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971.
972.
Monitoring the Dynamic Process of Formation of Plasmonic Molecular Junctions during Single Nanoparticle Collisions 下载免费PDF全文
Jing Guo Jie Pan Shuai Chang Xuewen Wang Na Kong Wenrong Yang Jin He 《Small (Weinheim an der Bergstrasse, Germany)》2018,14(15)
The capability to study the dynamic formation of plasmonic molecular junction is of fundamental importance, and it will provide new insights into molecular electronics/plasmonics, single‐entity electrochemistry, and nanooptoelectronics. Here, a facile method to form plasmonic molecular junctions is reported by utilizing single gold nanoparticle (NP) collision events at a highly curved gold nanoelectrode modified with a self‐assembled monolayer. By using time‐resolved electrochemical current measurement and surface‐enhanced Raman scattering spectroscopy, the current changes and the evolution of interfacial chemical bonding are successfully observed in the newly formed molecular tunnel junctions during and after the gold NP “hit‐n‐stay” and “hit‐n‐run” collision events. The results lead to an in‐depth understanding of the single NP motion and the associated molecular level changes during the formation of the plasmonic molecular junctions in a single NP collision event. This method also provides a new platform to study molecular changes at the single molecule level during electron transport in a dynamic molecular tunnel junction. 相似文献
973.
Ke Wang Baodan Liu Jing Li Xiaoyuan Liu Yang Zhou Xinglai Zhang Xiaoguo Bi Xin Jiang 《材料科学技术学报》2019,35(4):615-622
TiO_2 nanostructures with strong interfacial adhesion and diverse morphologies have been in-situ grown on Ti foil substrate through a multiple-step method based on conventional plasma electrolytic oxidation(PEO) technology, hydrothermal reaction and ion exchange process. The PEO process is critical to the formation of TiO_2 seeding layer for the nucleation of Na_2Ti_3O_7 and H_2Ti_3O_7 mediates that are strongly attached to the Ti foil. An ion exchange reaction can finally lead to the formation of H_2Ti_3O_7 nanostructures with diverse morphologies and the calcination process can turn the H_2Ti_3O_7 nanostructures into TiO_2 nanostructures with enhanced crystallinity. The morphology of the TiO_2 nanostructures including nanoparticles(NP), nanowhiskers(NWK), nanowires(NW) and nanosheets(NS) can be easily tailored by controlling the NaOH concentration and reaction time during hydrothermal process. The morphology, composition and optical properties of TiO_2 photocatalysts were analyzed using scanning electron microscope(SEM), X-ray diffraction(XRD), photoluminescence(PL) spectroscopy and UV–vis absorption spectrum. Photocatalytic tests indicate that the TiO_2 nanosheets calcined at 500?C show good crystallization and the best capability of decomposing organic pollutants. The decoration of Ag cocatalyst can further improve the photocatalytic performance of the TiO_2 nanosheets as a result of the enhanced charger separation efficiency. Cyclic photocatalytic test using TiO_2 nanostructures grown on Ti foil substrate demonstrates the superior stability in the photodegradation of organic pollutant, suggesting the promising potential of in-situ growth technology for industrial application. 相似文献
974.
Yixing Tian Huiling Liu Brian W.Sheldon Thomas J.Webster Sichen Yang Huilin Yang Lei Yang 《材料科学技术学报》2019,35(5):817-823
Nanostructured diamond have potential applications in many biomedical related fields and demonstrated extraordinary capacity to influence cellular responses. Studying the surface property of nanodiamond and its influence to protein adsorption and subsequent cellular responses along with the mechanism behind such capacity becomes more important. Here the role of surface energy associated with nanostructured diamond in modulating fibronectin and osteoblast(OB, bone forming cells) responses was investigated. Nanocrystalline diamond(NCD) and submicron crystalline diamond(SMCD) films with controllable surface energy were prepared by microwave-enhanced plasma chemical vapor deposition(MPCVD) techniques. Fibronectin adsorption on the diamond films with varied surface energy values was measured via the enzyme-linked immunosorbent assay(ELISA) and the relationship between the surface energy and fibronectin adsorption was studied. The result indicated that fibronectin adsorption on nanostructured surfaces was closely related to both surface energy and material microstructures. The spreading and migration of OB aggregates(each containing 30–50 cells) on the NCD with varied surface energy values were also studied. The result indicates a correlation between the cell spreading and migration on nanodiamond and the surface energy of nanostructured surface. 相似文献
975.
Jiang Lei Ding Yang Xue Xialin Zhou Sensen Li Cheng Zhang Xiaoke Jiang Xiqun 《Nano Research》2018,11(11):6062-6073
Nano Research - Developing multifunctional nanoparticles to support new therapy models is a promising and challenging task to address the current dilemma on antitumor treatment. Herein, we... 相似文献
976.
利用参数互异的Fitzhugh-Nagumo神经元构建了含耦合时滞的无标度神经元网络模型,通过数值模拟的方法,提出研究参数异质性和耦合时滞影响下神经元网络的共振动力学.结果发现,当耦合项中不含时滞时,适中的参数异质性能够使得神经元网络对外界弱周期信号的响应达到最优,即适中的参数异质性能够诱导神经元网络的共振响应,而且异质性诱导共振对耦合强度具有鲁棒性.更重要的是,耦合时滞对参数异质性作用下神经元网络的共振特性也有着显著性影响.当时滞约为信号周期的整数倍时,神经元网络能够周期性地出现共振现象,即适当的耦合时滞能够诱导神经元网络的多重共振,而且这种现象在异质性参数的适当范围内都能明显出现. 相似文献
977.
随着电力、电气设备的日益复杂化,对于其安全性能也有了更高的要求,数字兆欧表作为测量绝缘阻值的重要工具,已在工业领域中广泛应用;为了满足测量精度以及兆欧表的可靠性,通过基于S3C2440的嵌入式平台,提出了一种基于数字兆欧表的自动切换档位的实现方案,以达到更加精确的测量;此方案通过判断采集到的电压值选择相应的采样电阻来实现,并结合硬件平台和软件设计,分别介绍了驱动程序和应用程序的编写与测试,并很好地应用到了实际电路中;经测试,能够达到预期的效果,测量精度高,测量误差控制在±2%。 相似文献
978.
针对热释电红外传感器(PIR)在人体探测领域中越来越广泛的应用,研究设计了一种基于PIR的检测定位系统,可实时完成对人员目标入侵探测区域时的检测与定位,并预推出人员目标的行进轨迹;该系统由多个PIR感知节点组成,每个感知节点通过传感在动、静两种状态下对探测区域进行信息采集;最终融合多节点与不同状态下传感器采集的数据,算出各个传感器的探测角度值,以交叉定位的算法,得到目标的定位坐标;经实验证明,该系统运行稳定,检测灵敏,定位效果很好,拓宽了热释电传感器在定位定向方面的使用范围。 相似文献
979.
一体化保障技术是目前提高复杂武器系统测试和保障能力的研究重点,为解决一体化保障技术中存在的指标冗余问题,结合粗糙集相关理论,提出了基于属性重要性和属性间影响度的约简算法;通过在某型一体化保障设备的柴油发电机子模块中应用该算法,在精简测试指标的同时,保证了较高的测试准确性,缩短了测试时间,验证并说明该理论可以有效地解决一体化保障技术中的指标冗余问题。 相似文献
980.