Experimental validation of post-filling flow in vacuum assisted resin transfer molding processes

In Liquid Composite Molding (LCM) processes with compliant tool, such as Vacuum Assisted Resin Transfer Molding Process (VARTM), resin flow continues even after the inlet is closed due to the preform deformation and pressure gradient developed during infusion. The resin flow and thickness changes continue until the resin pressure becomes uniform or the resin gels. This post-filling behavior is important as it will determine the final thickness and fiber volume fraction distribution in the cured composite. In this paper, a previously proposed one dimensional coupled flow and deformation process model has been compared with the experimental data in which the resin pressure and part thickness at various locations during the post-filling stage is recorded. Two different post-infusion scenarios are examined in order to determine their impact on the final part fiber volume fraction and thickness. The effects of different venting arrangements are demonstrated. The model predictions compare favorably with the experimental data, with the minor discrepancies arising due to the variability of material properties.     

基于混合网格方法的VARTM工艺充模仿真与实验验证

针对VARTM工艺的特点,建立了充模过程树脂流动和预成型体变形行为数学模型。提出了基于混合网格方法的VARTM充模仿真算法,在该算法中,模具型腔几何模型进行二维或三维网格划分,在每个真空袋表面单元上增加一个一维附属单元,用于在仿真过程中实时地吸收或挤出因真空袋变形而产生的局部树脂体积变化,形成混合网格仿真模型;求解过程中,对树脂流动和预成型体变形分别进行求解后,基于上述混合网格模型进行两者耦合操作,实现了仿真精度和速度的统一。搭建了VARTM充模实验平台,进行了一维充模实验,通过仿真结果与实验测量结果对比,验证了本文算法的正确性。最后,通过三维仿真算例,验证了算法对三维复杂结构和顺序浇口策略仿真的可行性。     

Flow control using localized induction heating in a VARTM process

Voids formed during the mold filling stage of the vacuum assisted resin transfer molding (VARTM) process become defects in the fabricated parts. Active flow control is one way to eliminate these defects by guiding the flow along a desired path during the mold filling stage of the process. Building upon previous work of the authors [Johnson R, Pitchumani R. In: Proceedings of the thirty-fourth international SAMPE technical conference, MD, USA, vol. 34(1); 2002, p. 250–61; Johnson R, Pitchumani R. Enhancement of flow in VARTM using localized induction heating. Compos Sci Technol 2003;63(15):2202–15; Johnson R., Pitchumani R. In: Proceedings of the fourteenth international conference on composite materials, CA, USA; 2003, Paper# 0861; Johnson R, Pitchumani R. Simulation of active flow control based on localized preform heating in a VARTM process. Compos Part A-Appl Sci Manuf, in press doi:10.1016/j.compositesa.2005.09.007], this paper presents implementation of an active flow control using induction heating as a means of locally reducing viscosity to counteract the effects of nonhomogeneity in the permeability of preform layups in a prototype VARTM process. Feedback of flow front locations during the filling stage of the process is used together with a numerical process model to arrive at decisions on the trajectories of the induction coil and the coil voltage, so as to maintain a uniform flow progression without exceeding a prescribed maximum temperature limit. A flow front following control strategy is implemented in a lab-scale experimental setup and tested on several preform layups exhibiting spatial permeability variation, as well as in the case of preforms with mold inserts. Results of these studies demonstrate that active flow control is capable of reducing the fill time, improving the flow front uniformity throughout the duration of the mold fills, and eliminating dry spot formation.     

Mechanical properties of composite structures fabricated with the vacuum induced preform relaxation process

A new technique called vacuum induced preform relaxation (VIPR) can be used to improve the processing of composite parts manufactured using vacuum resin infusion methods. The VIPR process is a method for manipulating and guiding the resin filling pattern during a vacuum assisted resin transfer molding (VARTM) manufacturing process with a relatively small external vacuum chamber. This VIPR chamber can be sealed against the flexible molding surface of a VARTM mold and used to create vacuum above the preform. This causes the compressive forces compacting the fabric to decrease allowing the resin to flow faster in the effected region under the chamber. Thus the chamber can influence the resin flow pattern as well as avoid the formation of voids due to merging flow fronts. When the regulated vacuum in the chamber is applied it temporarily decreases the fiber volume fraction of the preform. It is important to investigate if this relaxation has a permanent adverse effect on the mechanical properties of the composite. The results of these tests strongly suggest that the use of the VIPR process does not compromise the mechanical properties of composite structures.     

嵌入加强筋的缝合泡沫夹芯结构复合材料VARTM工艺树脂充填模拟及验证

在缝合泡沫夹芯结构复合材料的泡沫中嵌入轻质的加强筋板,可以在不增加缝合密度并且在只增加较少质量的前提下,增强复合材料制品整体的强度和刚性。文中对真空辅助树脂传递模塑成型(VARTM)工艺树脂在嵌入加强筋的缝合泡沫夹芯结构复合材料预成型体中充填过程进行模拟和验证研究。采用一种矩形流道模型代替沿加强筋与泡沫空隙间的树脂流动,并对其等效渗透率及孔隙率进行计算;通过PAM-RTM软件模拟了嵌入加强筋板的缝合泡沫夹芯结构VARTM工艺的树脂充填过程,并建立了流动可视化实验装置与模拟对比,结果表明模拟与实验相当吻合。而模拟与实验的结果均表明加强筋的引入可以在局部加强树脂沿厚度方向的流动,但是会延缓树脂对整个预成型体的充填。     

真空辅助成型工艺中预成型体的厚度变化与过流控制

采用无接触式电涡流位移传感系统, 对真空辅助成型工艺中预成型体的厚度变化进行了实时监测。揭示了该成型工艺过程中预成型体的厚度变化规律, 并考察了树脂过流控制时间对制件厚度与纤维体积含量的影响。结果表明, 在整个工艺过程中预成型体的厚度变化可分为三个阶段: 在树脂浸入后, 预成型体厚度迅速增加; 在树脂过流控制阶段, 预成型体厚度变化较小且保持在较高水平; 在树脂管关闭后, 预成型体厚度迅速下降并逐渐趋于稳定。制件厚度与树脂过流控制时间的变化关系类似于正弦曲线, 在树脂过流控制时间约为10 min时, 纤维体积分数最低, 较无过流控制降低1.7%; 在树脂过流控制时间约为40 min时, 纤维体积分数最高, 较无过流控制提高1.6%。     

A Two-layer Model for the Simulation of the VARTM Process with Resin Distribution Layer

Vacuum assisted resin transfer molding (VARTM) is one of the important processes to fabricate high performance composites. In this process, resin is drawn into the mold to impregnate the fiber reinforcement to a form composite. A resin distribution layer with high permeability was often introduced on top of the fiber reinforcement to accelerate the filling speed. Due to the difference of the flow resistance in the resin distribution layer and the reinforcement as well as the resulting through thickness transverse flow, the filling flow field is intrinsically three-dimensional. This study developed a two-layer model with two-dimensional formulation to simulate the filling flow of the VARTM process with a resin distribution layer. Two-dimensional flow was considered in each layer and a transverse flow in the thickness direction was estimated between the two layers. Thermal analysis including the transverse convection was also performed to better simulate the temperature distribution.     

Flow modeling of the VARTM process including progressive saturation effects

Modeling of vacuum based liquid composite molding methods (e.g., VARTM) relies on good understanding of closely coupled phenomena. The resin flow depends on the preform permeability, which in turn depends on the local fluid pressure; the preform compaction behavior, and the membrane stresses in the vacuum bag. It has also been shown that for many preforms there is a significant unsaturated region behind the flow front, and that the flow in this region affects the overall flow behavior of the process. Studies of preform compaction have shown that the preform stiffness, as well as being non-linear and exhibiting significant hysteresis, is dependant on the fluid saturation. For this reason most researchers model the preform compaction based on the pressure-compaction behavior of saturated preforms during unloading. This assumption leads to an effective discontinuity in preform thickness at the flow front, which is not observed in actual experiments. In this paper an improved compaction model incorporating the saturation dependence of the compaction pressure in the partially saturated region, is used in a one-dimensional model of the VARTM process. The model gives physically more realistic results for the thickness in the flow front region, and an improved model for the consolidation of the preform at the end of infusion.     

A numerical study of filling process through multilayer preforms in resin injection/compression molding

In resin injection/compression molding (RI/CM), a preform often comprises layers of different fiber reinforcements. Each fiber reinforcement has unique through thickness and in-plane permeabilities as well as compressibility, creating a heterogeneous porous medium in the mold cavity. In the present article, numerical simulation is utilized to investigate the filling process of RI/CM in such a heterogeneous porous medium. The filling stage is simulated in a full three-dimensional space by using control volume/finite element method and based upon an appropriate filling algorithm. The flow in the open gap which may be present in the mold cavity is modeled by Darcy’s law using an equivalent permeability. Numerical simulations of filling process for preforms containing two and three layers of different reinforcements in various stacking sequences are conducted with the aid of computer code developed in this study. Results show that the injection time as well as flow front progression depends on fiber types in the whole preform, fiber stacking sequence and open gap provided in the mold cavity. Simulated results also suggest that the presence of open gap at top of reinforcement can lead to both low injection time and uniform flow pattern.     

Numerical simulation of injection/compression liquid composite molding. Part 2: preform compression

In the injection/compression liquid composite molding process (I/C-LCM), a liquid polymer resin is injected into a partially open mold, which contains a preform of reinforcing fibers. After some or all of the resin has been injected, the mold is closed, compressing the preform and causing additional resin flow. This paper addresses compression of the preform, with particular emphasis on modeling three-dimensional mold geometries and multi-layer preforms in which the layers have different mechanical responses. First, a new constitutive relation is developed to model the mechanical response of fiber mats during compression. We introduce a new form of nonlinear elasticity for transversely isotropic materials. A special case of this form is chosen that includes the compressive stress generated by changes in mat thickness, but suppresses all other responses. This avoids the need to model slip of the preform along the mold surface. Second, a finite element method, based on the principle of virtual displacement, is developed to solve for the deformation of the preform at any stage of mold closing. The formulation includes both geometric and material nonlinearities, and uses a full Newton–Raphson iteration in the solution. An open gap above the preform can be incorporated by treating the gap as a distinct material layer with a very small stiffness. Examples show that this approach successfully predicts compression in dry preforms for three-dimensional I/C-LCM molds.     

Flow analysis during compression of partially impregnated fiber preform under controlled force

Compression resin transfer molding (CRTM) is an alternative solution to conventional resin transfer molding processes. It offers the capability to produce net shape composites with fast cycle times making it conducive for high volume production. The resin flow during this process can be separated into three phases: (i) metered amount of resin injection into a partially closed mold containing dry fiber preform, (ii) closure of the mold until it is in contact with the fiber preform displacing all the resin into the preform and (iii) further mold closure to the desired thickness of the part compacting the preform and redistributing the resin. Understanding the flow behavior in every phase is imperative for predictive process modeling that guarantees full preform saturation within a given time and under specified force constraints.     

Analysis of non-isothermal mold filling process in resin transfer molding (RTM) and structural reaction injection molding (SRIM)

In this paper, we present a modeling and numerical simulation of a mold filling process in resin transfer molding/structural reaction injection molding utilizing the homogenization method. Conventionally, most of the mold filling analyses have been based on a macroscopic flow model utilizing Darcy's law. While Darcy's law is successful in describing the averaged flow field within the mold cavity packed with a porous fiber preform, it requires experiments to obtain the permeability tensor and is limited to the case of porous fiber preform-it can not be used to model the resin flow through a double porous fiber preform. In the current approach, the actual flow field is considered, to which the homogenization method is applied to obtain the averaged flow model. The advantages of the current approach are: parameters such as the permeability and effective heat conductivity of the impregnanted fiber preform can be calculated; the actual flow field as well as averaged flow field can be obtained; and the resin flow through a double porous fiber preform can be modelled. In the presentation, we first derive the averaged flow model for the resin flow through a porous fiber preform and compare it with that of other methods. Next, we extend the result to the case of double porous fiber preform. An averaged flow model for the resin flow through a double porous fiber preform is derived, and a simulation program is developed which is capable of predicting the flow pattern and temperature distribution in the mold filling process. Finally, an example of a three dimensional part is provided.     

Modeling forces generated within rigid liquid composite molding tools. Part A: Experimental study

The term liquid composite molding (LCM) encompasses a growing list of processes, including resin transfer molding (RTM), injection/compression molding (I/CM), and resin infusion (a.k.a. VARTM). All LCM techniques involve compressive deformation of the fiber reinforcement prior to, and in many cases during mold filling. Forces acting on molds are primarily due to the requirement to compact the reinforcement, and pressure generated due to resin flow through these fibrous structures. An experimental study of the forces exerted on a mold during the RTM and I/CM processes is presented here. Two reinforcing materials have been considered, exhibiting significantly different resistance to compaction. The evolution of mold clamping force has been shown to be strongly influenced by the complex, non-elastic compaction behaviour of fiber reinforcements. The important effects include stress relaxation, an apparent lubrication by the injected fluid, and permanent deformation. Efforts to simulate the experiments will be presented in Part B of this study.     

Simulation of the reinforcement compaction and resin flow during the complete resin infusion process

Resin infusion (a.k.a. VARTM) is one of the LCM processes, for which liquid resin is drawn into dry reinforcements. Significant cavity thickness changes occur during processing, due to the flexibility of the vacuum bag used as one side of the tool, and the complex stress balance within the laminate. While the magnitude of thickness change is often small, the influence is significant on reinforcement properties. Changes in permeability during filling and post-filling have the potential to significantly affect the process. To simulate this behaviour, it is important to accurately model compaction and unloading of reinforcement in dry and wet states. A series of tests were completed to determine compaction behaviour of an isotropic glass fibre mat. From these tests several non-linear elastic compaction models have been determined, and applied within a resin infusion simulation which addresses pre-filling, filling and post-filling. This simulation was then used to assess different post-filling strategies.     

Laminate thickness and resin pressure evolution during axisymmetric liquid composite moulding with flexible tooling

This paper presents experimental observations from the filling and post-filling stages of 1D axisymmetric Resin Infusion (VARTM) and RTM Light. A series of experiments have been performed to investigate the influence of mould flexural stiffness and fill mode on fluid pressure, cavity thickness, filling stage time, and post-filling stage time. Observations are also made on the effect of those parameters on the repeatability of nominally identical experiments. This paper helps identify the circumstances where a RTM simulation would be sufficiently accurate for an RTM Light process, and consequently where a full flexible tooling simulation is necessary.     

Application of calcium carbonate in resin transfer molding process: An experimental investigation

The resin transfer molding (RTM) process is used to manufacture advanced composite materials made of continuous glass or carbon fibers embedded in a thermoset polymer matrix. In this process, a fabric preform is prepared, and is then placed into a mold cavity. After the preform is compacted between the mold parts, thermoset polymer is transferred from an injection machine to the mold cavity through injection gate(s). Resin flows through the porous fabric, and eventually flows out through the ventilation port(s). After the resin cure process (cross‐linking of the polymer), the mold is opened and the part is removed. The objective of this study is to verify the application of calcium carbonate mixed in resin in the RTM process. Several rectilinear infiltration experiments were conducted using glass fiber mat molded in a RTM system with cavity dimensions of 320 × 150 × 3.6 mm, room temperature, maximum injection pressure 0.202 bar and different content of CaCO₃ (10 and 40%) and particle size (mesh opening 38 and 75 µm). The results show that the use of filled resin with CaCO₃ influences the preform impregnation during the RTM molding, changing the filling time and flow front position, however it is possible to make composite with a good quality and low cost.     

Three-dimensional process cycle simulation of composite parts manufactured by resin transfer molding

A process cycle of resin transfer molding (RTM) consists of two sequential stages, i.e. filling and curing stages. These two stages are interrelated in non-isothermal processes so that the curing stage is dominated by the resin flow as well as temperature and conversion distributions during the filling stage. Therefore, it is necessary to take into account both filling and curing stages to analyze the process cycle accurately. In this paper, a full three-dimensional process cycle simulation of RTM is performed. Full three-dimensional analysis is necessary for thick parts or parts having complex shape. A computer code is developed based on the control volume/finite element method (CV/FEM). The resulting computer code can provide information regarding flow progression and pressure field during mold filling; and temperature distribution and degree of cure distribution for a process cycle. The computer code can also be used for process cycle simulation of composite structures with complex geometry and with various molding strategies including switching injection strategy, multiple gate injection strategy and variable mold wall temperature. Numerical examples provided in the present work show the capabilities of the computer code in analyzing the process cycle.     

导流介质对真空导入模塑工艺树脂流动行为的影响

采用可视化流动实验方法研究了高渗透率导流介质对真空导入模塑工艺中树脂流动行为的影响。结果表明: 导流介质能较大幅度地减少树脂的充模流动时间, 且充模时间随着导流介质使用比例的增加而呈线性减少的关系; 导流介质的提速作用随着预成型体厚度的增加而逐渐减弱; 预成型体上下表面树脂流动前沿位置差距与预成型体厚度呈良好的线性增加关系, 说明导流介质的影响作用具有明显的厚度效应。厚度效应原理为真空导入模塑工艺过程的参数优化和保证制品质量提供了理论依据。      

The effect of fabric and fiber tow shear on dual scale flow and fiber bundle saturation during liquid molding of textile composites

In Liquid Composite Molding (LCM) processes, a fibrous reinforcement preform is placed or draped over a mold surface, the mold is closed and a resin is either injected under pressure or infused under vacuum to cover all the spaces in between the fibers of the preform to create a composite part. LCM is used in a variety of manufacturing applications, from the aerospace to the medical industries. In this manufacturing process, the properties of the fibrous reinforcement inside the closed mold is of great concern. Preform structure, volume fraction, and permeability all influence the processing characteristics and final part integrity. When preform fabrics are draped over a mold surface, the geometry and characteristics of both the bulk fabric and fiber tow bundles change as the fabric shears to conform to the mold curvature. Numerical simulations can predict resin flow in dual scale fabrics in which one can separately track the filling of the fiber tows in addition to flow of resin within the bulk fabric. The effect of the deformation of the bulk fabric due to draping over the tool surface has been previously addressed by accounting for the change in fiber volume fraction and permeability during the filling of a mold. In this work, we investigate the effect of shearing of the fiber tows in addition to bulk deformation during the dual scale filling. We model the influence of change in fiber tow characteristics due to draping and deformation on mold filling and compare it with the results when the fiber tow deformation effect is ignored. Model experiments are designed and conducted with a dual scale fabric to characterize the change in permeability of fiber tow with deformation angle. Simulations which account for dual scale shear demonstrate that the tow saturation rate is affected, requiring longer fill times, or higher pressures to completely saturate fiber tows in areas of a mold with high local shear. This should prove useful in design of components for applications in which it is imperative to ensure that there are no unfilled fiber tows in the final fabricated component.