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1.
乙酰二茂铁缩4-苯氨基硫脲(C19H19N3SFe)与某些金属离子在无水乙醇中反应得到了希夫碱配合物M.L.X2.nH2O(M为UO^2+2,Hg^2+,Ni^2+,Zn^2+,L为C19H19N3SFe;NO^-3,Cl^-,1/2SO^2-4;n=0-6)并对配合物的组成及某些物理化学质进行了测试和表征。 相似文献
2.
低能重离子及其碰撞产生的级联原子在生物材料中的直接作用范围 总被引:10,自引:6,他引:4
用Monte Carlo法模拟计算了30keV和200keV的N^+与110keV的Fe^+在模拟细胞中的射程分布和径迹结构,并将110keVFe^+模拟计算的结果与RSB测量的结果相比较,发现计算与测量的结果吻合较好,离子的作用范围小于1μm。计算和实验的结果都说明能量相当低的重离子不大可能直接作用引起麦胚深层生物效应。 相似文献
3.
注入低能重离子在模拟细胞中的能量沉积 总被引:7,自引:2,他引:5
用Monte Carlo法模拟计算了30keV和200keV的N^+与110keV的Fe^+模拟细胞中本身及级联离子非弹性散射产生的电子,分子振动的能量沉积;讨论了电子分子振动的总能量沉积的深度分布。 相似文献
4.
用Monte Carlo方法模拟计算了30keV的N^+在模拟细胞中溅射级联推进的影响。从计算结果看,在用10^17个/cm^2的30keV的N^+注入生物材料时,溅射级联推进约为034μm,故得出溅射级推进作用不大可能造成植物诱变的结论。 相似文献
5.
In^+离子注入蓝宝石(α—Al2O3单晶)的表面改性研究 总被引:2,自引:2,他引:0
研究了〈0001〉和〈1^-210〉晶向蓝宝石(α-Al2O3单昌)在注入360keV、1×10^16cm^-2或100keV、6×10^16cm^-1的In^+后产生的损伤、注入层的性能变化和退火行为。实验结果表明,退火过程中损伤的恢复和In的分布与退火气氛有关:在100keV、6×10^16cm^-2的In^+注入时,注入层电阻率降低了10个量级,大小为6.8×10^3Ω·cm,表面损伤层的显 相似文献
6.
对离子能量进行校刻的快离子激光光谱学方法利用多普勒效应把离子能量与离子的共振激发联系起来,可应用于1eV-100MeV能区,在几十keV范围内,测量准确度优于2×10^-3,用这种方法校刻了^144Nd^+的能量。 相似文献
7.
8.
高能离子注入对聚酰亚胺薄膜硬度的影响 总被引:1,自引:0,他引:1
报道了聚酰亚胺薄膜在高能(650keV-2MeV)B^+、C^+和Cu^+离子注入后硬度的变化。对注入样品进行了显微硬度测量和XPS及RBS分析,观察了硬度与离子种类、能量及注入剂量的依赖关系。结果表明,离子注入之后薄膜样品的显微硬度值明显提高,注入离子在样品中的电子能量损失对聚合物材料改性起着关键作用。XPS和RBS分析显示,离子注入之后聚酰亚胺薄膜中C的含量增加,形成了以苯环结构为主的新的交联 相似文献
9.
10.
^13N—NH3.H2O的制备与质量控制 总被引:6,自引:0,他引:6
利用^16O(p,α)^13N核反应,以小体积^16O-H2O靶生产^13N正电子核素,即用16.5MeV的质子束轰击^16O-H2O靶5-20min后,以戴氏合金(Devard.sAlloy)还原靶水,可得么1.9-6.7GBq的^13N-NH3.H2O。产品经HPLC分析,放化纯度〉95%,载体NH3的浓度〈1mmol/L,比活度为4.4PBq/mol,适用于临床PET的研究。 相似文献
11.
The performance characteristics of silicon surface barrier detectors have been investigated for detecting H+, He+, N+, Ne+ and Ar+ in the energy interval 6-100 keV. For a cryogenically cooled, 50 mm2, 1325? depletion depth detector the resolution for protons was 1.65 keV (FWHM). The resolution decreased as the particle mass increased being 6.5 keV for 40 keV Ar+. All particles exhibit pulse height linearity throughout the energy range. 相似文献
12.
《Journal of Nuclear Science and Technology》2013,50(12):991-1005
The measurement of angular neutron spectrum in a quasi-spherical pile of Ti was carried out by the linac time-of-flight method for the assessment of neutron cross sections for Ti in the energy range from a few keV to a few MeV. The measured spectrum in the pile is generally in good agreement with the calculated one from ENDF/B-IV (MAT = 1,286 for Ti) except in the energy range from about 60 keV to a few 100 keV, where the calculation gives considerably lower neutron flux than the measurement. In order to investigate the cause of this discrepancy between the measured and calculated spectra, the total cross sections for Ti were measured by the transmission method. The results give larger values of total cross sections for Ti by about 30% than ENDF/B-IV below 200 keV, and smaller values by about 10% above 200 keV. These results were ensured at 55 and 147 keV by the measurement using a Si-filtered neutron beam. The calculation based on the measured cross sections shows better agreement with the measured spectrum than that based on ENDF/B-IV. The discrepancy is still observed around 100 keV. The sensitivity analysis shows the importance of cross sections above 1 MeV and elastic cross sections in the resonance energy region to solve the disagreement between the measured spectrum and the calculated one. 相似文献
13.
Neutron Total Cross Sections of 239Pu from Transmission Measurements in the Energy Range of 1–500keV
《Journal of Nuclear Science and Technology》2013,50(8):794-804
The average neutron total cross sections of 239Pu were obtained in the energy range of 1~500 keV from the high resolution transmission measurements performed by Harvey et al. at the Oak Ridge Electron Linear Accelerator (ORELA). In the energy range of 1~10 keV, the average effective cross sections of three samples were extrapolated to the total cross section for zero sample thickness. Above 10 keV the resonance self-shielding corrections to the effective cross sections of the thick sample were calculated by simulation of the cross sections from the resonance parameters. The results are given with 2% to 4% accuracy in the energy range of 1~10 keV and with better than 1% accuracy in the energy range above 10 keV. They are particularly useful to meet the needs of accurate experimental data in the energy range of 1~50 keV. 相似文献
14.
Y. Wu Z. AnY.M. Duan M.T. LiuJ. Wu 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2011,269(2):117-121
The absolute K-shell ionization cross sections of Cl and Lα, Lβ X-ray production cross sections of Ba by 6-30 keV electron impact have been measured. The target was prepared by evaporating the thin film of compound BaCl2 to the thick pure carbon substrate. The effects of multiple scattering of electrons penetrating the target films, electrons reflected from the thick pure carbon substrates and Bremsstrahlung photons produced when incident electrons impacted on the targets are corrected by using Monte Carlo method. For Ba L-shell X-ray characteristic peaks, the spectra were fitted by using spectrum-fitting program ALLFIT to extract more accurately the Lα and Lβ peak counts. The experimental results, reported here for the first time in the energy region of 6-30 keV, were compared with some theoretical results developed recently. 相似文献
15.
《Journal of Nuclear Science and Technology》2013,50(5):744-750
The neutron capture cross section of 96Zr at incident neutron energies from 15 to 100 keV has been measured by the time-of-flight method. Capture γ-rays were detected with an anti-Compton NaI(Tl) spectrometer, and the pulse-height weighting technique was applied to derive the neutron capture cross section. The present measurement provided the capture cross section as a function of incident neutron energy in the keV region. The results were compared with previous measurements and cross section data in the evaluated nuclear data libraries, JENDL-4.0, JENDL-3.3, ENDF/B-VII.0, and ENDF/B-VI.8. The present results revealed considerable underestimation of the evaluated cross sections in the high-energy region of 35–100 keV. 相似文献
16.
The aim of this paper is to obtain relevant sets of collision cross sections of the parent ions in low pressure discharges in argon, oxygen, and nitrogen, i.e., Ar+ in Ar, O2+ in O2 and N2+ in N2. These ion data are first discussed and then validated from comparisons between the calculated transport coefficients and those measured in the literature. The elastic momentum transfer collision cross sections are determined from a semi-classical approximation for the phase shift calculation based on a 12-6-4 inter-particle potential while ion transport coefficients are determined versus the reduced electric field from Monte Carlo simulations. 相似文献
17.
《Journal of Nuclear Science and Technology》2013,50(9):1131-1141
New evaluation of neutron-induced nuclear data for five stable isotopes of zinc (mass numbers A = 64, 66, 67, 68, and 70) was consistently carried out in the incident neutron energy range from 10?5 eV up to 20MeV. In the low energy region up to about 100keV, the resonance parameters were evaluated by taking account of the available measured data. In the fast neutron region, the comprehensive calculations with nuclear reaction models, in which compound, preequilibrium, and direct processes are taken into account, were performed to estimate cross sections for various reactions and double differential cross sections of emitted neutrons and γ-rays. The comparisons of the evaluated cross sections with the experimental data and existing evaluated nuclear data libraries are made and show a good agreement with the measurements. 相似文献
18.
E. Rauhala 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》1985,12(4):447-452
Differential elastic scattering cross sections of 0.7—2.5 MeV protons for carbon, nitrogen and silicon have been determined at a scattering angle θ = 170°. Results from previous measurements near θ = 170° show large variations, of the order of 10–30% in the nonresonant regions. The purpose of the present investigations is to tabulate cross section data for backscattering analysis at a single scattering angle for many elements. Proton backscattering in the non-Rutherford energy region is more sensitive in the detection of C, N and many other light elements than other ion beam methods when a high background from the matrix is absent. Proton backscattering by using the present scattering cross sections and computer data analysis are outlined. The possible interference from other nuclear reactions is considered. 相似文献
19.
《Journal of Nuclear Science and Technology》2013,50(4):406-412
The capture cross sections and capture γ-ray spectra of 209Bi were measured in a neutron energy region from 5 to 80keV and at 520 keV, using pulsed keV neutrons from the 7Li(p, n)7Be reaction and a time-of-flight method. The capture γrays from a bismuth or standard gold sample were detected with a large anti-Compton NaI(Tl) spectrometer. The capture yield of the bismuth or gold sample was obtained by applying a pulse-height weighting technique to the corresponding capture y-ray pulse-height spectrum. The derived capture cross sections from 5 to 80 keV were in good agreement with recent measurements, but that at 520 keV was about half of previous measurements. This large discrepancy at 520 keV was ascribed to the incorrect background-subtraction in the previous measurements from a comparison between the present and previous capture γray spectra. Strong transitions from the capture states to low lying states of 210Bi were observed in the present γray spectra. The multiplicities of observed y rays were obtained from the γray spectra. 相似文献
20.
V. A. Khryachkov B. D. Kuz’minov M. V. Dunaev I. V. Dunaeva N. N. Semenova A. I. Sergachev 《Atomic Energy》2006,101(4):760-765
The cross sections of the reactions 14N(n, α)11B and 14N(n, t)12C have been measured for neutron energies 5.46–7.2 MeV. The neutrons are generated in the reaction D(d, n) on a solid titanium
target. The work employs digital spectrometry. The charged-particle detector is a pulsed ionization chamber with a Frisch
grid, filled with a kyrpton-nitrogen mixture. The cross sections are measured for four groups of α particles α0, α1, α2, and α3 from the reaction 14N(n, α)11B and for tritium from the reaction 14N(n, t)12C. The energy resolution of the spectrometer was 60 keV. The errors in determining the cross sections for the reactions (n,
α) and (n, t) are 10–15%. The measurement results are compared with the ENDF/V VI evaluation. Good agreement is obtained in
the neutron energy range 5.45–6.5 MeV. At higher energies, the discrepancy reaches 30%.
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Translated from Atomnaya énergiya, Vol. 101, No. 4, pp. 307–311, October, 2006. 相似文献