Metal halide perovskite single crystals are promising for diverse optoelectronic applications due to their outstanding properties. In comparison to the bulk, the crystal surface suffers from high defect density and is moisture sensitive; however, surface modification strategies of perovskite single crystals are relatively deficient. Herein, solar cells based on methylammonium lead triiodide (MAPbI3) thin single crystals are selected as a prototype to improve single-crystal perovskite devices by surface modification. The surface trap passivation and protection against moisture of MAPbI3 thin single crystals are achieved by one bifunctional molecule 3-mercaptopropyl(dimethoxy)methylsilane (MDMS). The sulfur atom of MDMS can coordinate with bare Pb2+ of MAPbI3 single crystals to reduce surface defect density and nonradiative recombination. As a result, the modified devices show a remarkable efficiency of 22.2%, which is the highest value for single-crystal MAPbI3 solar cells. Moreover, MDMS modification mitigates surface ion migration, leading to enhanced reverse-bias stability. Finally, the cross-link of silane molecules forms a protective layer on the crystal surface, which results in enhanced moisture stability of both materials and devices. This work provides an effective way for surface modification of perovskite single crystals, which is important for improving the performance of single-crystal perovskite solar cells, photodetectors, X-ray detectors, etc. 相似文献
LTE-A network offers data rates up to 1 Gbps which is 10?×?faster than LTE catering to growing demand of users. LTE improves user experience by reducing latency and increasing bandwidth efficiency. The emerging services and key enhancements such as Further Enhancement of Downlink Multiple-Input Multiple-Output (MIMO), Heterogeneous Networks, and Carrier Aggregation (CA) in LTE-A has improved performance of LTE-A networks. Scheduling optimization still remains one of the biggest challenges in high speed data transmission network. Scheduling in LTE-A networks are performed at various levels; User Equipment (UE), Serving Gateway (SGW), Air Interface and eNodeB. Remote Radio Head (RRH) is an extremely specialized device installed at antenna of eNodeB for optical to electrical signal conversion, amplification of signals and Uplink and Downlink Scheduling. Resource scheduling at Antenna of eNodeB module is constituted as a significant research optimization area. This paper proposes a soft computing based scheduler for RRH. Results of proposed technique are evaluated on Fairness Index, Throughput, Spectral Efficiency and Rank Indicator Distribution. The proposed algorithm aims to improve performance of scheduling. From experimental results, it is observed that proposed model succeeds to achieve significantly better performance as compared to state-of-art algorithms.