Simultaneous stereo particle image velocimetry and double-pulsed planar laser-induced fluorescence of turbulent premixed flames

A new technique was developed and applied to the study of flame structure and flame-vortex interaction in turbulent premixed flames. Turbulent premixed flames were probed using simultaneous stereo particle image velocimetry (PIV) and a double-pulsed acetone planar laser-induced fluorescence system (PLIF). Two double-pulsed Nd:YAG lasers operating at 532 and 266 nm were used for the PIV and acetone PLIF measurements, respectively. The stereo PIV images were acquired using two double-frame CCD cameras, and two ICCD cameras were used to capture the PLIF signal. The diagnostic system was applied to study turbulent methane-air stoichiometric premixed flames at relatively high Reynolds numbers. Flame merging and the creation of pockets of both products and reactants were detected, and a very strong interaction between the flame front and the vortex structures was suggested in the simultaneous PIV/PLIF images. Double-pulsed PLIF data obtained for different time delays allowed statistical study of flame development. Three-dimensional turbulent fluxes of mean progress variable were obtained. It was shown that the fluxes obey the gradient diffusion hypothesis. The proposed diagnostic increases flexibility and range of measurements available for premixed flames.     

Effects of strain rate,turbulence, reactant stoichiometry and heat losses on the interaction of turbulent premixed flames with stoichiometric counterflowing combustion products

Intense strain, turbulence, heat transfer, and mixing with combustion products can affect premixed flames in practical combustion devices. These effects are systematically studied in turbulent premixed CH₄/N₂/O₂ flames using a reactant versus product counterflow system and independently varying bulk strain rate, turbulent Reynolds number, equivalence ratio of the reactant mixture, and temperature of the stoichiometric counterflowing combustion products. The flow field and the turbulent flames are investigated using particle image velocimetry (PIV) measurements and laser-induced fluorescence (LIF) imaging of OH. The OH-LIF images are used to identify the interface between the counterflowing streams, referred to here as the gas mixing layer interface (GMLI). The flame response for different flow conditions is compared in terms of the probability of localized extinction along the GMLI, the turbulent flame brush thickness, and flame position relative to the GMLI, by using an OH-LIF-based progress variable. The probability of localized extinction at the GMLI increases as the separation between the turbulent flame brush and the GMLI decreases. Flame fronts in the vicinity of the GMLI are more likely to extinguish as a result of heat losses, dilution of the reaction zone by the product stream, and large local strain rates. A higher probability of localized extinction at the GMLI is induced by either a larger bulk strain rate or a slower flame speed. As the turbulent Reynolds number increases, the corresponding increase in turbulent flame brush thickness enhances the interactions of the flame fronts with the GMLI. Heat losses are substantially less significant for cases in which the turbulent flame brush is sufficiently separated from the GMLI. For flames in close proximity to the GMLI, the effects of the product stream on the flame front differ for lean and rich reactant mixtures. These disparities are attributed in part to differences in the ignitibility of the reactant mixtures by the hot product stream.     

Tubular premixed and diffusion flames: Effect of stretch and curvature

Tubular flames are ideal for the study of stretch and curvature effects on flame structure, extinction, and instabilities. Tubular flames have uniform stretch and curvature and each parameter can be varied independently. Curvature strengthens or weakens preferential diffusion effects on the tubular flame and the strengthening or weakening is proportional to the ratio of the flame thickness to the flame radius. Premixed flames can be studied in the standard tubular burner where a single premixed gas stream flows radially inward to the cylindrical flame surface and products exit as opposed jets. Premixed, diffusion and partially premixed flames can be studied in the opposed tubular flame where opposed radial flows meet at a cylindrical stagnation surface and products exit as opposed jets. The tubular flame flow configurations can be mathematically reduced to a two-point boundary value solution along the single radial coordinate. Non-intrusive measurements of temperature and major species concentrations have been made with laser-induced Raman scattering in an optically accessible tubular burner for both premixed and diffusion flames. The laser measurements of the flame structure are in good agreement with numerical simulations of the tubular flame. Due to the strong enhancement of preferential diffusion effects in tubular flames, the theory-data comparison can be very sensitive to the molecular transport model and the chemical kinetic mechanism. The strengthening or weakening of the tubular flame with curvature can increase or decrease the extinction strain rate of tubular flames. For lean H₂-air mixtures, the tubular flame can have an extinction strain rate many times higher than the corresponding opposed jet flame. More complex cellular tubular flames with highly curved flame cells surrounded by local extinction can be formed under both premixed and non-premixed conditions. In the hydrogen fueled premixed tubular flames, thermal-diffusive flame instabilities result in the formation of a uniform symmetric petal flames far from extinction. In opposed-flow tubular diffusion flames, thermal-diffusive flame instabilities result in cellular flames very close to extinction. Both of these flames are candidates for further study of flame curvature and extinction.     

Experimental annular stratified flames characterisation stabilised by weak swirl

A burner for the investigation of lean stratified premixed flames propagating in intense isotropic turbulence has been developed. Lean pre-mixtures of methane at different equivalence ratios were divided between two concentric co-flows to obtain annular stratification. Turbulence generators were used to control the level of turbulence intensity in the oncoming flow. A third annular weakly swirling airflow provided the flame stabilisation mechanism. A fundamental characteristic was that flame stabilisation did not rely on flow recirculation. The flames were maintained at a position where the local mass flux balanced the burning rate, resulting in a freely propagating turbulent flame front. The absence of physical surfaces in the vicinity of the flame provided free access for laser diagnostics. Stereoscopic Planar Image Velocimetry (SPIV) was applied to obtain the three components of the instantaneous velocity vectors on a vertical plane above the burner at the point of flame stabilisation. The instantaneous temperature fields were determined through Laser Induced Rayleigh (LIRay) scattering. Planar Laser Induced Fluorescence (PLIF) of acetone was used to calculate the average equivalence ratio distributions. Instantaneous turbulent burning velocities were extracted from SPIV results, while flame curvature and flame thermal thickness were calculated using the instantaneous temperature fields. The PDFs of these quantities were analysed to consider the separate influence of equivalence ratio stratification and turbulence. Increased levels of turbulence resulted in the expected higher turbulent burning velocities and flame front wrinkling. Flames characterised by higher fuel gradients showed higher turbulent burning velocities. Increased fuel concentration gradients gave rise to increased flame wrinkling, particularly when associated with positive small radius of curvature.     

Effects of Lewis number on flame surface density transport in turbulent premixed combustion

The transport of flame surface density (FSD) in turbulent premixed flames has been studied using a database obtained from Direct Numerical Simulation (DNS). Three-dimensional freely propagating developing statistically planar turbulent premixed flames have been examined over a range of global Lewis numbers from 0.6 to 1.2. Simplified chemistry has been used and the emphasis is on the effects of Lewis number on FSD transport in the context of Reynolds-averaged closure modelling. Under the same initial conditions of turbulence, flames with low Lewis numbers are found to exhibit counter-gradient transport of FSD, whereas flames with higher Lewis numbers tend to exhibit gradient transport of FSD. Stronger heat release effects for lower Lewis number flames are found to lead to an increase in the positive (negative) value of the dilatation rate (normal strain rate) term in the FSD transport equation with decreasing Lewis number. The contribution of flame curvature to FSD transport is found to be influenced significantly by the effects of Lewis number on the curvature dependence of the magnitude of the reaction progress variable gradient, and on the combined reaction and normal diffusion components of displacement speed. The modelling of the various terms of the FSD transport equation has been analysed in detail and the performance of existing models is assessed with respect to the terms assembled from corresponding quantities extracted from DNS data. Based on this assessment, suitable models are identified which are able to address the effects of non-unity Lewis number on FSD transport, and new or modified models are suggested wherever necessary.     

Measurement of the instantaneous flame front structure of syngas turbulent premixed flames at high pressure

Instantaneous flame front structure of syngas turbulent premixed flames including the local radius of curvature, the characteristic radius of curvature, the fractal inner cutoff scale and the local flame angle were derived from the experimental OH-PLIF images. The CO/H₂/CO₂/air flames as a model of syngas/air combustion were investigated at pressure of 0.5 MPa and compared to that of CH₄/air flames. The convex and concave structures of the flame front were detected and statistical analysis including the PDF and ADF of the local radius of curvature and local flame angle were conducted. Results show that the flame front of turbulent premixed flames at high pressure is a wrinkled flame front with small scale convex and concave structures superimposed with large scale flame branches. The convex structures are much more frequent than the concave ones on flame front which reflects a general characteristic of the turbulent premixed flames at high pressure. The syngas flames possess much wrinkled flame front with much smaller fine cusps structure compared to that of CH₄/air flames and the main difference is on the convex structure. The effect of turbulence on the general wrinkled scale of flame front is much weaker than that of the smallest wrinkled scale. The general wrinkled scale is mainly dominated by the turbulence vortex scale, while, the smallest wrinkled scale is strongly affected by the flame intrinsic instability. The effect of flame intrinsic instability on flame front of turbulent premixed flame is mainly on the formation of a large number of convex structure propagating to the unburned reactants and enlarge the effective contact surface between flame front and unburned reactants.     

Flame brush characteristics and burning velocities of premixed turbulent methane/air Bunsen flames

The flame brush characteristics and turbulent burning velocities of premixed turbulent methane/air flames stabilized on a Bunsen-type burner were studied. Particle image velocimetry and Rayleigh scattering techniques were used to measure the instantaneous velocity and temperature fields, respectively. Experiments were performed at various equivalence ratios and bulk flow velocities from 0.7 to 1.0, and 7.7 to 17.0 m/s, respectively. The total turbulence intensity and turbulent integral length scale were controlled by the perforated plate mounted at different positions upstream of the burner exit. The normalized characteristic flame height and centerline flame brush thickness decreased with increasing equivalence ratio, total turbulence intensity, and longitudinal integral length scale, whereas they increased with increasing bulk flow velocity. The normalized horizontal flame brush thickness increased with increasing axial distance from the burner exit and increasing equivalence ratio. The non-dimensional leading edge and half-burning surface turbulent burning velocities increased with increasing non-dimensional turbulence intensity, and they decreased with increasing non-dimensional bulk flow velocity when other turbulence statistics were kept constant. Results show that the non-dimensional leading edge and half-burning surface turbulent burning velocities increased with increasing non-dimensional longitudinal integral length scale. Two correlations to represent the leading edge and half-burning surface turbulent burning velocities were presented as a function of the equivalence ratio, non-dimensional turbulence intensity, non-dimensional bulk flow velocity, and non-dimensional longitudinal integral length scale. Results show that the half-burning surface turbulent burning velocity normalized by the bulk flow velocity decreased as the normalized characteristic flame height increased.     

Experimental analysis of an oblique turbulent flame front propagating in a stratified flow

This paper details the experimental study of a turbulent V-shaped flame expanding in a nonhomogeneous premixed flow. Its aim is to characterize the effects of stratification on turbulent flame characteristics. The setup consists of a stationary V-shaped flame stabilized on a rod and expanding freely in a lean premixed methane-air flow. One of the two oblique fronts interacts with a stratified slice, which has an equivalence ratio close to one and a thickness greater than that of the flame front. Several techniques such as PIV and CH^* chemiluminescence are used to investigate the instantaneous fields, while laser Doppler anemometry and thermocouples are combined with a concentration probe to provide information on the mean fields. First, in order to provide a reference, the homogeneous turbulent case is studied. Next, the stratified turbulent premixed flame is investigated. Results show significant modifications of the whole flame and of the velocity field upstream of the flame front. The analysis of the geometric properties of the stratified flame indicates an increase in flame brush thickness, closely related to the local equivalence ratio.     

A DNS study of hydrogen/air swirling premixed flames with different equivalence ratios

Hydrogen/air swirling premixed flames with different equivalence ratios are studied using direct numerical simulation. A fourth-order explicit Runge–Kutta method for time integration and an eighth-order central differencing scheme for spatial discretization are used to solve the full Navier–Stokes (N–S) equation system. A 9 species 19-step reduced mechanism for hydrogen/air combustion is adopted. The flames are stabilized with the help of a recirculation zone characterizing a high swirling flow. The vortex structures of the swirling premixed flames are presented. The flame structures are investigated in terms of the flame front curvature and tangential strain rate probability density functions (pdfs). The local flamelet temperature profiles are also extracted randomly along the flame front and compared with the corresponding laminar flame temperature profile. In order to study preferential diffusion effects, direct numerical simulation of two additional freely propagating planar flames in isotropic turbulence is conducted. Preferential diffusion effects observed in the planar flames are suppressed in the swirling flames. Further analysis confirms that the coherent small-scale eddies play important roles in the interactions between turbulence and the flame front. They are able to change the dynamic properties of the flame font and lead to enhanced burning intensity in the flame front with negative curvature for both stoichiometric and fuel-lean flames.     

Characterization of the effects of hydrogen addition in premixed methane/air flames

The use of hydrogenated fuels shows considerable promise for applications in gas turbines and internal combustion engines. In the present work, the effects of hydrogen addition in methane/air flames are investigated using both a laminar flame propagation facility and a high-pressure turbulent flame facility. The aim of this research is to contribute to the characterization of lean methane/hydrogen/air premixed turbulent flames at high pressures, by studying the flame front geometry, the flame surface density and the instantaneous flame front thermal thickness distributions. The experiments and analyses show that a small amount of hydrogen addition in turbulent premixed methane–air flames introduces changes in both instantaneous and average flame characteristics.     

Comprehensive study of the evolution of an annular edge flame during extinction and reignition of a counterflow diffusion flame perturbed by vortices

The structure of a time-dependent methane/enriched-air flame established in an axisymmetric, laminar counterflow configuration is investigated, as the flame interacts with two counterpropagating toroidal vortices. Computationally, the time-dependent equations are written using a modified vorticity–velocity formulation, with detailed chemistry and transport, and are solved implicitly on a nonstaggered, nonuniform grid. Boundary conditions are chosen to create local extinction and reignition in the vicinity of the axis of symmetry. Experimentally, CO planar laser-induced fluorescence (PLIF), OH PLIF, and an observable proportional to the forward reaction rate (RR) of the reaction CO+OH→CO₂+H are measured. Particle image velocimetry (PIV) is used to characterize the velocity field of the vortical structures and to provide detailed boundary conditions for the simulations. Excellent agreement is found between model and experiments to the minutest morphological details throughout the interaction. The validated model is then used to probe the dynamics of the two-dimensional extinction process with high temporal resolution. During the initial phase of the interaction, the flame is locally extinguished by the two vortices. The resulting edge flame propagates outward as an extinction front, with a structure that does not depart significantly from that of a diffusion flame. The front recedes from the axis of symmetry with a negative propagation speed that reaches a value as large as six times that of the freely propagating laminar flame with the same reactant concentrations found at the stoichiometric surface. As the front propagates outward, it transitions to an ignition front, and it reaches a positive propagation speed comparable to that of the freely propagating laminar flame. During this transition, it develops a characteristic premixed “hook,” with a lean premixed branch, a stoichiometric segment that evolves into the remnant of the original primary diffusion flame, and a much weaker secondary diffusion flame resulting from a secondary peak in heat release in the original unperturbed diffusion flame. No evidence of a distinct rich premixed flame is found. The edge flame stabilizes at a radial location where the local gaseous speed equals the propagation speed of the front. When the local perturbation has decayed below the flame propagation speed, the flame edge starts reigniting the mixing layer as an ignition wave that propagates with an essentially frozen structure along the stoichiometric surface until the original diffusion flame structure is fully recovered. Implications for flamelet modeling of turbulent flames with local extinction are discussed.     

Investigation of local flame structures and statistics in partially premixed turbulent jet flames using simultaneous single-shot CH and OH planar laser-induced fluorescence imaging

We report on the application of simultaneous single-shot imaging of CH and OH radicals using planar laser-induced fluorescence (PLIF) to investigate partially premixed turbulent jet flames. Various flames have been stabilized on a coaxial jet flame burner consisting of an outer and an inner tube of diameter 22 and 2.2 mm, respectively. From the outer tube a rich methane/air mixture was supplied at a relatively low flow velocity, while a jet of pure air was introduced from the inner one, resulting in a turbulent jet flame on top of a laminar pilot flame. The turbulence intensity was controlled by varying the inner jet flow speed from 0 up to 120 m/s, corresponding to a maximal Reynolds number of the inner jet airflow of 13,200. The CH/OH PLIF imaging clearly revealed the local structure of the studied flames. In the proximity of the burner, a two-layer reaction zone structure was identified where an inner zone characterized by strong CH signals has a typical structure of rich premixed flames. An outer reaction zone characterized by strong OH signals has a typical structure of a diffusion flame that oxidizes the intermediate fuels formed in the inner rich premixed flame. In the moderate-turbulence flow, the CH layers were very thin closed surfaces in the entire flame, whereas the OH layers were much thicker. In the high-intensity-turbulence flame, the CH layer remained thin until it vanished in the upper part of the flame, showing local extinction and reignition behavior of the flame. The single-shot PLIF images have been utilized to determine the flame surface density (FSD). In low and moderate turbulence intensity cases the FSDs determined from CH and OH agreed with each other, while in the highly turbulent case a locally broken CH layer was observed, leading to a significant difference in the FSD results determined via the OH and CH radicals. Furthermore, the means and the standard deviations of CH and OH radicals were obtained to provide statistical information about the flames that may be used for validation of numerical calculations.     

Time-resolved blowoff transition measurements for two-dimensional bluff body-stabilized flames in vitiated flow

Flame holding and blowoff characteristics of bluff-body stabilized, turbulent flames were measured in an enclosed rectangular duct with a triangular flame holder in vitiated, premixed flows. Blowoff stability margins were characterized with chemiluminescence measurements performed by high-speed imaging to capture flame dynamics during the approach to flame blow off. As the equivalence ratio was decreased, local extinctions along the flames interacting with shear layers surrounding the bluff body recirculation zone occurred with greater frequency and proximity to the wake stagnation zone. Decreased equivalence ratio resulted in extinction events at the trailing edge of the stagnation zone, which allowed reactants to be convected into the recirculation zone and burned behind the bluff body. Increasing reactant dilution of the recirculation zone eventually resulted in flame lift-off or extinction of the flame in the neighboring shear layer. These near field shear layer flames convected to the wake stagnation zone, and were eventually quenched. Simultaneous particle imaging velocimetry (PIV) and OH planar laser-induced fluorescence (PLIF) measurements captured the flame edge location and aerodynamic behavior as blowoff was approached. Two-dimensional hydrodynamic stretch along the flame front and flow field vorticity maps were extracted from the combined PIV/OH PLIF data. The distribution of flame stretch shifted to greater values as the equivalence ratio decreased and is believed to be the cause of local flame extinction in the wake stagnation zone that starts the blowoff process.     

Numerical simulations of premixed flame cellular instability for a simple chain-branching model

Two-dimensional direct numerical simulations are performed to investigate the non-linear dynamics of low Lewis number premixed flames, in the context of a two-step chain-branching chemistry model. This consists of a thermally-neutral, but temperature sensitive, chain-branching step which produces intermediates such as radicals and an exothermic, zero activation energy chain-completion step which converts the intermediates into products. Emphasis is on examining the role of intermediates in the flame structure on the cellular instability and in comparing and contrasting with previous one-step chemistry model solutions. When intermediates are present only in small concentrations in the underlying one-dimensional flame structure, the two-step cellular dynamics are qualitatively similar to those of the one-step model, including cell-splitting and re-merging, symmetry breaking bifurcations and formation of asymmetric cells, localized quenching of the flame front and a significant enhancement of the flame speed. However, a higher peak value of the intermediates concentration, corresponding to a more distributed heat release, is shown to have a significant stabilizing effect, e.g., in a domain of fixed transverse size, the fully developed cellular structure and flame speed remain closer to those of the one-dimensional flame.     

Pressure influence on the flame front curvature of turbulent premixed flames: comparison between experiment and theory

In gas turbines, lean premixed combustion is executed in strongly turbulent flow fields and under high-pressure to allow large thermal loads within small-size combustors. Previous research on turbulent premixed flames has revealed the vital importance of flame-vortex interactions, but most of these investigations have been performed only at atmospheric pressure disregarding the large pressure dependency of the flame front dynamics. We report about spatially high-resolved laser-induced predissociation fluorescence imaging of OH (OH-LIPF) in premixed, high-pressure bluff-body stabilized methane/air flames. For each of the two measurement series with different equivalence ratio (φ = 0.7 and φ = 1.0), the planar flame topology at different pressures (0.1 to 1.1 MPa) but constant exit velocity was detected and stored for analysis. As the pressure was increased, the flame front contour of both equivalence ratios became strongly wrinkled with formation of highly curved flame front elements. For quantification of this phenomenon, the probability density function of flame curvature was evaluated with definition of the mean curvature radius as representative folding scale. To discuss different mechanisms of flame front disturbances according to their relevance, the flame curvature is compared with characteristic turbulence scales of the flow field and with the expected folding scale derived with Sivashinsky‘s formulation of linear flame instability theory. Significant changes become obvious especially if the pressure is increased up to 0.5 MPa. The mean curvature radius decreases distinctly and can be linked to the decreasing size of the Taylor length. Additionally, the formation of highly convoluted flame front elements is enforced by the increasing flame instability behavior. As the results show, the flame stoichiometry has a strong impact on the flame front topology at increasing pressures due to the differences of their flame dynamics.     

Heat release rate variations in high hydrogen content premixed syngas flames at elevated pressures: Effect of equivalence ratio

Three-dimensional direct numerical simulations with detailed chemistry were performed to investigate the effect of equivalence ratio on spatial variations of the heat release rate and flame markers of hydrogen/carbon monoxide syngas expanding spherical premixed flames under turbulent conditions at elevated pressures. The flame structures and the heat release rate were analysed and compared between fuel-lean, stoichiometric and fuel-rich centrally ignited spherical flames. The equivalence ratio changes the balance among thermo-diffusive effects, Darrieus–Landau instability and turbulence, leading to different flame dynamics and the heat release rate distribution, despite exhibiting similar cellular and wrinkling flames. The Darrieus–Landau instability is relatively insensitive to the equivalence ratio while the thermo-diffusive process is strongly affected by the equivalence ratio. As the thermo-diffusive effect increases as the equivalence ratio decreases, the fuel-lean flame is more unstable than the fuel-rich flame with the stoichiometric flame in between, under the joint effects of the thermo-diffusive instability and the Darrieus–Landau instability. The local heat release rate and curvature display a positive correlation for the lean flame, no correlation for the stoichiometric flame, and negative correlation for the rich flame. Furthermore, for the fuel-lean flame, the low and high heat release rate values are found in the negative and positive curvature zones, respectively, while for the fuel-rich flame, the opposite trends are found. It is found that heat release rate markers based on species concentrations vary strongly with changing equivalence ratio. The results suggest that the HCO, HO₂ concentrations and product of OH and CH₂O concentrations show good correlation with the local heat release rate for H₂/CO premixed syngas-air stoichiometric flame under turbulent conditions at elevated pressures.     

Flame front structure of turbulent premixed flames of syngas oxyfuel mixtures

In order to investigate oxyfuel combustion characteristics of typical composition of coal gasification syngas connected to CCS systems. Instantaneous flame front structure of turbulent premixed flames of CO/H₂/O₂/CO₂ mixtures which represent syngas oxyfuel combustion was quantitatively studied comparing with CH₄/air and syngas/air flames by using a nozzle-type Bunsen burner. Hot-wire anemometer and OH-PLIF were used to measure the turbulent flow and detect the instantaneous flame front structure, respectively. Image processing and statistical analyzing were performed using the Matlab Software. Flame surface density, mean progress variable, local curvature radius, mean flame volume, and flame thickness, were obtained. Results show that turbulent premixed flames of syngas possess wrinkled flame front structure which is a general feature of turbulent premixed flames. Flame surface density for the CO/H₂/O₂/CO₂ flame is much larger than that of CO/H₂/O₂/air and CH₄/air flames. This is mainly caused by the smaller flame intrinsic instability scale, which would lead to smaller scales and less flame passivity response to turbulence presented by Markstain length, which reduce the local flame stretch against turbulence vortex. Peak value of Possibility Density Function (PDF) distribution of local curvature radius, R, for CO/H₂/O₂/CO₂ flames is larger than those of CO/H₂/O₂/air and CH₄/air flames at both positive and negative side and the corresponding R of absolute peak PDF is the smallest. This demonstrates that the most frequent scale is the smallest for CO/H₂/O₂/CO₂ flames. Mean flame volume of CO/H₂/O₂/CO₂ flame is smaller than that of CH₄/air flame even smaller than that of CO/H₂/O₂/air flame. This would be due to the lower flame height and smaller flame wrinkles.     

Effect of high hydrogen enrichment on the outer-shear-layer flame of confined lean premixed CH4/H2/air swirl flames

In this study, we investigated the H₂-induced transition of confined swirl flames from the “V” to “M” shape. H₂-enriched lean premixed CH₄/H₂/air flames with H₂ fractions up to 80% were conducted. The flame structure was obtained with Planar Laser-Induced Fluorescence (PLIF) of the OH radical. Flow fields were measured with Particle Image Velocimetry (PIV). It was observed that the flame tip in the outer shear layer gradually propagated upstream and finally anchored to the injector with the hydrogen fractions increase, yielding the transition from the “V” to “M” flame. We examined the flame structures and the flame flow dynamics during the transition. The shape transition was directly related to the evolution of the corner flame along the outer shear layer. With H₂ addition, the outer recirculation zone first appeared downstream where the corner flame started to propagate upstream; then, the recirculation zone expanded upward to form a stable “M” flame gradually. The flow straining was observed to influence the stabilization of the outer shear layer flame significantly. This study can be useful for the understanding of recirculation-stabilized swirling flames with strong confinement. The flame structure and the flow characteristics of flames with a high H₂ content are also valuable for model validation.     

Turbulence and combustion interaction: High resolution local flame front structure visualization using simultaneous single-shot PLIF imaging of CH, OH, and CH2O in a piloted premixed jet flame

High resolution planar laser-induced fluorescence (PLIF) was applied to investigate the local flame front structures of turbulent premixed methane/air jet flames in order to reveal details about turbulence and flame interaction. The targeted turbulent flames were generated on a specially designed coaxial jet burner, in which low speed stoichiometric gas mixture was fed through the outer large tube to provide a laminar pilot flame for stabilization of the high speed jet flame issued through the small inner tube. By varying the inner tube flow speed and keeping the mixture composition as that of the outer tube, different flames were obtained covering both the laminar and turbulent flame regimes with different turbulent intensities. Simultaneous CH/CH₂O, and also OH PLIF images were recorded to characterize the influence of turbulence eddies on the reaction zone structure, with a spatial resolution of about 40 μm and temporal resolution of around 10 ns. Under all experimental conditions, the CH radicals were found to exist only in a thin layer; the CH₂O were found in the inner flame whereas the OH radicals were seen in the outer flame with the thin CH layer separating the OH and CH₂O layers. The outer OH layer is thick and it corresponds to the oxidation zone and post-flame zone; the CH₂O layer is thin in laminar flows; it becomes broad at high speed turbulent flow conditions. This phenomenon was analyzed using chemical kinetic calculations and eddy/flame interaction theory. It appears that under high turbulence intensity conditions, the small eddies in the preheat zone can transport species such as CH₂O from the reaction zones to the preheat zone. The CH₂O species are not consumed in the preheat zone due to the absence of H, O, and OH radicals by which CH₂O is to be oxidized. The CH radicals cannot exist in the preheat zone due to the rapid reactions of this species with O₂ and CO₂ in the inner-layer of the reaction zones. The local PLIF intensities were evaluated using an area integrated PLIF signal. Substantial increase of the CH₂O signal and decrease of CH signal was observed as the jet velocity increases. These observations raise new challenges to the current flamelet type models.