Theoretical Study on the Characteristics of Atmospheric Radio Frequency Discharges by Altering Electrode Gap

In this paper, we present a theoretical study on the discharge characteristics of radio-frequency discharges at atmospheric pressure driven by a higher frequency of 40.68 MHz while the electrode gap is altered. Based on the analytical equations and simulation data from a one-dimensional fluid model, an optimal gap between electrodes, at which the largest electron density is obtained, can be observed under a constant power condition; however, as the electrode gap increases the time-averaged electron temperature decreases, and the underpinning physics is also discussed based on the simulation results. This study indicates that at a constant power by choosing an appropriate electrode spacing, the rf discharge can be effectively optimized at atmospheric pressure.     

An Experimental Study on Atmospheric Pressure Glow Discharge in Different Gases

Usually,the electrical breakdown of dielectric barrier discharge(DBD) at atmospheric pressure leads to a filamentary non-homogeneous discharge,However,it is also possible to obtain a diffuse DBD in homogeneous form,called atmospheric pressure glow discharge(APGD).We obtained a uniform APGD in helium and in the mixture of argon with alcohol,and studied the electrical characteristics of helium APGD.It if found that the relationship between discharge current and source frequency is different depending on the difference in gas gap when the applied voltage is kept constant.The discharge current shows an increasing trend with the increased frequency when gas gap is 0.8cm ,but the discharge current tends to decrease with the increased frequency when the gas gap increases.The discharge current always increases with the increased applied voltage when the source frequency is kept constant.We also observed a glow-like discharge in nitrogen at atmospheric pressure.     

Investigation on discharge characteristics of a coaxial dielectric barrier discharge reactor driven by AC and ns power sources

A coaxial dielectric barrier discharge(DBD) reactor with double layer dielectric barriers has been developed for exhaust gas treatment and excited either by AC power or nanosecond(ns)pulse to generate atmospheric pressure plasma. The comparative study on the discharge characteristics of the discharge uniformity, power deposition, energy efficiency, and operation temperature between AC and ns pulsed coaxial DBD is carried out in terms of optical and electrical characteristics and operation temperature for optimizing the coaxial DBD reactor performance. The voltages across the air gap and dielectric layer and the conduction and displacement currents are extracted from the applied voltages and measured currents of AC and ns pulsed coaxial DBDs for the calculation of the power depositions and energy efficiencies through an equivalent electrical model. The discharge uniformity and operating temperature of the coaxial DBD reactor are monitored and analyzed by optical images and infrared camera. A heat conduction model is used to calculate the temperature of the internal quartz tube. It is found that the ns pulsed coaxial DBD has a much higher instantaneous power deposition in plasma, a lower total power consumption, and a higher energy efficiency compared with that excited by AC power and is more homogeneous and stable. The temperature of the outside wall of the AC and ns pulse excited coaxial DBD reaches 158 ℃ and 64.3 ℃ after 900 s operation, respectively.The experimental results on the comparison of the discharge characteristics of coaxial DBDs excited by different powers are significant for understanding of the mechanism of DBDs,reducing energy loss, and optimizing the performance of coaxial DBD in industrial applications.     

Simulated and experimental studies on the array dielectric barrier discharge of water electrodes

A kind of dielectric barrier discharge(DBD) device composed of water electrodes with 3×3forms can produce large-area low-temperature plasmas at atmospheric pressure.To reflect the discharge characteristics of DBD better,a dynamic simulation model,which is based on the voltage controlled current source(CCS),is established,then the established model in Matlab/Simulink is used to simulate the DBD in air.The voltage-current waves and Lissajous at a voltage of 10 kV,11 kV and 12 kV peak value with a frequency of 15 kHz are studied.The change of the discharge power of DBD with a different amplitude and frequency of applied voltage is also analyzed.The result shows the voltage-current waves,Lissajous and discharge power of DBD under different conditions from the simulation agree well with those of the experiment.In addition,we propose a method to calculate the dielectric barrier capacitance C_d and the gap capacitance C_g,which is valid through analyzing the variation of capacitance at different voltage amplitudes.     

Numerical simulation and analysis of lithium plasma during low-pressure DC arc discharge

Alkali metal DC arc discharge has the characteristics of easy ionization, low power consumption, high plasma temperature and ionization degree, etc, which can be applied in aerospace vehicles in various ways. In this paper, we calculate the physical property parameters of lithium vapor, one of the major alkali metals, and analyze the discharge characteristics of lithium plasma with the magnetohydrodynamic (MHD) model. The discharge effects between constant current and voltage sources are also compared. It is shown that the lithium plasma of DC arc discharge has relatively high temperature and current density. The peak temperature can reach tens of thousands of K, and the current density reaches 6×10 ⁷ A⁻² . Under the same rated power, the plasma parameters of the constant voltage source discharge are much higher than those of the constant current source discharge, which can be used as the preferred discharge mode for aerospace applications.     

Effects of O2 addition on the plasma uniformity and reactivity of Ar DBD excited by ns pulsed and AC power supplies

Dielectric barrier discharges (DBDs) have been widely used in ozone synthesis, materials surface treatment, and plasma medicine for their advantages of uniform discharge and high plasma-chemical reactivity. To improve the reactivity of DBDs, in this work, the O₂ is added into Ar nanosecond (ns) pulsed and AC DBDs. The uniformity and discharge characteristics of Ar ns pulsed and AC DBDs with different O₂ contents are investigated with optical and electrical diagnosis methods. The DBD uniformity is quantitatively analyzed by gray value standard deviation method. The electrical parameters are extracted from voltage and current waveforms separation to characterize the discharge processes and calculate electron density n_e. The optical emission spectroscopy is measured to show the plasma reactivity and calculate the trend of electron temperature T_e with the ratio of two emission lines. It is found that the ns pulsed DBD has a much better uniformity than AC DBD for the fast rising and falling time. With the addition of O₂, the uniformity of ns pulsed DBD gets worse for the space electric field distortion by O₂⁻, which promotes the filamentary formation. While, in AC DBD, the added O₂ can reduce the intensity of filaments, which enhances the discharge uniformity. The ns pulsed DBD has a much higher instantaneous power and energy efficiency than AC DBD. The ratio of Ar emission intensities indicates that the T_e drops quickly with the addition of O₂ both ns pulsed and AC DBDs and the ns pulsed DBD has an obvious higher T_e and n_e than AC DBD. The results are helpful for the realization of the reactive and uniform low temperature plasma sources.     

Multiple current peaks and spatial characteristics of atmospheric helium dielectric barrier discharges with repetitive unipolar narrow pulse excitation

Atmospheric dielectric barrier discharges driven by repetitive unipolar narrow pulse excitation are investigated numerically by using one-dimensional fluid models.The one-dimensional simulation focuses on the effects of applied voltage amplitude,pulse repetition frequency,gap width and γ coefficient on the multiple-current-pulse (MCP) discharge.The results indicate that the MCP behavior will lead to the stratification of electron density distribution in axial direction.Traditional MCP manipulating methods,such as reducing the applied voltage amplitude,increasing the applied voltage frequency,adjusting the gap width,cannot regulate MCPs exhibiting in this work.Further analyses reveal that the increasing electric field of the cathode fall region is the basis for the emergence of MCP behavior.     

On peak current in atmospheric pulse-modulated microwave discharges by the PIC-MCC model

Pulse modulation provides a new way to tailor the electron density,electron energy and gas temperature in atmospheric radio-frequency (rf) discharges.In this paper,by increasing the rf frequency to several hundreds of MHz,or even much higher to the range of GHz,a very strong peak current in the first period (PCFP) with much larger electron energy can be formed during cthe power-on phase,which is not observed in the common pulse modulation discharges at a rf frequency of 13.56 MHz.The PIC-MCC model is explored to unveil the generation mechanism of PCFP,and based on the simulation data a larger voltage increasing rate over a quarter of a period and the distribution of electron density just before the power-on phase are believed to play key roles;the PCFP is usually produced in the rnicroplasma regime driven by the pulsed power supply.The effects of duty cycle and pulse modulation frequency on the evolution of PCFP are also discussed from the computational data.Therefore,the duty cycle and pulse modulation frequency can be used to optimize the generation of PCFP and high-energy electrons.     

Investigation of operating parameters on CO2 splitting by dielectric barrier discharge plasma

Experiments of CO2 splitting by dielectric barrier discharge (DBD) plasma were carried out,and the influence of CO2 flow rate,plasma power,discharge voltage,discharge frequency on CO2 conversion and process energy efficiency were investigated.It was shown that the absolute quantity of CO2 decomposed was only proportional to the amount of conductive electrons across the discharge gap,and the electron amount was proportional to the discharge power;the energy efficiency of CO2 conversion was almost a constant at a lower level,which was limited by CO2 inherent discharge character that determined a constant gap electric field strength.This was the main reason why CO2 conversion rate decreased as the CO2 flow rate increase and process energy efficiency was decreased a little as applied frequency increased.Therefore,one can improve the CO2 conversion by less feed flow rate or larger discharge power in DBD plasma,but the energy efficiency is difficult to improve.     

A comparison of power measurement techniques and electrical characterization of an atmospheric pressure plasma jet

In the last two decades a growing interest has been shown in the investigation of atmospheric pressure plasma jets (APPJs) that operate in contact with liquid samples. In order to form a complete picture about such experimental systems, it is necessary to perform detailed diagnostics of plasma jets, as one step that will enable the adjustment of system properties for applications in different areas. In this work, we conducted a detailed electrical characterisation of a plasma system configuration used for water treatment. A helium plasma jet, with a pin electrode powered by a continuous sine wave at a frequency of 330 kHz, formed a streamer that was in contact with a distilled water sample. An electrical circuit allowed the monitoring of electrical signals supplied to the jet and also to the plasma itself. An electrical characterisation together with power consumption measurements was obtained by using two different methods. The first method was based on the direct measurements of voltage and current signals, while in the second method we used 'Lissajous figures'. We compared these two methods when used for discharge power estimation and addressed their advantages and limitations. The results showed that both of these methods could be used to successfully determine power consumed by a discharge in contact with water, but only when taking into account power dissipation without plasma.     

Mode transition induced by gas pressure in dusty acetylene microdischarges: two-dimensional simulation

Radio-frequency microdischarge in acetylene is investigated by use of a fluid model and an aerosol dynamics model in a cylindrical discharge chamber. In this article, the results at a pressure of 100–500 Torr, a voltage of 80–150 V, and an electrode gap of 400–1000 μm are carefully analyzed and discussed. It is shown that two electron heating modes α and γ appear in the microdischarge, and the pressure-dependent transition from α to γ was accompanied by the abrupt decrease of electron density and electron temperature. The mode transition phenomenon is further confirmed by the variation of the electron temperature axial profiles, the profiles vary continuously from a center high at the pressure of 100 Torr to an edge high at the pressure of500 Torr. Furthermore, in the α mode(100 Torr) the plasma density increases linearly with the increase of electrode gap, but decreases sharply with the increase of electrode gap in the γ mode(100 Torr). The gas pressure and applied voltage effects on the nanoparticle density and degree of nonuniformity are also investigated. It has been shown that the gas pressure greatly influences the axial profiles of nanoparticle density and the values of the degree of nonuniformity, while the values of the plasma parameters(electron density and nanoparticle density) strongly depend on the applied voltage.     

Methane conversion using a dielectric barrier discharge reactor at atmospheric pressure for hydrogen production

In the present paper,we carried out a theoretical study of dielectric barrier discharge (DBD) filled with pure methane gas.The homogeneous discharge model used in this work includes a plasma chemistry unit,an electrical circuit,and the Boltzmann equation.The model was applied to the case of a sinusoidal voltage at a period frequency of 50 kHz and under a gas pressure of 600 Torr.We investigated the temporal variation of electrical and kinetic discharge parameters such as plasma and dielectric voltages,the discharge current density,electric field,deposited power density,and the species concentration.We also checked the physical model validity by comparing its results with experimental work.According to the results discussed herein,the dielectric capacitance is the parameter that has the greatest effect on the methane conversion and H2/CH4 ratio.This work enriches the knowledge for the improvement of DBD for CH4 conversion and hydrogen production.     

Measurements of plasma parameters in a hollow electrode AC glow discharge in helium

Measurements of the plasma parameters of coaxial gridded hollow electrode alternating current(AC)discharge helium plasma were carried out using an improved probe diagnostic technology.The measurements were performed under well-defined discharge conditions(chamber geometry,input power,AC power frequency,and external electrical characteristics).The problems encountered in describing the characteristics of AC discharge in many probe diagnostic methods were addressed by using an improved probe diagnostics design.This design can also be applied to the measurement of plasma parameters in many kinds of plasma sources in which the probe potential fluctuates with the discharge current.Several parameters of the hollow electrode AC helium discharge plasma were measured,including the plasma density,electron temperature,plasma density profiles,and changes in plasma density at different input power values and helium pressures.The characteristics of the coaxial gridded hollow electrode plasma determined by the experiments are suitable for comparison with plasma simulations,and for use in many applications of hollow cathode plasma.     

Study of Various Modes of Operation of an IEC Device

Inertial electrostatic confinement fusion devices are compact sources of neutrons, protons, electrons and X-rays. Such sources have many applications. Improving the efficiency of the device also increases the number of applications of this device. Hence a thorough understanding of the operation of this device is needed. In this paper we study the various modes in which an IEC device can be operated. The device seems to perform better when RF power is used. Furthermore, the amount of current that the power source can drive at a given pressure and grid voltage is dependent on the frequency applied to the grid—the higher the frequency the higher the cathode current. The device has been tested up to 320 kHz and the power supply current kept increasing up to this frequency. The higher limit was not reached by the present RF power supply. Another effect observed with the use of RF power is that the ionization source is more homogeneous relative to electron source ionization. This could mean that the heat load on the cathode is more evenly distributed. Such an even heat distribution would allow higher power operation.     

Kinetic simulation of the transition from a pulse-modulation microwave discharge to a continuous plasma

The generation of a very strong peak current in the first period(PCFP) in a pulse-modulated microwave discharge has been discussed in previous studies. In this paper we focus on the transition process from a pulsed discharge to a fully continuous one driven by the pulsed microwave power source by means of a kinetic model. The computational results show that by increasing the duty cycle or voltage modulation rate(VMR), the discharge eventually becomes fully continuous and PCFP can no longer be observed. In the transition process, the distributions of the electric field, electron energy probability function(EEPF) and plasma density are discussed according to the simulation data, showing different discharge structures. The simulations indicate that many high-energy electrons with electron energy larger than 20 eV and low-energy electrons with electron energy less than 3 eV could be generated in a pulsed microwave discharge, together with a reversal electric field formed in the anode sheath when PCFP occurs. However, only medium-energy electrons could be observed in a fully continuous discharge. Therefore, by investigating the transition process the pulse-modulated microwave discharges can be further optimized for plasma applications at atmospheric pressure.     

正脉冲电镀法制备φ33 mm模拟镍源

mA量级直流恒流电源具有过保护电压较低的缺点,不适于制作大面积、高活度⁶³Ni放射源。本文以正脉冲电源为解决方案,系统研究在简单组分的镀镍溶液中,各工艺条件对电镀结果的影响。研究结果表明,在阴极电流密度为18 mA/cm²、室温、脉宽80%、频率5 kHz条件下电镀2.5 h,可获得95%以上的⁵⁸Ni沉积率。     

Particle Densities of the Atmospheric-Pressure Argon Plasmas Generated by the Pulsed Dielectric Barrier Discharges

Atmospheric-pressure argon plasmas have received increasing attention due to their high potential in many industrial and biomedical applications. In this paper, a 1-D fluid model is used for studying the particle density characteristics of the argon plasmas generated by the pulsed dielectric barrier discharges. The temporal evolutions of the axial particle density distributions are illustrated, and the influences of changing the main discharge conditions on the averaged particle densities are researched by independently varying the various discharge conditions. The calculation results show that the electron density and the ion density reach two peaks near the momentary cathodes during the rising and the falling edges of the pulsed voltage. Compared with the charged particle densities, the densities of the resonance state atom Ar~r and the metastable state atom Ar~mhave more uniform axial distributions, reach higher maximums and decay more slowly. During the platform of the pulsed voltage and the time interval between the pulses, the densities of the excited state atom Ar*are far lower than those of the Ar~r or the Ar~m. The averaged particle densities of the different considered particles increase with the increases of the amplitude and the frequency of the pulsed voltage. Narrowing the discharge gap and increasing the relative dielectric constant of the dielectric also contribute to the increase of the averaged particle densities. The effects of reducing the discharge gap distance on the neutral particle densities are more significant than the influences on the charged particle densities.     

Simulation of Electrical Discharge Initiated by a Nanometer-Sized Probe in Atmospheric Conditions

In this paper,a two-dimensional nanometer scale tip-plate discharge model has been employed to study nanoscale electrical discharge in atmospheric conditions.The field strength distributions in a nanometer scale tip-to-plate electrode arrangement were calculated using the finite element analysis(FEA) method,and the influences of applied voltage amplitude and frequency as well as gas gap distance on the variation of efective discharge range(EDR) on the plate were also investigated and discussed.The simulation results show that the probe with a wide tip will cause a larger efective discharge range on the plate;the field strength in the gap is notably higher than that induced by the sharp tip probe;the efective discharge range will increase linearly with the rise of excitation voltage,and decrease nonlinearly with the rise of gap length.In addition,probe dimension,especially the width/height ratio,afects the efective discharge range in diferent manners.With the width/height ratio rising from 1:1 to 1:10,the efective discharge range will maintain stable when the excitation voltage is around 50 V.This will increase when the excitation voltage gets higher and decrease as the excitation voltage gets lower.Furthermore,when the gap length is 5 nm and the excitation voltage is below 20 V,the diameter of EDR in our simulation is about 150 nm,which is consistent with the experiment results reported by other research groups.Our work provides a preliminary understanding of nanometer scale discharges and establishes a predictive structure-behavior relationship.     

数字化X荧光仪电源的最优化设计

针对数字化X荧光仪的低功耗、低噪声等要求进行了电源最优化设计。文中对数字梯形滤波器进行了Simulink仿真,根据仿真结果得到最佳的M,N系数,由此确定微分电路的时间常数,最后确定高压电源的最佳开关频率点,降低了高压偏置电源噪声对系统的干扰。还分析了数字梯形滤波器及高速ADC采样的特点,设计了最优化的低压供电系统,进一步降低低压电源对系统的干扰。为了提高Si-Pin探测器制冷电源的供电效率,采用了高效率DC-DC、LDO芯片与检流芯片完成高效率恒流源的设计。实测高压电源的交流纹波小于3.5 mV,带载功耗小于70 mW,恒流源的带载转换效率83%,纹波电压小于12 mV,相同条件下采用文中电源系统可提高谱线的能量分辨率。     

The study on grid-to-rod fretting wear models for PWR fuel

The fretting wear is found to be generated at grid-to-rod contact areas by flow-induced vibration. This flow-induced grid-to-rod fretting wear may be initiated at a certain critical grid-to-rod gap that strongly depends on the extent of flow-induced vibration and grid spring designs. Three fretting wear excitation mechanisms acting on the grid-to-rod fretting wear are summarized. In order to examine the impact of grid spring designs on the fretting wear rate, the fretting wear tests for three kinds of grid spring designs were carried out for 500 h, simulating the reactor flow conditions. In parallel, three grid-to-rod fretting wear models that include constant work rate model, constant work density rate model and linear work density rate model have been developed. The three fretting wear models were used to predict the fuel rod perforation times with the use of the fretting wear test results. It is said that the constant work density rate model or the linear work density rate model is quite effective in predicting the grid-to-rod fretting-induced rod failure time observed in commercial nuclear power plants.