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41.
Allemann C Gordillo R Clemente FR Cheong PH Houk KN 《Accounts of chemical research》2004,37(8):558-569
Computational studies have led to models to understand some classic and contemporary asymmetric reactions involving organocatalysts. The Hajos-Parrish-Eder-Sauer-Wiechert reaction and intermolecular aldol reactions as well as Mannich reactions and oxyaminations catalyzed by proline and other amino acids, and Diels-Alder reactions catalyzed by MacMillan's chiral amine organocatalysts have been studied with density functional theory. Quantitative predictions for several new catalysts and reactions are provided. 相似文献
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43.
The growing popularity of the Video on Demand service in the Internet Protocol Television environments and the demand for increased quality of the offered videos are becoming a serious threat for the service providers because the high amounts of video traffic are causing congestion in the delivery networks. One of the most acceptable approaches to solve this issue is the peer-assisted streaming, where the peers participate in the streaming process in order to alleviate the load on the streaming servers and in the core of the network. Although the reliability of the Peer-to-Peer service is considerably improved in the managed networks because of the control that the operators have over the clients’ Set-Top Boxes, the failures of the peers still cannot be completely eliminated. The operator can take advantage of the streaming and storage resources of the clients and use them for peer-assisted streaming only while they are watching a video, but not after they finish the streaming session because they may turn off their receiving devices until the next session. In this chapter, we address the issue of the failures of the peers in such environments and their influence on the traffic requested from the servers for providing uninterrupted video experience. For that purpose, we propose a precise mathematical tool for modelling a peer-assisted system for Video on Demand streaming in managed networks with non-cooperative peers, which may decide not to share their resources while they are not active. This tool calculates the performance of the system taking into consideration large variety of system parameters, including the failure probability and the time the peers spend until they decide to turn on the STB and join the network. As the results from the simulations verify the correctness of the mathematical model, we use it to analyse how the failures of the peers are affecting the system’s performance for different system parameters. 相似文献
44.
Roshan Lalintha Peiris Mili John Tharakan Owen Noel Newton Fernando Adrian David Cheok 《Multimedia Tools and Applications》2013,66(1):81-94
This paper presents, AmbiKraf, a non-emissive fabric display that subtly animates patterns on common fabrics. We use thermochromic inks and peltier semiconductor elements to achieve this technology. With this technology we have produced numerous prototypes from animated wall paintings to pixilated fabric displays. The ability of this technology to subtly and ubiquitously change the color of the fabric itself has made us able to merge different fields and technologies with AmbiKraf. In addition, with an animated room divider screen, Ambikraf merged its technology with Japanese Byobu art to tighten the gap between traditional arts and contemporary technologies. Through this AmbiKraf Byobu art installation and other installations, we discuss the impact of this technology as a ubiquitous fabric display. With focus to improvements of some limitations of the existing system, we present our future vision that enables us to merge this technology into more applications fields thus making this technology a platform for ubiquitous interactions on our daily peripherals. 相似文献
45.
In this paper, a fuzzy logic controller (FLC) based variable structure control (VSC) is presented. The main objective is to obtain an improved performance of highly non‐linear unstable systems. New functions for chattering reduction and error convergence without sacrificing invariant properties are proposed. The main feature of the proposed method is that the switching function is added as an additional fuzzy variable and will be introduced in the premise part of the fuzzy rules; together with the state variables. In this work, a tuning of the well known weighting parameters approach is proposed to optimize local and global approximation and modelling capability of the Takagi‐Sugeno (T‐S) fuzzy model to improve the choice of the performance index and minimize it. The main problem encountered is that the T‐S identification method can not be applied when the membership functions are overlapped by pairs. This in turn restricts the application of the T‐S method because this type of membership function has been widely used in control applications. The approach developed here can be considered as a generalized version of the T‐S method. An inverted pendulum mounted on a cart is chosen to evaluate the robustness, effectiveness, accuracy and remarkable performance of the proposed estimation approach in comparison with the original T‐S model. Simulation results indicate the potential, simplicity and generality of the estimation method and the robustness of the chattering reduction algorithm. In this paper, we prove that the proposed estimation algorithm converge the very fast, thereby making it very practical to use. The application of the proposed FLC‐VSC shows that both alleviation of chattering and robust performance are achieved. 相似文献
46.
A hybrid scheme for the inversion of the Rahman-Pinty-Verstraete (RPV) model is presented. It combines the inversion technique described by Lavergne et al. (Lavergne, T., Kaminski, T., Pinty, B., Taberner, M., Gobron, N., Verstraete, M.M., Vossbeck, M., Widlowski, J.L., Giering, R. (2007). Application to MISR land products of an RPV model inversion package using adjoint and Hessian codes. Remote Sensing of Environment, 107, 362-375.) and a multilayer backpropagation feedforward neural network. The RPV inversion package is applied to a sample set of pixels within the satellite scene. Subsequently the pairs of bidirectional reflectance factors (BRF) and model parameters estimated from the sample set of pixels are used to train the neural network. Since the mathematical formulation of the RPV model is embedded in these training data variables, the neural network can efficiently retrieve the model parameters for the whole satellite scene. This scheme has been tested for a MISR L2 BRF scene, MISR L1B2-derived BRF data corresponding to two different dates and a mosaic of MISR L2 BRF scenes acquired over Southern Africa covering a large extent of Miombo woodland. The results show this strategy retrieves the RPV model parameters and uncertainties with high accuracy and considerable speed over large areas. 相似文献
47.
48.
A steady-state interval operability methodology is introduced here for multivariable non-square systems with fewer inputs than output variables to be used in the design of model-based constrained controllers (MPC, DMC). For such systems, set-point control is not possible for all the outputs and interval control is needed. The proposed iterative approach enables the selection of the needed interval constraints systematically, so that the tightest possible control is achieved without rendering the control problem infeasible. The application of this methodology to high-dimensional industrial problems characterizing processes of Air Products and Chemicals and DuPont shows that very significant reduction of the constrained region can be achieved from the steady-state point of view. Ratios of the initial to the calculated volume of the constrained regions examined range between 104 and 108. 相似文献
49.
Raquel Santos Mauler Fernando Guaragna Martins Dimitrios Samios 《Polymer Bulletin》1995,35(1-2):151-156
Summary The cleavage of styrene-butadiene rubber (SBR) with periodic acid (H5IO6) and simultaneous injection of ultrasonic radiation has been performed. Two frequencies, 25 and 40 kHz, respectively, have been used. The results demonstrate clearly that 40 kHz ultrasound radiation accelerates significantly the cleavage reaction. The Pearl String Model theory had been used to elucidate this process. 相似文献
50.