Sound Experiments on Superfluidity of 3He in Highly Porous Aerogels

We have carried out sound experiments on superfluid ³ He in three highly porous aerogels with different porosities. Two of the acoustic cells contain aerogels inside the pores in roughly sintered silver powder to avoid the vibration of the aerogel. In these acoustic cells we have detected fourth sound, and extracted the superfluid density from the fourth sound velocity. The effect of the sintered silver on superfluid ³ He was examined by using another acoustic cell which contains the sintered silver without aerogel. The size of the pores in the sintered silver was large enough not to show the size effect of superfluid ³ He and small enough to observe fourth sound of ³ He. In another cell without sintered silver, we have observed second-sound-like signal. The superfluid transition temperatures of ³ He are suppressed more in higher density aerogel. The aerogel density dependence of the suppression of the superfluid transition temperature of ³ He in aerogel can be explained qualitatively by the simple s-wave scattering approximation. However, the superfluid density shows quite different pressure-dependence in different porous aerogels. The reason of this phenomenon is not understood yet.     

A Preliminary Heat Capacity Measurement of 3He in Aerogel near its Superfluid Transition

We report simultaneous heat capacity and torsional oscillator measurement of ³ He in aerogel near the superfluid transition. The heat capacity has a peak at the temperature T_c where the torsional oscillator shows the onset of superfluid decoupling. The coincidence of these signatures suggests that ³ He in aerogel does undergo a true thermodynamic transition.     

Novel Oscillating Aerogel Experiments in Superfluid 3He at Ultralow Temperatures

We present novel experiments on a disk of 98% aerogel oscillating in superfluid ³ He at ultralow temperatures. The aerogel dik is attached to a goal post shaped vibrating wire resonator and immersed in liquid ³ He cooled by a Lancaster style nuclear cooling stage. At low pressures we see no evidence for superfluidity within the aerogel down to our base temperature of below <0.11T_c. At higher pressures we observe large temperature dependent frequency shifts, reminiscent of torsional oscillator experiments. We find the transition temperature at 5 bar to be around 600K. The response of the resonator is highly non linear when the helium in the aerogel is superfluid. The resonant frequency decreases strongly with increasing wire amplitude. This offers an exciting new technique for measuring the superfluid properties of ³ He in aerogel in the ultralow temperature regime.     

The Tricritical Region for Helium Mixtures in 0.87 Porosity Aerogel

We have used ultrasonic velocity measurements to study ³ He- ⁴ He mixtures in aerogel with a porosity 0.87. The phase diagram resembles that of bulk mixtures, with a single transition for ³ He-rich mixtures, in contrast to the detached phase separation curve seen in 0.98 porosity aerogel. A kink in the lambda line at a 3He concentration of X _C =0.51 suggests that the phase separation line meets it at a tricritical point. We have measured the amount of superfluid which decouples both at low temperature and close to the superfluid transition, as functions of ³ He concentration. Each showed a sudden change at the concentration where the kink appeared in the lambda line, suggesting an abrupt change in the morphology of the superfluid phase in the mixtures. Similar measurements were made for pure 4He films on the same aerogel. We discuss the nature of ³ He-rich mixtures in aerogels based on these experiments.     

Impurity Scattering Effect on Superfluidity of 3He in Aerogel

The impurity scattering effect on superfluid ³ He in aerogel is studied on the basis of the standard impurity theory within the weak coupling limit. We discuss the superfluid transition temperature and the superfluid density in the dirty Fermi liquid. The results are compared with recent experiments on the superfluidity of ³ He in aerogel. The low pressure data of the observed superfluid density are shown to be in better agreement with the results for the A-phase than for the B-phase. The B-phase results show considerable disagreement with the low pressure data.     

Effect of Strong Magnetic Fields on Superfluid 3He in 98% Porosity Aerogel

No Heading We report our results of shear acoustic impedance measurements performed on superfluid ³He in 98% porosity silica aerogel. Experiments in high porosity aerogel provide unique opportunity to study the influence of disorder on a p-wave superfluid and compare the behavior with that of the well understood pure bulk. Our experiment is designed to detect acoustic signatures from both bulk liquid and liquid in aerogel. In the past, experiments on ³He in aerogel have been conducted in zero or low magnetic fields (< 1 tesla). We made measurements in magnetic fields as high as 15 tesla at 28.4 and 33.5 bars and observed a new phase in aerogel induced by magnetic fields splitting the superfluid transition into two.PACS numbers: 67.57Pq, 67.80Mg     

Soliton-Like Spin State in the A-Like Phase of 3He in Anisotropic Aerogel

We have found a new stable spin state in the A-like phase of superfluid ³He confined to intrinsically anisotropic aerogel. The state can be formed by radiofrequency excitation applied while cooling through the superfluid transition temperature and its NMR properties are different from the standard A-like phase obtained in the limit of very small excitation. It is possible that this new state is formed by textural domain walls pinned by aerogel.      

Superfluid helium three in aerogel

We report measurements of the superfluid density and transition temperature of³He confined within 98.2% open aerogel. Both the superfluid fraction and the temperature at which the superfluid is manifested are suppressed strongly from their bulk values. The results suggest that the aerogel reduces the order parameter by a mechanism other than as a diffusely scattering surface.     

The Thermal Conductivity of Superfluid 3He in Aerogel: A Measurement of the Energy Gap

Transport properties of superfluid ³ He in aerogel are governed by a fixed mean free path set by the typical dimensions of the strand separation. We describe preliminary measurements of the thermal conductivity of superfluid ³ He confined in 98% silica aerogel. The majority of the measurements are made in relatively high magnetic fields where the superfluid within the aerogel is in the A-phase like state. Since the quasiparticle mean free path is fixed, the temperature dependence of the thermal conductivity depends only on the superfluid energy gap and on the texture in the case of the A-phase. The results so far obtained are broadly consistent with the aerogel-confined superfluid having a temperature dependent energy gap close to the BCS prediction although there are significant deviations at the lowest temperatures.     

Transverse Acoustic Spectroscopy of Superfluid 3He in Compressed Aerogel

The unique nanoporous structure of aerogel provides a rare opportunity to study the role of anisotropic disorder on an anisotropic superfluid ³He. It has been proposed that uniaxial deformation of compliant aerogel would induce global anisotropy and a few compelling effects of global anisotropy on nature of the superfluid phases have been predicted. We measured high frequency shear acoustic impedance in superfluid ³He at 32 bar in a commercially available 98% porosity aerogel under uniaxial compression. At 5% compression, we found evidence of an A-like phase stabilized in a wider temperature width than the A-like phase in uncompressed aerogel.     

NMR Study of Superfluid Phases of 3He Confined in 97.5% Porous Silica Aerogel

We have studied the scattering effect from aerogel strands on superfluid phases of ³He by a cw NMR method at 920 kHz. Liquid ³He at a pressure of 13 bar was confined in 97.5% porous aerogel from the same batch as that of a recent 4th sound study. The NMR experiment was performed in a magnetic field of 28.4 mT down to 0.3 mK. As temperature decreased, the NMR resonant frequency increased below 0.76 mK. The temperature of 0.76 mK agrees with the superfluid transition temperature T ^aerogel _c observed in the 4th sound study at the same pressure. Below T ^aerogel _c the behavior of thefrequency shift as a function of temperature indicates that there is no phasetransition to the other superfluid phase down to about 0.4 T ^aerogel _c . Owing to a very large surface solid ³He magnetization, we could not determine the superfluid phase of ³He in the aerogel in the magnetization measurement.     

The Equilibrium A-B Transition in Low Density Aerogels

No Heading We have measured in detail the NMR spectra of superfluid ³ He inside two different silica aerogels, one with a porosity of 99.3% and the other 98.6%. From these spectra, we are able to determine the equilibrium A-B transition temperatures in both aerogel samples as a function of hydrostatic pressure. We find that the slope of the reduced A-B transition temperature, 1- T_AB/T_c, vs. pressure is only about one third that seen for the bulk A-B transition, despite the fact the T_c for the two samples is suppressed very modestly, by only 4% and 8% at 34 bars. We argue from this that the presence of the aerogel stabilizes an equal-spin pairing which is district from that stable in the bulk.PACS numbers: 67.57 Pq, 67.57 Lm     

Capture of Superfluid Helium by Porous Structures

We have studied superfluid helium capture in a sample of silica aerogel of 98.2% porosity in the temperature range from 1.22 K up to 1.89 K. The high retention of He in the aerogel sample corresponds to a similar phenomenon in impurity-helium condensates, in which very high values of the ratio of helium atoms to impurity atoms (up to 60) have been seen. We have observed that removing the aerogel sample from superfluid helium in a cylindrical glass beaker caused a decrease of the helium level corresponding to the geometrical volume of the sample (≈1 cm³). This observation has allowed us to conclude that superfluid helium is completely captured by the porous sample. Superfluid helium filling aerogel and impurity-helium samples (porous structures) serves as a dispersive medium of gel-like samples which interacts strongly with impurity nanoclusters forming the dispersing system.      

3He-4He Mixtures in 95% Porous Aerogel

Torsional oscillator measurements of ³ He- ⁴ He mixtures in 95% porous aerogel found a phase diagram similar to that in 98% porous aerogel. The coexistence boundary on the ³ He rich side resides very close to, but nevertheless is detached from the superfluid transition line. Together with the findings in 98%, 87%, and 99.5% porous aerogel, this result supports the interpretation that the phase separation of ³ He- ⁴ He mixture in aerogel is induced by the capillary condensation of ⁴ He films from neighboring silica strands into ⁴ He rich domains.     

Impurity Scattering Effect on Superfluid Phases of 3He in 97.5% Porous Silica Aerogel

No Heading NMR studies of superfluid ³He in 97.5% aerogel have been performed in a magnetic field of 28.4 mT. A small-angle neutron scattering experiment on the structure of the aerogel shows that the average separation distance of silica strands is 54 nm. The aerogel strands were covered with a few layers of solid ³He whose magnetization shows Curie-Weiss behaviour. On cooling process A-like phase appeared at suppressed superfluid transition temperature T_C^aero and B-like phase appeared at lower temperatures although only the B-like phase was observed up to T_C^aero on warming process above 2.1 MPa. The superfluid transitions in aerogel always occur below the AB phase transition temperature of bulk liquid at all pressures. An isotropic inhomogeneous scattering model(IISM) proposed by Thuneberg et al. explained well the observed suppressed T_C^aero in 97.5% with the radius 59 nm of voids in this model. This radius is similar with the average strand separation distance of 54 nm measured in the structural analysis. This similarity of two lengths shows the connection of the suppression of T_C^aero with the actual average separation distance of the silica strands.PACS numbers: 67.57.Pq, 67.80.Jd     

Acoustic Spectroscopy of Superfluid 3He in Aerogel in the Presence of a Magnetic Field

We have constructed a silver alloy cell to investigate low frequency sound propagation in ³ He-filled aerogel at various magnetic fields. In this apparatus, two sound modes were observed in the superfluid phase. We observed both the first sound-like mode (fast mode) which is a compression wave also seen in the normal state and the second sound-like mode (slow mode) which is attributed to the out-of-phase oscillation of the superfluid and normal components of ³ He clamped to the aerogel matrix. The values of T_c and _s can be extracted from the analysis of these two modes. In addition, a Helmholtz resonance provides an in-situ signature of the bulk superfluid transition and allows us to also determine the bulk _s. By measuring these quantities over a range of applied magnetic fields we hope to explore the P, T, H phase diagram of ³ He in aerogel.     

Phase separation of3He-4He mixture in aerogel

Torsional oscillator measurements of ³ He- ⁴ He mixtures confined in aerogel show evidence of a well defined phase separation region. This region is detached from the superfluid transition line, opening up a region of miscible superfluid mixture at high ³ He concentration.     

Phase Transition of Superfluid 3He in Aerogel

We have studied phase transition of superfluid ³He in 97.5% porosity aerogel by NMR method. Above 1.0 MPa, superfluid phase transition has been observed. The transition temperature T _c ^a is strongly suppressed from its bulk value. The Pressure-Temperature diagram suggests that superfluid phase will not appear below near 0.8 MPa. The A-B phase transition has been observed above 1.3 MPa, below which a state of superfluid phases remains to be identified. The temperature dependence of NMR frequency shifts Δf in the A-like and the B-like phases are almost linear at pressures below 2.4 MPa. We obtained the differential coefficient of NMR frequency shifts ∂(Δf)/∂(T/T _c ^a ) at 0.9T _c ^a as a function of pressure, and it suggests that superfluid phase will not appear below near 0.8 MPa which is the same pressure estimated by P-T diagram.     

Acoustical Experiments on Superfluid 3He-4He Mixtures in Aerogel

This report discusses our results on the superfluidity of ³ He- ⁴ He mixtures in a 98% porosity silica aerogel. We have used low frequency sound to probe helium mixtures confined to aerogel, and have observed both the slow mode of superfluid ³ He in aerogel, which is manifested only below T_c, and an additional sound mode present only in the mixture. We attribute this novel sound mode to the slow-mode in the ⁴ He rich phase of the dilute ³ He- ⁴ He mixture. This mode exhibits positive frequency shifts below T_c in aerogel, while above T_c the mode is observed at a temperature independent frequency until close to T where it shifts to zero frequency.     

Absolute Ultrasound Attenuation Measurements in Superfluid 3He in 98% Aerogel by Direct Transmission

Systematic investigations on the effect of static disorder on p-wave superfluid ³He have been made possible by utilizing the unique structure of high porosity silica aerogel. For the past 10 years, a burst of experimental efforts revealed that three distinct superfluid phases exists. We have performed longitudinal ultrasound (9.5 MHz) attenuation measurements in the B-phase of the superfluid ³He in 98% aerogel. The absolute attenuation was determined by direct propagation of sound pulses through the medium in a wide range of temperatures, down to 200 μK, for sample pressures of 10 and 29 bars. Our results provide direct information on the zero-energy density of states of the superfluid phase in aerogel originating from impurity scattering.