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1.
A method to identify core documents within a given subject domain has been developed by the author. The method builds on the
concept of polyrepresentation by using different search rationales in several databases and isolating the overlaps between
them. This paper delineates the ideas behind the method and describes the study done to measure its effectiveness.
This revised version was published online in June 2006 with corrections to the Cover Date. 相似文献
2.
Summary
We report the synthesis of some new backbone fluorinated
polymers of the poly(phenylenevinylene) type. The new polymers
were characterised by NMR, SEC and X-ray powder diffraction. The
charge carrier mobilities were determined using pulse radiolysis
time resolved microwave conductivity (PR-TRMC) and the carrier
mobilities were compared to the similar non-fluorinated
analogues. The changes in charge carrier mobilities as a
function of molecular substitution pattern is discussed in terms
of other materials properties such as electronic structure and
absorption properties. The major result is that it was found
possible for this type of material to alter the electronic
energy levels by molecular substitution without imparting
significant changes in the magnitude of the charge carrier
mobilities and the optical properties. 相似文献
3.
Meng Li Clara Seinsche Samuel Jansson Julio Hernandez Jadranka Rota Eric Warrant Mikkel Brydegaard 《Journal of the Royal Society Interface》2022,19(191)
There are hundreds of thousands of moth species with crucial ecological roles that are often obscured by their nocturnal lifestyles. The pigmentation and appearance of moths are dominated by cryptic diffuse shades of brown. In this study, 82 specimens representing 26 moth species were analysed using infrared polarimetric hyperspectral imaging in the range of 0.95–2.5 µm. Contrary to previous studies, we demonstrate that since infrared light does not resolve the surface roughness, wings appear glossy and specular at longer wavelengths. Such properties provide unique reflectance spectra between species. The reflectance of the majority of our species could be explained by comprehensive models, and a complete parametrization of the spectral, polarimetric and angular optical properties was reduced to just 11 parameters with physical units. These parameters are complementary and, compared with the within-species variation, were significantly distinct between species. Counterintuitively to the aperture-limited resolution criterion, we could deduce microscopic features along the surface from their infrared properties. These features were confirmed by electron microscopy. Finally, we show how our findings could greatly enhance opportunities for remote identification of free-flying moth species, and we hypothesize that such flat specular wing targets could be expected to be sensed over considerable distances. 相似文献
4.
Shreesha Rao D.S Mikkel Jensen Lars Grüner-Nielsen Jesper Toft Olsen Peter Heiduschka Bj?rn Kemper Jürgen Schnekenburger Martin Glud Mette Mogensen Niels M?ller Israelsen Ole Bang 《光:科学与应用(英文版)》2021,10(7):1372-1384
We present the first demonstration of shot-noise limited supercontinuum-based spectral domain optical coherence tomography (SD-OCT) with an axial resolution of ... 相似文献
5.
Song J Chen M Olesen MB Wang C Havelund R Li Q Xie E Yang R Bøggild P Wang C Besenbacher F Dong M 《Nanoscale》2011,3(12):4966-4971
Core-sheath silver nanowire/polyvinylpyrrolidone (AgNW/PVP) nanocables have been fabricated via an efficient single-spinneret electrospinning method. The core-sheath structure is revealed by combining several characterization methods. A possible formation mechanism of the AgNW/PVP nanocable involving a strong stretching during the electrospinning process is proposed. Further, electrical measurements were performed on AgNW/PVP nanocables as well as bare AgNWs, which indicated the nanocables became insulating due to the isolation of highly conductive AgNWs by insulating PVP sheath. Therefore, the described fabrication method holds potential for the fabrication of low-cost metal/polymer composite materials for nanoelectronic applications in general. 相似文献
6.
Kacper Januchta Theany To Mikkel S. Bødker Tanguy Rouxel Morten M. Smedskjaer 《Journal of the American Ceramic Society》2019,102(8):4520-4537
Due to an increasing demand for oxide glasses with a better mechanical performance, there is a need to improve our understanding of the composition-structure-mechanical property relations in these brittle materials. At present, some properties such as Young's modulus can to a large extent be predicted based on the chemical composition, while others—in particular fracture-related properties—are typically optimized based on a trial-and-error approach. In this work, we study the mechanical properties of a series of 20 glasses in the quartenary Na2O–Al2O3–B2O3–SiO2 system with fixed soda content, thus accessing different structural domains. Ultrasonic echography is used to determine the elastic moduli and Poisson's ratio, while Vickers indentation is used to determine hardness. Furthermore, the single-edge precracked beam method is used to estimate the fracture toughness (KIc) for some compositions of interest. The compositional evolutions of Vickers hardness and Young's modulus are in good agreement with those predicted from models based on bond constraint density and strength. Although there is a larger deviation, the overall compositional trend in KIc can also be predicted by a model based on the strength of the bonds assumed to be involved in the fracture process. 相似文献
7.
Dr. Michael R. Mortensen Dr. Mikkel B. Skovsgaard Prof. Kurt V. Gothelf 《Chembiochem : a European journal of chemical biology》2019,20(21):2711-2728
The plethora of methods developed for the creation of protein conjugates often differs significantly with regard to the heterogeneity of the resulting products, in the degree of genetic manipulation of the protein required, and in the technical skills required to perform the conjugation procedure. Affinity-guided protein conjugation is a protein labeling methodology based on noncovalent binding interactions between a labeling probe and the protein of interest. These interactions increase the local concentration of a reactive group in the probe on the protein surface thus facilitating the conjugation in proximity of the complexation site. The ability to produce high-quality conjugates from nongenetically modified proteins both in vitro, but also in cells, demonstrates the power of affinity-guided protein conjugation. Here, we present the progress of affinity-guided protein conjugation in relation to selective protein labeling in living systems and the formation of high-quality protein conjugates. Furthermore, the probe design will be discussed in relation to the utility of the probe for labeling in vitro or in living systems. 相似文献
8.
Mie Lillethorup Mikkel Kongsfelt Marcel Ceccato Bjarke B. E. Jensen Bjarke Jørgensen Steen U. Pedersen Kim Daasbjerg 《Small (Weinheim an der Bergstrasse, Germany)》2014,10(5):922-934
Electrografting using aryldiazonium salts provides a fast and efficient technique to functionalize commercially available 3?5 layered graphene (vapour‐deposited) on nickel. In this study, Raman spectroscopy is used to quantify the grafting efficiency of cyclic voltammetry which is one of the most versatile, yet simple, electrochemical techniques available. To a large extent the number of defects/substituents introduced to the basal plane of high‐quality graphene by this procedure can be controlled through the sweeping conditions employed. After extended electrografting the defect density reaches a saturation level (~1013 cm?2) which is independent of the quality of the graphene expressed through its initial content of defects. However, it is reached within fewer voltammetric cycles for low‐quality graphene. Based on these results it is suggested that the grafting occurs (a) directly at defect sites for, in particular, low‐quality graphene, (b) directly at the basal plane for, in particular, high‐quality graphene, and/or (c) at already grafted molecules to give a mushroom‐like film growth for all films. Moreover, it is shown that a tertiary alkyl bromide can be introduced at a given surface density to serve as radical initiator for surface‐initiated atom transfer radical polymerization (SI‐ATRP). Brushes of poly(methyl methacrylate) are grown from these substrates, and the relationship between polymer thickness and sweeping conditions is studied. 相似文献
9.
Frederik C. Krebs Kristian O. Sylvester‐Hvid Mikkel Jrgensen 《Progress in Photovoltaics: Research and Applications》2011,19(1):97-112
A compact platform for testing solar cells is presented. The light source comprises a multi‐wavelength high‐power LED (light emitting diode) array allowing the homogenous illumination of small laboratory solar cell devices (substrate size 50 × 25 mm) within the 390–940 nm wavelength range. The spectrum can be synthesized by independent tuning of the 18 different wavelengths to mimic AM1.5G as well as various indoor lamp spectra. The intensity can be controlled with a 214‐bit accuracy and intensities up to 3 suns are possible with an approximate AM1.5G spectral distribution. For several wavelengths intensities up to 10 suns is possible, and for a few wavelengths up to 30 suns can be reached. The setup is equipped with reference diodes and an optical fibre coupling enabling calibration, monitoring and control of the light impinging on the sample. Through a computer controlled interface, it is possible to perform all the commonly employed measurements on the solar cell at very high speed without moving the sample. In particular, the LED‐based illumination system provides an alternative to light‐biased incident photon‐to‐current efficiency measurement to be performed which we demonstrate. Both top and bottom contact is possible and the atmosphere can be controlled around the sample during measurements. The setup was developed for the field of polymer and organic solar cells with particular emphasis on enabling different laboratories to perform measurements in the same manner and obtain a common basis for comparing data. The use of the platform is demonstrated using a standard P3HT:PCBM polymer solar cell but is generally applicable to any solar cell technology with a spectral response in the 390–950 nm region. Copyright © 2010 John Wiley & Sons, Ltd. 相似文献
10.
Mikkel Eske Nørgaard Sørensen Søren Hansen Morten Breivik Mogens Blanke 《Journal of Intelligent and Robotic Systems》2017,87(1):187-207
This paper combines fault-dependent control allocation with three different control schemes to obtain fault tolerance in the longitudinal control of unmanned aerial vehicles. The paper shows that fault-dependent control allocation is able to accommodate actuator faults that would otherwise be critical and it makes a performance assessment for the different control algorithms: an \(\mathcal {L}_{1}\) adaptive backstepping controller; a robust sliding mode controller; and a standard PID controller. The actuator faults considered are the partial to total loss of the elevator, which is a critical component for the safe operation of unmanned aerial vehicles. During nominal operation, only the main actuator, namely the elevator, is active for pitch control. In the event of a partial or total loss of the elevator, fault-dependent control allocation is used to redistribute control to available healthy actuators. Using simulations of a Cessna 182 aircraft model, controller performance and robustness are evaluated by metrics that assess control accuracy and energy use. System uncertainties are investigated over an envelope of pertinent variation, showing that sliding mode and \(\mathcal {L}_{1}\) adaptive backstepping provide robustness, where PID control falls short. Additionally, a key finding is that the fault-dependent control allocation is instrumental when handling actuator faults. 相似文献