide interesting information about building materials as radon source. In fact, a method based on analyses of gamma spectra data has been developed by the authors to provide, in field, quantitative estimation of disequilibrium in 226Ra and 228Ac sub-chains due to 222Rn and 220Rn exhalation. The method has been applied to data of gamma spectroscopy measurements carried out with HPGe detector (26%) in seven dwellings and one office in Rome. The first results of the data analysis show that, as regards especially the 226Ra sub-chain disequilibrium, different building materials (tuff, concrete, etc.) can show very different characteristics. If, in addition to the spectrometric data, other indoor environment parameters (indoor gamma dose rates, room dimensions, wall thickness, etc.) (Bochicchio et al., Radiat Prot Dosim 1994;56(1-4):137-140; Bochicchio et al., Environ Int 1996a;22:S633-S639) are utilized in a room model, an evaluation of 226Ra, 228Ac and 40K activity concentration and an indication of the exhalation features, by means of estimation of exhaled 222Rn activity concentration, can be achieved.     

Mapping the geogenic radon potential in Germany

Mapping the geogenic radon potential in Germany is a research project initiated by the German Federal Ministry for the Environment, Conservation and Reactor Safety. The project was aimed to develop a standard methodology for the estimation of a geogenic radon potential and to apply this method to map the region of Germany as an overview for planning purposes. The regionalisation results from a distance-weighted interpolation of the site-specific values of radon concentration in soil gas and in situ gas permeability of soils on a regular grid considering the corresponding geological units. The map of Germany in a scale of 1:2 million is based on the radon concentration in soil gas as an estimator of the geogenic radon potential assuming the 'worst case' of uniform highest permeability. The distribution is subdivided into categories of low (< 10 kBq/m3), medium (10-100 kBq/m3), increased (100-500 kBq/m3) and high (> 500 kBq/m3) radon concentration. High values occur especially in regions with granites and basement rocks of Paleozoic age, and are proven by measurements in 0.03% of the total area. Many of these regions are also known for their enhanced indoor values. The class with increased values takes a portion of 7.86% and likewise occurs mainly in regions with outcrops of folded and metamorphic basement, but also of some Meso- and Cenozoic sediments with increased uranium contents and/or higher emanation coefficients. For 67.3% of the country, the radon concentration is classified as 'medium', and an assignment to specific geological units cannot be made at the map scale considered. Low radon contents, where protective measures against radon are usually not considered, are found in the geologically rather homogeneous part of northern Germany with unconsolidated Cenozoic sediments, covering approximately 25% of the total country. It is of course not possible to predict the indoor radon concentration of single houses from these maps, because construction type and structural fabric of houses are essentially governing the extent to which subsoil radon potential affects the indoor concentration. Besides this, in places with site-specific geochemical, structural and soil-physical properties, local radon anomalies may occur which were not recorded in the course of the wide-meshed screening study.     

广州市土壤天然放射性水平调查

本文主要分析了广州市土壤天然放射性水平的调查数据。本次土壤氡浓度调查基本采用2km×2km的网格对广州市老八区均匀布点,采用GPS（卫星定位）定位。本次调查的结果表明：广州市的γ辐射剂量率平均值高于全国水平,是高放射性本底地区;氡浓度水平虽然在不同的季节变化较大,但两次不同季节的调查结果均与全国土壤氡平均值相当,属于中等水平。     

Investigations in Special “High Radon Areas” In Germany

The main source of high radon concentration indoors is the exhalation of radon from the soil. In the western part of Germany, two interesting regions, “Eifel” and “Hunsrück”, are selected for these radon investigations. The first region is an area with silt and sandstone of low uranium content but with tectonic fractures caused by postvolcanic activity, whereas in the part of the “Hunsrück” under consideration, the uranium concentration in the ground formerly allowed the extraction of uranium ores. An electrostatic deposit of the first radon daughter (Polonium-218-ion) onto a surface barrier detector and the subsequent analysis of the measured alpha spectra enables the determination of the concentration of radon in dwellings, its diffusion through and its exhalation rate from the soil. A maximum indoor concentration of radon of 8 kBq★m^?3 in a bedroom and approximately 35 kBq★m^?3 in a cellar room were determined in a house built in 1976. The daily variation between the minimum and the maximum concentration indoors amounts to a factor of ten. In these regions the radon concentration outdoors varies between 20 and 150 Bq★m^?3. The exhalation rates of radon from the soil are found to range from 0.002 to 1 Bq★m^?2★S^?1 The effects of sealing the ground slab with polyurethane and removing the air under the ground slab by suction will be presented.     

Variation in residential radon levels in new Danish homes

Radon‐222 gas arises from the radioactive decay of radium‐226 and has a half‐life of 3.8 days. This gas percolates up through soil into buildings, and if it is not evacuated, there can be much higher exposure levels indoors than outdoors, which is where human exposure occurs. Radon exposure is classified as a human carcinogen, and new Danish homes must be constructed to ensure indoor radon levels below 100 Bq/m³. Our purpose was to assess how well 200 newly constructed single detached homes perform according to building regulations pertaining to radon and identify the association between indoor radon in these homes and municipality, home age, floor area, floor level, basement, and outer wall and roof construction. Median (5–95 percentile) indoor radon levels were 36.8 (9.0–118) Bq/m³, but indoor radon exceeded 100 Bq/m³ in 14 of these new homes. The investigated variables explained nine percent of the variation in indoor radon levels, and although associations were positive, none of these were statistically significant. In this study, radon levels were generally low, but we found that 14 (7%) of the 200 new homes had indoor radon levels over 100 Bq/m³. More work is needed to determine the determinants of indoor radon.     

Population dose in the vicinity of old Spanish uranium mines

Regional surveys were conducted to determine exposure to natural sources of radiation for people in the vicinity of old Spanish uranium mines. The surveys evaluated indoor radon concentrations and outdoor and indoor external gamma dose rates. Indoor radon concentrations were measured in 222 dwellings by means of nuclear track-etched detectors. The terrestrial gamma ray dose rate was measured outdoors and indoors at a total of 256 points and 115 points, respectively. Estimates mean annual effective doses for the six areas studied ranged from 3.2 to 5.1 mSv per year, which is between 1.2 and 2 times higher than the average national value.     

Radon and Natural Ventilation in Newer Danish Single-Family Houses

Abstract To investigate the effect of ventilation on indoor radon (²²²Rn), simultaneous measurements of radon concentrations and air change rates were made in 117 Danish naturally ventilated slab-on-grade houses built during the period 1984–1989. Radon measurements (based on CR-39 alpha-track detectors) and air change rate measurements (based on the perfluorocarbon tracer technique; PFT) were in the ranges 12–620 Bq m^?3 and 0.16?0.96 h^?1, respectively. Estimates of radon entry rates on the basis of such time-averaged results are presented and the associated uncertainty is discussed. It was found that differences in radon concentrations from one house to another are primarily caused by differences in radon entry rates whereas differences in air change rates are much less important (accounting for only 80,0% of the house-to-house variation). In spite of the large house-to-house variability of radon entry rates it was demonstrated, however, that natural ventilation does have a significant effect on the indoor radon concentration. Most importantly, it was found that the group of houses with an air change rate above the required level of 0.5 h^?1 on average had an indoor radon concentration that was only 50% (0.5±0.1) of that of the group of houses with air change rates below 0.5 h^?1. The reducing effect of increased natural ventilation on the indoor radon concentration was found to be due mainly to dilution of indoor air. No effect could be seen regarding reduced radon entry rates.     

Radiation exposure in German dwellings,some results and a proposed formula for dose limitation

The results of our investigations in the Federal Republic of Germany on the indoor and outdoor exposure to natural radiation from gamma rays and radon and thoron daughters are presented. Indoor the median Rn-222 concentration was approximately four times higher than outdoors. A correlation analysis of the data obtained showed that indoors the equilibrium factor F is almost independent of ventilation, Rn-222 concentration and other parameters. The mean equilibrium factor was measured to be F = 0.3 in dwellings and approximately F = 0.4 outdoors. The results of our investigations on diffusion coefficients and exhalation rates showed, that the activity concentration in dwellings and in cellars can generally be explained by the radon exhalation from the building materials. Only in areas of high radon concentrations, the exhalation from the soil was a decisive factor. The mean effective dose equivalent by residence in dwellings amounted to 0.2 – 0.8 mSv/a for Rn-222 daughters and approximately 0.1 mSv/a for Rn-220 daughters. A relationship has been derived which permits the calculation of the expected average radiation exposure in dwellings by gamma radiation and by radon inhalation as function of the radionuclide concentration in building materials.     

Seasonal variations in soil gas radon concentration

We have been studying seasonal variations in soil gas radon concentration in southern Finland since 1982.To detect the radon we employ liquid scintillation solution in an open glass vial placed in a plastic tube set in a hole drilled in the ground.The results from an esker area show that there may be an appreciable seasonal variation in soil gas radon concentration, similar to that in houses. Because of the varying permeability and radium concentration of the ground, small changes in the building may have a large impact.     

Environmental gamma dose rates and influencing factors in buildings

Environmental gamma radiation measured in buildings in Dhaka shows a cosinusoidal variation of indoor dose rate with time mainly due to seasonally varied ventilation and air exchange rates of the houses. In connection, the nature and characteristics of the buildings were also discussed. As expected, a maximum dose rate was found in winter and a minimum in summer. The variations of indoor dose rates between buildings were observed. This study indicates that the higher air exchange rates of the houses may play an important role in providing a healthy and safe indoor environment for their inhabitants by reducing indoor exposure.     

Analytical quantification of airflows from soil through building substructures

Soil gas pollutants (VOCs, radon, …) have long been known to intrude into buildings through various openings, e.g., cracks and gaps in the foundations. As yet no model has been developed which can quantify this rate of flow whilst taking into account various substructure configurations. This is due to the complex phenomena that need to be consider and particularly to the difficulty in estimating pollutant flows at soil-building interfaces. In this paper analytical models have been developed to quantify these flows. The models have been developed for some typical substructure configurations: slab-on-grade, basement and crawlspace. The inputs of these models include particularly the foundation wall depth and the slab permeability. The analytical models have been compared to existing analytical models for one of the configurations. Moreover a 2-D finite element model has been used for numerical comparison. The models are presented as pressure-flow relationships and can be integrated into risk assessment tools in order to study the impact of soil gas pollutants on indoor air quality.     

Radon concentration in houses over a closed Hungarian uranium mine

High radon concentration (average 410 kBq m-3) has been measured in a tunnel of a uranium mine, located 15-55 m below the village of Kovágószolos, Hungary. The mine was closed in 1997; the artificial ventilation of the tunnel was then terminated and recultivation works begun. In this paper, a study has been made as to whether the tunnel has an influence on the radon concentration of surface dwellings over the mining tunnel. At different distances from the surface projection of the mining tunnel, radon concentration, the gamma dose, radon exhalation and radon concentration of soil gas were measured. The average radon concentration in the dwellings was 483 Bq m-3. Significantly higher radon concentrations (average 667 Bq m-3) were measured in houses within +/-150 m from the surface projection of the mining tunnel +50 m, compared with the houses further than the 300-m belt (average 291 Bq m-3). The average radon concentration of the soil gas was 88.8 kBq m-3, the average radon exhalation was 71.4 Bq m-2 s-1 and higher values were measured over the passage as well. Frequent fissures crossing the passage and running up to the surface and the high radon concentration generated in the passage (average 410 kBq m-3) may influence the radon concentration of the houses over the mining tunnel.     

Modeling Radon Entry into Houses with Basements: The Influence of Structural Factors

Where indoor concentrations are high, radon entry into houses with basements is usually due primarily to the convective transport of soil gas through openings in the subsurface part of the building shell. The factors determining the rate of entry may conveniently be divided into those associated with the undisturbed soil and those associated with the structure and its surroundings. This paper uses a numerical model to determine the influence of the latter factors on the soil gas and radon entry rates. The most important of these is the presence or absence of a gravel layer below the slab; the presence of the gravel can increase the radon entry rate through the perimeter gap betureen the foundation footer, slab, and wall (slab-footer gap) by as much as a factor of 5 over that for homogazeous soil. The permeability of the gravel becomes important when the soil permeability is unusually high, i.e., greater than 10^?10 m². Of lesser importance are the thickness of the gravel layer and the radium content of the gravel. The sizes and numbers of openings in the slab are relatively unimportant so long as the total opening area is vey small compared to the slab area. If cracks in the basement walls are major radon entry paths, as in concrete-block construction, the permeability of the soil restored to the region adjacent to the walls after completion of construction (backfill) is the determining factor in convective radon entry through these openings; if the soil is packed loosely, so that there is a gap between wall and soil, radon entry through a wall crack may be further increased by as much as a factor of 7.5. Radon entry rates through the slab-footer gap and through openings in the slab are only weakly influenced by the permeability of the backfill. The resistance of the perimeter gap to soil gas entry becomes significant when the gap width falls below 0.001 m, assuming a soil permeability of 10^?11 m².     

Modeling ventilation and radon in new Dutch dwellings

Indoor radon concentrations were estimated for various ventilation conditions, the differences being mainly related to the airtightness of the dwelling and the ventilation behavior of its occupants. The estimations were aimed at describing the variation in air change rates and radon concentrations to be expected in the representative newly built Dutch dwellings and identifying the most important parameters determining air change rate and indoor radon concentration. The model estimations were compared with measurements. Most of the air was predicted to enter the model dwelling through leaks in the building shell, independent of the ventilation conditions of the dwelling. Opening the air inlets was shown to be an efficient way to increase infiltration and thus to decrease radon concentration. The effect of increasing the mechanical ventilation rate was considerably less than opening the air inlets. The mechanical ventilation sets the lower limit to the air change rate of the dwelling, and is effective in reducing the radon concentration when natural infiltration is low. Opening inside doors proved to be effective in preventing peak concentrations in poorly ventilated rooms. As the airtightness of newly built dwellings is still being improved, higher radon concentrations are to be expected in the near future and the effect of occupant behavior on indoor radon concentrations is likely to increase. According to the model estimations soil-borne radon played a moderate role, which is in line with measurements.     

氡与室内空气环境

氡是一种放射性气体，在室内空气中广泛存在，并对人体造成极大伤害，因此倍受人们关注。本文主要介绍室内空气中氡的特性，来源，健康影响和防治措施。     

Radon Risk Mapping using Indoor Monitoring Data - A Case Study of the Lahti Area,Finland

An empirical statistical model is described for the use of indoor radon monitoring data as an indicator of the areal radon risk from soil and bedrock. The percentages of future homes expected to have radon concentrations exceeding the design level of 200 Bq/m³ unless constructed to provide protection against the entry of radon were assessed. The radon prognosis was made for different subareas, soil types and foundation types. This kind of report is used by the health and building authorities. In this study, 2689 indoor radon measurements were made in one of Finland's most radon-prone areas, consisting of eleven municipalities with a total area of 4600 km² and a population of 186,000. Radon concentrations were seasonally adjusted. Data on the location, geology and construction of buildings were determined from maps and questionnaires. The measurements covered different kinds of geological units in the area. The radon risk is highest in the gravel-dominated subarea in an ice-marginal formation and lowest in the northern half of the area in buildings constructed on bedrock. In these two areas, the design level of 200 Bq/m³ would be exceeded in 99% and 39% of new houses with slab-on-grade.