全文获取类型
收费全文 | 1110篇 |
免费 | 52篇 |
国内免费 | 19篇 |
专业分类
电工技术 | 59篇 |
综合类 | 3篇 |
化学工业 | 329篇 |
金属工艺 | 37篇 |
机械仪表 | 33篇 |
建筑科学 | 21篇 |
能源动力 | 72篇 |
轻工业 | 69篇 |
水利工程 | 2篇 |
石油天然气 | 1篇 |
无线电 | 79篇 |
一般工业技术 | 233篇 |
冶金工业 | 84篇 |
原子能技术 | 46篇 |
自动化技术 | 113篇 |
出版年
2023年 | 19篇 |
2022年 | 44篇 |
2021年 | 56篇 |
2020年 | 30篇 |
2019年 | 31篇 |
2018年 | 39篇 |
2017年 | 25篇 |
2016年 | 43篇 |
2015年 | 26篇 |
2014年 | 45篇 |
2013年 | 83篇 |
2012年 | 55篇 |
2011年 | 100篇 |
2010年 | 55篇 |
2009年 | 55篇 |
2008年 | 62篇 |
2007年 | 43篇 |
2006年 | 34篇 |
2005年 | 39篇 |
2004年 | 21篇 |
2003年 | 25篇 |
2002年 | 28篇 |
2001年 | 18篇 |
2000年 | 14篇 |
1999年 | 20篇 |
1998年 | 32篇 |
1997年 | 28篇 |
1996年 | 14篇 |
1995年 | 14篇 |
1994年 | 15篇 |
1993年 | 12篇 |
1992年 | 5篇 |
1991年 | 11篇 |
1990年 | 6篇 |
1989年 | 5篇 |
1988年 | 5篇 |
1987年 | 3篇 |
1986年 | 1篇 |
1985年 | 3篇 |
1984年 | 4篇 |
1983年 | 2篇 |
1981年 | 1篇 |
1980年 | 3篇 |
1979年 | 1篇 |
1978年 | 1篇 |
1977年 | 1篇 |
1976年 | 4篇 |
排序方式: 共有1181条查询结果,搜索用时 0 毫秒
91.
Mayuko Iriguchi Hiroki Koda Takamasa Koyama Nobuo Masataka 《Color research and application》2020,45(1):178-182
Women might experience modulation in their perception and cognition of colours and odours during the menstrual cycle, but how women's impressions of and correspondence between colours and odours differ according to the cycle changes remains unknown. Here, we experimentally examined women's performance of several tasks, including evaluation of impressions of colours and odours, matching/nonmatching of colours with odours, and identification of odours, comparing two phases: the beginning of menstruation and ovulation. The results showed that participants had similar impressions of colours and odours and made similar colour choices for odours in both the menstrual and ovulation phases, while “pleasant-unpleasant” impressions of colour and odour might vary according to the menstrual cycle. We found no significant differences in odour identification between the phases. The findings imply that hormonal changes during the menstrual cycle might affect “pleasant-unpleasant” impressions of colour and odour but not other features regarding impressions or crossmodal correspondence. In future studies, examination with a large number of participants is necessary. 相似文献
92.
Methylcyclohexane dehydrogenation for hydrogen production via a bimodal catalytic membrane reactor 下载免费PDF全文
Lie Meng Xin Yu Takuya Niimi Hiroki Nagasawa Masakoto Kanezashi Tomohisa Yoshioka Toshinori Tsuru 《American Institute of Chemical Engineers》2015,61(5):1628-1638
The dehydrogenation of methylcyclohexane (MCH) to toluene (TOL) for hydrogen production was theoretically and experimentally investigated in a bimodal catalytic membrane reactor (CMR), that combined Pt/Al2O3 catalysts with a hydrogen‐selective organosilica membrane prepared via sol‐gel processing using bis(triethoxysilyl) ethane (BTESE). Effects of operating conditions on the membrane reactor performance were systematically investigated, and the experimental results were in good agreement with those calculated by a simulation model with a fitted catalyst loading. With H2 extraction from the reaction stream to the permeate stream, MCH conversion at 250°C was significantly increased beyond the equilibrium conversion of 0.44–0.86. Because of the high H2 selectivity and permeance of BTESE‐derived membranes, a H2 flow with purity higher than 99.8% was obtained in the permeate stream, and the H2 recovery ratio reached 0.99 in a pressurized reactor. A system that combined the CMR with a fixed‐bed prereactor was proposed for MCH dehydrogenation. © 2015 American Institute of Chemical Engineers AIChE J, 61: 1628–1638, 2015 相似文献
93.
Koji Honda Ikuo Yamamoto Masamichi Morita Hiroki Yamaguchi Hiroshi Arita Ryohei Ishige Yuji Higaki Atsushi Takahara 《Polymer》2014
The effect of α-substituent on the molecular motion and wetting behavior of poly{2-(perfluorobutyl)ethyl acrylate} [PFA-C4], poly{2-(perfluorobutyl)ethyl methacrylate} [PFMA-C4], poly{2-(perfluorobutyl)ethyl α-fluoroacrylate} [PFFA-C4], and poly{2-(perfluorobutyl)ethyl α-chloroacrylate} [PFClA-C4] films were characterized by dynamic contact angle measurement, lateral force microscopy (LFM), wide angle X-ray diffraction (WAXD), and X-ray photoelectron spectroscopy (XPS). WAXD of oriented PFClA-C4 fiber suggested the presence of rod-like chain due to the presence of bulky α-substituent. The glass transition temperature (Tg) of PFFA-C4 and PFClA-C4 were well above the room temperature. The water repellencies of PFFA-C4 and PFClA-C4 were as high as that of PFMA-C4 and their oil repellency of PFFA-C4 and PFClA-C4 was higher than the PFMA-C4. This result was originated from the low main chain mobility of PFFA-C4 and PFClA-C4 due to the presence of bulky α-substituents. The effect of molecular motion on water repellency was clarified by the results of temperature dependence studies of dynamic contact angle, LFM, and surface chemical composition measured by XPS. 相似文献
94.
Hiroki Noguchi Atsuhiko TeradaKaoru Onuki Ryutaro Hino 《Chemical Engineering Research and Design》2014
The Japan Atomic Energy Agency has been conducting research and development on the thermo-chemical iodine–sulfur (IS) process, which is one of the most attractive water-splitting hydrogen production methods that uses nuclear thermal energy. The sulfuric acid decomposer is one of the key components of the IS process. The boiling heat transfer coefficients of sulfuric acid solutions are required to design the sulfuric acid decomposer. These coefficients were measured in aqueous solutions where the mole fraction of H2O ranged from 0.17 to 0.37 (heat flux range from 16.9 kW/m2 to 5.6 kW/m2) and compared with the empirical correlations formulated for binary mixtures. A combination of the Stephan–Körner correlation, using the empirical constant A0 = 2.00, and the Nishikawa–Fujita correlation was used to predict the experimental results with an accuracy of ±10%. 相似文献
95.
Qing Wang Liang Yu Hiroki Nagasawa Masakoto Kanezashi Toshinori Tsuru 《Journal of the American Ceramic Society》2020,103(8):4473-4488
Polytitanocarbosilane (TiPCS)-derived ceramic membranes were fabricated using a pre-ceramic polymer. Special attention was focused on a process of thermal-oxidative curing that was used to induce cross-linking and the effect of this process on the ceramic yield, thermal stability, oxidation resistance, and microstructure of TiPCS. The cross-linked TiPCS powders showed a ceramic yield and thermal stability that were higher than that from the non-cross-linked version. In addition, the cross-linked TiPCS with uniform micropores showed higher levels of N2 and CO2 adsorption capacity, BET surface area, and micropore volume than the non-cross-linked versions, and the cross-linking process enhanced the stability of the pore structure at high temperature. The cross-linked TiPCS membranes showed high H2 permeance (1.49 × 10−6 mol/(m2 s Pa)) with sub-nanopores (H2/SF6 selectivity: 12 000, H2/N2: 10), and in addition higher oxidation resistance than their non-cross-linked counterparts. Furthermore, the influence of the concentration of the TiPCS precursor coating solution was optimized and the hydrothermal stability of the membranes at high temperatures was also evaluated. The optimized membrane demonstrated great performance for the pervaporation removal of methanol in binary azeotropic systems of either MeOH/butyl acetate or MeOH/toluene, and it also showed high hydrothermal stability with excellent dehumidification performance under high temperatures. 相似文献
96.
Aiichiro Nagaki Yiyuan Jiang Hiroki Yamashita Naoshi Takabayashi Yusuke Takahashi Jun-ichi Yoshida 《化学工程与技术》2019,42(10):2113-2118
The lithiation of 5,5′‐dibromo‐2,2′‐bithiophene with one equivalent of an alkyllithium such as n‐BuLi or s‐BuLi was studied by varying the residence time in flow microreactors. With a short residence time, the product 2,2′‐bithiophene (3) derived from dilithiation was obtained preferentially and a significant amount of the starting material 5,5′‐dibromo‐2,2′‐bithiophene remained unchanged. An increase in the residence time caused a higher yield of the product 5‐bromo‐2,2′‐bithiophene derived from monolithiation with expense in the yields of 2,2′‐bithiophene and 5,5′‐dibromo‐2,2′‐bithiophene. The lithiation using MeLi gave the product 5‐bromo‐2,2′‐bithiophene preferentially even with a very short residence time. 相似文献
97.
98.
Development of biobased microwave absorbing composites with various magnetic metals and carbons 下载免费PDF全文
Shinji Kanehashi Hiroki Oyagi Toraki Iwamaru Shota Ando Kazukiyo Nagai Shinichiro Uekusa Tetsuo Miyakoshi 《应用聚合物科学杂志》2016,133(44)
The preparation and characterization of a biobased electromagnetic absorbing composites derived from natural lacquer as a renewable resource with microwave‐absorption fillers, including Ni–Zn ferrite and carbonyl iron (CI) as magnetic metals and soot and carbon nanotube (CNT) as carbon materials, were investigated in terms of the gel content, hardness, drying properties, and electromagnetic absorption properties. Interestingly, composites with ferrite and CI contained up to 320 and 550 wt %, respectively, of these compounds. This quite high loading capacity of the metal fillers in a natural‐lacquer base could have been due to the high compatibility between the filler and the natural lacquer; this indicated that the natural lacquer worked as a binder for these metals. The morphology of the biobased composite was characterized by scanning electron microscopy. The electromagnetic absorption properties of composites were characterized in the frequency range from 0.05 and 20 GHz by the reflection loss (RL) measurement method in terms of the kind of fillers and filler loading. The natural lacquer did not affect the absorption properties of the fillers. Biobased composites showed over 99% electromagnetic absorption in the frequency range 3.0–4.0 GHz for 280 wt % ferrite and 8.9–9.7 GHz for 200 wt % CI. Conversely, 10 and 20 wt % soot exhibited good performance (RL < ?20 dB) between 16.5 and 17.3 and between 8.8 and 9.2 GHz, respectively. The areas with RL values of less than ?20 dB of the CNT composites were 10.4–11.0 GHz for 5 wt % and 14.6–15.2 GHz for 10 wt %. Hence, natural lacquer can be used as a binder material for electromagnetic absorption composites. © 2016 Wiley Periodicals, Inc. J. Appl. Polym. Sci. 2016 , 133, 44131. 相似文献
99.
Fast Labelling of Natural Scenes Using Enhanced Knowledge 总被引:1,自引:0,他引:1
Hiroki Hayashi Mineichi Kudo Jun Toyama Masaru Shimbo 《Pattern Analysis & Applications》2001,4(1):20-27
A new technique for labelling natural scenes is proposed. This technique labels disjoint regions on an image of a natural
scene on the basis of knowledge about the relationship among objects. The proposed technique consists of three stages: (1)
segmentation, (2) initial labelling, and (3) label improvement. One of the most promising previous techniques uses simulated
annealing to find the solution, while our technique uses local hill-climbing with enhanced knowledge for speeding up the processing.
Local hill-climbing is known to be easy to be captured by a local minimum. We solved this problem by enhancing the knowledge
being used as constraints for the search. Our knowledge represents 1-to-n relationships among regions, pair-wise relationships of regions, and relative locations of the regions to the image. In addition,
we introduced two region features: an entropy in intensity; and a linearity of contours of each region. The linearity evaluation
aims to distinguish artificial objects from natural objects. The validity of the technique is supported by some experiments.
These experiments showed that the proposed technique is much faster with the almost same accurate. 相似文献
100.
Miyajima H. Asaoka N. Arima M. Minamoto Y. Murakami K. Tokuda K. Matsumoto K. 《Journal of microelectromechanical systems》2001,10(3):418-424
This paper presents a moving-coil electromagnetic optical scanner with newly developed hinge structure consisting of multilayered polyimide films with aluminum lead wires in between. The main purpose is to obtain a scanner with good durability and shock resistance for practical use. Polyimide has both features, and the aluminum lead wires, connecting the moving-coils and fixed electrode pads, are more reliable, because they are located inside the hinge, where the stress caused by torsional deformation and atmospheric degradation are minimal. An electromagnetic actuator is used to satisfy the following requirements; a millimeter-sized mirror, resonant and galvanometric operation, and scan angle control. Scanner prototypes with two different specifications (i.e., fast scanner and slow scanner) were fabricated and characterized. Driven with a sinusoidal current of ±20 mA, the fast scanner and the slow one vibrated with an optical scan angle (&thetas;o) of 1° at the resonant frequency (fr) of 1.7 kHz and &thetas;o of 60° at fr of 72 Hz, respectively. Durability was demonstrated with a shock test of 2500 G and a life test of over 13 000 h. By substituting sputtered aluminum driving coil with electroplated copper coil, improved &thetas;o of 16.8° was obtained at fr of 2.7 kHz 相似文献