Neutronic analysis of PROMETHEUS reactor fueled with various compounds of thorium and uranium

In this study, neutronic performance of the DT driven blanket in the PROMETHEUS-H (heavy ion) fueled with different fuels, namely, ThO₂, ThC, UO₂, UC, U₃Si₂ and UN is investigated. Helium is used as coolant, and SiC is used as cladding material to prevent fission products from contaminating coolant and direct contact fuel with coolant in the blanket. Calculations of neutronic data per DT fusion neutron are performed by using SCALE 4.3 Code. M (energy multiplication factor) changes from 1.480 to 2.097 depending on the fuel types in the blanket under resonance-effect. M reaches the highest value in the blanket fueled with UN. Therefore, the investigated reactor can produce substantial electricity in situ. UN has the highest value of ²³⁹Pu breeding capability among the uranium fuels whereas UO₂ has the lowest one. ²³⁹Pu production ratio changes from 0.119 to 0.169 according to the uranium fuel types, and ²³³U production values are 0.125 and 0.140 in the blanket fueled with ThO₂ and ThC under resonance-effect, respectively. Heat production per MW (D,T) fusion neutron load varies from 1.30 to 7.89 W/cm³ in the first row of fissile fuel breeding zone depending on the fuel types. Heat production attains the maximum value in the blanket fueled with UN. Values of TBR (tritium breeding ratio) being one of the most important parameters in a fusion reactor are greater than 1.05 for all type of fuels so that tritium self-sufficiency is maintained for DT fusion driver. Values of peak-to-average fission power density ratio, Γ, are in the range of 1.390 and ∼1.476 depending on the fuel types in the blanket. Values of neutron leakage out of the blanket for all fuels are quite low due to SiC reflector. The maximum neutron leakage is only ∼0.025. Consequently, for all cases, the investigated reactor has high neutronic performance and can produce substantial electricity in situ, fissile fuel and tritium required for (D,T) fusion reaction.     

Performance of the gas turbine-modular helium reactor fuelled with different types of fertile TRISO particles

Preliminary studies have been performed on operation of the gas turbine-modular helium reactor (GT-MHR) with a thorium based fuel. The major options for a thorium fuel are a mixture with light water reactors spent fuel, mixture with military plutonium or with with fissile isotopes of uranium. Consequently, we assumed three models of the fuel containing a mixture of thorium with ²³⁹Pu, ²³³U or ²³⁵U in TRISO particles with a different kernel radius keeping constant the packing fraction at the level of 37.5%, which corresponds to the current compacting process limit. In order to allow thorium to act as a breeder of fissile uranium and ensure conditions for a self-sustaining fission chain, the fresh fuel must contain a certain quantity of fissile isotope at beginning of life; we refer to the initial fissile nuclide as triggering isotope. The small capture cross-section of ²³²Th in the thermal neutron energy range, compared to the fission one of the common fissile isotopes (²³⁹Pu, ²³³U and ²³⁵U), requires a quantity of thorium 25–30 times greater than that one of the triggering isotope in order to equilibrate the reaction rates. At the same time, the amount of the triggering isotope must be enough to set the criticality condition of the reactor. These two conditions must be simultaneously satisfied. The necessity of a large mass of fuel forces to utilize TRISO particles with a large radius of the kernel, 300 μm. Moreover, in order to improve the neutron economics, a fuel cycle based on thorium requires a low capture to fission ratio of the triggering isotope. Amid the common fissile isotopes, ²³³U, ²³⁵U and ²³⁹Pu, we have found that only the uranium nuclides have shown to have the suitable neutronic features to enable the GT-MHR to work on a fuel based on thorium.     

Optimized fissile and fusile breeding in a laser-fusion fissile-enrichment flux trap blanket

Optimization of fissile and fusile production in the SOLASE-H laser-fusion fissile-enrichment fuel-factory blanket is carried out. The objective is maximizing fissile breeding with the constraints of maintaining self-sufficiency in tritium production, and realistically accounting in the modeling for structural and coolant compositions and configurations imposed by the thermal-hydraulic and mechanical designs. The effect of radial and axial blanket zone thicknesses on fusile and fissile breeding is studied using a procedure which modifies the zones' effective optical thicknesses, rather than the actual three-dimensional geometrical configurations. A tritium yield per source neutron of 1.08 and a Th (n, ) reaction yield per source neutron of 0.43 can be obtained in such a concept, where ThO₂ Zircaloy-clad fuel assemblies for light water reactors (LWRs) are enriched in the²³³U isotope by irradiating them in a lead flux trap. This corresponds to 0.77 kg/[MW(th)-year] of fissile fuel production, and 1.94 years of irradiation in the fusion reactor to attain an average 3 w/o fissile enrichment in the fuel assemblies. For a once-through LWR cycle, a support ratio of 2–3 is estimated. However, with fuel recycling, more attractive support ratios of 4–6 may be attainable for a conversion ratio of 0.55, and of 5–8 for a conversion ratio of 0.70. These estimates are lower than those reported, around 20, for related designs.     

Effect of Transplutonium Doping on Approach to Long-life Core in Uranium-fueled PWR

The present paper advertises doping of transplutonium isotopes as an essential measure to improve proliferation-resistance properties and burnup characteristics of UOX fuel for PWR. Among them ²⁴¹Am might play the decisive role of burnable absorber to reduce the initial reactivity excess while the short-lived nuclides ²⁴²Cm and ²⁴⁴Cm decay into even plutonium isotopes, thus increasing the extent of denaturation for primary fissile ²³⁹Pu in the course of reactor operation. The doping composition corresponds to one discharged from a current PWR. For definiteness, the case identity is ascribed to atomic percentage of ²⁴¹ Am, and then the other transplutonium nuclide contents follow their ratio as in the PWR discharged fuel. The case of 1 at% doping to 20% enriched uranium oxide fuel shows the potential of achieving the burnup value of 100GWd/tHM with about 20% ²³⁸Pu fraction at the end of irradiation. Since so far, americium and curium do not require special proliferation resistance measures, their doping to UOX would assist in introducing nuclear technology in developing countries with simultaneous reduction of accumulated minor actinides stockpiles.     

The fusion-supported decentralized nuclear energy system

A decentralized nuclear energy system is proposed comprising mass-produced pressurized water reactors in the size range 10 to 300 MW (thermal), to be used for the production of process heat, space heat, and electricity in applications where petroleum and natural gas are presently used. Special attention is given to maximizing the refueling interval with no interim batch shuffling in order to minimize fuel transport, reactor downtime, and opportunity for fissile diversion. The smallest reactors could be deployed as nuclear batteries, kept in the equivalent of spent-fuel shipping casks and returned to nuclear fuel centers for refueling. These objectives demand a substantial fissile enrichment (7 to 15%). The preferred fissile fuel is U-233, which offers an order of magnitude savings in ore requirements (compared with U-235 fuel), and whose higher conversion ratio in thermal reactors serves to extend the period of useful reactivity and relieve demand on the fissile breeding plants (compared with Pu-239 fuel). Application of the neutral-beam-driven tokamak fusion-neutron source to a U-233 breeding pilot plant is examined. This scheme can be extended in part to a decentralized fusion energy system, wherein remotely located large fusion reactors supply excess tritium to a distributed system of relatively smallnonbreeding D-T reactors.     

Studies on the Feasibility of the LWRs Waste-Thorium In-Core Fuel Cycle in the Gas Turbine-Modular Helium Reactor

The capability to operate on LWRs waste constitutes one of the major benefits of the Gas Turbine-Modular Helium Reactor; in this paper, it has been evaluated the possibility to incinerate the LWRs waste and to simultaneously breed fissile ²³³U by fertile thorium. Since a mixture of pure ²³⁹Pu-thorium has shown a quite poor neutron economy, the LWRs waste-thorium fuel performance has been also tested when plutonium and thorium are allocated in different TRISO particles. More precisely, when fissile and fertile actinides share the same TRISO kernel, the resonance at 0.29 eV of the fission and capture microscopic cross sections of ²³⁹Pu diminishes also the absorption rate of fertile ²³²Th and thus it degrades the breeding process. Consequently, in the present studies, two different types of fuel have been utilized: the Driver Fuel, made of LWRs waste, and the Transmutation Fuel, made of fertile thorium. Since, in the thermal neutron energy range, the microscopic capture cross section of ²³²Th is about 80-100 times smaller than the fission one of ²³⁹Pu, setting thorium in particles with a large kernel and LWRs waste in particles with a small one makes the volume integrated reaction rates better equilibrated. At the light of the above consideration, which drives to load as much thorium as possible, for the Transmutation Fuel they have been selected the JAERI TRISO particles packed 40%; whereas, for the Driver Fuel they have been tested different packing fractions and kernel radii. Since no configuration allowed the reactor to work, the above procedure has been repeated when fertile particles are packed 20%; the latter choice permits over one year of operation, but the build up of ²³³U represents only a small fraction of the depleted ²³⁹Pu. Finally, the previous configuration has been also investigated when the fertile and fissile fuels share the same kernel or when the fertile fuel axially alternates with the fissile one.     

Neutronic design of a sub-critical, source driven reactor at the RA-8 facility

We present a LEU-ADS design based on an existing Argentine experimental facility, the RA-8 pool type zero power reactor. The versatility of this reactor allows measurement of different core configurations using different fuel enrichment, burnable poison rods, water perturbations, different control rods types in critical or subcritical configurations with an external source.To assess the feasibility of the LEU-ADS, multiplication factors, kinetic parameters, spectra, and time flux evolution were computed. Two external sources were considered: an isotopic source, and a D-D pulsed neutron source.Parameters for different core configurations were calculated, and the feasibility of using continuous and pulsed neutron sources was verified.     

Application of Fusion Neutron Source for Denaturing of Plutonium

Potential of DT fusion neutron source to enhance proliferation resistance properties of plutonium by means of its isotopic denaturing is addressed. The approach is exemplified by denaturing of pure ²³⁹Pu and plutonium of typical LWR spent fuel through transmutation of neptunium. The essential feature of a fusion driven system proposed in the study is a zero mass balance of plutonium: total plutonium inventory is constant during irradiation. The system is capable to convert pure ²³⁹Pu into plutonium composition with more than 20% fraction of key ²³⁸Pu isotope during 1,000 d of irradiation under initial neutron loading of 1 MW.m^?2. Denaturing of LWR spent fuel plutonium under the same conditions would increase its ²³⁸Pu content up to 10-12%.     

Optimization of a radially cooled pebble bed reactor

By altering the coolant flow direction in a pebble bed reactor from axial to radial, the pressure drop can be reduced tremendously. In this case the coolant flows from the outer reflector through the pebble bed and finally to flow paths in the inner reflector. As a consequence, the fuel temperatures are elevated due to the reduced heat transfer of the coolant. However, the power profile and pebble size in a radially cooled pebble bed reactor can be optimized to achieve lower fuel temperatures than current axially cooled designs, while the low pressure drop can be maintained.The radial power profile in the core can be altered by adopting multi-pass fuel management using several radial fuel zones in the core. The optimal power profile yielding a flat temperature profile is derived analytically and is approximated by radial fuel zoning. In this case, the pebbles pass through the outer region of the core first and each consecutive pass is located in a fuel zone closer to the inner reflector. Thereby, the resulting radial distribution of the fissile material in the core is influenced and the temperature profile is close to optimal.The fuel temperature in the pebbles can be further reduced by reducing the standard pebble diameter from 6 cm to a value as low as 1 cm. An analytical investigation is used to demonstrate the effects on the fuel temperature and pressure drop for both radial and axial cooling.Finally, two-dimensional numerical calculations were performed, using codes for neutronics, thermal-hydraulics and fuel depletion analysis, in order to validate the results for the optimized design that were obtained from the analytical investigations. It was found that for a radially cooled design with an optimized power profile and reduced pebble diameter (below 3.5 cm) both a reduction in the pressure drop ( bar), which increases the reactor efficiency with several percent, and a reduction in the maximum fuel temperature (C) can be achieved compared to present axially cooled designs.     

Effective Hamiltonian for metallic Pu

We derive a low-energy effective Hamiltonian for metallic Pu by assuming that intra-atomic Coulomb and spin-orbit interactions are much stronger than the kinetic energy terms. An important property of is the exact cancellation of the effective f-f hopping tensor that places Pu closer to lanthanide systems such as Ce or mixed valent Sm than to the rest of the actinides. The similarity between the low-energy models of Pu and these mixed valent lanthanide systems could be the common root for explaining the large volume expansions observed in all of them.