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Large‐Size 2D β‐Cu2S Nanosheets with Giant Phase Transition Temperature Lowering (120 K) Synthesized by a Novel Method of Super‐Cooling Chemical‐Vapor‐Deposition
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Bo Li Le Huang Guangyao Zhao Zhongming Wei Huanli Dong Wenping Hu Lin‐Wang Wang Jingbo Li 《Advanced materials (Deerfield Beach, Fla.)》2016,28(37):8271-8276
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2D Materials: Large‐Area and High‐Quality 2D Transition Metal Telluride (Adv. Mater. 3/2017)
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Jiadong Zhou Fucai Liu Junhao Lin Xiangwei Huang Juan Xia Bowei Zhang Qingsheng Zeng Hong Wang Chao Zhu Lin Niu Xuewen Wang Wei Fu Peng Yu Tay‐Rong Chang Chuang‐Han Hsu Di Wu Horng‐Tay Jeng Yizhong Huang Hsin Lin Zexiang Shen Changli Yang Li Lu Kazu Suenaga Wu Zhou Sokrates T. Pantelides Guangtong Liu Zheng Liu 《Advanced materials (Deerfield Beach, Fla.)》2017,29(3)
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2D Materials: C3N—A 2D Crystalline,Hole‐Free,Tunable‐Narrow‐Bandgap Semiconductor with Ferromagnetic Properties (Adv. Mater. 16/2017)
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Siwei Yang Wei Li Caichao Ye Gang Wang He Tian Chong Zhu Peng He Guqiao Ding Xiaoming Xie Yang Liu Yeshayahu Lifshitz Shuit‐Tong Lee Zhenhui Kang Mianheng Jiang 《Advanced materials (Deerfield Beach, Fla.)》2017,29(16)
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2D Materials: A Free‐Standing and Self‐Healable 2D Supramolecular Material Based on Hydrogen Bonding: A Nanowire Array with Sub‐2‐nm Resolution (Small 21/2017)
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Ming Li Mengyao Song Guitai Wu Zhenyu Tang Yunfeng Sun Yunbin He Jinhua Li Lei Li Haoshuang Gu Xiong Liu Chuang Ma Zefei Peng Zhaoquan Ai David J. Lewis 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(21)
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2D Materials: Synaptic Barristor Based on Phase‐Engineered 2D Heterostructures (Adv. Mater. 35/2018)
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Woong Huh Seonghoon Jang Jae Yoon Lee Donghun Lee Donghun Lee Jung Min Lee Hong‐Gyu Park Jong Chan Kim Hu Young Jeong Gunuk Wang Chul‐Ho Lee 《Advanced materials (Deerfield Beach, Fla.)》2018,30(35)
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Pan Jia Qi Wen Dan Liu Min Zhou Xiaoyan Jin Liping Ding Huanli Dong Diannan Lu Lei Jiang Wei Guo 《Small (Weinheim an der Bergstrasse, Germany)》2019,15(50)
The unique feature of nacre‐like 2D layered materials provides a facile, yet highly efficient way to modulate the transmembrane ion transport from two orthogonal transport directions, either vertical or horizontal. Recently, light‐driven active transport of ionic species in synthetic nanofluidic systems attracts broad research interest. Herein, taking advantage of the photoelectric semiconducting properties of 2D transition metal dichalcogenides, the generation of a directional and greatly enhanced cationic flow through WS2‐based 2D nanofluidic membranes upon asymmetric visible light illumination is reported. Compared with graphene‐based materials, the magnitude of the ionic photocurrent can be enhanced by tens of times, and its photo‐responsiveness can be 2–3.5 times faster. This enhancement is explained by the coexistence of semiconducting and metallic WS2 nanosheets in the hybrid membrane that facilitates the asymmetric diffusion of photoexcited charge carriers on the channel wall, and the high ionic conductance due to the neat membrane structure. To further demonstrate its application, photonic ion switches, photonic ion diodes, and photonic ion transistors as the fundamental elements for light‐controlled nanofluidic circuits are further developed. Exploring new possibilities in the family of liquid processable colloidal 2D materials provides a way toward high‐performance light‐harvesting nanofluidic systems for artificial photosynthesis and sunlight‐driven desalination. 相似文献
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Semiconductors: Growth of Large‐Area 2D MoS2(1‐x)Se2x Semiconductor Alloys (Adv. Mater. 17/2014)
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Qingliang Feng Yiming Zhu Jinhua Hong Mei Zhang Wenjie Duan Nannan Mao Juanxia Wu Hua Xu Fengliang Dong Fang Lin Chuanhong Jin Chunming Wang Jin Zhang Liming Xie 《Advanced materials (Deerfield Beach, Fla.)》2014,26(17):2763-2763
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Jiadong Zhou Fucai Liu Junhao Lin Xiangwei Huang Juan Xia Bowei Zhang Qingsheng Zeng Hong Wang Chao Zhu Lin Niu Xuewen Wang Wei Fu Peng Yu Tay‐Rong Chang Chuang‐Han Hsu Di Wu Horng‐Tay Jeng Yizhong Huang Hsin Lin Zexiang Shen Changli Yang Li Lu Kazu Suenaga Wu Zhou Sokrates T. Pantelides Guangtong Liu Zheng Liu 《Advanced materials (Deerfield Beach, Fla.)》2017,29(3)
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Miika Mattinen Peter J. King Leonid Khriachtchev Kristoffer Meinander James T. Gibbon Vin R. Dhanak Jyrki Räisänen Mikko Ritala Markku Leskelä 《Small (Weinheim an der Bergstrasse, Germany)》2018,14(21)
Semiconducting 2D materials, such as SnS2, hold immense potential for many applications ranging from electronics to catalysis. However, deposition of few‐layer SnS2 films has remained a great challenge. Herein, continuous wafer‐scale 2D SnS2 films with accurately controlled thickness (2 to 10 monolayers) are realized by combining a new atomic layer deposition process with low‐temperature (250 °C) postdeposition annealing. Uniform coating of large‐area and 3D substrates is demonstrated owing to the unique self‐limiting growth mechanism of atomic layer deposition. Detailed characterization confirms the 1T‐type crystal structure and composition, smoothness, and continuity of the SnS2 films. A two‐stage deposition process is also introduced to improve the texture of the films. Successful deposition of continuous, high‐quality SnS2 films at low temperatures constitutes a crucial step toward various applications of 2D semiconductors. 相似文献
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A Free‐Standing and Self‐Healable 2D Supramolecular Material Based on Hydrogen Bonding: A Nanowire Array with Sub‐2‐nm Resolution
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Ming Li Mengyao Song Guitai Wu Zhenyu Tang Yunfeng Sun Yunbin He Jinhua Li Lei Li Haoshuang Gu Xiong Liu Chuang Ma Zefei Peng Zhaoquan Ai David J. Lewis 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(21)
In many 2D materials reported thus far, the forces confining atoms in a 2D plane are often strong interactions, such as covalent bonding. Herein, the first demonstration that hydrogen (H)‐bonding can be utilized to assemble polydiacetylene (a conductive polymer) toward a 2D material, which is stable enough to be free‐standing, is shown. The 2D material is well characterized by a large number of techniques (mainly different microscopy techniques). The H‐bonding allows splitting of the material into ribbons, which can reassemble, similar to a zipper, leading to the first example of a healable 2D material. Moreover, such technology can easily create 2D, organic, conductive nanowire arrays with sub‐2‐nm resolution. This material may have potential applications in stretchable electronics and nanowire cross‐bar arrays. 相似文献
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Twinned Growth of Metal‐Free,Triazine‐Based Photocatalyst Films as Mixed‐Dimensional (2D/3D) van der Waals Heterostructures
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Dana Schwarz Yu Noda Jan Klouda Karolina Schwarzová‐Pecková Ján Tarábek Jiří Rybáček Jiří Janoušek Frank Simon Maksym V. Opanasenko Jiří Čejka Amitava Acharjya Johannes Schmidt Sören Selve Valentin Reiter‐Scherer Nikolai Severin Jürgen P. Rabe Petra Ecorchard Junjie He Miroslav Polozij Petr Nachtigall Michael J. Bojdys 《Advanced materials (Deerfield Beach, Fla.)》2017,29(40)
Design and synthesis of ordered, metal‐free layered materials is intrinsically difficult due to the limitations of vapor deposition processes that are used in their making. Mixed‐dimensional (2D/3D) metal‐free van der Waals (vdW) heterostructures based on triazine (C3N3) linkers grow as large area, transparent yellow‐orange membranes on copper surfaces from solution. The membranes have an indirect band gap (E g,opt = 1.91 eV, E g,elec = 1.84 eV) and are moderately porous (124 m2 g?1). The material consists of a crystalline 2D phase that is fully sp2 hybridized and provides structural stability, and an amorphous, porous phase with mixed sp2–sp hybridization. Interestingly, this 2D/3D vdW heterostructure grows in a twinned mechanism from a one‐pot reaction mixture: unprecedented for metal‐free frameworks and a direct consequence of on‐catalyst synthesis. Thanks to the efficient type I heterojunction, electron transfer processes are fundamentally improved and hence, the material is capable of metal‐free, light‐induced hydrogen evolution from water without the need for a noble metal cocatalyst (34 µmol h?1 g?1 without Pt). The results highlight that twinned growth mechanisms are observed in the realm of “wet” chemistry, and that they can be used to fabricate otherwise challenging 2D/3D vdW heterostructures with composite properties. 相似文献