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1.
This paper presents numerical simulations and laser diagnostic experiments of a swirling lean premixed methane/air flame with an aim to compare different Large Eddy Simulations (LES) models for reactive flows. An atmospheric-pressure laboratory swirl burner has been developed wherein lean premixed methane/air is injected in an unconfined low-speed flow of air. The flame is stabilized above the burner rim in a moderate swirl flow, triggering weak vortex breakdown in the downstream direction. Both stereoscopic (3-component) PIV and 2-component PIV are used to investigate the flow. Filtered Rayleigh scattering is used to examine the temperature field in the leading flame front. Acetone-Planar Laser Induced Fluorescence (PLIF) is applied to examine the fuel distribution. The experimental data are used to assess two different LES models; one based on level-set G-equation and flamelet chemistry, and the other based on finite rate chemistry with reduced kinetics. The two LES models treat the chemistry differently, which results in different predictions of the flame dynamic behavior and statistics. Yet, great similarity of flame structures was predicted by both models. The LES and experimental data reveal several intrinsic features of the low swirl flame such as the W-shape at the leading front, the highly wrinkled fronts in the shear layers, and the existence of extinction holes in the trailing edge of the flame. The effect of combustion models, the numerical solvers and boundary conditions on the flame and flow predictions was systematically examined.  相似文献   

2.
The stability characteristics of a premixed, swirl-stabilized flame were studied to determine the effects of hydrogen addition on flame stability under fuel-lean conditions. The burner configuration consisted of a centerbody with an annular, premixed methane/air jet introduced through five, 45° swirl vanes. Flame stability was studied over a range of operating conditions. Under fuel-rich conditions the flame was lifted from the burner surface due to the mixing with entrained ambient air that was needed to form a flammable mixture. As the fuel/air mixture ratio was decreased toward stoichiometric, the resulting increase in flame speed allowed the flame to propagate upstream through the low-velocity wake region and attach to the centerbody face. The maximum blowout velocity occurred at stoichiometric conditions, and decreased as the mixture became leaner. OH PLIF measurements were used to study the behavior of OH mole fraction as the lean stability limit was approached. Near the lean stability limit the overall OH mole fraction decreased, the flame decreased in size and the high OH region took on a more shredded appearance. The addition of up to 20% hydrogen to the methane/air mixture resulted in a significant increase in the OH concentration and extended the lean stability limits of the burner.  相似文献   

3.
《Combustion and Flame》2003,132(1-2):58-72
The possible burning structures existing in two co-flowing combustible mixtures with different compositions, and their implications to the field of turbulent combustion are examined in this study. A coaxial burner with a quartz plate was used to experimentally investigate the flames of methane/air and propane/air mixtures propagating in a coaxial flow impinging onto a stagnation surface. The possible burning structures were observed to be: (1) a single-flame (a lean or rich premixed flame); (2) a double-flame (two lean or rich premixed flames, or a rich premixed flame and a diffusion flame); and (3) a triple-flame (a rich premixed flame, a diffusion flame and a lean premixed flame). An inner (or outer) mixture, far beyond the flammability limit, can still burn if a stronger outer (or inner) flame supports it. The extinction limit of the top part of the inner hat-shaped premixed flame is nearly independent of the burning intensity of the outer flame. It was found that the inner flame has a wider flammable region than the outer flame, and that the latter has a narrower flashback region than the former. Both propane and methane flames may exhibit flame-front instability, although the former displays much more clearly than the latter. Cellular and polyhedral instabilities can exist individually or appear simultaneously in the inner flame. However, only polyhedral (stripped-pattern) instability was observed in the outer flame. Finally, the experiments were analyzed theoretically using a simple geometrical model incorporated with the numerical simulations. The predicted shapes and locations of the flames are in good agreement with the experimental observations qualitatively.  相似文献   

4.
Experimental and numerical techniques to characterize the response of premixed methane-air flames to acoustic waves are discussed and applied to a multi-slit Bunsen burner. The steady flame shape, flame front kinematics and flow field of acoustically exited flames, as well as the flame transfer function and matrix are computed. The numerical results are compared with experiments. The influence of changes in the mean flow velocity, mixture equivalence ratio, slit width and distance between the slits on the transfer function is studied, both numerically and experimentally. Good agreement is found which indicates the suitability of both the experimental and numerical approach and shows the importance of predicting the influence of the flow on the flame and vice versa. On the basis of the results obtained, the role and physical nature of convective flow structures, heat transfer between the flame and burner plate and interaction between adjacent flames are discussed. Suggestions for analytical models of premixed flame-acoustics interaction are formulated.  相似文献   

5.
This paper describes a mechanism for the stabilization of ultra lean premixed methane/air flames by pulsed nonequilibrium plasma enhancement. It is shown that the pulsed discharge plasma produces a cool (~500–600 K) stream of relatively stable intermediate species including hydrogen (H2) and carbon monoxide (CO), which play a central role in enhancing flame stability. This stream is readily visualized by ultraviolet emission from electronically excited hydroxyl (OH) radicals. The rotational and vibrational temperature of this “preflame” are determined from its emission spectrum. Qualitative imaging of the overall flame structure is obtained by planar laser-induced fluorescence measurements of OH. Preflame nitric oxide (NO) concentrations are determined by gas sampling chromatography. A simple numerical model of this plasma enhanced premixed flame is proposed that includes the generation of the preflame through plasma activation, and predicts the formation of a dual flame structure that arises when the preflame serves to pilot the combustion of the surrounding non-activated premixed flow. The calculation represents the plasma through its ability to produce an initial radical yield, which serves as a boundary condition for conventional flame simulations. The simulations also capture the presence of the preflame and the dual flame structure, and predict preflame levels of NO comparable to those measured. A subsequent pseudo-sensitivity analysis of the preflame shows that flame stability is most sensitive to the concentrations of H2 and CO in the preflame. As a consequence of the role of H2 and CO in enhancing the flame stability, the blowout limit extensions of methane/air and hydrogen/air mixtures in the absence/presence of a discharge are investigated experimentally. For methane/air mixtures, the blowout limit of the current burner is extended by ~10% in the presence of a discharge while comparable studies carried out in lean hydrogen/air flames fail to extend this limit.  相似文献   

6.
为深入分析不同壁面导热率对微尺度燃烧器稳燃性能的影响,使用基于OpenFOAM框架开发的低马赫数反应流求解器,并结合DRM-19化学反应机理对正交各向热异性的微型平行平板内甲烷/空气预混火焰稳定性开展了数值模拟。模拟结果表明:相比于各向热同性壁面材料,正交各向热异性材料能够显著提升壁面对通道上游附近未燃气体的预热作用,同时减少燃烧器向外界环境的热损失,可达到提高火焰吹出极限的效果。  相似文献   

7.
Flame shapes and their transitions of premixed hydrogen enriched methane flames in a 3D-printed low-swirl burner are studied using simultaneous OH×CH2O planar laser induced fluorescence and stereoscopic particle image velocimetry. Three different flame shapes are observed, namely bowl-shape, W-shape, and crown-shape. The bowl-shaped flame has its base stabilized through flame-flow velocity balance and its sides stabilized in the inner shear layer. While the bulges of the W-shaped flame rely on a similar stabilization mechanism in the central flow, its outer edges are stabilized by large-scale eddies in the outer shear layer. The crown-shaped flame is also aerodynamically stabilized in the center, but its outer edges are anchored to the burner hardware. At a fixed equivalence ratio, the statistical transitions between flame shapes across test conditions are jointly dominated by hydrogen fraction and bulk velocity. Dynamically, W-to-crown transition is attributed to the upstream propagation and attachment of the flame outer edges.  相似文献   

8.
In the present paper, experimental investigations on the characterization of flame stabilization behavior in a 2.0 mm wide diverging channel are carried out with premixed methane–air mixtures. The effect of mixture equivalence ratio (Ф) and flow rate on flame shape, position, stability and emissions are reported in this work. The diverging portion of channel is preheated from the bottom side with a sintered metal burner to provide a positive temperature gradient along the direction of fluid flow which helps in stabilizing a flame in the channel. For a range of velocities and equivalence ratios, different types of stable and partially stable flame propagation modes were observed. Flames obtained for rich mixtures exhibited more stable nature as compared to lean mixtures. The flame stability limits were observed to vary between 0.2 m/s and 1.9 m/s for a range of mixture equivalence ratios.  相似文献   

9.
Experimental results are presented on the effect of methane content in a non-aromatic fuel mixture on the formation of aromatic hydrocarbons and soot in various fundamental combustion configurations. The systems considered consist of a laminar flow reactor, a laminar co-flow diffusion flame burner, and a laminar, premixed flame burner, all of which operate at atmospheric pressure. In the flow reactor, the experiments are performed at 1430 K, constant C-atom flow rates, 98% nitrogen dilution, C/O ratio = 2, and with fuel mixtures consisting of ethylene and methane. The diffusion flames are performed with fuel mixtures of methane and ethylene diluted in nitrogen to maintain a constant adiabatic flame temperature. The premixed flame experiments are performed with n-heptane and methane mixtures at a C/O ratio = 0.67 with nitrogen-impoverished air. The results show the existence of synergistic chemical effects between methane and other alkanes in the production of aromatics, despite reduced acetylene concentrations. This effect is attributable to the ability of methane to enhance the production of methyl radicals that will then promote production channels of aromatics that rely on odd-carbon-numbered species. Benzene, naphthalene, and pyrene show the strongest sensitivity to the presence of added methane. This synergy on aromatics trickles down to soot via enhanced inception and surface growth rates by polycyclic aromatic hydrocarbon condensation, but the overall effects on soot volume-fraction are smaller due to a compensating reduction in surface growth from acetylene. These results are observed under the very fuel-rich environments existing in the flow reactor and diffusion flames. In the premixed flames, however, instabilities did not permit investigation of conditions with sufficiently high equivalence ratios to perturb the aromatic and soot-growth regions.  相似文献   

10.
In premixed turbulent combustion, reaction rates can be estimated from the flame surface density. This parameter, which measures the mean flame surface area available per unit volume, may be obtained from algebraic expressions or by solving a transport equation. In this study, detailed measurements were performed on a Bunsen-type burner fed with methane/air mixtures in order to determine the local flame surface density experimentally. This burner, located in a high-pressure combustion chamber, allows investigation of turbulent premixed flames under various flow, mixture, and pressure conditions. In the present work, equivalence ratio was varied from 0.6 to 0.8 and pressure from 0.1 to 0.9 MPa. Flame front visualizations by Mie scattering laser tomography are used to obtain experimental data on the instantaneous flame front dynamics. The exact equation given by Pope is used to obtain flame surface density maps for different flame conditions. Some assumptions are made in order to access three-dimensional information from our two-dimensional experiments. Two different methodologies are proposed and tested in term of global mass balance (what enters compared to what is burned). The detailed experimental flame surface data provided for the first time in this work should progressively allow improvement of turbulent premixed flame modeling approaches.  相似文献   

11.
Formation of NOx in counterflow methane/air triple flames at atmospheric pressure was investigated by numerical simulation. Detailed chemistry and complex thermal and transport properties were employed. Results indicate that in a triple flame, the appearance of the diffusion flame branch and the interaction between the diffusion flame branch and the premixed flame branches can significantly affect the formation of NOx, compared to the corresponding premixed flames. A triple flame produces more NO and NO2 than the corresponding premixed flames due to the appearance of the diffusion flame branch where NO is mainly produced by the thermal mechanism. The contribution of the N2O intermediate route to the total NO production in a triple flame is much smaller than those of the thermal and prompt routes. The variation in the equivalence ratio of the lean or rich premixed mixture affects the amount of NO formation in a triple flame. The interaction between the diffusion and the premixed flame branches causes the NO and NO2 formation in a triple flame to be higher than in the corresponding premixed flames, not only in the diffusion flame branch region but also in the premixed flame branch regions. However, this interaction reduces the N2O formation in a triple flame to a certain extent. The interaction is caused by the heat transfer and the radical diffusion from the diffusion flame branch to the premixed flame branches. With the decrease in the distance between the diffusion flame branch and the premixed flame branches, the interaction is intensified.  相似文献   

12.
In the present study, the air turbulator, which is a part of a nonpremixed burner, is investigated numerically in terms of its effects on the diffusion methane flame structure and NOX emissions. A computational fluid dynamics (CFD) code was used for the numerical analysis. At first, four experiments were conducted using natural gas fuel. In the experimental studies, the excess air ratio was taken constant as 1.2, while the fuel consumption rate was changed between 22 and 51 Nm3/h. After the experimental studies, the CFD studies were carried out. Pure methane was taken as fuel for the simulations. The nonpremixed combustion model with the steady laminar flamelet model (SFM) approach was used in the combustion analyses. Methane‐air extinction mechanism with 17 species and 58 reactions was used for the simulations. The results obtained from the CFD studies were confronted with the measurements of the flue gas emissions in the experimental studies. Then, a modified burner head was analysed numerically for the different air turbulator blade numbers and angles. The CFD results show that increasing the air turbulator blade number and angle causes the thermal NO emissions to be reduced in the flue gas by making the flame in the combustion chamber more uniform than the original case. This new flame structure provides better mixing of the fuel and combustion air. Thus, the diffusion flame structure in the combustion chamber takes the form of the partially premixed flame structure. The maximum reduction in the thermal NO emissions in the flue gas is achieved at 38% according to the original case.  相似文献   

13.
Preferential species diffusion is known to have important effects on local flame structure in turbulent premixed flames, and differential diffusion of heat and mass can have significant effects on both local flame structure and global flame parameters, such as turbulent flame speed. However, models for turbulent premixed combustion normally assume that atomic mass fractions are conserved from reactants to fully burnt products. Experiments reported here indicate that this basic assumption may be incorrect for an important class of turbulent flames. Measurements of major species and temperature in the near field of turbulent, bluff-body stabilized, lean premixed methane–air flames (Le = 0.98) reveal significant departures from expected conditional mean compositional structure in the combustion products as well as within the flame. Net increases exceeding 10% in the equivalence ratio and the carbon-to-hydrogen atom ratio are observed across the turbulent flame brush. Corresponding measurements across an unstrained laminar flame at similar equivalence ratio are in close agreement with calculations performed using Chemkin with the GRI 3.0 mechanism and multi-component transport, confirming accuracy of experimental techniques. Results suggest that the large effects observed in the turbulent bluff-body burner are cause by preferential transport of H2 and H2O through the preheat zone ahead of CO2 and CO, followed by convective transport downstream and away from the local flame brush. This preferential transport effect increases with increasing velocity of reactants past the bluff body and is apparently amplified by the presence of a strong recirculation zone where excess CO2 is accumulated.  相似文献   

14.
We report on the application of simultaneous single-shot imaging of CH and OH radicals using planar laser-induced fluorescence (PLIF) to investigate partially premixed turbulent jet flames. Various flames have been stabilized on a coaxial jet flame burner consisting of an outer and an inner tube of diameter 22 and 2.2 mm, respectively. From the outer tube a rich methane/air mixture was supplied at a relatively low flow velocity, while a jet of pure air was introduced from the inner one, resulting in a turbulent jet flame on top of a laminar pilot flame. The turbulence intensity was controlled by varying the inner jet flow speed from 0 up to 120 m/s, corresponding to a maximal Reynolds number of the inner jet airflow of 13,200. The CH/OH PLIF imaging clearly revealed the local structure of the studied flames. In the proximity of the burner, a two-layer reaction zone structure was identified where an inner zone characterized by strong CH signals has a typical structure of rich premixed flames. An outer reaction zone characterized by strong OH signals has a typical structure of a diffusion flame that oxidizes the intermediate fuels formed in the inner rich premixed flame. In the moderate-turbulence flow, the CH layers were very thin closed surfaces in the entire flame, whereas the OH layers were much thicker. In the high-intensity-turbulence flame, the CH layer remained thin until it vanished in the upper part of the flame, showing local extinction and reignition behavior of the flame. The single-shot PLIF images have been utilized to determine the flame surface density (FSD). In low and moderate turbulence intensity cases the FSDs determined from CH and OH agreed with each other, while in the highly turbulent case a locally broken CH layer was observed, leading to a significant difference in the FSD results determined via the OH and CH radicals. Furthermore, the means and the standard deviations of CH and OH radicals were obtained to provide statistical information about the flames that may be used for validation of numerical calculations.  相似文献   

15.
The structures and dynamics of unsteady laminar partially premixed methane/air Bunsen flames are studied by means of numerical simulations, OH and CH PLIF imaging, and high speed chemiluminescence imaging employing a high framing speed intensified charge coupled device camera. The Bunsen burner has a diameter of 22 mm. Rich methane/air mixtures with an equivalence ratio of 1.5 are injected from the burner into atmosphere at different flow speeds ranging from 0.77 to 1.7 m/s, with Reynolds numbers based on the nozzle flow ranging from 1100 to 2500. The numerical simulations are based on a two-scalar flamelet manifold tabulation approach. Detailed chemistry is used to generate the flamelet manifold tabulation which relates the species concentrations, reaction rates, temperature and density to a distance function G and mixture fraction Z. Two distinct reaction zones are identified using CH and OH PLIF imaging and numerical simulations; one inner reaction zone corresponds to premixed flames on the rich side of the mixture and one outer reaction zone corresponds to mixing controlled diffusion flames on the lean side of the mixture. Under normal gravity conditions both the inner premixed flames and the outer diffusion flames are unsteady. The outer diffusion flames oscillate with a flickering frequency of about 15 Hz, which slightly increases with the burner exit velocity. The inner premixed flames are more random with much more small-scale wrinkling structures. Under zero gravity conditions the outer diffusion flames are stable whereas the inner premixed flames are unstable and highly wrinkled. It appears that the outer diffusion flames are governed by the Rayleigh-Taylor instability whereas the inner premixed flames are dictated by Landau-Darrieus instability. The two-scalar flamelet approach is shown to capture the basic structures and dynamics of the investigated unsteady partially premixed flames.  相似文献   

16.
Measuring the velocities of premixed laminar flames with precision remains a controversial issue in the combustion community. This paper studies the accuracy of such measurements in two-dimensional slot burners and shows that while methane/air flame speeds can be measured with reasonable accuracy, the method may lack precision for other mixtures such as hydrogen/air. Curvature at the flame tip, strain on the flame sides and local quenching at the flame base can modify local flame speeds and require corrections which are studied using two-dimensional DNS. Numerical simulations also provide stretch, displacement and consumption flame speeds along the flame front. For methane/air flames, DNS show that the local stretch remains small so that the local consumption speed is very close to the unstretched premixed flame speed. The only correction needed to correctly predict flame speeds in this case is due to the finite aspect ratio of the slot used to inject the premixed gases which induces a flow acceleration in the measurement region (this correction can be evaluated from velocity measurement in the slot section or from an analytical solution). The method is applied to methane/air flames with and without water addition and results are compared to experimental data found in the literature. The paper then discusses the limitations of the slot-burner method to measure flame speeds for other mixtures and shows that it is not well adapted to mixtures with a Lewis number far from unity, such as hydrogen/air flames.  相似文献   

17.
The effect of hydrogen addition in methane–air premixed flames has been examined from a swirl-stabilized combustor under unconfined flame conditions. Different swirlers have been examined to investigate the effect of swirl intensity on enriching methane–air flame with hydrogen in a laboratory-scale premixed combustor operated at 5.81 kW. The hydrogen-enriched methane fuel and air were mixed in a pre-mixer and introduced into the burner having swirlers of different swirl vane angles that provided different swirl strengths. The combustion characteristics of hydrogen-enriched methane–air flames at fixed thermal load but different swirl strengths were examined using particle image velocimetry (PIV), OH chemiluminescence, gas analyzers, and micro-thermocouple diagnostics to provide information on flow field, combustion generated OH radical and gas species concentration, and temperature distribution, respectively. The results show that higher combustibility of hydrogen assists to promote faster chemical reaction, raises temperature in the reaction zone and reduces the recirculation flow in the reaction zone. The upstream of flame region is more dependent on the swirl strength than the effect of hydrogen addition to methane fuel. At lower swirl strength condition the NO concentration in the reaction zone reduces with increase in hydrogen content in the fuel mixture. Higher combustibility of hydrogen accelerates the flow to reduce the residence time of hot product gases in the high temperature reaction zone. At higher swirl strength the NO concentration increases with increase in hydrogen content in the fuel mixture. The effect of dynamic expansion of the gases with hydrogen addition appears to be more dominant to reduce the recirculation of relatively cooler gases into the reaction zone. NO concentration also increases with decrease in the swirl strength.  相似文献   

18.
The utilization of hydrogen as a fuel in free jet burners faces particular challenges due to its special combustion properties. The high laminar and turbulent flame velocities may lead to issues in flame stability and operational safety in premixed and partially premixed burners. Additionally, a high adiabatic combustion temperature favors the formation of thermal nitric oxides (NO). This study presents the development and optimization of a partially premixed hydrogen burner with low emissions of nitric oxides. The single-nozzle burner features a very short premixing duct and a simple geometric design. In a first development step, the design of the burner is optimized by numerical investigation (Star CCM+) of mixture formation, which is improved by geometric changes of the nozzle. The impact of geometric optimization and of humidification of the combustion air on NOx emissions is then investigated experimentally. The hydrogen flame is detected with an infrared camera to evaluate the flame stability for different burner configurations. The improved mixture formation by geometric optimization avoids temperature peaks and leads to a noticeable reduction in NOx emissions for equivalence ratios below 0.85. The experimental investigations also show that NOx emissions decrease with increasing relative humidity of combustion air. This single-nozzle forms the basis for multi-nozzle burners, where the desired output power can flexibly be adjusted by the number of single nozzles.  相似文献   

19.
A two-dimensional laminar premixed flame is stabilized over a burner in a confined duct and is subjected to external acoustic forcing from the downstream end. The equivalence ratio of the flame is 0.7. The flame is stabilized in the central slot of a three-slotted burner. The strength of the shear layer of the cold reactive mixture through the central slot is controlled by the flow rate of cold nitrogen gas through the side slots. The frequency range of acoustic excitation is 400-1200 Hz, and the amplitude levels are such that the acoustic velocity is less than the mean flow velocity of the reactants. Time-averaged chemiluminescence images of the perturbed flame front display time-mean changes as compared to the unperturbed flame shape at certain excitation frequencies. Prominent changes to the flame front are in the form of stretching or shrinkage, asymmetric development of its shape, increased/preferential lift-off of one or both of the stabilization points of the flame, and nearly random three-dimensional fluctuations over large time scales under some conditions. The oscillations of the shear layer and the response of the confined jet of the hot products to the acoustic forcing, such as asymmetric flow development and jet spreading, are found to be responsible for the observed mean changes in the flame shape. A distinct low-frequency component (∼60-90 Hz) relative to the excitation frequency is observed in the fluctuations of the chemiluminescent intensity in the flame under most conditions. It is observed that fluctuations in the flame area predominantly contribute to the origin of the low-frequency component. This is primarily due to the rollup of vortices and the generation of enthalpy waves at the burner lip. Both of these processes are excited at the externally imposed acoustic time scale, but convect/propagate downstream at the flow time scale, which is much larger.  相似文献   

20.
A combined experimental and numerical study has been conducted to determine the stagnation point heat transfer for laminar methane/air flame impinging on a flat surface. Effects of Reynolds number, equivalence ratio and burner diameter on stagnation point heat flux were examined experimentally at different separation heights. Maximum stagnation point heat flux was obtained when the flat surface was closest to the tip of the inner premixed reaction zone. Heat flux decreased along the axial direction when the separation distance was further increased from the tip of inner reaction zone. There was a secondary rise in heat flux at the stagnation point at larger separation distances. Correlations were developed for stagnation point Nusselt number. Numerical simulations were carried out using a commercial CFD code (FLUENT) for laminar methane/air flame impinging on a flat surface for various separation distances. Results were compared with those found experimentally. The reason for conducting the simulations was to (a) gain more insight into how the presence of the plate affects the flame and the flow and temperature fields and (b) to explain the reason for high heat flux when the tip of the inner reaction zone was very close to the stagnation point.  相似文献   

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