Pool boiling of perfluorocarbon mixtures on silicon surfaces

The need for higher pool boiling critical heat flux (CHF) in electronic cooling applications has turned attention to the use of binary mixtures of dielectric liquids. The available literature demonstrates that the addition of a liquid with higher saturation temperature, higher molecular weight, higher viscosity and higher surface tension can lead to significant enhancement of CHF, beyond what can be achieved through changes in pressure, liquid subcooling, and the product of surface effusivity and heater thickness. The current study focuses on extending the available data on mixture CHF enhancement, as well as pool boiling, on polished silicon surfaces to FC-72/FC-40 mixture ratios of 10%, 15%, and 20% of FC-40 by weight, a pressure range of between 1 and 3 atm, and fluid temperature from 22 to 45 °C, leading to high subcooling conditions. It is found that peak heat flux can be increased to as high as 56.8 W/cm² compared to 25.2 W/cm² for pure FC-72 at 3 atm and 22 °C. It is believed that the increase in the mixture latent heat of evaporation and surface tension, accompanying the depletion of the lower boiling point fluid in the wall region plays the major role in enhancing the critical heat flux for binary mixtures.     

Enhancement of pool boiling critical heat flux in dielectric liquids by microporous coatings

An experimental investigation into the effects of pressure and subcooling on the pool boiling critical heat flux from a bare silicon chip-like heater and from a silicon heater coated with microporous layers, is reported. The dual inline heater package was immersed in FC-72, a dielectric fluid, and the experiments were performed in the horizontal orientation, with subcooling varying between 0 K and 72 K, and the pressure between 101.3 kPa and 303.9 kPa. The maximum CHF values on the diamond-base microporous-coated silicon heater were found to reach 47 W/cm², at 3 atm and nearly 50 K of subcooling, and to provide an average enhancement of approximately 60% over the values attained with un-treated silicon surfaces. An available CHF correlation, with a reported standard deviation of 12.5% for un-treated surfaces over a large range of pressures, subcoolings, and surface conditions, was shown to predict the pressure and subcooling effects on CHF from the surface-enhanced chip with a standard deviation of 12%.     

Theoretical and experimental study of the effects of spray inclination on two-phase spray cooling and critical heat flux

Experiments were conducted with PF-5052 liquid sprays impacting a 1.0 × 1.0 cm² heated test surface at different inclination angles, flow rates, and subcoolings. Inclination angle had no noticeable effect on the single-phase or two-phase regions of the boiling curve. Maximum CHF was always achieved with the spray impinging normal to the test surface; increasing angle of inclination away from the normal decreased CHF appreciably. Video analysis showed inclined sprays produced lateral liquid film flow towards the farthest downstream region of the test surface. The film liquid provided partial resistance to dryout despite the weak volumetric spray flux in the downstream region. A new theoretical model of the spray’s impact area and volumetric flux proves this decrease is the result of a sharp reduction in the fraction of the test surface area that is directly impacted by the spray. Combining the model and video results with a previous point-based CHF correlation for normal sprays is shown to accurately predict the effects of orientation angle on CHF for different nozzles and operating conditions.     

Enhanced flow boiling heat transfer of FC-72 on micro-pin-finned surfaces

For the purpose of cooling electronic components with high heat flux efficiently, some experiments were conducted to study the flow boiling heat transfer performance of FC-72 on silicon chips. Micro-pin-fins were fabricated on the chip surface using a dry etching technique to enhance boiling heat transfer. Three different fluid velocities (0.5, 1 and 2 m/s) and three different liquid subcoolings (15, 25 and 35 K) were performed, respectively. A smooth chip (chip S) and four micro-pin-finned chips with the same fin thickness of 30 μm and different fin heights of 60 μm (chip PF30–60) and 120 μm (chip PF30–120), respectively, were tested. All the micro-pin-finned surfaces show a considerable heat transfer enhancement compared to the smooth one, and the critical heat flux increases in the order of chip S, PF30–60 and PF30–120. For a lower ratio of fin height to fin pitch and/or higher fluid velocity, the fluid velocity has a positive effect on the nucleate boiling curves for the micro-pin-finned surfaces. At the velocities lower than 1 m/s, the micro-pin-finned surfaces show a sharp increase in heat flux with increasing wall superheat, and the wall temperature at the critical heat flux (CHF) is less than the upper limit, 85 °C, for the reliable operation of LSI chips. The CHF values for all surfaces increase with fluid velocity and subcooling. The maximum CHF can reach nearly 150 W/cm² for chip PF30–120 at the fluid velocity of 2 m/s and the liquid subcooling of 35 K.     

Subcooled flow boiling heat transfer and associated bubble characteristics of FC-72 on a heated micro-pin-finned silicon chip

Experiments are conducted here to investigate subcooled flow boiling heat transfer and associated bubble characteristics of FC-72 on a heated micro-pin-finned silicon chip flush-mounted on the bottom of a horizontal rectangular channel. In the experiments the mass flux is varied from 287 to 431 kg/m² s, coolant inlet subcooling from 2.3 to 4.3 °C, and imposed heat flux from 1 to 10 W/cm². Besides, the silicon chips contain three different geometries of micro-structures, namely, the smooth, pin-finned 200 and pin-finned 100 surfaces. The pin-finned 200 and 100 surfaces, respectively, contain micro-pin-fins of size 200 μm × 200 μm × 70 μm (width × length × height) and 100 μm × 100 μm × 70 μm. The measured data show that the subcooled flow boiling heat transfer coefficient is reduced at increasing inlet liquid subcooling but is little affected by the coolant mass flux. Besides, adding the micro-pin-fin structures to the chip surface can effectively raise the single-phase convection and flow boiling heat transfer coefficients. Moreover, the mean bubble departure diameter and active nucleation site density are reduced for rises in the FC-72 mass flux and inlet liquid subcooling. Increasing coolant mass flux or reducing inlet liquid subcooling results in a higher mean bubble departure frequency. Furthermore, larger bubble departure diameter, higher bubble departure frequency, and higher active nucleation site density are observed as the imposed heat flux is increased. Finally, empirical correlations for the present data for the heat transfer and bubble characteristics in the FC-72 subcooled flow boiling are proposed.     

Correlation of critical heat flux and two-phase friction factor for subcooled convective boiling in structured surface microchannels

Critical heat flux (CHF) and pressure drop of subcooled flow boiling are measured for a microchannel heat sink containing 75 parallel 100 μm × 200 μm structured surface channels. The heated surface is made of a Cu metal sheet with/without 2 μm thickness diamond film. Tests and measurements are conducted with de-ionized water, de-ionized water +1 vol.% MCNT additive solution, and FC-72 fluids over a mass velocity range of 820–1600 kg/m² s, with inlet temperatures of 15(8.6)°C, 25(13.6)°C, 44(24.6)°C, and 64(36.6)°C for DI water (FC-72), and heat fluxes up to 600 W/cm². The CHF of subcooled flow boiling of the test fluids in the microchannels is measured parametrically. The two-phase pressure drop is also measured. Both CHF and the two-phase friction factor correlation for one-side heating with two other side-structured surface microchannels are proposed and developed in terms of the relevant parameters.     

Single-phase and two-phase cooling with an array of rectangular jets

Experiments were performed to explore the effects of jet width, impingement velocity, and inlet subcooling on the cooling performance of an array of three confined rectangular FC-72 and ethanol jets impacting a 3.0 cm × 3.0 cm heated surface. The single-phase heat transfer coefficient increased with increasing jet velocity and/or jet width. A correlation for single-phase cooling was constructed by dividing the flow into impingement zones and confinement channel flow regions that are dominated by wall jet flow. Increases in jet velocity, jet width, and/or subcooling broadened the single-phase region preceding the commencement of boiling and enhanced critical heat flux (CHF). A new correlation was developed which fits the CHF data with good accuracy. Overall, better cooling performance was realized for a given flow rate by decreasing jet width. Pressure drop was for the most part quite modest, even for the smallest jet width and highest velocity tested. Overall, these results prove the present cooling scheme is highly effective at maintaining fairly isothermal surface conditions, with spatial variations of less than 1.2 and 2.6 °C for the single-phase and boiling regions, respectively. These results demonstrate the effectiveness of the present jet-impingement scheme for thermal management of next generation electronics devices and systems.     

A new mechanistic model for pool boiling CHF on horizontal surfaces

This work proposes a new mechanistic model for predicting the critical heat flux (CHF) in horizontal pool boiling systems. It is postulated that when the vapor momentum flux is sufficient to lift the liquid macrolayer from the heating surface, wetting is no longer feasible, and a transition from nucleate to film boiling occurs. This is the same mechanism that has found success in predicting CHF in flow boiling systems. An experimental investigation of CHF with pentane, hexane, and FC-72 in saturated horizontal pool boiling with chamber pressures of 150, 300, and 450 kPa provides evidence that the new model captures the variation of CHF with pressure reasonably well compared with other well known models. The new model is also compared with existing data from the literature over a reduced pressure range of 2 × 10^?5–2 × 10^?1. The mean deviation between the predicted and measured CHF is typically within 20% over the parameter space covered.     

Local heat transfer distribution and effect of instabilities during flow boiling in a silicon microchannel heat sink

Flow boiling of the perfluorinated dielectric fluid FC-77 in a silicon microchannel heat sink is investigated. The heat sink contains 60 parallel microchannels each of 100 μm width and 389 μm depth. Twenty-five evenly distributed temperature sensors in the substrate yield local heat transfer coefficients. The pressure drop across the channels is also measured. Experiments are conducted at five flow rates through the heat sink in the range of 20–80 ml/min with the inlet subcooling held at 26 K in all the tests. At each flow rate, the uniform heat input to the substrate is increased in steps so that the fluid experiences flow regimes from single-phase liquid flow to the occurrence of critical heat flux (CHF). In the upstream region of the channels, the flow develops from single-phase liquid flow at low heat fluxes to pulsating two-phase flow at high heat fluxes during flow instability that commences at a threshold heat flux in the range of 30.5–62.3 W/cm² depending on the flow rate. In the downstream region, progressive flow patterns from bubbly flow, slug flow, elongated bubbles or annular flow, alternating wispy-annular and churn flow, and wall dryout at highest heat fluxes are observed. As a result, the heat transfer coefficients in the downstream region experience substantial variations over the entire heat flux range, based on which five distinct boiling regimes are identified. In contrast, the heat transfer coefficient midway along the channels remains relatively constant over the heat flux range tested. Due to changes in flow patterns during flow instability, the heat transfer is enhanced both in the downstream region (prior to extended wall dryout) and in the upstream region. A previous study by the authors found no effect of instabilities during flow boiling in a heat sink with larger microchannels (each 300 μm wide and 389 μm deep); it appears therefore that the effect of instabilities on heat transfer is amplified in smaller-sized channels. While CHF increases with increasing flow rate, the pressure drop across the channels has only a minimal dependence on flow rate once boiling is initiated in the microchannels, and varies almost linearly with increasing heat flux.     

Nucleate boiling heat transfer enhancement for water and FC-72 on titanium oxide and silicon oxide surfaces

An experimental study was performed to investigate the nucleate boiling and critical heat flux (CHF) of water and FC-72 dielectric liquid on hydrophilic titanium oxide (TiO₂) nanoparticle modified surface. A 1 cm² copper heater with 1 μm thick TiO₂ coating was utilized in saturated pool boiling tests with water and highly-wetting FC-72, and its performance was compared to that of a smooth surface. Results showed that TiO₂ coated surface increased CHF by 50.4% and 38.2% for water and FC-72, respectively, and therefore indicated that boiling performance enhancement depends on the level of wettability improvement. A silicon oxide (SiO₂) coated surface, exhibiting similar surface topology, was tested to isolate the roughness related enhancement from the overall enhancement. Data confirmed that hydrophilicity of TiO₂ coated surface provides an additional mechanism for boiling enhancement.     

Enhanced boiling of HFE-7100 dielectric liquid on porous graphite

Enhanced boiling of HFE-7100 dielectric liquid on porous graphite measuring 10 mm × 10 mm is investigated, and results are compared with those for smooth copper (Cu) of the same dimensions. Although liquid is out-gassed for hours before performing the pool boiling experiments, air entrapped in re-entrant type cavities, ranging in size from tens to hundreds of microns, not only enhanced the nucleate boiling heat transfer and the critical heat flux (CHF), but also, the mixing by the released tiny air bubbles from the porous graphite prior to boiling incipience enhanced the natural convection heat transfer by ∼19%. No temperature excursion is associated with the nucleate boiling on porous graphite, which ensues at very low surface superheat of 0.5–0.8 K. Conversely, the temperature overshoot at incipient boiling on Cu is as much as 39.2, 36.6, 34.1 and 32.8 K in 0 (saturation), 10, 20 and 30 K subcooled boiling, respectively. Nucleate boiling ensues on Cu at a surface superheat of 11.9, 10.9, 9.5 and 7.5 K in 0 (saturation), 10, 20 and 30 K subcooled boiling, respectively. The saturation nucleate boiling heat flux on porous graphite is 1700% higher than that on Cu at a surface superheat of ∼10 K and decreases exponentially with increased superheat to ∼60% higher near CHF. The CHF values of HFE-7100 on porous graphite of 31.8, 45.1, 55.9 and 66.4 W/cm² in 0 (saturation), 10, 20 and 30 K subcooled boiling, are 60% higher and the corresponding superheats are 25% lower than those on Cu. In addition, the rate of increase in CHF with increased liquid subcooling is 50% higher than that on Cu.     

Correlation of high critical heat flux during flow boiling for water in a small tube at various subcooled conditions

High critical heat fluxes (CHFs) for subcooled boiling of water in a small tube were investigated experimentally. A platinum tube with an inner diameter of 1.0 mm and a length of 40.9 mm was used in the experiment. The upward flow velocity, the subcooling of water, and the outlet pressure of the experimental tube were varied to enable a parametric study of the CHFs. The flow velocity ranged from 9 to 13 m/s and the inlet subcooling ranged from 69 to 148 K. The boiling number decreased with increasing Weber number. The boiling number is also dependent on a non-dimensional parameter and the density ratio of liquid to vapor. A correlation for the high CHF of the small tube was obtained based on the experimental data. Finally, the high CHF correlation was evaluated using the CHF data obtained by other researchers.     

Flow boiling CHF enhancement with surfactant solutions under atmospheric pressure

Surfactant effect on CHF (critical heat flux) was determined during water flow boiling at atmospheric pressure in closed loop filled with solution of tri-sodium phosphate (TSP, Na₃PO₄ · 12H₂O). TSP was added to the containment sump water to adjust pH level during accident in nuclear power plants. CHF was measured for four different water surfactant solutions in vertical tubes, at different mass fluxes (100–500 kg/m² s) and two inlet subcooling temperatures (50 °C and 75 °C). Surfactant solutions (0.05–0.2%) at low mass flux (～100 kg/m² s) showed the best CHF enhancement. CHF was decreased at high mass flux (500 kg/m² s) compared to the reference plain water data. Maximum increase in CHF was about 48% as compared to the reference data. Surfactant caused a decrease in contact angle associated with an increase of CHF from surfactant addition.     

Subcooled flow boiling CHF enhancement with porous surface coatings

The effect of micro/nanoporous inside surface coated vertical tubes on CHF was determined during water flow boiling at atmospheric pressure. CHF was measured for smooth and three different coated tubes, at mass fluxes (100–300 kg/m² s) and two inlet subcooling temperatures (50 °C and 75 °C). Greater CHF enhancement was found with microporous coatings than with nanoporous coatings. Al₂O₃ microporous coatings with particle size <10 μm and coatings thickness of 50 μm showed the best CHF enhancement. Maximum increase in CHF was about 25% for microporous Al₂O₃. A wettability test was performed to study an increase of CHF with microporous coated surfaces.     

High heat flux spray cooling with ammonia: Investigation of enhanced surfaces for CHF

A spray cooling study was conducted to investigate the effect of enhanced surfaces on Critical Heat Flux (CHF). Test surfaces involved micro-scale indentations and protrusions, macro (mm) scale pyramidal pin fins, and multi-scale structured surfaces, combining macro and micro-scale structures, along with a smooth surface that served as reference. Tests were conducted in a closed loop system using a vapor atomized spray nozzle with ammonia as the working fluid. Nominal flow rates were 1.6 ml/cm² s of liquid and 13.8 ml/cm² s of vapor, resulting in a pressure drop of 48 kPa. Results indicated that the multi-scale structured surface helped increase maximum heat flux limit by 18% over the reference smooth surface, to 910 W/cm² at nominal flow rate. During the additional CHF testing at higher flow rates, most heaters experienced failures before reaching CHF at heat fluxes above 950 W/cm². However, some enhanced surfaces can achieve CHF values of up to ≈1100 W/cm² with ≈67% spray cooling efficiency based on liquid usage. The results also shed some light on the current understanding of the spray cooling heat transfer mechanisms. Enhanced surfaces are found to be capable of retaining more liquid compared to a smooth surface, and efficiently spread the liquid film via capillary force within the structures. This important advantage delays the occurrence of dry patches at high heat fluxes, and leads to higher CHF. The present work demonstrated ammonia spray cooling as a unique alternative for challenging thermal management tasks that call for high heat flux removal while maintaining a low device temperature with a compact and efficient cooling scheme.     

Pool boiling heat transfer on horizontal rectangular fin array in saturated FC-72

The flow patterns and pool boiling heat transfer performance of copper rectangular fin array surfaces immersed in saturated FC-72 were experimentally investigated. The effects of the geometry parameters (fin spacing and fin length) on boiling performance were also examined. The test surfaces were manufactured on a copper block with a base area of 10 mm × 10 mm with three fin spacing (0.5 mm, 1.0 mm and 2.0 mm) and four fin lengths (0.5 mm, 1.0 mm, 2.0 mm and 4.0 mm). All experiments were performed in the saturated state at 1 atmospheric condition. A plain surface was used as the reference standard and compared with the finned surfaces. The photographic images showed different boiling flow patterns among the test surfaces at various heat fluxes. The test results indicated that closer and higher fins yielded a greater flow resistance that against the bubble/vapor lift-off in the adjacent fins. Moreover, as the heat flux approached to critical heat flux (CHF), numerous vapor mushrooms periodically appeared and extruded from the perimeter of the fin array, causing dry-out in the center of the fin array. Closer and higher fins provide more heat transfer. The results also showed that overall heat transfer coefficient decayed rapidly as the fin spacing decreased or the fin length increased. The maximum value of CHF on the base area was 9.8 × 10⁵ W m⁻² for the test surface with a 0.5 mm fin spacing and a 4.0 mm fin length, which has a value five times greater than that of the plain surface.     

Enhancement of pool-boiling heat transfer using nanostructured surfaces on aluminum and copper

Enhanced pool-boiling critical heat fluxes (CHF) at reduced wall superheat on nanostructured substrates are reported. Nanostructured surfaces were realized using a low temperature process, microreactor-assisted-nanomaterial-deposition. Using this technique we deposited ZnO nanostructures on Al and Cu substrates. We observed pool-boiling CHF of 82.5 W/cm² with water as fluid for ZnO on Al versus a CHF of 23.2 W/cm² on bare Al surface with a wall superheat reduction of 25–38 °C. These CHF values on ZnO surfaces correspond to a heat transfer coefficient of ～23,000 W/m² K. We discuss our data and compare the behavior with conventional boiling theory.     

Experimental study of saturated flow boiling heat transfer in an array of staggered micro-pin-fins

This study concerns water saturated flow boiling heat transfer in an array of staggered square micro-pin-fins having a 200 × 200 μm² cross-section by a 670 μm height. Three inlet temperatures of 90, 60, and 30 °C, six mass velocities for each inlet temperature, ranging from 183 to 420 kg/m² s, and outlet pressures between 1.03 and 1.08 bar were tested. Heat fluxes ranged from 23.7 to 248.5 W/cm². Heat transfer coefficient was fairly constant at high quality, insensitive to both quality and mass velocity. Heat transfer was enhanced by inlet subcooling at low quality. Possible heat transfer mechanism was discussed.     

An experimental study on CHF enhancement in flow boiling using Al2O3 nano-fluid

The critical heat flux (CHF) is one of the most important thermal hydraulic parameters in heat transfer system design and safety analyses. CHF enhancement allows higher limits of operation conditions such that heat transfer equipment can be operated safely with greater margins and better economy. The application of nano-fluids is thought to have strong potential for enhancing the CHF. In this study, zeta potentials of Al₂O₃ nano-fluids were measured and flow boiling CHF enhancement experiments using Al₂O₃ nano-fluids were conducted under atmospheric pressure. The CHFs of Al₂O₃ nano-fluids were enhanced up to ～70% in flow boiling for all experimental conditions. Maximum CHF enhancement (70.24%) was shown at 0.01 vol% concentration, 50 °C inlet subcooling, and a mass flux of 100 kg/m² s. Inner surfaces of the test section tube were observed by FE–SEM and the zeta potentials of Al₂O₃ nano-fluids were measured before and after the CHF experiments.     

Subcooled flow boiling and microbubble emission boiling phenomena in a partially heated microchannel

A simultaneous visualization and measurement study has been carried out to investigate subcooled flow boiling and microbubble emission boiling (MEB) phenomena of deionized water in a partially heated Pyrex glass microchannel, having a hydraulic diameter of 155 μm, which was integrated with a Platinum microheater. Effects of mass flux, inlet water subcooling and surface condition of the microheater on subcooled flow boiling in microchannels are investigated. It is found that MEB occurred at high inlet subcoolings and at high heat fluxes, where vapor bubbles collapsed into microbubbles after contacting with the surrounding highly subcooled liquid. In the fully-developed MEB regime where the entire microheater was covered by MEB, the mass flux, the inlet water subcooling and the heater surface condition have only small effects on the boiling curves. The occurrence of MEB in microchannel can remove a large amount of heat flux, as high as 14.41 MW/m² at a mass flux of 883.8 kg/m² s, with only a moderate rise in wall temperature. Therefore, MEB is a very promising method for cooling of microelectronic chips. Heat transfer in the fully-developed MEB in the microchannel is presented, which is compared with existing subcooled flow boiling heat transfer correlations for macrochannels.