Optical gain calculation of mid-infrared InAsN/GaSb quantum-well laser for tunable absorption spectroscopy applications

We report on optical gain calculations of a dilute-nitride mid-infrared laser structure designed to be grown on InAs substrate. The active region is composed of several strain-compensated type-II “W”-like InAsN/GaSb/InAsN quantum wells adapted to operate near 3.3 μm at room temperature. For typical injected carrier density σ = 1.1012 cm^− 2, the theoretical laser structure performances reveal a gain value at around 1000 cm^− 1 at 300 K, inducing a modal gain value equal to 50 cm^− 1. Low radiative current densities lower than 100 A/cm² are predicted, indicating that this dilute-nitride structure could operate at 300 K with small threshold current density.     

HPGe detectors for low-temperature nuclear orientation

Using the Low-Temperature Nuclear Orientation (LTNO) technique one can study various interesting properties of atomic nuclei and nuclear decay which can be deduced from the measurements of the angular distributions of charged particles emitted during the decay. However, the use of particle detectors working in conditions of LTNO devices (which are generally not available commercially) is a necessary precondition for the realization of these experiments.

Planar HPGe detectors for detection of charged particles at “liquid helium” temperatures were developed and produced at NPI e . Relatively simple technology using vacuum evaporation and diffusion was employed. The performance of detectors at low temperatures was tested and their characteristics measured in a testing cryostat before using them in real experiments.

The HPGe detectors were extensively used in a whole range of LTNO experiments with various physical objectives — in offline (IKS Leuven) as well as online (CERN-ISOLDE, Louvain-la-Neuve — LISOL) experiments. In frame of the project “Meson-Exchange Enhancement of First-Forbidden Beta Transitions in the Lead Region”, the measurements of angular distribution of emitted β-particles allowed to determine experimentally the “meson-exchange currents” contribution to the β-decay. In the project “Isospin Mixing in NZ nuclei”, the isospin-forbidden β-transitions of the nuclei in region (A=50–100) were studied in order to obtain information on the isospin structure of the nuclear states. A new project looking for the possible presence of the tensor currents contribution to the β-decay is being prepared for the CERN-ISOLDE facility.     

Scintillating and particle discrimination properties of selected crystals for low-temperature bolometers: from LiF to BGO

Selected crystals have been investigated at 20 mK for their properties of scintillation produced under irradiation. A scintillation signal is found in preliminary studies of YAP:Ce, GSO:Ce, CaF₂:Eu and Al₂O₃:Ti crystals thanks to high sensitivity light detectors. The full mixed “light-and-heat” bolometric technique has been applied to further characterize materials already employed in rare event researches: CaWO₄, BGO, undoped Al₂O₃ (sapphire). All these crystals show powerful discrimination properties for /γ or nuclear recoil/γ detection, with a special mention to undoped Al₂O₃, hitherto untested, which revealed an unexpected strong light emission. A weaker light signal has been found on LiF and TeO₂ bolometers too, sufficient to separate alpha from gamma events in these crystals.     

Approaching the fundamental noise limit in Mo/Au TES bolometers with transverse normal metal bars

Recent efforts in the Transition Edge Sensor (TES) bolometer/calorimeter community have focused on developing detectors whose noise properties are near the fundamental limits. These include the in-band phonon noise, the out-of-band Johnson noise, and the 1/f noise. We have investigated the noise performance of Mo/Au-bilayer TES bolometers designed for infrared detectors. These detectors use normal metal regions for the suppression of excess noise, which are oriented either parallel to (“bars”) or transverse to (“stripes”) the direction of current flow. Two nearly identical detectors, one with stripes and one with bars, were fabricated at the NASA/GSFC detector development facility. Significantly lower noise is found with the normal metal regions oriented transversely. We compare the detailed noise measurement and quantitative analysis of the noise level in each device as a function of the detector resistance. Our preliminary result is that the best detector features only moderate excess noise in both the in-band region and in the out-of-band region. This noise performance is suitable for instruments with multiplexed TES arrays, such as GSFC's FIBRE and SAFIRE.     

Spectroscopic evidence of inhomogeneous distribution of Nd in YVO4, YPO4 and YAsO4 crystals

Nd³⁺ : YVO₄ is one of the most interesting laser hosts for micro and diode-pumped solid state lasers. We have studied magnetic and optical properties of Nd³⁺ in three zircon type crystals YMO₄ (M=V, As, P). In particular, Nd³⁺ ions exhibit in the three hosts a multisite character observed in the absorption and emission spectra. However, the emission and its dynamics are strongly dependant on the reabsorption mechanisms. In Nd : YVO₄, single crystals containing 7 ± 1 × 10¹⁸ Nd³⁺ ions/cm³, the lifetime is 95 ± 2 μs in good agreement with the calculated radiative lifetime. Electron Paramagnetic Resonance (EPR) measurements are performed to identify the nature of the different substitution sites for Nd³⁺ ions. Nd³⁺ ions are found to be inhomogeneously distributed in tetragonal D_2d symmetry sites, in isolated ions, “shallow clusters” and pairs. Proportions of the different local environments depend on the total neodymium concentration. For instance, 15% of the Nd³⁺ ions are gathered in Nd³⁺–Nd³⁺ pairs for 7.2 ± 0.2 × 10¹⁹ Nd³⁺ ions/cm³.     

CdWO4 scintillator as a compact gamma ray spectrometer for planetary lander missions

The objective of this work is to develop a gamma ray spectrometer (GRS) suitable for use on planetary rover missions. The main characteristics of this detector are low weight, small volume low power and resistance to cosmic ray radiation over a long period of time. We describe a 3 cm diameter by 3 cm thick CdWO₄ cylindrical scintillator coupled to a PMT as a GRS for the energy region 0.662–7.64 MeV. Its spectral performance and efficiency are compared to that of a CsI(Tl) scintillator 2.5 cm diameter by 6 cm thick coupled to a 28 mm×28 mm PIN photodiode. The comparison is made experimentally using ¹³⁷Cs, ⁶⁰Co, 6.13 MeV gamma rays from a ¹³C(,γn)O¹⁶* source, 7.64 MeV thermal neutron capture gamma rays emitted from iron bars using a ²⁵²Cf neutron source, and natural radioactivity 1.46 MeV ⁴⁰K and 2.61 MeV ²³²Th gamma rays. We use a Monte Carlo method to calculate the total peak efficiency of these detectors and the full energy, first and second escape peak efficiencies. The experimental and calculated results agree well. We investigated the usefulness of these detectors for a GRS on a Mars lander mission. Although both detectors meet desired specifications, it was found that CdWO₄ has advantages over CsI(Tl) being a more compact detector of higher efficiency. Using a shaping amplifier of 24 ms, CdWO₄ spectrometer exhibited a 6.8% FWHM at 662 keV. At 6.13 MeV, CdWO₄ detector possesses an intrinsic total and full energy peak efficiencies of 16.7% and 6.3%, respectively. These efficiencies are nearly a factor of 1.6 and 4 greater than the corresponding efficiencies of the CsI(Tl) detector.

A proposed gamma ray spectroscopy system to be placed on a rover, consists of a central detector surrounded by a Compton suppressor shield. The central detector is a cylindrical CdWO₄ detector and the Compton suppressor shield is made of segmented CdWO₄, coupled to PIN photodiodes. The shield also prevents thermal neutron activation of the central detector.     

Design considerations for thin film coated semiconductor thermal neutron detectors—I: basics regarding alpha particle emitting neutron reactive films

Semiconductor-based thermal neutron detectors provide a compact technology for neutron detection and imaging. Such devices can be produced by externally coating semiconductor-charged-particle detectors with neutron reactive films that convert free neutrons into charged-particle reaction products. Commonly used films for such devices utilize the ¹⁰B(n,)⁷Li reaction or the ⁶Li(n,)³H reaction, which are attractive due to the relatively high energies imparted to the reaction products. Unfortunately, thin film or “foil” type thermal neutron detectors suffer from self-absorption effects that ultimately limit neutron detection efficiency. Design considerations that maximize the efficiency and performance of such devices are discussed. Theoretical and experimental results from front coated, back coated, and “sandwich” designs are presented.     

Attenuation of a non-parallel beam of gamma radiation by thick shielding—application to the determination of the U enrichment with NaI detectors

The traditional method used to determine the Uranium enrichment by nondestructive analysis is based on the “enrichment meter principle” [1]. It involves measuring the intensity of the 186 keV net peak area of ²³⁵U in “quasi-infinite” samples. A prominent factor, which affects the peak intensity, is the presence of gamma absorbing material (e.g., container wall, detector cover) between the sample and the detector. Its effect is taken into consideration in a commonly called “wall thickness” correction factor. Often calculated on the basis of approximations, its performance is adequate for small attenuation factors applicable to the case of narrow beams. However these approximations do not lead to precise results when wide non-parallel beams are attenuated through thick container walls.

This paper is dedicated to the calculation by numerical integration of the geometrical correction factor (K_wtc) which describes the effective mean path length of the radiation through the absorbing layer. This factor was calculated as a function of various measurement parameters (types and dimensions of the detector, of the collimator and of the shielding) for the most commonly used collimator shapes and detectors. Both coherent scattering (Rayleigh) and incoherent scattering (Compton) are taken into account for the calculation of the radiation interaction within the detector.     

Particle launch to 19 km/s for micro-meteoroid simulation using enhanced three-stage light gas gun hypervelocity launcher techniques

Particle launch experiments were performed to study application of the enhanced hypervelocity launcher (EHVL), i.e. the third-stage addition to the two-stage gun, for launching micron to millimeter sized particulates at velocities unobtainable with a standard two-stage light gas gun launch. Three types of particles or fliers were tested along with several barrel designs. For micron scale particles fine-grain polycrystalline ceramics were impacted and fractured, launching particulate clouds at velocities of 15 km/s. Multiple titanium particles 400 μm diameter embedded in plastic were “shotgun” launched to velocities of 10 km/s. Flier plates of 3 mm diameter by 1 mm thick Ti6Al4V were launched to 19 km/s. All experiments used a second-stage projectile with graded density facing impacting a flier in an impact generated acceleration reservoir. This paper describes the modification and adaptation of the Sandia EHVL to provide micrometeoroid simulation capabilities.     

Grain size effects on the tensile properties and deformation mechanisms of a magnesium alloy, AZ31B, sheet

The grain size dependence of the tensile properties and the deformation mechanisms responsible for those properties are examined for Mg alloy, AZ31B, sheet. Specifically, the Hall–Petch effect and strain anisotropy (r-value) are characterized experimentally, and interpreted using polycrystal plasticity modeling. {1 0 . 2} extension twins, {1 0 . 1} contraction twins, and so-called “double-twins” are observed via microscopy and diffraction-based techniques, and the amount of twinning is found to increase with increasing grain size. For the sheet texture and tensile loading condition examined, {1 0 . 2} extension twinning is not expected, yet the polycrystal plasticity model predicts the observed behavior, including this ‘anomalous’ tensile twinning. The analysis shows that the Hall–Petch strength dependence, of the polycrystal as a whole, is primarily determined by the grain size dependence of the strength of the prismatic slip systems.     

A comparative study of Co thin film deposited on GaAs (1 0 0) and glass substrates

The structural, magnetic and transport properties of Co/GaAs (1 0 0) and Co/glass thin films have been investigated. The structural measurements reveal the crystalline nature of Co thin film grown on GaAs, while microcrystalline nature in case of glass substrate. The film grown on GaAs shows higher coercivity (49.0 G), lower saturation magnetization (3.65 × 10⁻⁴) and resistivity (8 μΩ cm) values as compared to that on glass substrate (22 G, 4.77 × 10⁻⁴ and 18 μΩ cm). The grazing incidence X-ray reflectivity and photoemission spectroscopy results show the interaction between Co and GaAs at the interface, while the Co layer grown on glass remains unaffected. These observed results are discussed and interpreted in terms of different growth morphologies and structures of as grown Co thin film on both substrates.     

Effect of ferroic domain pattern changes on the Raman spectra of some ferroic crystals

The influence of changes in the pattern of ferroic domain structure on the Raman spectra of β-LiNH₄SO₄ and (NH₄)₃H(SO₄)₂ single crystals were studied. It was shown that the Raman spectra of β-LiNH₄SO₄ passed from the ferroelastic phase differ from those of “as-grown” crystal and those of the crystal, which was in the paraelectric phase. Significant changes could be observed in the Raman bands related to triply degenerated ν₃ and ν₄ vibrations of the SO₄ tetrahedron. Detailed temperature studies of the Raman spectra of β-LiNH₄SO₄ close to the paraelectric–ferroelectric phase transition, exhibit anomaly of some internal vibrations of SO₄ in the temperature range where a regular large-scale structure is observed. Different types of evolution of the ferroelastic domain structure and temperature behaviour of the donor and acceptor vibrations were shown while heating and cooling the (NH₄)₃H(SO₄)₂ crystal. Different values of temperature hysteresis were found in temperature studies of the ferroelastic domain structure (ΔT_S  3–5 K) and in Raman spectra studies (ΔT_S  12 K). No changes were observed in the pattern of ferroelastic domain structure at the temperature T_II–III  265 K, at which C2/c → P2/n structural phase transition takes place. On the other hand, at T_III–IV  135 K additional domains with W′-type of domain wall orientation were found.     

ΔE−E Telescope systems for detecting charged particles produced with a “white” neutron beam

Highly stable ΔE−E telescope systems consisting of plastic scintillation detectors are operated as flux monitors in a “white” neutron beam between 15 and 50 MeV. Multiple telescope systems consisting of large area silicon ΔE detectors and NaI E detectors are set up in a scattering chamber to investigate charged particle reactions induced by fast neutrons up to 50 MeV.     

Photon energy dependence of spatial non-uniformity in super-conducting tunnel junction detectors between 200 ev and 10 keV

It has been demonstrated by Low-Temperature Scanning Synchrotron Microscope that the spatial profiles of Nb/Al/AlO_x/Al/Nb detectors are abnormally large in an energy range between 2 and 10 keV, and thus the detectors produce no clear total absorption peaks. Below 2 keV, on the other hand, full illumination experiments have afforded the evidence that the spatial uniformity is significantly improved, for example, an 100 μm square junction has an intrinsic energy resolution of 5.4 eV at 200 eV. These results reconfirm that carefully designed junction detectors with a reasonable size are ideal for energy-dispersive spectroscopy in a soft X-ray range.     

A novel gamma-ray imaging concept using “edge-on” microchannel plate detector

The “edge-on” illuminated microchannel plate (MCP) position-sensitive detector (PSD) is used for gamma-ray imaging for the first time. The superior position resolution of the MCP is combined with high detection efficiency due to the “edge-on” illumination mode. The results of imaging a 15 μCi ¹³⁷Cs source (662 keV quantum energy) are presented.     

Edge sensitivity of “edgeless” silicon pad detectors measured in a high-energy beam

We report measurements in a high-energy beam of the sensitivity of the edge region in “edgeless” planar silicon pad diode detectors. The edgeless side of these rectangular diodes is formed by a cut and break through the contact implants. A large surface current on such an edge prevents the normal reverse biasing of this device above the full depletion voltage, but we have shown that the current can be sufficiently reduced by the use of a suitable cutting method, followed by edge treatment, and by operating the detector at a low temperature. A pair of these edgeless silicon diode pad sensors was exposed to the X5 high-energy pion beam at CERN, to determine the edge sensitivity. The signal of the detector pair triggered a reference telescope made of silicon microstrip detector modules. The gap width between the edgeless sensors, determined using the tracks measured by the reference telescope, was then compared with the results of precision metrology. It was concluded that the depth of the dead layer at the diced edge is compatible with zero within the statistical precision of ±8 μm and systematic error of ±6 μm.     

Development of a gamma compensated boron lined ionisation chamber for reactor safety and control applications

Boron lined ionisation chambers with an overall diameter of 85 mm and maximum length of 165 mm have been developed and tested. The chamber consists of 34 numbers of parallel plate aluminium electrodes spaced at a distance of 2 mm and mounted on SS rods and radiation resistant polyetheretherketone (PEEK) spacers. One surface of the signal electrode and both the surfaces of the +HT electrodes are dip coated with boron. It is filled with nitrogen gas at a pressure of 128 cm of Hg. Tests at the ⁶⁰Co source facility at gamma fields ranging from 200 R/h to 830 kR/h showed that the chamber required 500 V to obtain 90% of the saturation current at 830 kR/h. The gamma compensation factor was measured as 0.12–7% for various gamma fields for polarising voltages of +400 and −350 V. Neutron measurements at the Apsara Thermal Column showed that the linearity of the chamber response as a function of reactor power was within 2%. The neutron sensitivity was measured as 3.9 fA/nv.     

Comparison of sensing characteristics of ChemFEC devices based on spin-coated thin films of calix[n]arenes

ChemFECs (chemical field effect capacitors) or EIS (Electrolyte-Insulator-Semiconductor) devices were coated with calix[n]arene macrocycles for cation sensors development. Silicon nitride surface electrodes were spin-coated with p-tert-butylcalix[n]arene molecules for n = 8, 9 and 11. Electrochemical capacitance measurements were carried out to evaluate the sensitivity of the calix[n]arene layers towards specific cations as calcium and copper ions. Sensor responses were due to the “host-guest” specific interaction between the rigid cavity of calix[n]arene receptors (ligand) and chemical ion species. The developed chemical sensors have demonstrated good analytical characteristic in terms of: stability, selectivity and lifetime. In addition, experimental results were fitted using the site binding model in order to determine complex association constants, pK (1.9 ≤ pK ≤ 6.39) and surface density of ligands, N_L (9.10¹⁴ ≤ N_L ≤ 2.10¹⁶). All results obtained in this work were compared with those obtained using silicon dioxide EIS electrodes coated with the same calix[n]arene receptors using both spin-coating and thermal evaporation deposit processes.     

Construction and performance of one- and two-dimensional large position-sensitive liquid and plastic scintillation detectors — an application to a neutron polarimeter

Large one- and two-dimensional position-sensitive neutron detectors have been developed. Their shapes are a long block and a square and their sizes are 100×10×7.5 cm³ and 100×100×10 cm³ for one- and two-dimensional detectors, respectively. Both liquid and plastic scintillators are employed as detector materials. Position resolutions are examined by using monoenergetic neutron beams with energies of 61.6 MeV. The obtained position resolutions in FWHM are 3–5 cm and 4–14 cm for one- and two-dimensional detectors, respectively. Position resolutions are poor near the corner of the two-dimensional detector irrespective of scintillator materials. Scintillation light responses have been compared with predictions of Monte Carlo calculations. Neutron polarimeters at an intermediate energy have been developed by utilizing the position sensitivity of these detectors.     

X-ray imaging with “edge-on” microchannel plate detector: first experimental results

A novel scanning slit X-ray imaging system based on an “edge-on” microchannel plate detector was developed and tested. Images were acquired at 50 kV(p) X-ray tube voltage with a limiting spatial resolution of 7 lp/mm. The pixel noise was measured to be 0.3 count/pixel/s for a 50×70 μm² pixel size. This photon counting detector can be considered to be virtually noise free.